Theory of the synchronously pumped picosecond dye laser

The circulation of a synchronously mode locked dye laser pulse in a linear cavity configuration containing a dye cell as an active medium and a bandwidth-limiting element is treated. The condition that the pulse shape reproduces after each cavity round-trip provides a nonlinear integro-differential equation for the steady-state pulse shape. For the solution of this equation an approximate method, not limited to small pulse energies, is given and the pulse duration, intensity, energy, asymmetry of the pulse shape, stable regions and other interesting parameters are discussed.     

Temporal dynamics of high repetition rate pulsed single longitudinal mode dye laser

Theoretical and experimental studies of temporal dynamics of grazing incidence grating (GIG) cavity, single-mode dye laser pumped by high repetition rate copper vapour laser (CVL) are presented. Spectral chirp of the dye laser as they evolve in the cavity due to transient phase dynamics of the amplifier gain medium is studied. Effect of grating efficiency, focal spot size, pump power and other cavity parameters on the temporal behaviour of narrow band dye laser such as build-up time, pulse shape and pulse width is studied using the four level dye laser rate equation and photon evolution equation. These results are compared with experimental observations of GIG single-mode dye laser cavity. The effect of pulse stretching of CVL pump pulse on the temporal dynamics of the dye laser is studied.     

Pulse structure studies and absolute cavity length determination for a synchronously pumped picosecond dye laser

Second harmonic cross correlation functions of a pulse with its near neighbor have been studied in a synchronously pumped cw dye laser. Measurements were made both as a function of dye laser cavity length mismatch and the number of cavity round trips separating the correlated pulses. The pulse envelope is found to have a characteristic interpulse frequency determined by the pump laser, whereas the pulse substructure has a characteristic frequency determined by the dye laser cavity length. The cross correlation measurements allow experimental determination of the dye laser length corresponding to exact synchrony. In contrast to theoretical predictions the length of exact synchrony corresponds to optimum pulse shape and duration. Our results are discussed in terms of a simple model which leads to pulse duration estimates as much as twice those obtained by conventional analysis of autocorrelation traces.     

同步泵浦飞秒激光锁模理论研究

考虑到饱和增益、饱和吸收、群速弥散和自相位调制等效应对光脉冲的作用,我们给出了一个适用于飞秒脉冲激光系统的锁模方程。并且用这个方程初步地研究了同步泵浦被动锁模的染料激光器。结果表明,染料光脉冲的输出特性将极大地取决于腔内色散、S参数、饱和吸收体的浓度、腔长失谐量等因素。     

Rate equation simulation of a synchronously pumped dye laser

A simple rate equation model of a standing wave synchronously pumped dye laser yields output pulses which agree qualitatively and quantitatively with recent experimental observations. The shape, amplitude and temporal position of the simulated pulse varies dramatically, not only with cavity length detuning, but also with the gain to loss ratio. Features of pulse formation and stability are predicted which are precluded by the steady-state assumption present in most other models.     

碰撞锁模环形染料激光器动力学过程的研究

本文在建立碰撞锁模(CPM)激光器数学模型的基础上,对碰撞锁模激光器中激光锁模脉冲形成的动力学过程进行了计算机模拟计算,并对其结果进行了理论分析和讨论,得到了脉冲宽度、脉冲波形及对称性与泵浦速率、腔长、增益介质和可饱和吸收介质在腔内的相对位置等因素间的关系。     

相位对同步泵浦锁模染料激光系统参数的影响

本文讨论了同步泵浦锁模染料激光器系统输出脉冲形状的非对称性对该激光系统输出相位部分的贡献,还给出了腔内诸元件对输出相位的贡献,从而得到了激光输出脉冲的脉宽、峰值位置和振幅的解析表达式。 关键词：     

Combined AM and synchronous mode locking of CW dye laser

Theoretical analysis of an AM mode locked-synchronously pumped CW dye laser is presented. The pulsewidth and the pulse energy of the mode locked steady-state pulse are expressed as functions of system parameters. It is shown that the cavity length adjustment is not as critical as in the case of purely synchronously mode locked CW dye laser.     

A parametric study of negative feedback Nd:YAG laser

The output pulse parameters of a mode-locked Nd:YAG laser with a passive negative feedback element were studied experimentally. The pulse evolution within the train was experimentally recorded using a modified second harmonic generation autocorrelator. By comparing the laser operation with and without an acousto-optic modulator, we found that with the later there is a significant increase in the mode locking probability and the pulse acquires a temporally Gaussian symmetric pulse shape. Further with the active modulator there is a relaxation in alignment tolerances and increase in the range of permissible dye concentrations for stable mode locking. It was also observed that the pulse width of the negative feedback laser depends on the saturation intensity of the mode locking dye and reduces for a dye with higher saturation intensity. The pulse width was also found to reduce linearly as the initial transmission of the dye is reduced.     

Theory of synchronously pumped dye lasers

An analysis of cw synchronously pumped dye lasers is presented. Under the assumption that the cavity (tuning element) bandwidth is much wider than the bandwidth of the transform limited pulses generated, the pulse forming dynamics is rigorously treated. It is shown that for a finite mismatch between the lengths of the dye and the pump lasers, a steady-state pulse develops in the dye laser cavity with a conserved pulseshape. The characteristics (energy, shape, peak power, duration) of these pulses of ultimate width are quantitatively determined as a function of cavity mismatch. An analytical solution for the pulse envelope is determined, which yieldsI(t)∝Sech²(t/t _p ) to a good approximation.     

Rate equation simulation of temporal characteristics of a pulsed dye laser oscillator

A time-dependent, two-dimensional (in space) rate equation model of a transversely-pumped pulsed dye laser oscillator, which incorporates transverse pump intensity variation in the presence of intracavity dye laser radiation, is proposed to understand and predict its temporal behaviour. The model yields output pulses which agree well with experimental results using rhodamine 6G and kiton red dyes. The shape, amplitude and temporal position of the simulated pulse within the pump pulse vary dramatically across the tuning range of each dye depending on the relative gain and loss values.     

Generation of nearly transform-limited pulses in subnanosecond region with TEA nitrogen-laser-pumped dye laser

A dye laser is transversely pumped by a TEA nitrogen laser with 700 ps duration. The dye laser pulse has a spectral linewidth of 0.007 nm and a pulse width of ≈ 140 ps, giving a time-bandwidth product of 1.5. It is pointed out that the fluorescence lifetime of the laser dye plays an important role in generation of laser emission using a long laser cavity under subnanosecond pulse pumping.     

Spectrally Adjustable Picosecond Dye Laser Pulses Generated with Nanosecond Nitrogen Lasers

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Numerical calculations of intracavity dye Q-switched ruby laser

A mathematical model describing the dynamic emission of the Q-switched ruby laser has been adapted. The suggested model allows the investigation of the effects of a dye cell on the mode characteristics of the ruby laser and, moreover, the study of the effect of the laser input parameters on the output laser pulse. This model simulates the nonlinear effects of dye pulse modulation on the laser emission.In addition, a numerical solution of a nonlinear rate equation system of the adapted model is discussed. The solution estimates the density of the emitted radiation, population inversion and energy transfer processes of the ruby laser rod and dye cell for different emission regimes (one pulse regime, free running pulses, repetition periodic pulses). The estimated results of the laser output pulse characteristics are in a good agreement with the other calculated and experimental results.     

溴化亚铜激光泵浦的可调谐微微秒染料激光

本文首次报道了利用脉宽为25ns重复率为10kHz的溴化亚铜激光泵浦混有饱和吸收体DODCI的超短腔染料激光,产生出30ps光脉冲.在理论上对混入DODCI的超短腔染料激光脉冲压缩效应作了分析计算,计算结果与实验基本一致.在实验上又通过一个放大-色散系统实现对此染料激光脉冲的同步放大和调谐,并达到傅里叶变换极限.     

On noise and fluctuations in a synchronously mode-locked cw laser system

A single-shot and synchronously-scanned streak camera, autocorrelation and noise spectrum analysing techniques are utilized to study the output characteristics of synchronously mode-locked cw lasers. Four main conclusions are drawn: (i) the pulse train from a synchronously-pumped dye laser reveals, besides phase jitter, considerable pulse shape fluctuations; (ii) autocorrelation measurements may be highly misleading when actual pulse shapes are considered; (iii) both the phase jitter and pulse shape fluctuations of the dye laser output are caused by the phase fluctuations of the pumping ion laser pulse train; (iv) the phase jitter of the ion laser proceeds from the fluctuations in the cavity roundtrip time with a characteristic time of about 5 s. Under optimum conditions the rms noise of the dye laser output was 2% and the phase jitter with respect to the rf sine drive of the acousto-optical mode-locker, 30 ps. A qualitative explanation fo the noise properties is given.     

Numerical analysis of pulse generation in synchronously mode-locked cw dye lasers

We present theoretical results on the characteristics of pulses generated by a synchronously pumped dye laser. Our analysis indicates the important influence of spontaneous emission on shape and frequency chirp of the pulse. Dye-laser operation is possible within a wide range of cavity mismatch. A large mismatch of the lengths of the dye and the pump-laser cavity results in the generation of noise bursts caused by the influence of spontaneous emission. At small cavity mismatch pulse profile and frequency chirp of the pulse are directly generated in the steady-state regime by algebraic equations. Our formulas indicate that the sign of the pulse chirp depends only on the sign of the shift between laser frequency and centre frequency of the amplifying transition.     

2-NSEC pulses from double cavity dye laser

Short pulses fully adjustable between 2 and 20 nsec were obtained from a double cavity laser pumped dye laser using the same amplifying cell. The duration of the pulse (short cavity) is controlled using a lower threshold cavity with adjustable length. The spectrum of the laser emission was found to be larger in the secondary cavity of variable length. This effect is attributed to a wavelength shift during the dye laser emission due to a variation with time of the excited molecular population.     

Cavity detuning effects in the synchronously mode-locked CW dye laser

A detailed numerical model analysis of the synchronously mode-locked CW dye laser is presented. In the analysis, good mode-locking is found mainly for negative cavity detuning. The calculated cavity length detunig effects are compared with the results of experiments performed on the Oxazine-1 dye laser. The agreement between theory and experiment is satisfactory. The experimental good mode-locking regime is predicted correctly by this analysis. The present calculations are also compared with the hitherto reported qualitative model analyses with a gaussian dye pulse approximation. The validity of these model analyses is examined.     

Angularly resolved coherent Raman spectroscopy (ARCS)

This new crossed beam configuration produces an angularly separated Coherent Anti-Stokes Raman spectrum, eliminating the need for a spectrometer. Since one of the driving laser beams is always linearly opposed to the dye laser, it may also be used as a dye pump and the experiment performed within the dye cavity for efficient laser energy utilization. With this arrangement, a broad bandwidth dye laser produces a several wavenumber resolution spectrum from a small volume with relatively simple alignment. The spectrum is scanned by varying the incidence angle of the probe beam or taken is a single pulse using a fan shaped probe beam.