Selective excitation,coherent control,and attosecond spectrochronography of electron subshells in atomic systems

Optical field waveforms with an ultrabroad spectrum and a tailored phase are shown to enable selective excitation, coherent control, and attosecond spectrochronography of electron subshells in many-electron atomic systems. Analysis of the evolution of the density matrix of electron subshells in an atomic system driven by an ultrashort light pulse shows that the interference of different quantum pathways of electron dynamics plays a key role in the buildup of the nonlinear-optical response of such a system. Our analysis suggests a method whereby the attosecond dynamics of individual electron subshells in atoms can be coherently controlled with ultrashort laser pulses.     

Temporal coherent control of superfluorescent pulses

We demonstrate that collective atomic interferences can be investigated by measuring the superfluorescence (SF) time delay. A pair of broadband (≈20 nm), ultrashort (≈80 fs), collinear pulses with a variable delay coherently excites rubidium (Rb) atoms. The generated superfluorescent pulses at 420 nm on the cascade transition are recorded by a picosecond streak camera. Both intensity and SF time delay of the 420 nm pulse are altered as the delay between input pulses varies. In particular, the SF time delay of the normalized 420 nm pulse exhibits oscillations with different periods. This can be understood in terms of atomic and quantum interferences due to two possible two-photon excitation pathways through the intermediate levels (Rb D-lines).     

Manipulating light pulses via dynamically controlled photonic band gap

When a resonance associated with electromagnetically induced transparency in an atomic ensemble is modulated by an off-resonant standing light wave, a band of frequencies can appear for which light propagation is forbidden. We show that dynamic control of such a band gap can be used to coherently convert a propagating light pulse into a stationary excitation with nonvanishing photonic component. This can be accomplished with high efficiency and negligible noise even at the level of few-photon quantum fields thereby facilitating possible applications in quantum nonlinear optics and quantum information.     

Deterministic and storable single-photon source based on a quantum memory

A single-photon source is realized with a cold atomic ensemble (87Rb atoms). A single excitation, written in an atomic quantum memory by Raman scattering of a laser pulse, is retrieved deterministically as a single photon at a predetermined time. It is shown that the production rate of single photons can be enhanced considerably by a feedback circuit while the single-photon quality is conserved. Such a single-photon source is well suited for future large-scale realization of quantum communication and linear optical quantum computation.     

Test of the all-optical control of wave-particle duality of cavity photons by ordinary photodetection

The principle of complementarity refers to the ability of quantum entities to behave as particles or waves under different experimental conditions. We present a proposal for the experimental observation of the ultrafast all-optical control of the wave-particle duality of light. The device is constituted by a three-level quantum emitter strongly coupled to a microcavity (MC) and can be realized by exploiting a great variety of systems, ranging from atomic physics and semiconductor quantum dots to intersubband polaritons and Cooper pair boxes. The wavelike or particlelike behavior of MC photons can be probed by simply measuring the cavity output photon rate after excitation with pairs of phase-locked weak pulses with precise arrival times.     

Coherent control of stationary light pulses

We present a detailed analysis of the recently demonstrated technique to generate quasi-stationary pulses of light [M. Bajcsy, A.S. Zibrov, M.D. Lukin, Nature (London) 426 (2003) 638] based on electromagnetically induced transparency. We show that the use of counter-propagating control fields to retrieve a light pulse, previously stored in a collective atomic Raman excitation, leads to quasi-stationary light field that undergoes a slow diffusive spread. The underlying physics of this process is identified as pulse matching of probe and control fields. We then show that spatially modulated control-field amplitudes allow us to coherently manipulate and compress the spatial shape of the stationary light pulse. These techniques can provide valuable tools for quantum nonlinear optics and quantum information processing.     

Population transfer between two quantum states by piecewise chirping of femtosecond pulses: theory and experiment

We propose and experimentally demonstrate the method of population transfer by piecewise adiabatic passage between two quantum states. Coherent excitation of a two-level system with a train of ultrashort laser pulses is shown to reproduce the effect of an adiabatic passage, conventionally achieved with a single frequency-chirped pulse. By properly adjusting the amplitudes and phases of the pulses in the excitation pulse train, we achieve complete and robust population transfer to the target state. The piecewise nature of the process suggests a possibility for the selective population transfer in complex quantum systems.     

Quantum-control spectroscopy with exact state selectivity

A method of exact state-selective spectroscopy is introduced, based on quantum control through four specific short laser pulses. The exact conditions for the two pairs of ultrafast pulses are set by the feedback control for selective excitation to one specific resonance state while the other state is destructively interfered as the shadow pair, leading to a state-selective spectrum.     

A quantum computer in the scheme of an atomic quantum transistor with logical encoding of qubits

A scheme of a multiqubit quantum computer on atomic ensembles using a quantum transistor implementing two qubit gates is proposed. We demonstrate how multiatomic ensembles permit one to work with a large number of qubits that are represented in a logical encoding in which each qubit is recorded on a superposition of single-particle states of two atomic ensembles. The access to qubits is implemented by appropriate phasing of quantum states of each of atomic ensembles. An atomic quantum transistor is proposed for use when executing two qubit operations. The quantum transistor effect appears when an excitation quantum is exchanged between two multiatomic ensembles located in two closely positioned QED cavities connected with each other by a gate atom. The dynamics of quantum transfer between atomic ensembles can be different depending on one of two states of the gate atom. Using the possibilities of control for of state of the gate atom, we show the possibility of quantum control for the state of atomic ensembles and, based on this, implementation of basic single and two qubit gates. Possible implementation schemes for a quantum computer on an atomic quantum transistor and their advantages in practical implementation are discussed.     

Optimum conditions for superradiant damping

The conditions are investigated under which cooperative or superradiant effects are greatest in an inhomogeneously broadened atomic system that is excited by a coherent light pulse. The coupled non-linear atomic equations of motion are solved numerically for excitation pulses of various areas. It is shown that the absolute intensity of the response decreases strongly with decreasing pulse are below π, but that the relative superradiant contribution increases with decreasing pulse area. The reasons for this are discussed, and it is suggested that excitation by a pulse in the neighborhood of π/2 may represent an optimum compromise for the observation of superradiance.