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1.
相比单粒子阵列,金属纳米颗粒的二聚体阵列的共振效应受更多因素的影响,包括阵列的组成方式、二聚体的结构和朝向、粒子的形状、大小等,因此具有更好的可调性.本文基于修正长波近似法,通过引入两种粒子之间的阵列因子矩阵,修正了两种粒子的极化率,从而得到了二聚体阵列的消光截面的解析公式.在此基础上,讨论了整个阵列在不同偏振光激发下的共振的调制和偏振特性.  相似文献   

2.
郭艳芳  孔凡敏  李康 《光学技术》2012,38(3):317-322
采用离散偶极子近似(DDA)方法,研究了单体银纳米粒子和银纳米粒子阵列的光谱特性。研究结果发现,单体银纳米粒子的表面等离子体共振消光峰的位置随着周围介质折射率和粒子尺寸的增大逐渐红移,并且消光光谱的峰宽也越来越大。当银纳米粒子正方阵列的周期接近单体的共振波长时,阵列的消光光谱中会出现尖锐的共振峰,改变粒子尺寸的大小可以发现消光光谱中共振峰的峰值和位置有大幅度地改变,通过改变阵列在平行和垂直于入射光偏振方向上的周期,可以调节二维长方阵列共振峰的峰宽和峰位。该研究为纳米粒子在光学显微镜、生物传感元件、数据存储等领域中的应用提供有效地理论参考。  相似文献   

3.
本文利用离散点偶极子近似方法(DDA)研究了金和银纳米粒子二维周期阵列的光学性质。研究结果表明二维周期阵列的消光性质及其表面等离子共振(SPR)波长受到阵列内粒子组成材料、粒子形状尺寸、阵列周期和阵列排布方式等因素的影响。对于二维正方阵列,当周期较小时(一般小于300 nm),阵列的共振波长主要取决于粒子组成材料和形状尺寸;当周期与阵列单体的共振波长附近时,阵列的消光谱中会出现极窄且锐的SPR共振峰,峰位只与阵列的周期值相关。改变阵列在平行和垂直于入射光偏振方向的周期,可以方便地调节二维长方阵列的共振峰的峰位和峰宽。  相似文献   

4.
采用静电近似理论计算了Ag纳米棒阵列在不同偏振光入射下的消光光谱。当入射光偏振方向平行于纳米棒长轴时会激发表面等离激元纵向振动模式,而当入射光偏振方向垂直于纳米棒长轴时会激发表面等离激元横向振动模式。基于两种模式共振波长的不同,采用Ag纳米棒阵列可以用来设计高性能的表面等离激元微型偏振器。Ag纳米棒阵列的偏振性能在纵向共振波长明显优于在横向共振波长,通过调节纳米棒的纵横比可以对纵向模式的共振峰位进行大范围调控。结果表明这种微型偏振器所适用的波长能够通过纳米棒的纵横比在可见到近红外波段范围内调控,而消光比和插入损耗能够通过纳米棒的直径和长度实现调控。  相似文献   

5.
纳米颗粒及其阵列结构的光学性能与颗粒本身的表面等离子体共振及周期结构参数密切相关.本文根据Mie散射理论和多极子振荡理论,研究了光在银球型纳米颗粒及阵列中的传输性质.对于单个纳米颗粒,当颗粒半径小于50 nm时,消光峰由电偶极子共振产生;当半径大于50 nm时,除电偶极子振荡产生的消光峰外,在短波处将出现由电四极子共振产生的消光峰,且两种极子的共振频率随颗粒半径的增加而减小.由电偶极子共振产生的消光峰位置的理论计算结果与实验结果相符合.对于由球形颗粒组成的无限大二维周期阵列,消光峰主要由单个颗粒产生的消光峰和Wood-Rayleigh反常衍射造成的消光峰组成.通过控制纳米颗粒的尺寸、形状以及阵列的周期、排列方式,可以调节两种极子的共振峰位.本文的结果将对设计具有特定光学性能的纳米结构产生重要的实际意义.  相似文献   

6.
用Mie散射理论计算大气气溶胶光学特性   总被引:17,自引:5,他引:12  
本文在已知厦门海域气溶胶粒子谱分布的基础上,用MIE散射理论计算了该地区气溶胶粒子的光学特性,得到了气溶胶粒子的散射截面、吸收截面、消光截面与波长的关系,散射相函数以及偏振相函数,并用实验对两个相函数加以了验证。此结论为研究大气矢量辐射传输提供了很好的方法;尤其偏振相函数的提出为今后用偏振的方法研究大气提供了理论依据。  相似文献   

7.
金属纳米颗粒阵列中形成的四偶极晶格共振模式具有低辐射损耗、高品质因子的特性,因此广泛应用于纳米激光、传感、固态照明等领域.基于时域有限差分法在均匀环境下研究了银纳米圆柱阵列的光谱与近场特性.研究结果表明,在x偏振光直入射下,通过调节阵列x方向的周期,共振强度先增加后降低,当两个方向上的周期相等时,提出的阵列结构能够产生一个线宽约0.4 nm、品质因子高达1815的四偶极晶格共振模式,这种共振模式呈现出Fano线型的透射谷;调控y方向的周期能够实现从Fano线型的透射峰到透射谷的转变.本文说明了粒子大小、晶格周期对四偶极晶格共振模式的重要性,同时为银纳米颗粒在可见光波段设计高品质因子共振提供了优化策略.  相似文献   

8.
徐天宁  李翔  贾文旺  隋成华  吴惠桢 《物理学报》2015,64(24):245201-245201
五边形截面的单晶Ag纳米线对ZnO量子点荧光具有增强的现象. 为解释这一现象, 利用时域有限差分法对五边形截面的Ag纳米线的局域表面等离子体共振模式进行了理论模拟. 结果表明, 五边形截面的Ag纳米线在紫外区域存在两个消光峰, 分别由Ag纳米线的横向偶极共振(340 nm)和四极共振(375 nm)引起; 这两个消光峰与ZnO量子点荧光增强峰相一致, 而且随着Ag纳米线的半径增大而红移; 消光峰对应的共振模式取决于Ag纳米线的截面形状; 根据Ag纳米线电场增强倍数与激发光波长变化关系曲线可知, 最大增强电场位于五边形截面的顶点处, 而边线处电场增强较小. 理论模拟的结果较好地解释了Ag纳米线/ZnO量子点体系的荧光增强现象, 也为Ag纳米线在提高半导体材料发光效率、生物探测等方面的应用提供有益的参考.  相似文献   

9.
本文导出了e+e对撞实验中产生的共振态的辐射修正截面的近似解析公式.对于Z0粒子和J/ψ,Υ家族的粒子,在确定这些共振态参数的实验扫描能量范围内,该解析近似的精度达到0.1%量级.利用解析近似公式与对撞束能量分辨函数的卷积拟合实验观测到的共振截面数据,可得到比当前普遍采用的Jackson,Scharre方法更准确的共振参数值.  相似文献   

10.
孟田华  赵国忠 《光子学报》2013,(9):1061-1064
利用太赫兹时域光谱系统,测量了3种在硅衬底上淀积厚度为100nm金膜的椭圆环阵列结构后,并且分析了各样品在太赫兹波段的透射增强现象及产生机理.结果表明:在整个太赫兹波段,此组结构样品的透射系数均在0.68以上,产生明显的透射增强;当太赫兹波的偏振方向与椭圆环长轴之间的夹角为90°时,3个样品在1.67THz处的共振峰是由于短轴方向的电子形成偶极子振荡与入射太赫兹波进行耦合产生的;夹角为0°时,周期阵列样品无明显共振峰,而分形阵列样品的共振峰则不如斑图阵列样品的明显;样品结构的对称性越差,透射谱的信息越丰富.此外,分析相位差谱也验证了共振增强透射的存在.  相似文献   

11.
The energy extinction cross section of a concentrically layered sphere varies with velocity as the Doppler shift moves the spectral content of the incident signal in the sphere's co-moving inertial reference frame toward or away from resonances of the sphere. Computations for hollow gold nanospheres show that the energy extinction cross section is high when the Doppler shift moves the incident signal's spectral content in the co-moving frame near the wavelength of the sphere's localized surface plasmon resonance. The energy extinction cross section of a three-layer sphere consisting of an olivine-silicate core surrounded by a porous and a magnetite layer, which is used to explain extinction caused by interstellar dust, also depends strongly on velocity. For this sphere, computations show that the energy extinction cross section is high when the Doppler shift moves the spectral content of the incident signal near either of olivine-silicate's two localized surface phonon resonances at 9.7 μm and 18 μm.  相似文献   

12.
A completely relativistic mechanism for describing polarization bremsstrahlung caused by an elastic collision of a charged particle with a many-electron target was suggested. Multipole expansions for the amplitude and cross section of the process taking into account radiation lag effects were obtained. Including higher order multipoles was shown to result in substantial asymmetry of the angular distribution of emitted photons compared with the dipole case and in a noticeable change in the spectral characteristics of polarization radiation. The cross section of polarization bremsstrahlung was found to increase logarithmically as the energy of incident particles grew.  相似文献   

13.
A theoretical analysis of electromagnetic forces on neutral particles in a hollow waveguide is presented. We show that the effective scattering cross section of a very small (Rayleigh) particle can be strongly modified inside a waveguide. The coupling of the scattered dipolar field with the waveguide modes induces a resonant enhanced backscattering state of the scatterer-guide system close to the onset of new modes. The particle effective cross section can then be as large as the wavelength even far from any transition resonance. As we will show, a small particle can be strongly accelerated along the guide axis while being highly confined in a narrow zone of the cross section of the guide.  相似文献   

14.
随机取向烟尘团簇粒子的光学截面的数值计算   总被引:2,自引:2,他引:0  
采用蒙特卡罗方法根据团簇—团簇凝聚(CCA)模型对由球形原始微粒凝聚而成的烟尘团簇粒子进行了模拟,利用离散偶极子近似(DDA)方法数值计算了不同原始微粒粒径和数目组成的随机取向的烟尘团簇粒子的总消光截面、吸收截面及散射截面等光学特性参数,研究了原始微粒粒径及数目对随机取向烟尘团簇粒子光学特性的影响。结果表明:当入射波长一定时,随机取向烟尘団簇粒子的光学特性主要取决于原始微粒的粒径和数目;烟尘团簇粒子对不同波段激光的吸收和散射存在差别,这种差别随原始微粒粒径及数目变化而变化。这一工作为研究电磁波在烟尘中的传输特性提供重要参考数据。  相似文献   

15.
The metallic films perforated with a periodic array of air holes show extraordinary optical transmission properties. In this paper the influence of the incident light's polarization direction and the arrays’ period on the transmission through the rectangular hole arrays immersed in a metallic film is studied by utilizing the finite-difference time-domain method. The results show that the intensities and number of the transmission peaks can be adjusted by changing the incident light's polarization direction, while the intensities can keep constant for some particular frequencies. The transmission peak's wavelength can be easily controlled by altering the lattice period parallel to the electric field for the rectangular holes. These results maybe provide reference for the design of multiple-wavelength resonance devices.  相似文献   

16.
The extinction, integrated scattering, and absorption spectra of gold and silver nanorods with random and regular orientation are studied. The calculations are performed for spheroids, circular cylinders, circular cylinders with hemispherical ends (T-matrix method), and rectangular prisms (discrete dipole approximation). A new quadrupole resonance is discovered that arises between the usual plasmon dipole resonances excited by a field longitudinal or transverse with respect to the symmetry axis. The new resonance can be excited only by a TM incident wave and is the greatest for orientation of the symmetry axis of the particle at an angle of 54° with respect to the light beam.  相似文献   

17.
This work presents a new explanation for the extinction paradox and shows that the canonical explanations are incorrect. This paradox refers to the large size limit of a particle's extinction cross section. It is called a paradox because the geometrical optics approximation, which should be valid in this limit, predicts a cross section that is half of the true value. The new explanation is achieved by formulating the scattered wave in terms of an integral over the particle's surface where the seemingly unrelated Ewald-Oseen theorem appears in the formulation. By expressing the cross section in terms of this surface integral, the Ewald-Oseen theorem is analytically connected to the cross section. Several illustrations are used to reveal the significance of this connection: The paradox is seen to be a consequence of the requirement that the incident wave be canceled within the particle by secondary radiation from its own internal field. Following this, the canonical explanations are examined to reveal serious problems. In the process, the same asymptotic extinction behavior is shown to occur for small highly refractive dielectric particles, and thus is not just a large particle size or small wavelength effect as is often stated. The traditional explanations cannot account for this behavior while the new one actually predicts it. All in all, this work constitutes a fundamental reworking of 60 years of accepted understanding for the cause of the asymptotic behavior of the extinction cross section.  相似文献   

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