Collective excitations in148Gd populated in thep p′-reaction on a radioactive target

Collective excitations in the two-particle nucleus¹⁴⁸Gd up to 2.9 MeV have been investigated by thepp′-reaction at 25 MeV beam energy, and angular distributions have been analyzed with standard DWBA calculations. It is found that¹⁴⁸Gd has larger octupole- than quadrupole collectivity in the energy range investigated. The 3^? strength distribution is in quantitative agreement with predicted results for the levels formed by the coupling of two valence particles to the¹⁴⁶Gd core octupole phonon.     

Excited states in145Gd from the (3He, 2n) reaction

Medium and high spin states in¹⁴⁵Gd up to 3.5 MeV excitation energy have been studied by in-beam gamma ray and conversion electron spectroscopy bombarding enriched¹⁴⁴Sm target with a³He beam. For a part of the identified levels a configuration is proposed in terms of weak coupling of one neutron hole with the¹⁴⁶Gd core or of one neutron particle with the¹⁴⁴Gd core.     

Particle hole yrast states in146Gd and147Gd and the Z=64 shell closure

The level structures of¹⁴⁶Gd and¹⁴⁷Gd have been investigated by in-beamγ-ray ande ^? spectroscopy with (α, xn) reactions on enriched Sm targets. Detailed level schemes up to ～4 MeV, which differ radically from earlier schemes, are reported. The energy levels are characterized as particle-hole excitations using empirical single particle energies and two nucleon interactions. Analysis of pure 1p 1h proton excitations demonstrates that theZ=64 andN=82 energy gaps are about equally large.     

The ground state mass of147Gd from single-neutron-transfer reactions and its impact on derived mass values

Using a¹⁴⁸Gd radioactive target and the (p,d), (d,t), and (³He,α) single neutron pick-up reactions we have measured the¹⁴⁷Gd mass excess as — 75,366(4) keV, which differs by 139(24) keV from the adopted value of the 1983 mass table. From this result, and from recently reported first transfer-reaction mass determinations for¹⁴⁵Eu and¹⁴⁶Eu, we have recalculated the masses of nuclei above¹⁴⁶Gd from a previous shell model analysis of high-spin states.     

Production of high multiplicity yrast isomers in147Gd and146Gd in a-particle induced reactions

High spin isomers in ¹⁴⁷ Gd and ¹⁴⁶ Gd have been produced in (α, xn)reactions, and their half-lives, excitation energies and maximum spins have been determined. It is proposed that these isomers are identical with those recently observed in bombardments with ⁵⁰ Ti and ⁴⁰ Ar projectiles.     

Shell model isomers near Z = 64, N = 82: g-factors of Yrast states in 146Gd and 147Gd

Nuclear g-factors have been measured for the 7^? isomer in ¹⁴⁶Gd and for the $\text{27}\text{2}{}^{\mathrm{?}}$ isometer in ¹⁴⁷Gd. For ¹⁴⁷Gd the results is consistent with the expectation for a pure shell model configuration.     

Excited superdeformed band in146Gd

A non-yrast superdeformed band has been found in¹⁴⁶Gd using the¹¹⁰Pd(⁴⁰Ar, 4n)¹⁴⁶Gd reaction. The nuclear assignment was made from the analysis of an experiment using a backed target. This band and the previously identified yrast SD band are probably not signature partners.     

Shell model and octupole states in148Gd from in-beam experiments

Through (α, 4n) and (τ, 3n) reactions the high-spin states in the two-neutron nucleus¹⁴⁸Gd were populated up toI ^π=21? at 7.2 MeV, including numerous states above the yrast line. The¹⁴⁸Gd energy spectrum is interpreted in terms of the spherical shell model. Identification of the (νf _7/2 i _{1 3/2})_10? state gives the νi _13/2 single particle energy free of octupole admixtures as 2.1(1) MeV. Eight high-spin states between 1.2 and 3.7 MeV were identified as the couplings of the two valence-particles to the¹⁴⁶Gd octupole phonon, and three above-lying levels are assigned as double-octupole excitations including a 12⁺ state which decays by anE3-E3 stretched cascade. All these octupole levels can be quantitatively predicted from the one-particle x phonon spectrum of¹⁴⁷Gd. The high-spin states above 3 MeV are four-quasiparticle excitations ofπ ⁺¹ π ^?1 ν ² andπ ² ν ² type and their energies are in good accord with shell model estimates.     

Levels of146Ce studied through the decay of high-spin isomer of146La

The decay of 10.0 s high-spin isomer of¹⁴⁶La to levels of¹⁴⁶Ce has been studied using the on-line isotope separator KUR-ISOL. Gamma-ray singles,γ -γ coincidence and conversion-electron spectra have been measured. A level scheme containing 90 levels and 206γ-ray transitions has been constructed for¹⁴⁶Ce, populated in the decay of the high-spin isomer of¹⁴⁶La. Among these, 39 levels are reported for the first time. Spins and parities for some levels are proposed on the basis ofγ-decay mode, logft values and conversion-electron measurements. The band structure of the low-lying levels in¹⁴⁶Ce is discussed.     

Tentative level diagram of146Pm below 1.1 MeV

The level scheme of the doubly odd nucleus¹⁴⁶Pm was investigated by means of in-beam spectroscopy. The¹⁴⁶Nd(p, n) reaction in the 3.5–8 MeV proton energy interval on enriched targets has been used to populate the exited states of¹⁴⁶Pm. High resolutionγ-ray spectra using Ge(Li) and hyperpure Ge detectors and conversion electrons with a mini-orange spectrometer were measured. Withγ-exitation functions andnγ-coincidences usingnγ-discriminated NE231 neutron detectors transitions in¹⁴⁶Pm were identified,γγ-coincidences gave information aboutγ-cascades. With these data a level scheme of 38 levels below 1.1 MeV exitation energy has been deduced including 73 transitions. For 12 transitions experimental conversion coefficients have been evaluated, which agree with the expected values forM1/E2-transitions.     

On the Z = 64 shell closure

Spherical HFB calculations do not produce a Z = 64 shell closure in ¹⁴⁶Gd.     

The 3− state in the doubly closed shell nucleus 64 146 Gd82

Inbeam γ-ray angular distribution measurements establishI ^π = 3^? for the 1579 keV first excited state in¹⁴⁶Gd.     

Properties of the 3− first excited state in the doubly closed shell nucleus146Gd

Conversion electron measurements confirm the 3^? assignment recently proposed for the 1579 keV first excited state in¹⁴⁶Gd. Fromγγ- ande ^? γ-coincidence data the half life of that state has been determined asT _1/2=1.06±0.12 ns.     

The doubly-magic character of146Gd and its relation to208Pb

Recent experiments indicate the possibility of a doubly-magic character for the nucleus¹⁴⁶Gd (Z=64, N=82). In this work the results of a large-scale shell-model study on the nucleus¹⁴⁶Gd and its neighbouring nuclei¹⁴⁵Eu,¹⁴⁵Gd,¹⁴⁷Gd and¹⁴⁷Tb are presented. The configurations taken into account include up to 2p - 2h excitations for protons and/or neutrons. The calculated spectra and static moments are compared with the experimental data. Finally, the present results on shell closure in¹⁴⁶Gd are discussed in connection with those derived from a similar approach applied to the well-known doubly-magic nucleus²⁰⁸Pb.     

High spin states in the doubly-closed shell nucleus146Gd

High spin states of¹⁴⁶Gd, populated in heavyion induced reactions, have been investigated by means of in-beamγ-ray spectroscopy using the Compton-suppressed germanium detector arrays OSIRIS and ESSA30. 35 new levels and 47 new transitions could be placed in the level scheme. In addition to the extension to very high spins, a new cascade has been observed at intermediate spins.     

β + ratio andβ-delayedγ-decay of146Eu

The positron decay of¹⁴⁶Eu was investigated, firstly to derive for the allowed transition to the 2046 keV state in¹⁴⁶Sm the electron capture to positron decay ratio. The experimental valueEC/β ⁺=43.7(42) is found to be in agreement within the respective error intervals with the ones calculated from the formalism of allowed decay using the recentQ-values of¹⁴⁶Eu. Further on, theγ-decay properties of¹⁴⁶Eu have been reinvestigated with emphasis on implied modifications of the hitherto accepted decay scheme: 42 new levels and 33 newγ-transitions were placed in the revised level scheme, 12 of the previously reported levels were deleted. The level distribution of¹⁴⁶Sm is discussed within a statistical model. The indication for a non-statisticalβ-strength function is observed.     

Investigation of statistically perturbed angular correlations of154Gd and156Gd in different liquid sources

The statistical perturbations of γγ-angular correlations involving the first 2⁺ rotational state of¹⁵⁴Gd and¹⁵⁶Gd have been time differentially investigated. We used liquid sources of 3⁺ ions of Gadolinium in lN perchloric acid, 0.5 N and 1N hydrochloric acid, 1.3N and 2.6 N sulfuric acid. Influences of the various chemical surroundings on the ratio λ₄/λ₂ of the attenuation parameters have been found. A simultaneous measurement of the angular correlation of the 874 keV–123 keV cascade and the 2,098 keV–89 keV cascade of¹⁵⁴Gd and¹⁵⁶Gd, respectively, has been performed in perchloric solution. From the ratio of the attenuation parameters λ₂, obtained by this experiment, we have derived the ratio of the magneticg-factors of the first 2⁺ levels of these isotopes asg ¹⁵⁴/g ¹⁵⁶=1.11±0.08.     

Decay of149Gd and directional correlations of gamma cascades in149Eu

The decay of¹⁴⁹Gd(9.4d) to the levels of¹⁴⁹Eu has been studied using large volume high resolution Ge(Li) and NaI(Tl) detectors,γ-γ coincidence and directional correlation experiments have been performed. Newγ-rays at energies 131.9, 278.6, 384.7, 415.7, 599.2, 726.5, 734.7, 956.4 and 1,231.1 keV in¹⁴⁹Eu have been observed. Three new levels in¹⁴⁹Eu have been placed at 956.4, 1,082.0 and 1,231.1 keV. Spin-parity assignments have been made to some of the levels in¹⁴⁹Eu. Multipolarity assignments have been made for most of the electromagnetic transitions from the conversion coefficients obtained through the knowledge of ourγ-transition intensities and the published conversion-electron intensities. Based on the newγ-transitions observed in the singles and coincidence spectra, a revised level scheme has been proposed for¹⁴⁹Eu and compared with previously published level schemes. Radioactivity¹⁴⁹Gd; measuredT _1/2,T _γ,γγ coin, γγ(θ), I.C.C.,¹⁴⁹Eu deduced levels,J,γ-mixing,π. Enriched targets, Ge(Li) detectors.     

The level structure of the 153Gd nucleus studied in the 150Sm(α, n)153Gd reaction

The level structure of ¹⁵³Gd has been studied by means of the ¹⁵⁰Sm(α, n)¹⁵³Gd reaction. The experiment included measurements of γ-γ coincidences, γ-angular distributions, γ-ray yield at 17 MeV and 19 MeV beam energy, and γ-ray multiplicities. Favoured and unfavoured members of the positive-parity i_13,2, band were identified. States belonging to the h_9,2 and f_7,2 band structures have been located.Surprisingly low multiplicity numbers were deduced for ₁₅₃Gd γ-rays. This may indicate that the (α, n) reaction is not a pure compound reaction. The level structure of ¹⁵³Gd has been compared to the known structure of other odd-mass N = 89 nuclei, and a close similarity is found.The positive-parity band structure has been compared to calculations with the pairing-plus-recoil model. Good agreement is obtained without any ad hoc Coriolis attenuation.