Determination of absoluteK-internal conversion coefficients of some transitions in Ce140 by the internal-external conversion method

The internalK-conversion coefficients of the 331, 431, 815 and 933 keV transitions following the decay of La¹⁴⁰ have been determined absolutely by the method of comparing internal and external conversion lines measured in a double — focusing beta — ray spectrometers. TheK-internal conversion coefficients of the 4+→2+ 487 keV transition in Ce¹⁴⁰ was used to normalize relativeK-electron and gamma-ray intensities for these transitions. The results obtained are:α _K (331)=0.04432±0.00471,α _K (431)=0.28110±0.02913,α _K (815)=0.00396±0.00043,α _K (933)=0.00282±0.00031. Multipolarity assignments based on these values are suggested. The 815 keV transition is found to be pure magnetic dipole character in good agreement with the theoretical values calculated bySliv andBand. The 331 and 933 keV transitions are proved to have magnetic dipole character withE2/M1 equal 0.2852±0.0143 and 0.1750±0.0088 respectively. The 431 keV transition was found to have magnetic octupole character. The results obtained are most consistent with the assignment 2+, 4+, 2+, 3+ and 1+ for the 1597, 2084, 2184, 2410 and 2515 keV levels respectively.     

Untersuchung des Iridium-191m-Zerfalls

Theγ-radiation of the nuclear isomer Ir^191m (T _1/2=4.5 sec) has been investigated with the aid of a scintillation fast-slow coincidence-spectrometer. Theγ-rays of the 42 keV-transition have been measured for the first time. The conversion coefficient α of this transition was found to be α = 13500 ₊₂₁₁₀₀ ^?5200 in acceptable agreement with the value taken from the tables ofRose under the assumption of anE3-transition. Thus this assignment proposed earlier by other authors has been confirmed. TheK-conversion coefficient of the 129 keV-transition has been remeasured yielding α _K =2.32±0.06.     

Concerning internal conversion coefficients in Hf180

The gamma-ray relative intensities from transitions in Hf¹⁸⁰ following the 5.5 hour Hf^180m decay have been measured using a bent-crystal gamma-ray diffraction monochromator and a least-squares fitting technique. From these measurements it was possible to deduce a value for the internal conversion coefficient for the 93.3-keV transition of α _T ⁹³ =4.91±0.23. From previous measurements of conversion electron intensities byEdwards andBoehm and our gamma-ray relative intensities, internal conversion coefficients for all transitions except the 57.5-keV transition were obtained. These coefficients agree well with the previous determinations byEdwards andBoehm, however, our measurements have improved precision, particularly in the case of 501.3-keV transition. The present measurements of α _K for the 215.3-, 332.5-and 443.8-keVE2 transitions are 11% lower than theoretical values while α_K for 93.3 keV E2 transition agrees closely with the theoretical value. These results are in close agreement with the previous measurements ofEdwards andBoehm. The present experimental α_K for the 501-keV transition agrees closely with the theoretical α_K for an E3 multipolarity.     

Messungen derK-Konversionskoeffizienten und der Aktivierungsquerschnitte der isomeren Atomkerne Se77m,Se79m,Ge75m und Ge77m

TheK-conversion coefficients α _K of the nuclear isomers Se^77m , Se^79m , Ge^75m and Ge^77m have been measured by detecting theK-röntgen- andγ-radiation from neutron-irradiated Se- and GeO₂-samples with the aid of scintillation counters to be α _K =0.79±0.06, 7.4±0.6, 1.44±0.13, and 1.2±0.6, respectively. In all cases, the values obtained, are in agreement with those taken from the tables ofRose under the assumption of anE3-transition, thus confirming this assignment which was proposed earlier by other authors. In addition, the cross sectionsσ for inducing the activities by slowed down neutrons have been measured to beσ=22±2, 0.40±0.04, 0.20±0.02, and 0.12±0.03 barns, respectively, and are compared with earlier data of several authors.     

Dasβ-Spektrum des Cs137

Theβ-ray spectrum of Cs¹³⁷ has been measured with an iron-free spectrometer. The energy of the soft component was found to beE ₀=514±2 keV. The parameterk of the hard-component shape factorC _2VA ⁽²⁾ (W)=q ²+kp ² was determined to bek=0.015±0.004. Theβ intensities amount to 6.5% (hard component) and 93.5% (soft component). TheK conversion coefficient of the isomeric transition was measured to beα _K=0.093±0.003, in excellent agreement withSliv's theoretical value.     

Konversion der 238,6 keV-γ-Linie des ThB und Vergleich mit den Tabellen von Sliv und von Rose

The conversion ratiosK/L _I andK/L _II of the 238.6 keVγ transition of ThB have been measured with the new Heidelbergπ/2 √13Β-ray spectrometer. For this transition there are great discrepancies between the values as given bySliv andBand, and byRose. The experimental resultsK/L _I=5.96±0.26 andK/L _II=60.3±7.1 are in excellent agreement with the values ofSliv andBand.     

Zur Unsymmetrie der Impulshöhenverteilung in einem Szintillationsspektrometer für monoenergetische Röntgenstrahlung

For theK _α1-lines of the elements Ti, Fe, Cu and Mo the pulse-height distributions at the output of a Na I(Tl)-scintillation detector are recorded with an automatically recording single channel pulse-height analyser. The deviation to be observed in this low-energy region of the most probable from the mean value of these distributions is determined and is compared with the computations ofWright. The results may be described by an empirical formula with the energy dependenceE ^?2, whileWright predicts the dependenceE ^?1.     

Aufbau eines automatisch arbeitenden π√2-Spektrometers und Untersuchung des Konversionslinienspektrums von In114m und ThB mit Folgeprodukten

An automatically operatedπ√2 spectrometer is described. The regulated current supply is transistorized. With this spectrometer the electron spectra of In^114m and of ThB with daughter products have been investigated. TheK/L ratio of the 191 keV isomeric transition in In^114m was found to be 1·25±0·03, in excellent agreement with the theoretical value ofSliv andBand. In the electron spectrum of ThB and daughter products 46 lines were found betweenB?=1750Г cm andB?=10000Г cm. Some of them are new. Most important is a new weak line atB?=7030Г cm which fixes a new level atE=1·807 MeV in ThC′ (Po²¹²). Simultaneously the earlier reported discrepancy between electron andγ-ray intensities for 1·8 MeV transition energy is resolved. There is anE0 transition of 1·800 MeV while the new line is theK conversion line of a new radiative transition (most probablyM2). A spin ofI=2+ is assigned to the 1·680 MeV level of ThC′. The 0·953 MeV transition from this level isM1, withE0 admixture.     

L/K-Einfangverhältnis von65Zn

A multiwire proportional counter was constructed to measureL/K-capture ratios. The length of the counter is 90 cm, the diameter 14 cm, and it works with pressures from 1 to 6 atm. — The counter was proved by measuring theL/K-capture ratio of³⁷Ar. The result obtained is 0,098±0,003, in agreement with the calculated ratio 0,100 ofBahcall and the results of many other measurements with multiwire proportional counters. — Gaseous radioactiv Zincdiethyl was the substance to determine theL/K-capture ratio of⁶⁵Zn. The result obtained is 0,111±0,006, in agreement with the calculated ratio 0,109 ofBahcall, while 0,119±0,007 measured with a multiwire proportional counter bySantos Ocampo andConway is somewhat above the calculated ratio.     

Vergleich der Photoerzeugung von π0 am Proton mit der Voraussage nach der Dispersionstheorie

The real parts of the photoamplitudesE 1S _1/2,M 1P _1/2,M 1P _3/2 have been calculated from the angular distribution of the reactionγ+p→p+π⁰ recently measured byGoldansky et al. at 160 to 240 MeV. One of the solutions fits pretty well to the theoretical prediction for theM 1P _3/2-amplitude according to the dispersion method ofChew, Goldberger, Low andNambu. There is a discrepancy forM 1P _1/2 ifα ₁₁ is taken from the effective range formula, but the positive values ofα ₁₁, necessary to give agreement, are not excluded by the results of the phase shift analysis, especially sincePontecorvo et al. have recently found positive values at higher energies. The prediction for the real part of theE 1 S_1/2-amplitude agrees with the experimental data, if pretty large recoil corrections are added which had been neglected byChew et al.     

Quasielastic kaon knockout from a proton and momentum distribution of virtual kaons in the proton

The momentum distribution of kaons in the proton and the coupling-constant ratio fKΛN/fKΣN are determined on the basis of the ³P₀ quark model of meson-baryon coupling. The longitudinal cross section for kaon electroproduction is calculated. The results of the present study are compatible with available experimental data, but more detailed data on the longitudinal cross section would make it possible to refine the absolute values of the coupling constants fKΛN and fKΣN.     

Suche nach Zweiquantenprozessen beim Zerfall von Xe131m

The decay of Xe^131m was investigated in order to detect nuclear double decay processes, in which the transition energy is distributed either between twoγ-quanta or between oneγ-quantum and oneK-conversion electron or between twoK-conversion electrons. By analyzing the emittedγ-radiation in a two-dimensional way an upper limit of 2.2 · 10^?5 was derived for the ratio of theγγ- toγ-transition probability. An investigation of theγ-spectrum in coincidence withK-quanta yielded an upper limit of 3 · 10^?2 for the rate ofe _Kγ-transitions relative toγ-transitions. The simultaneous emission of twoK-quanta was actually observed. These doubleK-quanta result either from the doubleK-conversion that was sought or from the internal conversion of the internal Compton-effect. For the doubleK-electron emission toγ-emission probability a value of (3.6±0.7) · 10^?3 was obtained. TheK-conversion coefficient and the half-life of Xe^131m were measured to be 32.1±0.4 and 11.94±0.04 d, respectively.     

Das K-Auger-Spektrum von Neon

TheKLL-Auger spectrum of neon was investigated with an electrostatic spectrometer with an energy resolution of 0.12%. The ionization in theK-shell was caused by electron impact. The use of a gaseous target made it possible to measure the Auger electrons without any energy loss. The relative intensities of the KLL-lines were determined to be:KL ₁ L ₁(¹ S ₀)=1.0;KL ₁ L _2,3(¹ P ₁)=3.06±0.07;KL ₁ L _2,3(³ P _0,1,2)=0.98±0.05;KL _2,3 L _2,3(¹ S ₀)=1.67±0.08;KL _2,3 L _2,3(¹ D ₂)=13.1±0.6;KL _2,3 L _2,3(² P _0,2)=0. This is in agreement with an earlier measurement byKörber andMehlhorn but disagrees with all theoretical values calculated nonrelativistically for low Z. It is shown that agreement may be achieved by applying quantitatively the configuration interaction, introduced very recently byAsaad, and using improved wave functions for the calculation of the transition amplitudes. As a consequence of the ionization by electron impact also theKL-LLL Auger spectrum was caused. 10 lines of this spectrum were measured and identified. Moreover, from the Auger energies measured, the binding energyE(K) of neon was calculated to be E(K)=(870.0±0.4) eV.     

Study of Er171 decay by means of an electron-gamma coincidence technique

The decay scheme of Er¹⁷¹ (7.8 h) has been reinvestigated by means of an electron-gamma coincidence spectrometer and a scintillation spectrometer with a transistorized RIDL-400 channel analyser. A careful unfolding of the high energy region of the gamma-ray spectrum revealed the presence of photopeaks at energies of approximately 371, 404, 543, 572, 618, 675, 738, 796, 869, 910 and 962 keV. The existence of 32 transitions in Tm¹⁷¹ was confirmed. Also, it is proved that the 277, 362 keV transitions are in coincidence with the 210 keV and that the 175 keV transition is in coincidence with the 86 keV transition. We revealed the doubt for the existence of the 166, 210, 236, 277 and 419 keV transitions. From coincidence and single counting rates the followingK-conversion coefficients of the 111, 116, 124, 296 and 308 keV transitions were determined to be: α _K (111)=1.561±0.062, α _K (116)=0.699±0.035, α _K (124)=0.608±0.024, α _K (296)=0.0197±0.0010, α _K (308)=0.0183±0.0009, which give the 116, 124 keV transitions an electric quadrupole character; the 111 keV transition a magnetic dipole character withE2/M1 equal 0.4528; and the 296, 308 keV transitions an electric dipole character withM2/E1 equal 0.0058 and 0.0071 respectively.     

Aussagen der Theorie von Kraichnan für die isotrope hydromagnetische Turbulenz

The theory ofKraichnan is applied to quasi-stationary isotropic hydromagnetic turbulence. The average infinitesimal-impulse-response functionsg(k, τ), g _m (k, τ) and the time-correlationsr(k, τ), r _m (k, τ) are evaluated by the non-local direct-interaction approximation within the inertial range. For the range of ohmic but no viscous dissipation it is found that the magnetic energy spectrumE _m (k) obeys aE(k)k ^?2-law in accordance with results ofGolitsyn andMoffatt.     

Untersuchung derK-Strahlung beim Elektroneneinfang des Ge71 mit einem Diffraktionsspektrometer mit gebogenem Kristall

The intensity of satellites in the Gallium-x-rays emitted inK-capture of Ge⁷¹ has been measured and found to be (1,3±0,5)×10^?4 perK-capture. A curved-crystal X-ray spectrometer with a radius of curvature of 27 cm was used for the measurement. The satellites are found to be due to double ionisation ofK-shell accompanyingK-capture as described by the theory ofPrimakoff andPorter. The theoretically calculated intensity of X-ray satellites emitted due to double ionisation ofK-shell — (0,9)×10^?4 perK-capture — is in fair agreement with experiment.     

Octupole vibrations of deformed nuclei

The octupole vibrations of deformed nuclei are studied. A strong coupling between the harmonic octupole vibrations and the quadrupole ellipsoid is assumed. This interaction gives rise to a splitting of octupole bands with different projection quantum numberK. TheE1-transitions of the octupole states are explained within the frame of the Dynamic Collective Theory ofDanos andGreiner by calculating the Coulomb interaction between octupole vibrations and giant resonances. Furthermore, theE2- andE3-transitions of the octupole states are studied. The spectrum of W¹⁸² is investigated in detail. A fair agreement between theory and experiment is obtained. Predictions for the octupole spectra of Sm¹⁵² and Gd¹⁵⁶ are given.     

Relativistic Slater's integrals for theK andL shells

TheZ-dependent form of theSlater's integrals for electrons in theK andL shells is studied by expanding the relativistic hydrogenic radial wave functions in the manner explained byLayzer andBahcall. When screening is not taken into consideration, theseSlater's integrals can be put in the form AZ(1+a Z²) wherea is positive for all integrals considered except G¹(1s, 2p) and G²(2¯p, 2p). Values ofA anda are given.     

Winkelkorrelationsmessungen an >30y Holmium 166 und Bestimmung desg R -Faktors des 4+-Rotationsniveaus von Erbium 166

The spins of several excited states of Er¹⁶⁶ have been investigated byγγ-angular correlation measurements. The spin sequence 0+, 2+, 4+, 6+ for the ground state rotational band was presumed to be correct. Unique assignments were derived for the states of 1076 keV, 1377 keV and 1785 keV asI=5, 7 and 6 respectively. These results are in agreement with the spins proposed byGallagher jr. andSoloviev. The multipolarities of theγ-transitions of 408 keV, 709 keV, 811 keV and 831 keV were derived as 95%E1+(5±1)%M2, 99·6%E1+(0·4±0·5)%M2, 99·1%E2+(0·9±0·3)%M1, and 96·1%E2+(3·9±1)%M1 respectively. The unusual mixing ratios of the transitions of 811 keV and 831 keV can be understood as a consequence of theK-selection rule. Eachγ-transition from the 1785 keV state should be stronglyK-forbidden and one expects a half-life ofT _1/2≈3·10^?9s. A measurement of the time spectrum of the coincidences between theβ-radiation and the high energyγ-lines gave however:T _1/2(1785 keV state)≦3·10^?10s. The rotation of the angular correlation between the 184 keV line and theγ-group at 820 keV has been measured in an external magnetic field of 53000 gauss as:ω·τ(4+)=0·083±0·006. This value contains small corrections for an additional rotation of the angular correlation of the 831 keV–184 keV triple cascade in the 6+state and for a small attenuation by internal fields. WithT _1/2(4+state)=1·23·10^?10s, andβ=7·08 one gets for theg-factorg _R=+0·266±0·024 in good agreement with recent results for the 2+ state.     

Einfluß der Pion-Pion-Wechselwirkung auf Pion-Nukleon-Streuphasen

The isospin dependent part of theS-wave pion-nucleon amplitude is calculated according to the CGLN approach, but recoil and projection on the partial waves are treated exactly. Then the difference against the experimental data is approximately a constant up to 100 MeV and amounts to 1/3 of the total value. It is shown, that at low energies the main corrections of the CGLN equations are taken into account by a subtraction of theπ+π→?+\(\overline \Re \),J=I=1 amplitudesf _± ¹ (t) as proposed byMandelstam andFrazer. Calculations have been done forS, P andD pion-nucleon amplitudes. The main result is a prediction of theS-wave amplitude obtained without adjusting free parameters up to 100 MeV. The relations of this method to the equations derived byBowcock, Cottingham andLurié according to the Cini-Fubini approach are discussed.