Penning collisions of laser-cooled metastable helium atoms

We present experimental results on the two-body loss rates in a magneto-optical trap of metastable helium atoms. Absolute rates are measured in a systematic way for several laser detunings ranging from -5 to -30 MHz and at different intensities, by monitoring the decay of the trap fluorescence. The dependence of the two-body loss rate coefficient β on the excited state ( 2³ P ₂) and metastable state ( 2³ S ₁) populations is also investigated. From these results we infer a rather uniform rate constant K _sp = (1±0.4)×10^-7 cm³/s. Received 8 September 2000 and Received in final form 19 December 2000     

Mixture of ultracold lithium and cesium atoms in an optical dipole trap

We present the first simultaneous trapping of two different ultracold atomic species in a conservative trap. Lithium and cesium atoms are stored in an optical dipole trap formed by the focus of a CO₂ laser. Techniques for loading both species of atoms are discussed and observations of elastic and inelastic collisions between the two species are presented. A model for sympathetic cooling of two species with strongly different mass in the presence of slow evaporation is developed. From the observed Cs-induced evaporation of Li atoms we estimate a cross-section for cold elastic Li-Cs collisions. Received: 1 August 2001 / Published online: 23 November 2001     

Cross-section for collisions of ultracold Li with Na

In a magneto-optical trap (MOT) we are able to simultaneously trap and cool ⁷Li and Na. We investigated the loading behavior of the cloud of Li atoms in presence of the overlapped cloud of cold Na atoms, and, by blocking the weak repumping beam for Na, compared it with the loading curve for Li atoms only. Out of these loading curves we calculated the collision cross-section of Na on Li to be 10^-11 cm ³ /s. Received 11 January 2002 / Received in final form 5 April 2002 Published online 24 September 2002     

An atom faucet

We present a simple and efficient source of slow atoms. From a background vapour loaded magneto-optical trap (MOT), a thin laser beam extracts a continuous jet of cold rubidium atoms. The jet that is typical to leaking MOT systems is created without any optical parts placed inside the vacuum chamber. We also present a simple three dimensional numerical simulation of the atomic motion in the presence of these multiple saturating laser fields combined with the inhomogeneous magnetic field of the MOT. At a pressure of P _Rb87 = 10^-8 mbar and with a moderate laser power of 10 mW per beam, we generate a flux Φ = 1.3×10⁸ atoms/s with a mean velocity of 14 m/s and a divergence of 10 mrad. Received 13 January 2001     

Photoassociation of heteronuclear lithium

Photoassociation of ultracold heteronuclear ⁶Li⁷Li molecules is observed inside a combined magneto-optical trap for ⁶Li and ⁷Li. The trapped atomic cloud is illuminated by a tunable single-mode laser and the number of trapped ⁷Li atoms is monitored by absorption spectroscopy. Characteristic hyperfine resolved spectra have been recorded for singlet spin orientation. Interesting saturation effects have been observed. Received: 12 July 2001 / Revised version: 1 October 2001 / Published online: 23 November 2001     

Sisyphus cooling of rubidium atoms on the line: The role of the neighbouring transitions

We study one-dimensional Sisyphus cooling on the transition of ⁸⁷ Rb atoms in the electric field created by two counter-propagating linearly polarized laser beams with an angle of between the polarization directions. The neighbouring F '=0 and F '=2 excited states are found to play an important role in the cooling mechanism, e.g., by inhibiting a significant population of the velocity-selective dark state. Our experimental data, such as temperatures and probe absorption coefficients, agree well with the results of quantum Monte-Carlo wavefunction simulations. Received 26 November 1998 and Received in final form 20 April 1999     

Cold inelastic collisions between lithium and cesium in a two-species magneto-optical trap

We investigate collisional properties of lithium and cesium which are simultaneously confined in a combined magneto-optical trap. Trap-loss collisions between the two species are comprehensively studied. Different inelastic collision channels are identified, and inter-species rate coefficients as well as cross-sections are determined. It is found that loss rates are independent of the optical excitation of Li, as a consequence of the repulsive Li^*-Cs interaction. Li and Cs loss by inelastic inter-species collisions can completely be attributed to processes involving optically excited cesium (fine-structure changing collisions and radiative escape). By lowering the trap depth for Li, an additional loss channel of Li is observed which results from ground-state Li-Cs collisions changing the hyperfine state of cesium. Received 28 December 1998 and Received in final form 16 February 1999     

Optimizing the production of metastable calcium atoms in a magneto-optical trap

We investigate the production of long-lived metastable (4³ P ₂ ) calcium atoms in a magneto-optical trap (MOT) operating on the 4¹ S ₀ ?4¹ P ₁ transition at 423 nm. For excited 4¹ P ₁ atoms a weak decay channel into the triplet states 4³ P ₂ and 4³ P ₁ exists via the 3¹ D ₂ state. The undesired 4³ P ₁ atoms decay back to the ground state within 0.4 ms and can be fully recaptured if the illuminated trap volume is sufficientlylarge. We obtain a flux of above 10¹⁰ atoms/s into the 4³ P ₂ state. We find that our MOT lifetime of 23 ms is mainly limited by this loss channel, and thus the 4³ P ₂ production is not hampered by inelastic collisions. If we close the loss channel by repumping the 3¹ D ₂ atoms with a 671 nm laser back into the MOT cycling transition, a non-exponential 72 ms trap decay is observed, indicating the presence of inelastic two-body collisions between 4¹ S ₀ and 4¹ P ₁ atoms. Received: 10 July 2001 / Revised version: 22 October 2001 / Published online: 23 November 2001     

A continuous cold atomic beam from a magneto-optical trap

We have developed and characterized a new method to produce a continuous beam of cold atoms from a standard vapour-cell magneto-optical trap (MOT). The experimental apparatus is very simple. Using a single laser beam it is possible to hollow out in the source MOT a direction of unbalanced radiation pressure along which cold atoms can be accelerated out of the trap. The transverse cooling process that takes place during the extraction reduces the beam divergence. The atomic beam is used to load a magneto-optical trap operating in an ultra-high vacuum environment. At a vapour pressure of 10^-8mbar in the loading cell, we have produced a continuous flux of 7×10⁷atoms/s at the recapture cell with a mean velocity of 14 m/s. A comparison of this method with a pulsed transfer scheme is presented. Received 19 February 2001     

Production of a bose einstein condensate of metastable helium atoms

We recently observed a Bose-Einstein condensate in a dilute gas of ⁴He in the 2³S₁ metastable state. In this article, we describe the successive experimental steps which led to the Bose-Einstein transition at 4.7 μK: loading of a large number of atoms in a MOT, efficient transfer into a magnetic Ioffé-Pritchard trap, and optimization of the evaporative cooling ramp. Quantitative measurements are also given for the rates of elastic and inelastic collisions, both above and below the transition. Received 15 October 2001     

Acceleration of cold Rb atoms by frequency modulated light pulses

The displacement of Rb atoms in a magneto-optical trap (MOT) caused by the force of a finite time series of counter-propagating frequency modulated light pulse pairs is measured as a function of the chirp of the pulses. The frequency modulated light pulses induced ⁸⁵Rb 5²S_1/2 F=3 ↔ ⁸⁵Rb 5²P_3/2 F'=2, 3, 4 excitation and de-excitation of the atoms. The result of this excitation de-excitation process is a force causing the acceleration and, consequently, the displacement of the maximum of the spatial distribution of the trap atoms. The time dependence of the populations of the levels of the atom are calculated — including also the ⁸⁵Rb 5²S_1/2 F=2 and F'=1 states — as the result of the interaction with the finite train of counter propagating frequency modulated light pulses by the solution of the Bloch equations. As the result of the measurement the interval of the chirp of the frequency modulated light of given intensity where the transitions take place, are determined. The results of the experiment and the expectation on the basis of model calculations are in qualitative agreement.     

Spin-polarized Dirac-Slater calculations on the energies of hollow argon atom

In this work, the multiplet splitting in terms of a spin-dependent model is analyzed. The spin-polarized and unpolarized single configuration Dirac-Fock-Slater wavefunctions have been used in the evaluation of the total energies of highly ionized argon with different L shell population The transition energies of hollow argon atom with initial configurations 1s ⁰ _1/22s ^m _1/22p ⁿ _1/22p ^l _3/2 with m = 0 to 2 and n + l varying from 6 to 1 are reported in this work. The calculations have been carried out by taking into account a relativistic exchange potential in the Dirac-Slater potential. To account for the correlation effects, a correction term has also been considered perturbatively. The present calculations show that the spin-polarized technique which is mainly applied to the ground states of atoms may also be applied to atoms ionized in the inner shells with a good degree of accuracy. Received 5 December 2000 and Received in final form 9 April 2001     

Interaction of frequency modulated light pulses with rubidium atoms in a magneto-optical trap

The spatial displacement of the ⁸⁵Rb atoms in a Magneto-Optical Trap (MOT) under the influence of series of frequency modulated light pulse pairs propagating opposite to each other is measured as a function of the time elapsed after the start of the pulse train, and compared with the results of simulations. Adiabatic excitation and consecutive de-excitation take place between the ground 5²S_1/2 (F=3) and the 5²P_3/2 (F'=2, 3, 4) excited levels as the result of the interaction. The displacement of the ⁸⁵Rb atoms is calculated as the solution of simple equation of motion where the expelling force is that arising from the action of the frequency modulated light pulses. The restoring and friction forces of the MOT are taken into account also. The system of Bloch equations for the density matrix elements is solved numerically for transitions between six working hyperfine levels of the atom interacting with the sequence of the frequency modulated laser pulses. According to these simulations, the momentum transferred by one pulse pair is always smaller than the expected 2ħk, (1) where ħ is the Plank constant and k=2π/λ where λ is the wavelength, (2) having a maximum value in a restricted region of variation of the laser pulse peak intensity and the chirp.     

Accumulation of chromium metastable atoms into an optical trap

We report the fast accumulation of a large number of metastable ⁵²Cr atoms in a mixed trap, formed by the superposition of a strongly confining optical trap and a quadrupolar magnetic trap. The steady state is reached after about 400 ms, providing a cloud of more than one million metastable atoms at a temperature of about 100 μK, with a peak density of 10¹⁸ atoms m^-3. We have optimized the loading procedure, and measured the light shift of the ⁵D₄ state by analyzing how the trapped atoms respond to a parametric excitation. We compare this result to a theoretical evaluation based on the available spectroscopic data for chromium atoms.     

Cold rubidium molecule formation through photoassociation: A spectroscopic study of the 0 g - long-range state of 87 Rb 2

We report the detailed analysis of translationally cold rubidium molecule formation through photoassociation. Cold molecules are formed after spontaneous decay of photoexcited molecules from a laser cooled atomic sample, and are detected by selective mass spectroscopy after two-photon ionization into Rb ₂ ⁺ ions. A spectroscopic study of the 0 _g ^- (5 S + 5 P _3/2 ) pure long-range state of ⁸⁷Rb₂ is performed by detecting the ion yield as a function of the photoassociation laser frequency; the spectral data are theoretically analyzed within the semiclassical RKR approach. Molecular ionization is resonantly enhanced through either the 2 ³ Π _g or the 2 ³ Σ ⁺ _g intermediate molecular states. Some vibrational levels of the latter electronic state are observed and assigned here for the first time. Finally, cold molecules formation rates are calculated and compared to the experimentally measured ones, and the vibrational distribution of the formed molecules in the a ³ Σ ⁺ _u ground triplet state is discussed. Received 18 January 2001 and Received in final form 10 April 2001     

Decay rate measurement of lithium in a magneto-optical trap

A detailed account of various experimental techniques developed during the study on the decay rate coefficient of laser trapped ⁷Li atoms are presented. The frequency of a dye laser is stabilized using a simple sealed-off cell specially designed for Li vapor. The accurate number of trapped atoms are obtained by measuring the fluorescence intensity and the population ratio between the ground and the excited states by absorption coefficient measurement. The absolute value of the collisional lossrate coefficient of trapped ⁷Li atoms is determined by analyzing the temporal change of the fluorescence intensity when the supply of the Li beam is turned off.     

Dynamics of resonant energy transfer in a cold Rydberg gas

We investigate excitation transfer and migration processes in a cold gas of rubidium Rydberg atoms. Density-dependent measurements of the resonant population exchange for atoms initially excited into the 32P_3/2(|m_J|=3/2) state are compared with a Monte Carlo model for coherent energy transfer. The model is based on simulations of small atom subensembles involving up to ten atoms interacting via coherent pair processes. The role of interatomic mechanical forces due to the resonant dipole-dipole interaction is investigated. Good agreement is found between the experimental data and the predictions of the model, from which we infer that atomic motion has negligible influence on the energy transfer up to Rydberg densities of 10⁸ cm^-3, that the system has to be described in terms of many-body dynamics, and that the energy transfer preserves coherence on microsecond timescales.     

Pulsed polarization gradient cooling in an optical dipole trap with a Laguerre-Gaussian laser beam

We utilized a blue-detuned Laguerre-Gaussian (doughnut) laser beam to trap cold rubidium atoms by optical dipole force. ”Pulsed” polarization gradient cooling was applied to the trapped atoms to suppress the trap loss due to heating caused by random photon scattering of the trapping light. In this trap about 10⁸ atoms were initially captured and the trap lifetime was 1.5 s, which was consistent with losses due to background gas collisions. This trap can readily be applied to atom guiding, compression, and evaporative cooling. Received: 10 July 1997 / Received in final form: 5 January 1998 / Accepted: 16 January 1998     

Alternate technique for simultaneous measurement of photoionization cross-section of isotopes by TOF mass spectrometer

New measurements of photoionization cross-sections of the lithium isotopes are reported employing a Time of Flight (TOF) mass spectrometer in conjunction with an atomic beam apparatus. Using a two-step selective photoionization and saturation technique, we have simultaneously measured the photoionization cross-section of the 2p excited state of both the isotopes Li⁶ and Li⁷ as 15±2.5 Mb and 18 ±2.5 Mb where as the corresponding number densities have been determined as N₀≈5.3×10¹⁰ atoms/cm³ and N₀≈6.2×10¹¹ atoms/cm³ respectively.     

Direct measurement of fine structure changing collisional losses in cold trapped 85Rb

Using a technique that consists in ionizing atoms out of the 5P _1/2 fragments originated in the cold collision process, we have measured the contribution of the fine structure changing collision (FS) to the total trap loss rate of cold ⁸⁵Rb. Our results show that FS contribution is responsible for about 4% of the total trap loss. This result should stimulate new theoretical discussions involving exoergic cold collisions. Received 26 October 1998 and Received in final form 2 February 1999