小缺陷铁纳米环的磁特性

用蒙特卡罗方法与快速傅里叶变换微磁学相结合的方法模拟小缺陷铁纳米环的磁化动力学.研究发现小缺陷铁纳米环的磁滞回线出现"双稳态"特征，与实验结果一致.能量研究表明：涡旋态出现的区间为能量局域极小区间.缺陷系统的剩磁随着缺陷位置的变化而变化：剩磁随着Y值的增加先增大后减小，并在中间区域保持相对稳定.系统的自旋组态可以解释上述现象.     

Y_(1-x)Gd_xCrO_3(x=0～0.3)的负磁化和磁化反转行为研究（英文）

用固相反应法制备了Y1-xGdxCrO3和YCrO3多晶样品,并对样品的磁特性进行了研究.100Oe的场冷和零场冷热磁曲线均出现了负磁化及磁化反转行为.这一行为来自于Gd3+和Cr3+的反铁磁相互作用且可以用Gd3+的顺磁效应来解释.随着冷却场的增大,场冷负磁化行为逐渐被抑制,当冷却场与拟合所得的内场大小一致时,负磁化行为消失.也就是说,当外场小于内场时,负磁化行为将会出现,反之则消失.     

各向同性纳米结构Fe-Pt薄膜的结构和磁性

采用直流溅射和热处理技术制备了两个各向同性的纳米结构Fe-Pt永磁合金薄膜系列,并研究了它们的结构和磁性.研究表明,在富Fe双相纳米结构Fe-Pt永磁合金薄膜中,仅由硬磁的FePt相与软磁的Fe₃Pt相组成;在同一系列中,随Fe层厚度的增加,饱和磁极化强度和剩磁明显增大.由Kelly-Henkel图研究指出,在上述Fe-Pt纳米结构永磁合金薄膜中,磁相互作用主要由近邻纳米晶粒间的铁磁交换相互作用控制. 关键词： 磁性薄膜 纳米结构 矫顽力     

纳米复合永磁材料中软磁性相交换硬化的研究

本文就纳米复合永磁材料中软磁相被交换硬化问题,从一维模型和三维模拟计算进行了分析研究. 一维和三维各向异性样品研究表明,在相同微结构下,当硬磁相的各向异性降低时,除矫顽力降低外,在磁矩全部反转之前退磁曲线是一样的. 因此,硬磁相各向异性的降低不会导致最大磁能积(BH)_max增大和剩磁增加. 对于三维各向同性样品的模拟计算表明,降低硬磁相的各向异性会使剩磁和(BH)_max都明显降低. 因此,增强硬磁相的各向异性并增大硬磁相晶粒尺寸是提高 关键词： 纳米复合永磁 矫顽力 剩磁 磁能积     

分子束外延生长Fe/Fe_(50)Mn_(50)双层膜的交换偏置

利用表面磁光克尔效应和铁磁共振对分子束外延生长的Fe/Fe50Mn50双层膜的交换偏置场和矫顽力进行了研究,实验结果表明,当反铁磁层厚度小于5.5!nm时,不出现交换偏置,而当大于这一厚度时,出现交换偏置;大约在7!nm时,达到极大值.随着反铁磁层厚度的继续增大,偏置场和矫顽力随Fe50Mn50膜厚的增大而下降.铁磁共振实验结果表明样品的磁性存在单向各向异性.并对上述结果进行了讨论.     

Au诱导形成有序Si纳米孔阵列及其应用

以自组装聚苯乙烯小球(PS)单层膜为掩膜,利用Au对Si表面的催化氧化作用以及KOH溶液对单晶Si的各向异性腐蚀特性,在Si(100)面上制备了一系列尺寸小于100 nm有序可控的Si纳米孔阵列.扫描电镜(SEM)和原子力显微镜(AFM)等的测试结果显示:当PS小球溶液与甲醇溶液的体积比为9:11时,可形成大面积无缺陷的单层膜;但当体积比过大时,会导致类似双层膜结构的形成;而当体积比过小时,会诱导形成点缺陷和线缺陷.对PS小球及溅射Au处理过的Si晶片进行KOH溶液腐蚀,随着腐蚀时间变长,纳米孔的横向尺寸和深度增大,其形貌由圆形逐渐变为倒金字塔型,当腐蚀时间超过10 min,纳米孔阵列的有序性遭到破坏.采用离子束溅射技术在倒金字塔型纳米孔衬底上获得了有序Ge/Si纳米岛,而在圆形纳米孔衬底上获得了有序Ge/Si纳米环.进一步对有序Ge/Si纳米岛及纳米环的形成机理进行了解释.     

YBa_2Cu_3O_(7-δ)超导体磁弛豫

我们用振动样品磁强计研究了多晶和熔融织构 YBa_2Cu_3O_(7-δ)样品磁弛豫特性.发现在液氮温度77K 下,两种样品的零场冷磁化强度 M 仍随时间 t 呈对数衰减.表明 P.W.Ander-son 的经典磁通蠕动理论在该温度下适用于高 T_c 氧化物超导体.实验还给出了磁弛豫S=-((?)M)/((?)lnt)随外场的变化关系.对于多晶样品,当外场 B>B~*(穿透场),S 正比于 B~(-α),文中对这一关系进行了解释.     

磁场中手性碳纳米环的类超导效应

利用导出的任意手性碳纳米环（TCNTs）的电子状态－能量关系式,对磁场中任意手性TCNTs所具有的类似超导环的性质及持续电流的手性效应进行理论探讨。在T＝0K时,金属型和半导体型TCNTs象介观一维正常金属环一样具有类似超导环的性质、即持续电流以磁通量子φ0为周期随φ线性变化,且对手性角θ、环半径R极为敏感。手性TCNTs类似超导环的性质比高对称TCNTs明显得多,但随R增大而减弱,且减弱的快慢也与手性角θ有关。     

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研究了电漂移对通行高能离子与新经典撕裂模(NTM)共振相互作用的影响。利用漂移动力论方法,在求解共振相互作用产生的作用在磁岛上的环向力矩的过程中重新考虑了电漂移的作用。结果表明,在与磁岛运动相关的环向动量平衡中v>0的通行高能离子与v<0的通行高能离子作用恰好相反,当磁岛沿电子抗磁漂移方向传播时,前者趋向于使磁岛传播频率减小,后者趋向于使磁岛传播频率增大,通行高能离子产生的总的环向力矩几乎为零。仅将v>0的通行高能离子所产生的环向力矩带入由环向动量平衡方程和修正的卢瑟福方程所组成的方程组中,数值计算结果表明,描述磁岛旋转频率与宽度随时间做非线性振荡的稳定极限环并不存在。     

界面原子扩散对SmCo/Fe交换弹簧双层膜磁性能影响的微磁学研究

本文通过三维微磁学数值模拟,研究了界面处原子扩散形成的界面层对易轴平行和垂直膜面取向SmCo/Fe双层膜磁性能的影响.当易轴取向平行膜面时,体系成核在第二象限.随着界面层厚度的增加,尽管剩磁逐渐减小,而成核场和钉扎场逐渐增加,以致最大磁能积先增加后减小,直至体系由交换弹簧磁体过渡到刚性磁体.当易轴取向垂直膜面时,随着界面层厚度的增加,体系成核由第一象限逐渐过渡到第二象限,虽然钉扎场从减小、不变到略有增加,但成核场和剩磁逐渐增加,导致最大磁能积逐渐增加.在退磁过程中,膜面内自旋偏转:易轴平行膜面取向系统显示了 flower态和C态的产生与消失的过程;而易轴垂直膜面取向系统显示了vortex态的产生与消失的过程.随着易轴平行膜面SmCo/Fe双层膜界面层中SmCo原子扩散比例的增加,成核场和钉扎场增加但剩磁减小,最大磁能积先增加后降低.当易轴两种取向时,对任一界面层厚度,成核场随界面交换耦合常数的增大而增大,这表明界面层的存在增强了硬磁/软磁层之间的交换耦合作用.本文建立的模型很好地模拟了相关的实验结果[2007 Appl. Phys. Lett. 91 072509].     

The role of dipolar interactions for the magnetic properties of ferromagnetic nanoring

We investigate numerically the effects of the dipolar interactions on magnetic properties in small ferromagnetic nanorings using a Monte Carlo technique. Our simulated results show that the strength of dipolar interaction in the magnetic nanoring has an important influence on the magnetization reversal processes and further the coercivity and the remanence. As the dipolar interaction increases, the transition of magnetization reversal processes from the onion-rotation state to the vortex state can occur, which results in an increase in coercivity and a decrease in remanence. On the other hand, it is found that the coercivity and the remanence depend more strongly on the strength of dipolar coupling for the relatively small size nanoring than for the large size nanoring in width. This can be attributed to the stable vortex state without core in smaller width nanoring in contrast to the metastable vortex state with core in larger width nanoring, induced by strong dipolar interactions. Additionally, the temperature dependence of coercivity and remanence in magnetic nanoring is also studied at a fixed dipolar interaction.     

Spin configurations in nanostructured magnetic rings: From DC transport to GHz spectroscopy

We report three different experiments performed on permalloy nanorings. They address either (a) the stray-field and (b) the magnetoresistance characteristics of an individual nanoring, or (c) the magnetization dynamics of a periodic array of identical rings. Interestingly, in all three properties covering the frequency range from DC to 20 GHz we observe irreversible switching and hysteretic behavior. Localized spin waves, which are excited by ferromagnetic resonance in different ring segments, are found to obey an intriguing magnetic field dispersion. We attribute this to the characteristic spin configurations in the nanorings, i.e., the onion and the vortex states, which are controlled by the external magnetic field.     

Electronic structure and magnetism of Fe-doped SiC nanotubes

The electronic structure and magnetic properties of Fe-doped SiC nanotubes are investigated by using the first-principles method based on density functional theory(DFT) in the local spin density approximation(LSDA).The calculation results indicate that the SiC nanotube of Fe substitution for C exhibits antiferromagnetism while ferromagnetism features prominently when Fe substitutes Si.This is a kind of half-metal magnetic material.The formation energy calculation results show that the formation energy of ferromagnetic structure is 3.2 eV lower than that of antiferromagnetic structure.Fe atoms are more likely to replace Si atoms.Spin-orbit coupling induces electron spin polarization in the ground state.Also,the doping Fe atoms make relaxation towards the outside of the tube to some extent and larger geometric distortion occurs when Fe substitutes C,but the whole geometric structure of SiC nanotubes is not damaged due to the doping.It is revealed in the calculation of energy band structure and density of states that more dispersed distribution of energy levels is produced near the Fermi level.For Fe substitution for Si,obviously there are spin-split and intense p-d hybrid effects by Si 3p electron spins and Fe 3d electron spins localized at the exchanging interactions between magnetic transitional metal(TM) impurities.Spin electronic density results indicate that system magnetic moments are mainly generated by the unpaired 3d electrons of Fe atoms.All these results show that the transition metal doping SiC nanotube could be a potential route to fabricating the promising magnetic materials.     

Magnetic properties for cobalt nanorings: Monte Carlo simulation

In this paper, two structure models of cobalt nanoring cells (double-nanorings and four-nanorings, named as D-rings and F-rings, respectively) have been considered. Base on Monte Carlo simulation, the magnetic properties of the D-rings and F-rings, such as hysteresis loops, spin configuration, coercivity, etc., have been studied. The simulated results indicate that both D-rings and F-rings with different inner radius (r) and separation of ring centers (d) display interesting magnetization behavior and spin configurations (onion-, vortex- and crescent shape vortex-type states) in magnetization process. Moreover, it is found that the overlap between the nearest single nanorings connect can result in the deviation of the vortex-type states in the connected regions. Therefore, the appropriate d should be well considered in the design of nanoring device. The simulated results can be explained by the competition between exchange energy and dipolar energy in Co nanorings system. Furthermore, it is found that the simulated temperature dependence of the coercivity for the D-rings with different d can be well described by H_c=H₀ exp[−(T/T₀)^p].     

Tunable dipolar magnetism in high-spin molecular clusters

We report on the Fe17 high-spin molecular cluster and show that this system is an exemplification of nanostructured dipolar magnetism. Each Fe17 molecule, with spin S=35/2 and axial anisotropy as small as D approximately -0.02 K, is the magnetic unit that can be chemically arranged in different packing crystals while preserving both the spin ground state and anisotropy. For every configuration, molecular spins are correlated only by dipolar interactions. The ensuing interplay between dipolar energy and anisotropy gives rise to macroscopic behaviors ranging from superparamagnetism to long-range magnetic order at temperatures below 1 K.     

Nonlinear light propagation in the defect band of one-dimensional defective structures

In this paper we numerically investigate the nonlinear propagation of defect state in one-dimensional structures with defects. We investigate the nonlinear transmission spectra and the bistable response for defective structures with different index gradients. The results show that positive Kerr nonlinearity can suppress the Wannier-Stark localization. And the nonlinear response of defect states band exhibits an optical switch behavior, which may be applied to all-optical devices. And the gap solitons from these defect states are presented.     

Vibration analysis of nanorings using nonlocal continuum mechanics and shear deformable ring theory

In this article, we use shear deformable ring theory (SDRT) for the analysis of free in-plane vibration of nanorings based on nonlocal elasticity theory. The equations of motion of the nanoring are derived for the aforementioned problem by considering the small scale effect. Analytical solutions for the natural frequencies of the nanorings are presented. It is shown that the nonlocal effects play an important role in the vibration of nanorings and cannot be neglected. The effects of the small scale on the natural frequencies considering various parameters such as the radius of the nanoring, the thickness of the nanoring and mode numbers are investigated.     

并苯纳米环[6]CA及其衍生物的电子结构和光物理性质的密度泛函理论研究

采用密度泛函理论PBE0方法在6-31G(d, p) 基组水平上对比研究并六苯纳米环[6]CA及BN取代纳米环[6]CA-BN的几何结构及电子性质. 同时探讨锂离子掺杂对不同体系的芳香性、前线分子轨道、电子吸收光谱及传输性质的影响. 通过电离势、亲合势及重组能的计算, 预测纳米环体系得失电子的能力及传输性能. 结果表明:[6]CA的能隙很小, BN取代后, 能隙明显增大; 锂离子掺杂到两种纳米环中, 在不明显改变前线分子轨道分布的前提下, 几乎同步降低了最高占据轨道、 最低未占据轨道能级, 锂离子掺杂使载流子传输性能得到很大改善; 电子吸收光谱拟合发现, BN取代使吸收光谱很大程度蓝移, 吸收强度明显减小; 而锂离子掺杂对光谱的强度及吸收范围没有明显影响. 关键词： 碳纳米环 硼氮纳米环 锂离子掺杂 密度泛函理论     

Micromagnetic simulations of 200-nm-diameter cobalt nanorings using a Reuleaux triangular geometry

Using micromagnetic simulations, we investigated the magnetic states and switching processes of Co nanorings with lateral dimensions of 200 nm. We propose a special geometry of nanorings that adopts different Reuleaux triangular shapes. Reuleaux's triangles (RT) combine both the equilateral triangle and circular geometries. We studied the magnetic spin configurations of individual nanorings by varying the thickness and geometry of the nanomagnets. Our results demonstrated that in most nanomagnets exhibiting a thickness of less than 4 nm, there exists an onion-type state, which precedes either a twisted, double twisted, or cardioid state, when studying the magnetization reversal process. The hysteresis loops and magnetic states found in these RTs are compared with circular nanorings.