The Yang-Lee distribution for a class of lattice gases

Classical lattice gases moving on a simple cubic lattice are considered. The lattice is assumed to grow only one-dimensionally. The gas particles have hard cores (of diameter greater than the lattice spacing) and are further subject to interactions of finite range and finite order. The interactions outside the hard cores may be represented as the components of av-dimensional vector, ?, which is initially allowed to be complex. Using a transfer matrix technique, an asymptotic expression is obtained for the grand canonical pressure (at complex values of the inverse absolute temperature β and the fugacityz). Let λ₁ ... λ _M denote the eigenvalues of the transfer matrix. Define ? to be aD*-interaction if and only if the quotients, λ _j /λ _k , 1≦j<k≦M, regarded as functions of β,z (with ? fixed) arenonconstant. In this paper it is assumed that there exists at least one allowable D*-interaction. With this assumption, the main result is that ifF denotes the set of interaction vectors for which the distribution, Ω, of limit points of zeros of the grand partition function in the complexz-plane at fixed β (res. complex β-plane at fixedz) contains a domain, thenF contains no product setA ₁×...×A _v ,A _k ??, 1≦k≦v unless one or more of theA _k consists of (at most) isolated points. This implies that the set of vectors for which Ω consists of arcs is dense in the set of all allowable vectors (in the usual topology for ?v).     

Exciton binding energy in GaAs quantum wells deduced from magneto-optical absorption measurement

Magneto-optical absorption spectra due to exciton states and Landau-levels were measured in GaAs/AlAs multi-quantum-wells. By extrapolating the photon energies of the absorption peaks to zero magnetic field, the lowest state (1S) heavy hole exciton binding energy, E^B_$\text{h}$(1S), was obtained as a function of well size L_z in the range $\text{58}\text{A}\text{?}\text{?}\text{L}{}_{\mathrm{z}}\text{?252}\text{A}\text{?}$. The L_z dependence of E^B_h showed the change of the exciton character from three-dimensional to two-dimensional with decreasing L_z. The diamagnetic shift observed for the heavy hole exciton peak was larger than that for the light hole exciton peak, showing the anisotropic nature of the Luttinger-Kohn Hamiltonian. The diamagnetic shift of the heavy hole exciton peak became smaller as L_z was decreased, suggesting the enhancement of the two-dimensional exciton character.     

Novel features of the fragment mass variance in fission of hot nuclei

On the basis of data obtained by the incomplete fusion reactions ⁷Li(43A MeV)+²³²Th and ¹⁴N(34A MeV)+¹⁹⁷Au, the energy dependence of the variance (σ _M ² ) of the fragment mass in fission of highly heated nuclei has been investigated for total excitation energies E _tot ^* ranging from 50 up to 350 MeV. The dependence σ _M ² E _tot ^* shows some unexpected features when E _tot ^* exceeds a value of about 70 MeV. After this value, the steady increase of σ _M ² expected from its temperature dependence changes to some kind of plateau between 100 and 200 MeV. Further on, at E _tot ^* in excess of about 250 MeV, the variance is found to increase again sharply. In order to analyze this behavior quantitatively, a dynamical stochastic model has been developed. The model employs the one-body dissipation mechanism and describes the decay of highly excited and rotating nuclei by fission and light-particle evaporation. It satisfactorily explains the measured prior-to-scission neutron multiplicities and the experimental mass variances up to E _tot ^* ?250 MeV, but the stochastic treatment does not reveal any increase in σ _M ² at higher excitation energies in contradiction with the data.     

Degenerate asymptotic perturbation theory

Asymptotic Rayleigh-Schrödinger perturbation theory for discrete eigenvalues is developed systematically in the general degenerate case. For this purpose we study the spectral properties ofm×m—matrix functionsA(κ) of a complex variable κ which have an asymptotic expansion εA _k κ ^k as τ→0. We show that asymptotic expansions for groups of eigenvalues and for the corresponding spectral projections ofA(κ) can be obtained from the set {A _κ} by analytic perturbation theory. Special attention is given to the case whereA(κ) is Borel-summable in some sector originating from κ=0 with opening angle >π. Here we prove that the asymptotic series describe individual eigenvalues and eigenprojections ofA(κ) which are shown to be holomorphic inS near κ=0 and Borel summable ifA _k ^* =A _k for allk. We then fit these results into the scheme of Rayleigh-Schrödinger perturbation theory and we give some examples of asymptotic estimates for Schrödinger operators.     

A study by E.S.R. of Mn2+ in potassium chromate

Divalent manganese ions are found in potassium chromate single crystals after heating at 600°C in the presence of iodine. These ions occupy three differently oriented sites with the same spin Hamiltonian parameters: g_z = 2·000, g_x = 2·008, g_y = 2·015; A_z = ?88·4 G, A_x = A_y = ?91 G; D = 190 and E = ?30 G.The authors suggest that Mn²⁺ occupies a substitutional (K⁺) position rather than an interstitial one. The influence of iodine is discussed.     

The reversibility of the Goos–Hänchen shift near the band-crossing structure of one-dimensional photonic crystals containing left-handed metamaterials

We perform a theoretical investigation on the Goos–Hänchen (GH) shift in one-dimensional photonic crystals (1DPCs) containing left-handed metamaterials (LHMs). We find an unusual effect of the GH shift near the photonic band-crossing structure, which is located at the condition, ?k _z ^(A) d _A =k _z ^(B) d _B =m π (m=1,2,3,…), under the inclined incident angle, here A denotes the LHM layer and B denotes the dielectric layer. Above the frequency of the band-crossing point (BCP), the GH shift changes from negative to positive as the incident angle increases, while the GH shift changes reversely below the BCP frequency. This effect is explained in terms of the phase property of the band-crossing structure.     

Nuclear magnetic relaxation of spin<Emphasis Type="Italic">I</Emphasis>=1/2 scalar coupled to a quadrupolar nucleus in the presence of cross-correlation effects

The rigorous treatment of relaxation for the dipolar-multipolarAX spin system (I=1/2,S>1/2) in the presence of the dipolarI-S coupling, anisotropy chemical shift and quadrupolar interaction ofS spin is proposed. The calculations of the spin evolution under the relaxation Hamiltonian are based on the second-order time-dependent perturbation theory and are carried out in the operator representation. For this task the double commutator identities of the type [[I _±S _z ⁿ ,A _q ^μp ]A _?q ^μp ] and [[I _zS _z ⁿ ,A _q ^μp ]A _?q ^μp. ] are derived. The fist-order differential equations for the evolution of longitudinal two-spin orderI _zS _z ⁿ , z=magnetization ofS spinS _z ⁿ and coherences <I _±S _z ⁿ > in the spin systemIS with scalar coupling between spin 1/2 and quadrupolar spinS>1/2 were obtained. These equations are used to get equations for the evolutions of each component of the multiplet structure of spinI. The imaginary part of the cross-correlation spectral density function and indirect spin-spin coupling Hamiltonian are taken into account. Equations for the longitudinal components of theI spin spectrum in the presence of cross-correlation effects were obtained also. Longitudinal and transverse relaxation times and cross-relaxation times in the presence of cross-correlation D-CSA, Q-CSA, Q-D were analyzed.     

Excitonic representation: Collective excitation spectra in the quantized Hall regime and spin biexciton

The excitonic representation method for describing collective excitations in the quantized Hall regime makes it possible to simplify analysis of the spectra and to obtain new results in the strong magnetic field limit, when E _C ??ω_c (ω_c is the cyclotron frequency and E_C is the characteristic Coulomb energy). For an integer odd filling factor ν greater than unity (i.e., for ν = 3, 5, 7,...), the spectra of one-cyclotron magneto-plasma excitations are calculated. For unit filling factor, the existence of a spin biexciton (bound state of two spin waves) corresponding to excitation with a spin change (δ_S = δ_Sz = ?2) is proved. The exact equation determining the ground state of the biexciton is derived in the thermodynamic limit N_Φ → ∞ (_N? is the system degeneracy). The exchange energy of this state is lower than for a single spin wave (with δ_S = δ_Sz = ?1) for the same value of the 2D wavevector q. In the limit q → ∞ corresponding to the decay of a biexciton into a pair of quasiparticles one of which is a trion with a spin of ?3/2, the energy is found to be lower than the energy (e²/εl _B )√π/2 required for exciting an electron-hole pair in the strictly 2D case (l_B is the magnetic length and ε is the dielectric constant), although this energy is higher than another “classical” result (e²/εl _B )√π/2, corresponding to the excitation of a skyrmion-antiskyrmion pair (|δS|=|δS _z |?1). The solution of the exact equation gives the trion binding energy and the activation gap for quasiparticles whose excitation corresponds to a change in the total spin by δS = δ S_z =?3. The energy of a spin biexciton is calculated for values of the wavevector such that ql _B ?1.     

Effect of the initial excitation energy on the average fission lifetime of nuclei

The dependence of the fission time on the initial nuclear excitation energy E _{tot 0} ^* is studied on the basis of a refined combined dynamical and statistical model. It is shown that this dependence may be nonmonotonic, in which case it features a broad maximum. It turns out that the form of the average fission time 〈t _f 〉 as a function of E _{tot 0} ^* depends greatly on the orbital angular momentum L _n carried away by prescission neutrons.     

Fission yields at different fission-product kinetic energies for thermal-neutron-induced fission of 239Pu

At the recoil spectrometer “Lohengrin” of the Institut Laue-Langevin in Grenoble, the yields of the light fission products from the thermal-neutron-induced fission of ²³⁹Pu were measured as a function of A, Z, the kinetic energy E and the ionic charge states q. The nuclear charge and mass distributions summed over all ionic charge states were determined for different light fissionproduct kinetic energies between 93 and 112 MeV. The proton odd-even effect which was measured to be (11.6 ± 0.6)% causes considerable fine structure in the yields. The average kinetic energy of even-Z elements in the light fission-product group is 0.3 ± 0.1 MeV larger than for odd-Z elements. The neutron odd-even effect is (6.5 ± 0.7)%. The comparison with previously published data ¹) for thermal-neutron-induced fission of ²³⁵U reveals a correlation between the proton odd-even effect in the yield and in the kinetic energy of the elements. The dependence of the proton odd-even effect on the fragmentation is very similar for ²³⁵U and ²³⁹Pu when it is considered as a function of the nuclear charge of the heavy fission products. The isobaric variances σ_z². for thermal-neutron fission of ²³⁵U and ²³⁹Pu coincide at all kinetic energies if the influence of the proton odd-even effect is averaged out. This supports the hypothesis that the magnitude of σ_z² is determined only by quantum-mechanical zero-point fluctuations. The influence of the spherical shells Z = 50 and N = 82 on the fragmentation is discussed.     

EPR spectra of the excited nitrogen state in 6H-SiC

A study is reported of donor EPR spectra in compensated 6H-SiC crystals with donor concentrations (N _D -N _A ) varied from 8×10¹⁷ to 5×10¹⁶ cm^?3, performed within a temperature interval from 77 to 170 K at a frequency of 37 GHz. A second paramagnetic state of nitrogen in silicon carbide has been found to exist, and it is associated with its excited 1S(E) state becoming paramagnetic after thermal ionization of the donor electrons from the 1S(A ₁) to 1S(E) level. The EPR spectrum of nitrogen in the 1S(E) state is a single line with an anisotropic width because of the unresolved hyperfine structure. A light-induced charge transfer between the ground, 1S(A ₁), and excited, 1S(E), nitrogen states has been observed. The valley-orbit splitting and the energy required to ionize donor electrons from the 1S(E) to higher lying excited states have been determined for the cubic nitrogen sites. The parameters of a structural defect, characteristic of n-type 6H-SiC compensated crystals, have been established.     

Nonfactorizable contributions to hadronic decays of charm mesons in the Cabibbo-suppressed modes

We investigate nonfactorizable contributions to charm meson decays into D → ππ/K K?/K K?*/K? K*/D → K*K?* modes. Obtaining the contributions from spectatorquark diagrams for N _c = 3, we determine the nonfactorizable isospin amplitudes required to explain the data for these modes. For these decays, we observe that ππ, πρ, decay modes favor a nonfactorizable-isospin-amplitudes ratio A ₀ ^nf /A ₂ ^nf equal to (1.123±0.158) and for K K?, K K?*, K? K* and K*K?* modes, the ratio of nonfactorizable amplitudes A ₀ ^nf and A ₁ ^nf turns out to be unity.     

Mass asymmetry dependence of angular distribution in237Np(α29 and 44 MeV,f): single particle effect

Angular distributions of fission products have been measured as a function of mass asymmetry in the odd-Z ²³⁷Np(α_{29 and 44 MeV},f) system using a recoil-catcher technique and off-line gamma spectrometry. Higher angular anisotropies were observed for the asymmetric mode products compared to the symmetric mode products at both energies. Average anisotropies for individual modes are lower than those for neighbouring even-even fissioning nucleus²⁴²Pu due to odd-nucleon spin effect. Present data have been analysed according to the transition state model assuming two modes of fission with characteristic saddle-shapes, barriers and multichance fission probabilities. It is seen that angular distributions for the symmetric and asymmetric modes are decided at and well past the corresponding saddle points respectively. Odd-nucleon spin contribution (〈k ²〉) to the tilting mode variance have been deduced. For (²⁴¹)Am fission, 〈k ²〉 values for the asymmetric and symmetric modes are ≤ 14 and > 14 ?² respectively. The 〈k ²〉 value averaged over several nuclei from preactinide (²⁰¹Ti) to actinide (²⁴⁸Cf) is 11.5 ± 4.2 ?². Average 〈k ²〉 value is in close agreement with the theoretical estimate.     

Emission and laser-excitation spectra of rotationally cooled methylcyanodiacetylene cation (A˜2EāX˜2 E) and photoelectron—photon

The A?²EāX?² E band system of rotationally cooled methylcyanodiacetylene cation has been studied by emission and excitation spectroscopies. Spectra were obtained by electron-impact ionisation of a seeded helium supersonic free jet and by Penning ionisation followed by laser excitation. These data enable the vibrational frequencies of most of the A₁ fundamentals to be inferred for the X?²E (to within ±2 cm^?1) andX?²E (to within ±4 cm?1) states. The fluorescence quantum yields and lifetimes of the cation prepared in selected levels of theA?²E andB?²A₁, excited states have been determined by photoelectron—photon coincidence measurements and yield a quantitative insight into the radiationless-decay pathways.     

Systematic behavior ofB(E2) values in the yrast bands of doubly even nuclei

The experimental information onB(E2) transition rates in the yrast bands of doubly even nuclei (126≦A≦184) is systematized. The strength functionS _exp≡B(E2,I→I?2)×E(I→I?2) is found to reveal characteristic behavior significant for structure studies of yrast bands. The energy-weightedB(E2,I→I?2) values (S _exp) and 2?/?²(?: moment of inertia) are plotted versus the rotational frequency squared ?²ω² for each nucleus. In strongly deformed nuclei (N≧90), theS _exp curves smoothly increase for low rotational frequencies suggesting that up to spin valuesI≈8 the ratioQ ₀ ² ? is nearly constant (Q ₀: quadrupole moment). This is not the case in nuclei with a soft core (N≦88). In the relevant discussion, the hydrodynamical model as well as the CAP effect are considered. The results in the backbending region are qualitatively discussed in terms of the two-band crossing model. Evidence is found supporting the prediction of an oscillating behavior of the yrast-yrare interaction.     

The effect of the nonplanarity of heterocyclic analogues of fluorene with the phosphorus atom on spin-orbit interactions

The transition dipole moments P ₀₀ ^S for the transitions from the sublevels s=z,y, and x of the triplet electronic states ³ A″, which are caused by intramolecular spin-orbit (SO) interactions, are calculated. The calculation is carried out for molecules of heterocyclic analogues of fluorene containing phosphorus and nitrogen (namely, the groups P-H, P-C₆H₅, and N-H). The influence that the planar and nonplanar models of the molecules, as well as the substituents ?C₆H₅ and ?H at the heteroatom (HA), exert on the values of (P ₀₀ ^S )² and on the directions of the corresponding vectors is considered. The values of the component \(k_{SO^ \sim } \sum _s (P_{00}^s )^2 \) of the radiative deactivation rate constant of the T ₁ state are calculated. It is ascertained that, in the series of molecules with HA = N, O, P, and S, both the calculated values of k _SO and those experimentally determined from an analysis of the intensity distribution in fine-structure phosphorescence spectra vary little, whereas the constant of the SO coupling in the heteroatom ?_HA increases substantially along this series. The reason for the weak influence of ?_HA on values of k _SO—common for both planar and nonplanar molecules—is found.     

Simplified closed form expressions for irreducible tensor operators

A general closed form expression is derived which enables one to write a spherical tensor of rank L and projection k, T_uk^L, in terms of the familiar angular momentum operators, S_z and S². The simplicity of this expression results from an intriguing relationship between these spherical tensor operators (diagonal operator equivalents) and successive derivatives of Tchebichef orthogonal polynomials.     

Analysis of fragment mass distribution in asymmetric area at fission of <Superscript>235</Superscript>U induced by thermal neutrons

The fragment mass yields in fission of ²³⁵U induced by thermal neutrons for A = 145–160 and E_K = 50–75 MeV were measured using a mass spectrometer. The fine structure is observed at A = 153, 154 and E_K = 50–60 MeV. The obtained results were described in the framework of a model based on the dinuclear system concept. The analyzed correlation between the total kinetic energy and mass distribution of fission fragments is connected with the shell structure of the formed fragments of fission. From this correlation and the time dependence of the calculated mass distribution of the binary reaction products, one can conclude that the descent time from a saddle point to a scission point for the more deformed fragments is longer than that for fragments of more compact shape.