Exciton-photon interaction in low-dimensional semiconductor microcavities

The structure of the photon states and dispersion of cavity polaritons in semiconductor microcavities with two-dimensional optical confinement (photon wires), fabricated from planar Bragg structures with a quantum well in the active layer, are investigated by measuring the angular dependence of the photoluminescence spectra. The size quantization of light due to the wavelength-commensurate lateral dimension of the cavity causes additional photon modes to appear. The dispersion of polaritons in photon wires is found to agree qualitatively with the prediction for wires having an ideal quantum well, for which the spectrum is formed by pairwise interaction between exciton and photon modes of like spatial symmetry. The weak influence of the exciton symmetry-breaking random potential in the quantum well indicates a mechanism of polariton production through light-induced collective exciton states. This phenomenon is possible because the light wavelength is large in comparison with the exciton radius and the dephasing time of the collective exciton state is long. Zh. éksp. Teor. Fiz. 114, 1329–1345 (October 1998)     

Pulse Transmission and State Conversion in Two-mode Optomechanical Cavity Coupled with Atomic Medium

We investigate the quantum state conversion between cavity modes of distinctively different wavelengths for the two-mode optomechanical cavity coupled with the three-level lambda atom. In the frequency domain, we show that the coherence of atom medium leads to the two maximum transmissions. We also show that the injected atom can interrupt the traveling photon pulses which is transmitted between the different input and output channels. Thus, the addition of atom provides us a way to control the transmission between the quantum states of two cavity modes and the photon information storage.     

Quantum state transfer between distant atoms via selectivity photon emission and absorption progresses

We proposed a simple scheme to deterministically generate three-dimensional (3D) quantum state transfer (QST) between two spatially atoms based on the selectivity photon emission and absorption progresses. In the present scheme, two M-type five-level atoms are trapped into two cavities connected by a fiber. By quantitatively discussing the evolution of system, we show that the effects of atom's spontaneous decay and photon leakage out of fiber can be suppressed in our scheme due to the presence of virtual excited processes in atom and fiber modes. Moreover, we also show that the present scheme can be extended to realize QST between distant nodes in a coupled array of optical cavity, which is very useful for the progress of the quantum information network.     

Inhibition and enhancement of the spontaneous emission of quantum dots in structured microresonators

Spontaneous emission of quantum dot systems in laterally structured microcavities that exhibit photon confinement in all three directions has been studied by time-resolved photoluminescence spectroscopy. For on-resonance conditions, we find that the dot emission rate is increased substantially over that of the unstructured planar cavity. For off-resonance conditions, we are able to suppress the emission rate by an order of magnitude by using cavities with metal coatings, which we attribute to the suppression of leaky optical modes in these structures.     

Photon bunching and anti-bunching with two dipole-coupled atoms in an optical cavity

We investigate the effect of the dipole–dipole interaction(DDI) on the photon statistics with two atoms trapped in an optical cavity driven by a laser field and subjected to cooperative emission. By means of the quantum trajectory analysis and the second-order correlation functions, we show that the photon statistics of the cavity transmission can be flexibly modulated by the DDI while the incoming coherent laser selectively excites the atom–cavity system's nonlinear Jaynes–Cummings ladder of excited states. Finally, we find that the effect of the cooperatively atomic emission can also be revealed by the numerical simulations and can be explained with a simplified picture. The DDI induced nonlinearity gives rise to highly nonclassical photon emission from the cavity that is significant for quantum information processing and quantum communication.     

Hybrid quantum processors: molecular ensembles as quantum memory for solid state circuits

We investigate a hybrid quantum circuit where ensembles of cold polar molecules serve as long-lived quantum memories and optical interfaces for solid state quantum processors. The quantum memory realized by collective spin states (ensemble qubit) is coupled to a high-Q stripline cavity via microwave Raman processes. We show that, for convenient trap-surface distances of a few microm, strong coupling between the cavity and ensemble qubit can be achieved. We discuss basic quantum information protocols, including a swap from the cavity photon bus to the molecular quantum memory, and a deterministic two qubit gate. Finally, we investigate coherence properties of molecular ensemble quantum bits.     

Quantum dots in photonic crystals: From quantum information processing to single photon nonlinear optics

Quantum dots in photonic crystals are interesting both as a testbed for fundamental cavity quantum electrodynamics (QED) experiments and as a platform for quantum and classical information processing. We describe a technique to coherently access the QD-cavity system by resonant light scattering. Among other things, the coherent access enables a giant optical nonlinearity associated with the saturation of a single quantum dot strongly coupled to a photonic crystal cavity. We explore this nonlinearity to implement controlled phase and amplitude modulation between two modes of light at the single photon level—a nonlinearity observed so far only in atomic physics systems. We also measured the photon statistics of the reflected beam at various detunings with the QD/cavity system. These measurements reveal effects such as photon blockade and photon-induced tunneling, for the first time in solid state. These demonstrations lie at the core of a number of proposals for quantum information processing, and could also be employed to build novel devices, such as optical switches controlled at the single photon level.     

Using coherent feedback loop for high quantum state transfer in optomechanics

We investigate the coherent feedback loop scheme to improve the quantum correlations transfer from optical to mechanical degrees of freedom in a double cavity optomechanical system. We use the Duan criterion to determine the separability of the two-mode mechanical states. The logarithmic negativity is employed to quantify the amount of the entanglement between mechanical modes in steady and dynamical regimes. We show that the entanglement can be significantly enhanced by a coherent feedback using a suitable tuning of the reflectivity parameter of the beam splitter located in each cavity. We also show that this enhancement is influenced by the temperature, the light squeezing parameter and the gain of the parameter amplifier. The entanglement dynamics in presence of the coherent feedback loop is also analyzed.     

Dicke quantum spin glass of atoms and photons

Recent studies of strongly interacting atoms and photons in optical cavities have rekindled interest in the Dicke model of atomic qubits coupled to discrete photon cavity modes. We study the multimode Dicke model with variable atom-photon couplings. We argue that a quantum spin-glass phase can appear, with a random linear combination of the cavity modes superradiant. We compute atomic and photon spectral response functions across this quantum phase transition, both of which should be accessible in experiments.     

Time-resolved and cw photoluminescence from strongly coupled organic microcavities

The optical properties of microcavities (MCs) are strongly dependent on both polarization of incident and emitted light and its angle of observation. Here we report the measurements of cw- and time-resolved photoluminescence (PL) observed at negative detuning and at resonance for s- and p-polarization in the strong coupling regime of a planar MC containing J-aggregates of a cyanine dye. Following non-resonant excitation, the emission spectra consist of three types of features: direct J-aggregate exciton emission, polariton emission, and uncoupled monomer emission through the transmission maxima of the distributed Bragg reflector beyond the stop-band. We compare our experimental results with a transfer-matrix calculation of the transmission for s- and p-polarization and explain the different positions of the polariton branches, the stop-band width, and the high- and low energy transmission maxima of the MC. Time-resolved PL experiments show an increase in the decay lifetime of the exciton-like mode when it is positioned far from the cavity mode. Close to resonance, the lower polariton branch decays with the natural lifetime of the J-aggregates.     

Spontaneous emission enhancement at a photonic wire miniband edge

In a multimode photonic-crystal waveguide, we observe strong enhancement of the photoluminescence of embedded quantum dots at the edges of the so-called mini-stopband that were opened by Bragg diffraction between two guided modes. Taking into account light collection, we relate this observation to the singular photon density of states that is characteristic of a one-dimensional photon system. Furthermore, we quantify by how much the radiation losses smooth the divergence. For the first time to our knowledge, a clear account of the control of spontaneous emission in a one-dimensional system is thus demonstrated.     

Transferring and Bounding Single Photon in Waveguide Controlled by Quantum Node Based on Atomic Ensemble

We study the scattering process of photons confined in a one-dimensional optical waveguide by a laser controlled atomic ensemble. The investigation leads to an alternative setup of quantum node controlling the coherent transfer of single photon in such one dimensional continuum. To exactly solve the effective scattering equations by using the discrete coordinate approach, we simulate the linear waveguide as a coupled resonator array at the high energy limit. We generally calculate the transmission coefficients and itsvanishing at resonace reflects the good controllability of our scheme. We also show that there exist two bound states to describe the localize photons around the cavity.     

Intracavity weak nonlinear phase shifts with single photon driving

We investigate a doubly resonant optical cavity containing a Kerr nonlinear medium that couples two modes by a cross phase modulation. One of these modes is driven by a single photon pulsed field, and the other mode is driven by a coherent state. We find an intrinsic phase noise mechanism for the cross phase shift on the coherent beam which can be attributed to the random emission times of single photons from the cavity. An application to a weak nonlinearity phase gate is discussed.     

Quantum coherence transfer between an optical cavity and mechanical resonators

This study highlights the theoretical investigation of quantum coherence in mechanical oscillators and its transfer between the cavity and mechanical modes of an optomechanical system comprising an optical cavity and two mechanical oscillators that,in this study, were simultaneously coupled to the optical cavity at different optomechanical coupling strengths. The quantum coherence transfer between the optical and mechanical modes is found to depend strongly on the relative magnitude of the two optomechanical couplings. The laser power, decay rates of the cavity and mechanical oscillators, environmental temperature, and frequency of the mechanical oscillator are observed to significantly influence the investigated quantum coherences. Moreover,quantum coherence generation in the optomechanical system is restricted by the system's stability condition, which helps sustain high and stable quantum coherence in the optomechanical system.     

Dynamics of entanglement transfer from radiation modes to localized qubits

We address the dynamics of entanglement transfer from two radiation modes to a pair of localized qubits implemented as atoms flying through or trapped in separated cavities. We first generalize previous results to include radiation in entangled mixed states and to describe the effect of cavity mirror transmittance. Then we investigate the transfer process by Monte Carlo Wave Function approach, which allows us to solve the whole system dynamics including cavity mode and atomic decays. We focus on flying modes prepared in coherently correlated states and we find realistic conditions for efficient entanglement transfer out of the weak and strong coupling regimes in the perspective of quantum memories realization.     

Controlling spontaneous emission and threshold-less laser oscillation with optical microcavities

We describe the alteration of spontaneous emission of materials in optical microcavities having dimensions on the order of the emitted wavelength. Particular attention is paid to one-dimensional optical confinement structures with pairs of planar reflectors (planar microcavities). The presence of the cavity causes great modifications in the emission spectrum and spatial emission intensity distribution accompanied by changes in the spontaneous emission lifetime. Experimental results are shown for planar microcavities containing GaAs quantum wells or organic dye-embedded Langmuir-Brodgett films as light emitting layers. Also discussed are the laser oscillation properties of microcavities. A remarkable increase in the spontaneous emission coupling into the laser oscillation mode is expected in microcavity lasers. A rate equation analysis shows that increasing the coupling of spontaneous emission into the cavity mode causes the disappearance of the lasing threshold in the input-output curve. Experimentally verification is presented using planar optical microcavities confining an organic dye solution. The coupling ratio of spontaneous emission into a laser mode increases to be as large as 0.2 for a cavity having a half wavelength distance between a pair of mirrors. At this point, the threshold becomes quite fuzzy. Differences between the spontaneous emission dominant regime and the stimulated emission dominant regime are examined with emission spectra and emission lifetime analyses.     

Phonon-mediated coupling of InGaAs/GaAs quantum-dot excitons to photonic crystal cavities

We demonstrate that the emission characteristics of site-controlled InGaAs/GaAs single quantum dots embedded in photonic crystal slab cavities correspond to single confined excitons coupled to cavity modes, unlike previous reports of similar systems based on self-assembled quantum dots. By using polarization-resolved photoluminescence spectroscopy at different temperatures and a theoretical model, we show that the exciton-cavity interaction range is limited to the phonon sidebands. Photon-correlation and pump-power dependence experiments under nonresonant excitation conditions further establish that the cavity is fed only by a single exciton.     

Coupled-resonator optical waveguides doped with nanocrystals

Microsphere resonators doped with semiconductor nanocrystals are explored as building blocks for coupled-resonator optical waveguides (CROWs). The evolution of individual cavity modes into coherently coupled waveguide modes is studied using polarization-sensitive microphotoluminescence spectroscopy. To demonstrate the formation of multisphere photon states, we use a bent linear array of microresonators and probe the properties of the cavity photon field by the spatially and spectrally resolved measurement of the nanocrystal emission. Photon mode coupling is evidenced by the observed mode splitting and emission intensity distributions along the CROW structure.     

Temperature dependent polariton emission from strongly coupled organic semiconductor microcavities

We investigated the absorption and photoluminescence (PL) of J-aggregates of a cyanine dye both in a thin film format and when used as the active layer in a strongly-coupled microcavity. We show that as temperature is reduced, the absorption linewidth of the J-aggregates narrows and shifts to higher energy. When the J-aggregate is placed in a microcavity we find that the energy of the polariton modes also shifts to higher energies as temperature is reduced. We compare the intensity of PL emission from the upper and lower branches at resonance as a function of temperature, and find that it can be described by an activation energy of 25 meV. PL emission spectra at resonance also suggest that uncoupled excitons inside the microcavity populate the upper polariton branch states.