High spin states in147Tb

The level scheme of¹⁴⁷Tb has been extended to 116 levels and 198 transitions in two experiments with the OSIRIS Compton suppressed detector array at the HMI Berlin with the reactions¹²²Sn(³¹P, 6n)¹⁴⁷Tb at 160 MeV and¹²⁰Sn(³¹P, 4n)¹⁴⁷Tb at 152 MeV. Evidence for a new high spin isomer atE=7664.1 keV with a life-time of the order of 2 ns has been found.     

Particle plus octupoleM2/E3 isomers and high-spin particle-hole states in147Tb and148Tb

The level structures of theN=82 andN=83 nuclei¹⁴⁷Tb and¹⁴⁸Tb have been studied by means of (α, 8n) and (α,7n) reactions induced by 68 to 110 MeVα particle bombardments of¹⁵¹Eu targets. In-beam conversion electron measurements have established that isomers withT _1/2=4.8(6)ns in¹⁴⁷Tb andT _1/2=22(1)ns in¹⁴⁸Tb decay byM2+E3 transitions to the ground states. The measuredB(E3) values show that the isomeric states arise from the coupling of the valence nucleon(s) to the¹⁴⁶Gd core octupole. Particlephonon coupling in these nuclei and in the one-neutron nucleus¹⁴⁷Gd is discussed and compared with well known cases involving the²⁰⁸Pb core. The higher lying yrast states in the two Tb nuclei are described as shell-model particle-hole excitations using empirical single particle energies and nucleon-nucleon interactions.     

Decay energies of the low-spin states of147Tb and148Tb

Using¹¹²Cd(⁴⁰Ar,pxn) reactions andγ-ray spectroscopy, the EC/β ⁺ and EC(K)/β ⁺ probability ratios were determined for individualβ-transitions in the¹⁴⁷Tb(1.6 h)→¹⁴⁷Gd and¹⁴⁸Tb(60 min)→¹⁴⁸Gd decays. Under assumption of applicability of theoretical ratios for allowedβ-decays on the first-forbidden nonunique transitions studied here, the experimental ratios were converted into information on decay energies. Combining the results with the known masses of^147,148Gd andQ _α values of neutron-deficient holmium-to-lutetium isotopes, mass excesses could be determined for¹⁴⁷Tb,¹⁴⁸Tb, low-spin¹⁵¹Ho, low-spin¹⁵²Ho,¹⁵⁵Tm,¹⁵⁶Tm and¹⁵⁹Lu.     

Precise atomic masses of147Eu,147Gd,and151Tb derived from their decay properties

Theβ-decay energies of¹⁴⁷Eu,¹⁴⁷Gd, and¹⁵¹Tb were determined by usingγ-spectroscopical methods. The comparison of experimental with calculatedK-capture probabilities yielded theQ _EC values 1.690( _?16 ⁺²¹ )MeV and 2.203( _?13 ⁺¹⁹ )MeV for¹⁴⁷Eu and¹⁴⁷Gd, respectively. By measuring the ratio of positron decay to electron capture for two branches in¹⁴⁷Eu decay, the decay energiesQ _EC=1.702(13) MeV andQ _EC=1.709(18)MeV were derived. Also fromEC/β ⁺ ratios the valuesQ _EC=2.225(75) MeV for¹⁴⁷Gd, andQ _EC=2.566(12)MeV for¹⁵¹Tb were obtained. Earlier discrepancies in the mass adjustment of these isotopes were removed. In course of the present studiesγ-decay properties of¹⁴⁷Eu and¹⁴⁷Gd were reinvestigated.     

Occupancy of single-proton orbitals in148Gd

The (³He,d) and (t, α) reactions on a radioactive Z=64¹⁴⁸Gd target were used to populate the single-proton states in¹⁴⁹Tb and¹⁴⁷Eu. In¹⁴⁹Tb the data establish the five single-proton states of the 51 to 82 major shell. The proton occupancies deduced from these experiments suggest that in the¹⁴⁸Gd ground state there are on average 1.8(3) proton pairs above the Z=64 shell gap.     

Atomic masses of147m, 148m, 149m Tb,148Dy,150m, 152m Ho derived from decay properties

Using nuclear fusion reactions of⁴⁰Ar ions with¹¹²Cd,¹¹⁴Sn and¹¹⁶Sn and subsequentγ-ray spectroscopy, the probability ratios of positron emission and electron capture,β ⁺/EC _k andβ ⁺/(EC+β ⁺), are determined for individualβ-transitions in the decay of^147m ,^148m ,^149m Tb,¹⁴⁸Dy and^150m ,^152m Ho. From comparison with theoretical ratios the followingQ _EC values, given in keV, are derived:^147m Tb, 4.620(60);^148m Tb, 5.730(30);^149m Tb, 3.610(50);¹⁴⁸Dy, 2.680(30);^150m Ho, 6.625(120) and^152m Ho, 6.470(80). The present decay-energy data are compared with earlier measurements and the new information obtained for the mass surface around¹⁴⁶Gd is discussed.     

Low-spin states of 64 147 Gd83 in the β-decay of 147gTb

Spectra of γ-rays, internal conversion electrons and γ?γ-coincidences in the β-decay of the isomeric 1/2⁺, 1.6 h, ¹⁴⁷Tb state are studied using semiconductor detectors. More than one hundred of new gamma-transitions are observed. Multipolarities of some gamma-transitions with energy up to 2MeV are established. The proposed decay scheme of ¹⁴⁷Tb, 1.6 h is discussed in framework of the shell model.     

Seniority-three yrast states in theN=82 nucleus147Tb

Firm spin-parity assignments for the high-spin states up to 3.5 MeV in the one-proton nucleus¹⁴⁷Tb were obtained from¹⁴⁴Sm(⁶Li, 3n) in-beamγ-ray and conversion electron measurements. The energies of these two-particle one-hole excitations were calculated from the shell model with empirical nucleon-nucleon interaction energies. The calculated energy splittings agree well with experiment, whereas the theoretical excitation energies disagree by ?1 MeV if recently measured ground state masses are used.     

High-spin levels in 147Tb

The high-spin states of ¹⁴⁷Tb have been studied with regard to their spins. The data were obtained by in-beam γ-ray spectroscopy using the reaction ¹²⁰Sn(³¹P,4n)¹⁴⁷Tb at 152 MeV performed at the Osiris spectrometer in Berlin. We obtained multipole mixing ratios for 60 transitions, and level spins up to 67/2ħ are introduced. Received: 30 March 1998     

Electromagnetic moments and nuclear charge radii for neutron-deficient Tb isotopes and the deformation jump nearZ=64,N=90

Optical isotope shifts and hyperfine structures of the^{147–153,155,157,159} Tb isotopes have been measured by the resonance ionization spectroscopy method. Nuclear moments and changes in nuclear charge radiiΔ 〈r ²〉 have been deduced. The “jump” inΔ 〈r ²〉 atN=88–90 has been revealed. It is compared with the relevant data for nuclei with other proton numbers.     

Applications of the total absorption <Emphasis Type="Italic">γ</Emphasis>-ray spectroscopy for <Emphasis Type="Italic">β</Emphasis>-decay study

Applications of total absorption γ-ray spectroscopy (TAS) for measurements of the beta-decay strength function, for completeness testing of decay schemes, and for determination of total beta-decay energy are discussed. Applications of TAS in combination with high-resolution γ spectroscopy for studying the fine structure of the beta-decay strength function are demonstrated. Results for ¹⁴⁷_gTb (T_1/2 ? 1.6 h) and for ¹⁵⁶Ho (T_1/2 ? 56 min) are presented.     

Gamow-Teller resonance in β+ decay of 147mDy and spin-isospin current renormalization

The total absorption spectrum of γ-rays following β⁺ decay of ^147mDy has been investigated. The decay energy Q_ε = 7.18 (10) MeV and an improved value of half-life $\text{T}{}_{\mathrm{<mtext>1</mtext><mtext>2</mtext>}}\text{= 55.7 (7)}\text{s}$ are determined. The intensity of the transitions from the isomeric state is 31 (3)%, the internal conversion being included. More than 40% of decays populate ¹⁴⁷Tb levels with the excitation energy E_ex ? 4.4 MeV. The β⁺ strength function S_β⁺ exhibits a pronounced narrow maximum at E_ex = 4.84 MeV and some structure at higher energy. The total probability of ^147mDy β⁺ decay corresponds to the value $\text{log}\text{?t = 3.67 (8)}$.The calculation of S_β carried out in the random-phase approximation gives the correct resonance energy. The coefficient of the spin-isospin current renormalization found from the comparison of the calculated β-decay probability with the experimental one is |;G_A/g_v|; = 0.7±0.1.     

Hydrothermal synthesis and luminescent properties of LnPO4:Tb,Bi (Ln=La,Gd) phosphors under UV/VUV excitation

Monoclinic LnPO₄:Tb,Bi (Ln=La,Gd) phosphors were prepared by hydrothermal reaction and their luminescent properties under ultraviolet (UV) and vacuum ultraviolet (VUV) excitation were investigated. LaPO₄:Tb,Bi phosphor and GdPO₄:Tb phosphor showed the strongest emission intensity under 254 and 147 nm excitation, respectively, because of the different energy transfer models. In UV region, Bi³⁺ absorbed most energy then transferred to Tb³⁺, but in VUV region it was the host which absorbed most energy and transferred to Tb³⁺.     

High spin states in148Tb

The level scheme of¹⁴⁸Tb has been extended to an excitation energyE _x =14.0 MeV and a spinI≈ 38? in two experiments with the OSIRIS Comptom suppressed detector array at the HMI Berlin using the reactions¹²²Sn(³¹P,5n)¹⁴⁸Tb at 160 MeV and¹²⁰Sn(³¹P,3n)¹⁴⁸Tb at 152 MeV.     

Energy transfer process in CaSO4:Tb,Ce phosphor

Thermoluminescence (TL) and photoluminescence studies have been carried out on CaSO₄:Tb, CaSO₄:Ce and CaSO₄:Tb,Ce phosphors with the aim of studying energy transfer process in the CaSO₄:Tb,Ce phosphor. CaSO₄:Tb,Ce shows TL peaks at 150, 220, 320 and 400°C. Changes in Tb and Ce concentrations influence the relative heights of these glow peaks. Co-doping with 0.1 mol% of Ce in CaSO₄:Tb enhances the sensitivity of 320^oC TL peak by a factor of 15. Fluorescence results show that there is energy transfer from Ce to Tb ion. The defect centres formed in CaSO₄:Tb,Ce phosphor are studied using electron spin resonance technique. The 320^oC glow peak correlates with a centre (SO₃⁻radical) with g-values: g_||=2.0061 and g_⊥=2.0026.     

The doubly-magic character of146Gd and its relation to208Pb

Recent experiments indicate the possibility of a doubly-magic character for the nucleus¹⁴⁶Gd (Z=64, N=82). In this work the results of a large-scale shell-model study on the nucleus¹⁴⁶Gd and its neighbouring nuclei¹⁴⁵Eu,¹⁴⁵Gd,¹⁴⁷Gd and¹⁴⁷Tb are presented. The configurations taken into account include up to 2p - 2h excitations for protons and/or neutrons. The calculated spectra and static moments are compared with the experimental data. Finally, the present results on shell closure in¹⁴⁶Gd are discussed in connection with those derived from a similar approach applied to the well-known doubly-magic nucleus²⁰⁸Pb.     

Der Zerfall des163Tb

The beta and gamma radiations of¹⁶³Tb have been investigated employing scintillation and semiconductor spectrometers and coincidence techniques. The sources were produced by the¹⁶³Dy(n,p)¹⁶³Tb reaction. A half-life of 19.5 min has been measured without evidence for an isomeric state in the half-life range of 2 sec to 7 d; especially a 6.5 h activity previously assigned to¹⁶³Tb could not be confirmed. 76 of the total of 82 gamma-ray transitions, representing 99.6% of the gamma-ray intensity, could be assigned to 23 levels in¹⁶³Dy. From beta and beta-gamma coincidence measurements aQβ-value of 1.7 ± 0.1 MeV has been determined. Spin and parity of 3/2⁺ are deduced for the ground state of¹⁶³Tb with the Nilsson configuration [411↑]. The level at 884 keV is interpreted as aJ ^π=1/2⁺ state with a high contribution of the three-quasiparticle configurationp[411↑]-p[523↑]-n[523↓] because of an allowed unhindered beta-ray transition to this level.     

Production of149gTb in deep inelastic transfer reactions: An approach to the angular momentum of fragments

The excitation functions for deep inelastic reactions in which two to six charges are transferred from⁴⁰Ar and⁶³Cu ions to rare earth targets have been measured using activation techniques, the observed radionuclides being^{150, 151}Dy and^149gTb. From the comparison of the curves relative to^149gTb and those relative to^{150, 151}Dy, it was deduced that the low spin isomer^149gTb was produced with significant probability for low incident energies. Using data from (heavy ions,xn) reactions, it was possible to attribute this production to the deexcitation of Tb fragments formed in deep inelastic transfers with angular momenta lower than 9?. This result is in good agreement with the angular momentum calculations performed under the hypothesis that the initial angular momentum window leading to deep inelastic reactions is situated between the critical angular momentum for fusion and that corresponding to grazing collisions. As far as Cu induced reactions are concerned, both hypothesis of rolling and sticking are consistent with the experimental data. For Ar induced reactions, the results indicate that the stage of sticking is not reached when the incident energy is lower than 200 MeV. Nuclear Reactions:^{142, 145}Nd,^{144, 148}Sm,¹⁵⁴Gd(Ar,X)^{151, 150}Dy,^149gTbE=160–280 MeV; measuredσ(E).¹⁴⁴Nd,¹⁴⁸Sm,¹⁵¹Eu,¹⁵⁴Gd(Cu, X)^{151, 150}Dy,^149gTb.E=280–420 MeV measuredσ(E). Enriched targets. Deduced angular momentum of Tb fragments.     

Study of high- lying states in 147Eu

The high-spin states of ¹⁴⁷Eu have been studied in the reaction ¹³⁹La(¹³C, 5n)¹⁴⁷Eu at a beam energy of 98 MeV. Based onthe in-beam measurements ofγ-γ-t coincidences and γ-ray angular distributions, the level scheme of ¹⁴⁷Eu has been extended from 4174 keVup to 8137 keV in excitation energies. A zeroth-order approximation of weak coupling model was applied to explain the observed level structure of ¹⁴⁷Eu.     

Negative-parity bands in the 88-neutron nuclei153Tb and155Ho

Bands of negative-parity levels have been observed in in-beam studies of¹⁵³Tb and¹⁵⁵Ho. The data are qualitatively accounted for in the rotation-alignment model as decoupled bands based on the h_11/2 proton orbital. Nuclear Reactions:¹⁵³Eu(α, 4nγ)¹⁵³Tb,E=45–55 MeV;¹⁵⁰Sm(¹⁰B, 5nγ)¹⁵⁵Ho,E=60–70 MeV; measuredE _γ,I _γ (0), γ ? γ coinc.,E _e, I _e ^K ,¹⁵³Tb and¹⁵⁵Ho deduced levels,J, π. Ge(Li) and Si(Li) detectors. Enriched targets.