克尔介质中脉冲宽度对瞬态热光非线性效应的影响

在纳秒时域，研究了激光脉冲宽度变化对克尔介质中瞬态热光非 线性效应的影响.通过不同脉冲宽度τp下得到的二硫化碳 苯胺黑溶液的Z_scan实验结果，对瞬态热光非线性效应和光克尔效应的共存过程进行了分析 .随着脉冲宽度的增加，观察到了热光非线性效应从瞬态到稳态变化过程和Z_scan峰谷特性 的转变.同时，从声波的传播方程和光波的非线性传播方程出发，用数值计算方法模拟了这 一非线性过程，结果表明数值模拟结果和实验结果是相符的. 关键词： 瞬态热光非线性效应 脉冲宽度 Z_scan 克尔效应     

克尔介质中瞬态热光非线性效应的作用

研究了介质中瞬态热光非线性效应对于克尔效应Z扫描测量结果的影响，观察到了Z扫描峰谷特性的转变，相应的数值模拟结果与实验结果很好地吻合.实验也发现，克尔效应和瞬态热光非线性效应相互抵消时Z扫描曲线呈现出新奇的单峰或平台状曲线.对于用纳秒脉冲激光进行的Z扫描测量结果的正确分析具有重要意义. 关键词： 瞬态热光非线性效应 克尔效应 Z扫描     

相位物体Z-扫描研究金属簇合物[Tp*W(μ3-S)3Cu3Py3(μ3-Br)](PF6)/DMF溶液的瞬态热致非线性折射

在纳秒时域,采用相位物体(PO)Z-扫描技术研究了一种新型金属簇合物溶液的瞬态热致非线性效应.该方法的最大优点是很容易区分瞬态热致非线性折射和三阶非线性折射.本文利用PO Z-扫描和传统Z-扫描研究了在8 ns脉宽、不同能量激光脉冲作用下[Tp*W(μ3-S)3Cu3Py3(μ3-Br)](PF6)/DMF溶液的光学非线性.从声波方程和热传导方程出发,对实验结果进行了理论分析和数值模拟,理论值和实验结果很好的吻合.研究结果表明,样品溶液的非线性折射主要来源于瞬态热致非线性效应.     

相位物体$lt;i$gt;Z$lt;/i$gt;-扫描研究金属簇合物［$lt;i$gt;Tp$lt;/i$gt;*W($lt;i$gt;μ$lt;/i$gt;$lt;sub$gt;3$lt;/sub$gt;-S)$lt;sub$gt;3$lt;/sub$gt;Cu$lt;sub$gt;3$lt;/sub$gt;$lt;i$gt;Py$lt;/i$gt;$lt;sub$gt;3$lt;/sub$gt;($lt;i$gt;μ$lt;/i$gt;$lt;sub$gt;3$lt;/sub$gt;-Br)］($lt;i$gt;PF$lt;/i$gt;$lt;sub$gt;6$lt;/sub$gt;)/DMF溶液的瞬态热致非线性折射

在纳秒时域,采用相位物体（PO）Z-扫描技术研究了一种新型金属簇合物溶液的瞬态热致非线性效应.该方法的最大优点是很容易区分瞬态热致非线性折射和三阶非线性折射.本文利用PO Z-扫描和传统Z-扫描研究了在8 ns脉宽、不同能量激光脉冲作用下［Tp*W（μ₃-S）₃Cu₃Py₃（μ₃-Br）］（PF₆）/DMF溶液的光学非线性.从声波方程和热传导方程出发,对实验结果进行了理论分析和数值模拟,理论值和实验结果很好的吻合.研究结果表明,样品溶液的非线性折射主要来源于瞬态热致非线性效应. 关键词： Z-扫描')" href="#">相位物体 Z-扫描 瞬态热致非线性折射 光克尔效应 DMF     

非线性偏振旋转锁模自相似脉冲光纤激光器的研究

利用耦合非线性薛定谔方程（CNLSE）为非线性偏振旋转（NPE）锁模自相似光纤激光器建立了一种新的数值模型.模型中,用CNLSE描述脉冲在单模光纤中的传播,在增益光纤中同时考虑了增益带宽和增益饱和作用,用传输矩阵描述构成NPE锁模的光学元件.优化了腔内净色散和光纤长度等参数,模拟了脉冲在激光腔内的演化特性,得到了典型的自相似脉冲运行区域及特点.在最佳自相似脉冲运行区域内,得到了能量约为7 nJ、脉宽约11 ps、线性啁啾的抛物脉冲.比较了不同腔内净色散条件下输出脉冲的特点,给出了三阶色散对输出脉冲的影响. 关键词： 自相似脉冲 非线性偏振旋转锁模 耦合非线性薛定谔方程 数值模拟     

应用非线性薛定谔方程模拟深海内波的传播

本文选取东沙岛以东深海区域,应用描述深海内波的非线性薛定谔方程,采用啁啾的思想,研究了频散和非线性效应之间的关系,模拟了深海内波的传播.数值模拟内波演变趋势与MODIS影像拍摄到的内波演变趋势基本符合,从而验证了应用非线性薛定谔方程模拟深海弱非线性内波传播的合理性. 关键词： 深海内波 啁啾 非线性薛定谔方程 频散和非线性     

高阶非线性效应对飞秒脉冲激光器的影响

本文以分段计算法用高阶非线性薛定谔方程讨论了激光器的传输过程,考虑了有三阶色散、高阶非线性效应-自陡峭效应存在时,激光器中飞秒脉冲的传输特性,给出了棱镜对的分离距离与激光器脉宽的关系,并用数值计算法模拟了脉冲在激光器中的传输过程.     

较高阶非线性抽运-探测过程中的空间效应

在飞秒抽运一探测光谱技术中,空间分辨的探测光信号反映了在不同空间位置的材料的非线性效应。当抽运光强度增大时,探测光信号中会出现明显的高阶特别是五阶非线性效应。利用劈裂算子方法直接解决了一维非线性传播方程的问题。在数值模拟中,研究了在不同抽运强度和位置下的抽运一探测过程中的五阶非线性效应。在足够高的抽运场下,探测信号出现清晰的振荡,显示了三阶和五阶非线性效应之间的干涉。当空间位置离抽运场中心足够远时,五阶比三阶非线性效应的衰减快得多,对其物理机制和趋势进行了定性的讨论。     

基于超快激光脉冲瞬态特征的非线性透射率

根据麦克斯韦方程,结合超快激光脉冲的瞬态特性,在忽略色散的影响下,推导并得出了三阶非线性各向同性系统中以光强表示的非线性吸收偏微分方程。以高斯脉冲激光为例,给出了该方程的一个近似解。基于该近似解的非线性透射率,不仅与脉冲激光的峰值强度、样品厚度以及介质的双光子吸收系数有关,而且还与描述脉冲主要特性的物理量——激光脉冲半峰全宽以及激发光的频率有关。数值拟合Rhodamine等物质的非线性透射率的实验曲线的结果显示,基于超短脉冲瞬态特性的非线性透射率得出的介质双光子吸收系数大于传统非线性透射率参考公式给出的相应结果,与双光子诱导荧光法的结果基本吻合。     

交叉相位调制对非线性光纤环镜中光脉冲传输的影响

基于耦合非线性薛定谔方程，采用分步傅里叶方法分析了在单波长信道和WDM（波分复用）4波长信道中XPM（交叉相位调制）对高速NOLM（非线性光纤环镜）光开关中脉冲传输的影响.数值计算表明：XPM造成NOLM中信号脉冲串扰与畸变，并造成NOLM开关性能的下降.WDM系统NOLM光纤环中的同向传播的各波长之间的XPM串扰比相向脉冲之间的XPM效应的影响更大，并且波长越短输出功率越低，中间信道受XPM的影响所导致的脉座现象和走离效应比两侧波长信道严重.     

A simple model of laser-induced fluorescence under arbitrary optical thickness conditions at the excitation wavelength

A simple model is worked out to investigate laser-induced fluorescence in media of arbitrary optical thicknesses at the excitation wavelength. Close-form expressions are obtained for laser fluence, absorbed energy density and emitted fluorescence signal as a function of optical thickness and incident laser fluence. It is shown that in optically thick media saturation curves are not proportional to density of the species excited by the laser, except at saturation, and that the saturation fluence increases with optical thickness. Experimental saturation curves of lead in laser-produced plasmas of brass are discussed in the light of this model.     

厚光学非线性介质Z扫描理论分析

采用高斯分解方法，对厚光学非线性材料的Ｚ扫描进行了理论分析，得到了对于实验工作者寻找优良的光学非线性材料和合理设计光学限制器时较有用的结果。 关键词：     

A boundary-based net-exchange Monte Carlo method for absorbing and scattering thick media

A boundary-based net-exchange Monte Carlo method was introduced (JQSRT 74 (2001) 563) that allows to bypass the difficulties encountered by standard Monte Carlo algorithms in the limit of optically thick absorption (and/or for quasi-isothermal configurations). With the present paper, this method is extended to scattering media. Developments are fully 3D, but illustrations are presented for plane parallel configuration. Compared to standard Monte Carlo algorithms, convergence qualities have been improved over a wide range of absorption and scattering optical thicknesses. The proposed algorithm still encounters a convergence difficulty in the case of optically thick, highly scattering media.     

厚高阶光学非线性介质Z扫描的变分法分析

利用变分法对具有五阶光学非线性介质的Z扫描特性进行了研究。通过比较，发现当介质在具有较大的五阶非线性系数或较大光强的情况下，五阶非线性项的作用是不可忽略的。这对光限制器的设计和Z扫描实验都具有一定的指导意义。     

Counterpropagating optical beams and solitons

Physics of counterpropagating optical beams and spatial optical solitons is reviewed, including the formation of stationary states and spatiotemporal instabilities. First, several models describing the evolution and interactions between optical beams and spatial solitons are discussed, that propagate in opposite directions in nonlinear media. It is shown that coherent collisions between counterpropagating beams give rise to an interesting focusing mechanism resulting from the interference between the beams, and that interactions between such beams are insensitive to the relative phase between them. Second, recent experimental observations of the counterpropagation effects and instabilities in waveguides and bulk geometries, as well as in one‐ and two‐dimensional photonic lattices are discussed. A variety of different generalizations of this concept are summarized, including the counterpropagating beams of complex structures, such as multipole beams and optical vortices, as well as the beams in different media, such as photorefractive materials and liquid crystals.     

非线性光学格子中的光束演化研究

研究光学格子中(即在光传输的横截面上存在周期格子势的调制)光束的演化，利用变分原理，求出了光束宽度、振幅、频率啁啾参量随传播距离的演化形式.发现光束宽度与调制周期的比值必须小于一定的值才能形成孤子的传输；同时，还得到了光束在不同的条件下存在着不同的传输过程.光学格子中周期格子的作用有类似非线性的良好的特性，周期格子的引入提供了可以更好地控制格子孤子的形成和传输的参考条件.     

Power saturation effects in thick single-element optical limiters

Optical limiters relying on nonlinear absorption or nonlinear refraction are most effective against an incoming laser beam when the active material is thicker than one Rayleigh length. We have found that a variety of thick optical limiter configurations can be modelled by integrating the formulae for optical transmission by thin media, and that the results are exact to the first order in power or irradiance. The limiter behaviour saturates as the optical power increases. For the case of thick irradiance-dependent absorbers and an incident Gaussian beam model, we have also found that the predictions of a simple saturation formula for the optical transmittance agree well with the transmittance values computed using a numerical technique. Under certain conditions this saturation formula is also suitable for describing the transmission of nonlinear refractors, thereby providing a straight-forward technique for modelling limiters over a broad parameter range.     

多维梯度折射率介质内辐射传递的扩散近似

推导多维梯度折射率介质内稳态辐射传递的扩散近似方程.使用有限元法对扩散近似进行离散和求解,利用两个二维半透明介质的稳态辐射传递问题验证该扩散近似的精度及适用性.算例考虑介质为均匀折射率及梯度折射率两种情况.利用扩散近似分别求解辐射平衡时的边界热流、介质内温度场分布,并与辐射传递方程的求解结果进行对比分析.结果表明:介质折射率变化、散射特性、光学厚度及散射反照率均直接影响扩散近似的精度;在光学厚及强散射条件下,该扩散近似可以作为一种快速算法应用于梯度折射率介质稳态辐射传递的求解.     

Structural,optical, spectroscopic and thermal investigations on novel semi-organic nonlinear optical material - Potassium boro-oxalate single crystal

In this work, a new semi-organic nonlinear optical material of Potassium boro-oxalate (KBO) is synthesized and subsequently a single crystal of size 7 × 5 × 3 mm³ is grown from the aqueous solution by slow evaporation technique at ambient temperature. Characterizations are performed on the single crystals to study the structural, thermal, linear and nonlinear optical (NLO) properties of the as-grown single crystals. Crystal and molecular structure of KBO are solved by direct method and further refinement is performed by full-matrix least-square method employing SHELXL-2014 software. Single crystal X-ray diffraction (SXRD) studies revealed that the grown crystal associates to triclinic crystal family with non-centrosymmetric space group P1. The Fourier transform infrared (FTIR) spectrum reflected the presence of various functional groups in the title compound. The Ultraviolet-visible-near infrared (UV-VIS-NIR) absorption and transmission spectrum are recorded to capture the suitability of the grown single crystals for various optical and NLO applications. The thermal decomposition and thermal stability of the KBO single crystals up to 187°C are investigated by TGA-DTG (Thermo Gravimetric - Differential Thermo Gravimetric), TGA-DTA (Thermo Gravimetric-Differential Thermal analysis) and DSC (Differential Scanning Calorimetry) curves. Kurtz-Perry powder technique is employed to explore the SHG (Second Harmonic Generation) efficiency of the KBO single crystals. SHG efficiency of KBO is found to be comparable to KDP.     

具有振幅调制的光学格子中光束的演化研究

利用变分原理和数值模拟的方法研究了光束在光传输方向的横截面上存在着具有振幅调制的光学格子时的演化,得到了光束宽度、振幅、光束的波阵面曲率随传播距离的演化形式.通过将光束的传输类比于粒子的运动,发现光束参量的条件存在三个区域,在不同的区域光束将在光格子的调制下有不同的传输形式,光格子振幅调制系数在各个区域起到了重要作用.光学格子中周期格子的作用有类似非线性的很好的特性,周期格子的引入提供了更好地控制格子孤子形成和传输的参考条件.