X-ray spectroscopy diagnostic of a plasma produced by femtosecond laser pulses irradiating a cluster target

The parameters of a plasma produced upon the interaction of ultrashort laser pulses with cluster targets are measured by the methods of X-ray spectroscopy. The dependence of the plasma parameters on the initial properties of a cluster target (the design of a supersonic nozzle, the average size of clusters, the spatial inhomogeneity) and the laser pulse properties (its duration and contrast) is studied. The plasma diagnostics is performed using the model of formation of emission spectra, which was proposed earlier and includes a number of fitting parameters, which provide good agreement with experimental spectra. The systematic experimental studies performed by us showed that our model of cluster heating by ultrashort pulses is indeed a physical model, and the fitting parameters represent the average values of plasma parameters in the corresponding space-time regions.     

Modeling cluster jets as targets for high-power ultrashort laser pulses

A hydrodynamic model is formulated that describes the formation of clusters in atomic gas jets expanding into vacuum, which are used as laser plasma targets. Detailed model calculations performed for an argon gas jet describe spatial distributions of the density of gas and cluster phases formed in the Laval nozzle at room temperature in a broad range of entrance gas pressures. The cluster density distribution is significantly inhomogeneous. The cluster distribution features revealed by the model calculations were qualitatively confirmed by the X-ray spectroscopic measurements of the spatial distribution of emission from the plasma created in the jet tar-gets by high-power ultrashort laser pulses.     

Generation of higher-order harmonics of chirped radiation from a titanium-sapphire laser in plasma generated by pulses of different durations

The frequency conversion of laser radiation in plasma created by pulses of different durations under conditions of the chirp variation of the radiation to be converted is investigated. It is shown that the chirp variation of the laser pulse during the generation of higher-order radiation harmonics of the femtosecond laser leads to a considerable change in the brightness, wavelength shift, and maximal order of generated harmonics. The long-and short-wavelength shifts of harmonics observed in these studies are attributed to the manifestation of a considerable concentration of free charge carriers in the plasma, as well as the self-modulation of the laser pulse. The generation of plasma by pulses whose durations vary from 160 fs to 20 ns is considered and it is shown that the generation efficiency of harmonics depends to a greater extent on the energy of the heating prepulse than on its intensity on the surface of a target to be ablated. The effect that the atomic number of the target has on the formation of optimal plasma at different delays between the heating prepulse and the femtosecond pulse to be converted is discussed.     

Excitation of low-lying nuclear states by the ion line emission in femtosecond laser plasma

A scheme of nuclear excitation by the ionic X-ray lines in laser plasma using two femtosecond laser pulses is proposed. The first pulse produces plasma with a given degree of ionization, allowing the X-ray line energies of the target ions to be tuned to resonance with the nuclear transition, while the second pulse generates hot electrons that are necessary for X-ray generation.     

Role of ambient gas in heating of metal samples by femtosecond pulses of laser radiation

In this work we consider an experimentally observed effect of significant increasing of the residual heat in metal targets at their irradiation with femtosecond laser pulses in an ambient gas in respect to the vacuum conditions. Numerical modelling of heating of a platinum target by femtosecond laser pulses in argon under normal conditions has been performed taking into account gas breakdown in the focussing region of the laser beam in front of the target. The applied model is based on a combination of a thermal model describing heating and phase transitions in irradiated samples and a hydrodynamic model to describe motion of the ambient gas perturbed by laser irradiation as a result of multiphoton ionization. The hot ambient gas is shown to heat efficiently the irradiated sample. The hydrodynamic processes in the ambient gas play an important role in heating. This work was financially supported by the Russian Foundation for Basic Research (Project 08-01-00264-a) and the INTAS/SB RAS Program (Project 06-1000013-8949).     

On the possibility of obtaining incoherent femtosecond X-ray pulses from a laser plasma

It is proposed to use a high rate of collisional ionization in a superdense laser plasma to generate incoherent femtosecond X-ray pulses. The calculations indicate that the use of picosecond laser pulses with a contrast of about 10¹⁰ will allow the generation of an X-ray pulse with a duration of about 10 fs. The adequacy of the proposed model of the excitation of linear X-ray radiation from the plasma has been tested in the experiments with a picosecond laser of a moderately high contrast.     

Direct simulation monte carlo of pulsed laser ablation of metals with clusterization processes in vapor

A mathematical model is proposed to describe laser ablation of metals in vacuum under the action of nanosecond laser pulses of moderate intensity taking into account the processes of cluster formation and decay in the vapor cloud. To describe the laser radiation absorption and metal heating, the thermal model based on the unsteady one-dimensional heat equation with a volume heat source is used, and the method of statistical modelling is employed for modelling vapor expansion and the processes of cluster formation. The efficiency of the proposed complex model is considered by the example of pulsed laser ablation of a niobium target. The work was supported financially by INTAS (grant No. 03-51-5208).     

Interference model of femtosecond laser pulse conical emission in dispersive medium

A simple interference model is proposed for conical emission frequency-angular spectrum formation during the filamentation of femtosecond laser pulse in a nonlinear dispersive medium. The model allows to obtain analytical expressions for frequency-angular distributions of the supercontinuum spectral components of pulses at different wavelengths in media with arbitrary material dispersion law. The model reproduces the supercontinuum frequency-angular spectrum transformation for the case of laser pulse splitting into several subpulses and for multiple refocusing of the light field in filament. Frequency-angular spectra analytically calculated from the proposed interference model are in good agreement with the results of numerical simulations performed for the filamentation of femtosecond laser pulses in fused silica.     

Explosions of xenon clusters in ultraintense femtosecond x-ray pulses from the LCLS free electron laser

Explosions of large Xe clusters ( ~ 11,000) irradiated by femtosecond pulses of 850 eV x-ray photons focused to an intensity of up to 10(17) W/cm(2) from the Linac Coherent Light Source were investigated experimentally. Measurements of ion charge-state distributions and energy spectra exhibit strong evidence for the formation of a Xe nanoplasma in the intense x-ray pulse. This x-ray produced Xe nanoplasma is accompanied by a three-body recombination and hydrodynamic expansion. These experimental results appear to be consistent with a model in which a spherically exploding nanoplasma is formed inside the Xe cluster and where the plasma temperature is determined by photoionization heating.     

Multistep ionization of argon clusters in intense femtosecond extreme ultraviolet pulses

The interaction of intense extreme ultraviolet femtosecond laser pulses (lambda = 32.8 nm) from the FLASH free electron laser (FEL) with clusters has been investigated by means of photoelectron spectroscopy and modeled by Monte Carlo simulations. For laser intensities up to 5x10(13) W/cm(2), we find that the cluster ionization process is a sequence of direct electron emission events in a developing Coulomb field. A nanoplasma is formed only at the highest investigated power densities where ionization is frustrated due to the deep cluster potential. In contrast with earlier studies in the IR and vacuum ultraviolet spectral regime, we find no evidence for electron emission from plasma heating processes.     

基于双相延迟模型的飞秒激光烧蚀金属模型

为了分析飞秒激光烧蚀过程,在双相延迟模型的基础上建立了双曲型热传导模型.模型中考虑了靶材的加热、蒸发和相爆炸,还考虑了等离子体羽流的形成和膨胀及其与入射激光的相互作用,以及光学和热物性参数随温度的变化.研究结果表明:等离子体屏蔽对飞秒激光烧蚀过程有重要的影响,特别是在激光能量密度较高时;两个延迟时间的比值对飞秒激光烧蚀过程中靶材的温度特性和烧蚀深度有较大的影响;飞秒激光烧蚀机制主要以相爆炸为主.飞秒激光烧蚀的热影响区域较小,而且热影响区域的大小受激光能量密度的影响较小.计算结果与文献中实验结果的对比表明基于双相延迟模型的飞秒激光烧蚀模型能有效对飞秒激光烧蚀过程进行模拟.     

Pulsed Gas Jet for Large Size Atomic Cluster Production

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Effect of laser spot size on fusion neutron yield in laser--deuterium cluster interactions

The effect of the laser spot size on the neutron yield of table-top nuclear fusion from explosions of a femtosecond intense laser pulse heated deuterium clusters is investigated by using a simplified model, in which the cluster size distribution and the energy attenuation of the laser as it propagates through the cluster jet are taken into account. It has been found that there exists a proper laser spot size for the maximum fusion neutron yield for a given laser pulse and a specific deuterium gas cluster jet. The proper spot size, which is dependent on the laser parameters and the cluster jet parameters, has been calculated and compared with the available experimental data. A reasonable agreement between the calculated results and the published experimental results is found.     

Guiding of intense laser pulses in plasma waveguides produced from efficient, femtosecond end-pumped heating of clustered gases

We demonstrate intense pulse guiding in efficient femtosecond end-pumped waveguides generated in clustered gases. This novel scheme provides a route to significantly lower on-axis plasma density (< 10(18) cm(-3)) more than is feasible in conventional hydrodynamic plasma waveguides. Self-focused propagation and strong absorption of intense femtosecond laser pulses are used to produce long centimeter scale channels in an argon cluster jet, and a subsequent pulse is guided with 3 x 10(17) W cm(-2) intensity and approximately 50% coupling efficiency. Preliminary results with hydrogen clusters also show guiding.     

Pulsed Gas Jet for Large Size Atomic Cluster Production

A pulsed gas jet of large size noble gas atomic clusters as targets for high intensity femtosecond laser pulses is reported. The jet can work for gas stagnation pressure in excess of 40 atmospheres and with a repetition rate of 10 Hz to fit 10 Hz table-top terrawatt femtosecond Ti∶Sapphire laser. The scaling law indicates that the monomer argon clusters produced in the jet can be as large as 22,000 atoms/cluster at room temperature. Preliminary experiments for argon ionic kinetic energy spectrum indicated that the argon clusters are produced in the jet.     

Angular distribution of ejected electrons at the laser-cluster interactions

The histograms of deflection angles of electrons ejected from Xe clusters irradiated by femtosecond super-intense laser pulses are presented. The dependence of the angular distribution on the peak laser intensity, the pulse duration, and the cluster position is considered. A clear relationship between the final electron energy and the deflection angle is shown. The deflection angles are calculated by solving the relativistic equation of motion taking into account the Lorentz force and the Coulomb field of the ionized cluster. The ions in the cluster undergo sequential multiple ionization up to charge multiplicity Z = 26. The measurements of the electron angular distributions allow us to reproduce the imaging dynamics of outer ionization of the cluster at the leading edge of the relativistic femtosecond laser pulse.     

Vacuum heating of solid target irradiated by femtosecond laser pulses

The interaction of femtosecond laser pulses with solid targets was studied through experiments and particle-in-cell (PIC) simulations. It is proved that the vacuum heating and the inverse bremsstralung process are the main mechanisms of the laser pulse absorption under such conditions. The distribution of hot electrons and that of X-ray are found to have double-temperature structure, which is confirmed by PIC simulations. While the lower temperature is attributed to the resonant absorption, the higher one, however, is caused by the laser-induced electric field in the target normal direction. The time-integrated spectra ofthe reflected laser pulse shows that the mechanism of electron acceleration is determined by the plasma density profile.