Temperature Dependence of Photoluminescence from Single and Ensemble InAs/GaAs Quantum Dots

We investigate the temperature dependence of photoluminescence from single and ensemble InAs/GaAs quantum dots systematically. As temperature increases, the exciton emission peak for single quantum dot shows broadening and redshift. For ensemble quantum dots, however, the exciton emission peak shows narrowing and fast redshift. We use a simple steady-state rate equation model to simulate the experimental data of photoluminescence spectra. It is confirmed that carrier-phonon scattering gives the broadening of the exciton emission peak in single quantum dots while the effects of carrier thermal escape and retrapping play an important role in the narrowing and fast redshift of the exciton emission peak in ensemble quantum dots.     

Dynamic dipole–dipole induction of coherence among a quantum dot ensemble

The quantum mechanical dynamic resonance due to dipole–dipole interaction is shown possibly to induce coherent modes of electrons within an ensemble of two-level systems or quantum dots. The physical origin of this coherence would naturally be postulated as the parity inheritance into a site being excited from another site being de-excited. An experimental spectrum suggestive of this dipole–dipole mode is also shown. This coherence is expected to be useful for quantum computing.     

Magneto-absorption in cylindrical quantum dots

The absorption of light in an ensemble of non-interacting cylindrical quantum dots in the presence of a magnetic field is discussed using a model consisting of dots with rectangular infinitely-high potential barriers. The ensemble’s absorption coefficient is calculated — as well as the threshold frequency of absorption — as a function of the applied magnetic field and the quantum dot size. Theoretical results are compared with experimental data on magneto-luminescence in an In_0.53Ga_0.47As/InP cylindrical quantum dot system. In addition, using a perturbation theory framework, the influence of excitonic effects on the behaviour of the electron-hole energetic spectrum of said system is discussed.     

Stimulated and spontaneous optical generation of electron spin coherence in charged GaAs quantum dots

We report on the coherent optical excitation of electron spin polarization in the ground state of charged GaAs quantum dots via an intermediate charged exciton (trion) state. Coherent optical fields are used for the creation and detection of the Raman spin coherence between the spin ground states of the charged quantum dot. The measured spin decoherence time, which is likely limited by the nature of the spin ensemble, approaches 10 ns at zero field. We also show that the Raman spin coherence in the quantum beats is caused not only by the usual stimulated Raman interaction but also by simultaneous spontaneous radiative decay of either excited trion state to a coherent combination of the two spin states.     

Quantum leakage of collective excitations of atomic ensemble induced by spatial motion

We generalize the conception of quantum leakage for the atomic collective excitation states. By making use of the atomic coherence state approach, we study the influence of the atomic spatial motion on the symmetric collective states of 2-level atomic ensemble due to inhomogeneous coupling. In the macroscopic limit, we analyze the quantum decoherence of the collective atomic state by calculating the quantum leakage for a very large ensemble at a finite temperature. Our investigations show that the fidelity of the atomic system will not be good in the case of atom numberN→∞. Therefore, quantum leakage is an inevitable problem in using the atomic ensemble as a quantum information memory. The detailed calculations shed theoretical light on quantum processing using atomic ensemble collective qubit.     

Inelastic interaction of ultrashort pulses of polarized light with an ensemble of isolated quantum dots

A system of equations is formulated describing the evolution of a slowly varying envelope of an arbitrarily polarized ultrashort pulse of electromagnetic radiation in a medium with its resonant properties determined by an ensemble of isolated quantum dots. It is assumed that the concentration of quantum dots is small and that the whole system is equivalent to a gas of resonant four-level atoms. Particular solutions are found that correspond to the propagation of a stationary optical pulse. It is shown by numerical solution of the generalized truncated Maxwell-Bloch equations that steady-state propagation is possible only for circularly polarized light pulses, whereas the pulses of arbitrary polarization either decay and experience the dispersion-related broadening or are converted into circularly polarized solitary waves.     

Onion like growth and inverted many-particle energies in quantum dots

Use of surfactants like antimony in MOCVD growth enables novel growth regimes for quantum dots (QDs). The quantum dot ensemble luminescence no longer appears as a single inhomogeneously broadened peak but shows a multi-modal structure. Quantum dot subensembles are forming which differ in height by exactly one monolayer. For the first time the systematic dependence of excitonic properties on quantum dot size and shape can be investigated in detail. Both biexcitonic binding energy and excitonic fine-structure splitting vary from large positive through zero to negative values. Correlation and piezoelectric effects explain the observations.     

Quasielastic scattering of light by a photoexcited electron-hole plasma induced in a GaAs layer in the presence of InAs quantum dots

The development of a method for registering quasielastic electronic light scattering spectra in the near-IR region, which makes it possible to detect light scattering by a photoexcited electron-hole plasma induced in a GaAs layer in the presence of a self-organized ensemble of InAs quantum dots, is reported. A substantial resonance intensification of such scattering, two orders of magnitude greater than the values established for the bulk material, is observed, and the main mechanism of such scattering is determined.     

The effect of nutation upon nonresonant propagation of electromagnetic wave in the ensemble of quantum dots

A new type of nutation oscillations is described arising only in the phase of a nonresonant electromagnetic wave (in the vicinity of its leading edge) propagating in the ensemble of quantum dots and producing electron transfer between the states of the quantum dots with approximately the same energy. It is shown that the period of the nutation oscillations can be used to determine main parameters of the nonresonant electron transfer between the quantum dots.     

Photoreflectance study of energy level structure of self-assembled InAs/GaAs quantum dots emitting at 1.3 μm

Photoreflectance and photoluminescence measurements were performed on the ensemble of self assembled InAs/GaAs quantum dots designed to emit at 1.3 μm. As many as six QDs-related optical transitions were observed in PR spectra, the energies of which were confirmed by high-excitation PL results. Numerical calculations allowed estimating the average size of the dots, which is larger than for standard InAs/GaAs QDs. This result is in agreement with structural data. Additionally, the energy level structure for such QDs was derived and compared with the electronic structure of standard InAs/GaAs dots. It was shown that the energy level structure of such large dots qualifies them for the active region of a laser emitting at 1.3 μm.     

Raman coherence beats from entangled polarization eigenstates in InAs quantum dots

The homodyne-detected transient four-wave-mixing response of InAs/GaAs self-assembled quantum dots shows temporal oscillations of the optically induced Raman coherence arising from two entangled polarization eigenstates of the exciton. The phase sensitive nature of the homodyne detection enables us to follow the time evolution of the nonradiative quantum coherence between the polarization states, providing a measurement of the fine-structure splitting in the dots, which is much less than the inhomogeneous broadening, and the corresponding decoherence rate of the entangled state.     

Dynamics of coherent and incoherent spin polarizations in ensembles of quantum dots

The temperature dependence of spin coherence in InGaAs quantum dots is obtained from quantum beats observed in polarization-resolved pump-probe experiments. Within the same sample we clearly distinguish between coherent spin dynamics leading to quantum beats and incoherent long-lived spin-memory effects. Analysis of the coherent data using a theoretical model reveals approximately 10 times greater stability of the spin coherence at high temperature compared to that found previously for exciton states in four-wave-mixing experiments by Borri et al. [Phys. Rev. Lett. 87, 157401 (2001)]]. The data on incoherent polarization reveal a new form of spin memory based on charged quantum dots.     

Pyramidal quantum dots: High uniformity and narrow excitonic emission

We report on the optical properties of site-controlled InGaAs dots in GaAs barriers grown in pre-patterned, large pitch, pyramidal recesses by metalorganic vapour phase epitaxy. The inhomogeneous broadening of excitonic emission from an ensemble of quantum dots is found to be extremely narrow, with a standard deviation of 1.19 meV. A dramatic improvement in the spectral purity of emission lines from individual dots is also reported (18–30 μeV ) when compared to the state-of-the-art for site controlled quantum dots.     

Quantum memory based on $\mathsf{\Lambda}$-atoms ensemble with two-photon resonance EIT

We study the -atoms ensemble based quantum memory for the quantum information carried by a probe light field. Two atomic Rabi transitions of the ensemble are coupled to the quantum probe field and classical control field respectively with a same detuning. Our analysis shows that the dark states and dark-state polaritons can still exist for the present case of two-photon resonance EIT. Starting from these dark states we can construct a complete class of eigen-states of the total system. A explicit form of the adiabatic condition is also given in order to achieve the memory and retrieve of quantum information.Received: 8 June 2004, Published online: 10 August 2004PACS: 03.67.-a Quantum information - 42.50.Gy Effects of atomic coherence on propagation, absorption, and amplification of light; electromagnetically induced transparency and absorption - 03.65.Fd Algebraic methods     

Hybrid quantum processors: molecular ensembles as quantum memory for solid state circuits

We investigate a hybrid quantum circuit where ensembles of cold polar molecules serve as long-lived quantum memories and optical interfaces for solid state quantum processors. The quantum memory realized by collective spin states (ensemble qubit) is coupled to a high-Q stripline cavity via microwave Raman processes. We show that, for convenient trap-surface distances of a few microm, strong coupling between the cavity and ensemble qubit can be achieved. We discuss basic quantum information protocols, including a swap from the cavity photon bus to the molecular quantum memory, and a deterministic two qubit gate. Finally, we investigate coherence properties of molecular ensemble quantum bits.     

Electron spin coherence in Si

We discuss pulsed electron spin resonance measurements of electrons in Si and determine the spin coherence from the decay of the spin echo signals. Tightly bound donor electrons in isotopically enriched ²⁸Si are found to have exceptionally long spin coherence. Placing the donors near a surface or interface is found to decrease the spin coherence time, but it is still in the range of milliseconds. Unbound two-dimensional electrons have shorter coherence times of a few microseconds, though still long compared to the Zeeman frequency or the typical time to manipulate a spin with microwave pulses. Longer spin coherence is expected in two-dimensional systems patterned into quantum dots, but relatively small dots will be required. Data from dots with a lithographic size of 400 nm do not yet show longer spin coherence.     

On‐chip single photon sources using planar photonic crystals and single quantum dots

We review the basic light‐matter interactions and optical properties of chip‐based single photon sources, that are enabled by integrating single quantum dots with planar photonic crystals. A theoretical framework is presented that allows one to connect to a wide range of quantum light propagation effects in a physically intuitive and straightforward way. We focus on the important mechanisms of enhanced spontaneous emission, and efficient photon extraction, using all‐integrated photonic crystal components including waveguides, cavities, quantum dots and output couplers. The limitations, challenges, and exciting prospects of developing on‐chip quantum light sources using integrated photonic crystal structures are discussed.     

基于电磁诱导透明机制的压缩光场量子存储

光场的量子存储不仅是构建量子计算机的重要基础,而且是实现量子中继和远距离量子通信的核心部分.由于存在不可避免的光学损耗,光学参量放大器产生的压缩真空态光场将变为压缩热态光场,不再是最小不确定态.因此,压缩热态光场的量子存储是实现量子互联网的关键.在原子系综中利用电磁诱导透明机制能够实现量子态在光场正交分量和原子自旋波之间的相互映射,即受控量子存储.本文根据量子存储的保真度边界,研究了实现压缩热态光场量子存储的条件.量子存储的保真度边界是通过经典手段能够达到的最大保真度,当保真度大于该边界时,就实现了量子存储.通过数值计算分析了不同情况下压缩热态光场的量子存储保真度边界,以及存储保真度随存储效率的变化关系,得到了实现量子存储的条件,为连续变量量子存储实验设计提供了直接参考.     

CdSe量子点“开关”的构建及其在药物分析中的应用

以CdCl₂·2.5H₂O,Na₂SeO₃和NaBH₄为反应物,制备巯基丁二酸稳定的CdSe量子点。在合成的量子点中加入一定浓度的铜离子,铜离子结合于量子点表面而使其荧光猝灭。在猝灭后的体系中加入青霉胺,由于青霉胺能使结合于量子点表面的铜离子释放出来而使量子点的荧光恢复。据此,建立了一种CdSe量子点"开关"测定青霉胺的新方法。在选定的实验条件下,方法的线性范围为1~72 μg/mL,检出限为0.031 μg/mL。应用于实际样品中青霉胺的测定,结果令人满意。     

Quantum beats of fine-structure states in InP quantum dots

Different types of quantum beats were experimentally observed in the photoluminescence kinetics of semiconductor nanostructures with InP quantum dots characterized by strong inhomogeneous broadening of the optical transitions. Specific types of beats were selected by varying the magnitude and orientation of the magnetic field, the applied bias voltage, and the frequencies of the exciting and detected light. Parameters of the fine structure of electrons and holes in the system under study and characteristic relaxation times of the spin coherence are determined from the experimental data.