Focusing effects in nonlinear resonant four-wave mixing (RFWM) MIR and FIR generation

Summary The influence of pump beam geometry in a NH₃ superradiant Raman FIR laser with RFWM generation of MIR emission has been analysed. We have observed that, in general, MIR radiation is emitted in a stimulated configuration, so pump and MIR beam overlap is basically important to exhibit an efficient RFWM. In particular, strong focusing, also in the presence of self-focusing, shows a lowering of the threshold of Raman FIR emission, as expected, plus a reduction of RFWM MIR emission. COMB-Arrich., CRE Frascati.     

Qualitative modification of the high energy atomic photoionization cross section

It is demonstrated that the nonrelativistic high energy omega-->infinity behavior of the photoionization cross section of an nl atomic subshell, sigma(nl)(omega), for l>0 is independent of l and is given by sigma(nl)(omega) approximately 1/omega(9/2), rather than the previously generally accepted sigma(nl)(omega) approximately 1/omega(l+7/2). Furthermore, for l = 1, although the exponent does not change, the coefficient is significantly altered. This modification of sigma(nl)(omega) is due to the interchannel interaction between ns photoionization channels and l not equal0 channels in the atom. As a result, for the photoionization of l not equal0 electrons, the single-particle approximation is never correct in the omega-->infinity limit. This has important consequences for sum rule calculations.     

2H(e,e(')p)n reaction at high recoil momenta

The 2H(e,e(')p)n cross section was measured in Hall A of the Thomas Jefferson National Accelerator Facility near the top of the quasielastic peak (x(Bj)=0.964) at a four-momentum transfer squared, Q(2)=0.665 (GeV/c) (2) (omega=0.368 GeV, W=2.057 GeV), and for recoil momenta up to 550 MeV/c. The measured cross section deviates by 1-2sigma from a state-of-the-art calculation at low recoil momenta. At high recoil momenta the cross section is well described by the same calculation; however, in this region, final-state interactions and interaction currents are predicted to be large, and alternative choices of nucleon-nucleon potential and nucleon current operator may result in significant spread in the calculations.     

Dynamical properties of the one-dimensional band insulator (NbSe4)3I

Optical and photoemission experiments reveal unexpected spectral signatures of one-dimensional band insulators. In the model compound (NbSe (4))3I the optical conductivity decays as a power law sigma(1)(omega) approximately omega(-4.25) above a sharp gap edge. Photoemission observes both the valence and a shadow band, produced by a commensurate superstructure. We identify an optical and photoemission band gap consistent with other measurements but much smaller than the energy scale defined by the dispersion of the band peak in the photoemission spectra.     

Transition behaviors in biased asymmetric quantum dot-in-double-well photodetector

A triple-band mid-/far-infrared (MIR/FIR) photodetector tunable by polarity is demonstrated by asymmetric quantum dot-in-double-well (DdWELL) structure that exhibits unique photoresponse (PR) transitions. In contrast to the MIR2 band with no dependence, the two MIR1/FIR PR bands are blue/red-shifted by the bias voltage, and the MIR2-FIR dual-band spectrum changes to a single-band feature due to the polarity. A four-level energy band model is proposed for the transition scheme, and the electric field dependence of the FIR band numerically calculated by a simplified DdWELL structure is in good agreement with the experimental PR spectra.     

Degenerate four-photon parametric interactions (DFPI) in optically pumped CH3F laser

Conclusion The results of the investigation make it possible to draw a conclusion that the DFPI processes do not influence significantly the spectral composition and the energy values of the output FIR emission in a superradiant CH₃F laser. They are determined in fact by the Raman processes. But anyway the DFPI processes are of great importance for the MIR emission generation and lead to the appearance of a large number of intensive MIR lines in the IR wavelength range.     

Performance improvements of ultraviolet/infrared dual-band detectors

Results are reported on dual-band detectors based on a GaN/AlGaN structure operating in both the ultraviolet–midinfrared (UV–MIR) and ultraviolet–farinfrared (UV–FIR) regions. The UV detection is due to an interband process, while the MIR/FIR detection is from free carrier absorption in the emitter/contact followed by internal photoemission over the barrier at the GaN/AlGaN interface. The UV detection, which was observed from 300 K to 4.2 K, has a threshold of 360 nm with a peak responsivity of 0.6 mA/W at 300 K. The detector shows a free carrier IR response in the 3–7 μm range up to 120 K, and an impurity response around 54 μm up to 30 K. A response in the range 7–13 μm, which is tentatively assigned to transitions from C impurities and N vacancies in the barrier region, was also observed. It should also be possible to develop a detector operating in the UV–visible–IR regions by choosing the appropriate material system. A dual-band detector design, which allows not only to measure the two components of the photocurrent generated by UV and IR radiation simultaneously but also to optimize the UV and IR responses independently, is proposed.     

Two-electron linear intersubband light absorption in a biased quantum well

We point out a novel manifestation of many-body correlations in the linear optical response of electrons confined in a quantum well. Namely, we demonstrate that along with the conventional absorption peak at a frequency omega close to the intersubband energy delta, there exists an additional peak at frequency h omega approximately = 2delta. This new peak is solely due to electron-electron interactions, and can be understood as excitation of two electrons by a single photon. The actual peak line shape is comprised of a sharp feature, due to excitation of pairs of intersubband plasmons, on top of a broader band due to absorption by two single-particle excitations. The two-plasmon contribution allows us to infer intersubband plasmon dispersion from linear absorption experiments.     

Infrared detection and photon energy up-conversion in graphene layer infrared photodetectors integrated with LEDs based on van der Waals heterostructures: Concept,device model,and characteristics

We propose the concept of the infrared detection and photon energy up-conversion in the devices using the integration of the graphene layer infrared detectors (GLIPs) and the light emitting diodes (LEDs) based on van der Waals (vdW) heterostructures. Using the developed device model of the GLIP-LEDs, we calculate their characteristics. The GLIP-LED devices can operate as the detectors of far- and mid infrared radiation (FIR and MIR) with an electrical output or with near-infrared radiation (NIR) or visible radiation (VIR) output. In the latter case, GLIP-LED devices function as the photon energy up-converters of FIR and MIR to NIR or VIR. The operation of GLIP-LED devices is associated with the injection of the electron photocurrent produced due to the interband absorption of the FIR/MIR photons in the GLIP part into the LED emitting NIR/VIR photons. We calculate the GLIP-LED responsivity and up-conversion efficiency as functions the structure parameters and the energies of the incident FIR/MIR photons and the output NIR/VIR photons. The advantages of the GLs in the vdW heterostructures (relatively high photoexcitation rate from and low capture efficiency into GLs) combined with the reabsorption of a fraction of the NIR/FIR photon flux in the GLIP (which can enable an effective photonic feedback) result in the elevated GLIP-LED device responsivity and up-conversion efficiency. The positive optical feedback from the LED section of the device lead to increasing current injection enabling the appearance of the S-type current-voltage characteristic with a greatly enhanced responsivity near the switching point and current filamentation.     

Measurements of the complex conductivity of NbxSi(1-x) alloys on the insulating side of the metal-insulator transition

We have conducted temperature and frequency dependent transport measurements in amorphous NbxSi1-x samples in the insulating regime. We find a temperature dependent dc conductivity consistent with variable range hopping in a Coulomb glass. The frequency dependent response in the millimeter-wave frequency range can be described by the expression sigma(omega) varies with (-iota omega)(alpha) with the exponent somewhat smaller than 1. Our ac results are not consistent with extant theories for the hopping transport.     

Frequency-dependent thermal response of the charge system and the restricted sum rules of La2-xSrxCuO4

In La2-xSrxCuO4 (LSCO) the spectral weight W=integralOmega0sigma(ab)1(omega,T)domega [where sigma(ab)1(omega,T) is the ab-plane conductivity] obeys the same law W=W0-BOmegaT2 as in a conventional metal such as gold, for any Omega up to the plasma edge. However, in LSCO BOmega points toward correlation effects and, unlike in gold, is related to an energy scale tT相似文献   

Transverse Josephson plasma mode in T* phase SmLa(1-x)Sr(x)CuO(4-delta) single crystals

Far-infrared reflectivity along the c axis in T* phase SmLa(1-x)Sr(x)CuO(4-delta) single crystals is measured down to 8 cm(-1). Below T(c), the conductivity peak is observed at 25 cm(-1) for x = 0.15 ( T(c) = 30 K) along with two reflectivity edges at 13 and 27 cm(-1). The conductivity peak is attributed to the transverse Josephson plasma mode between two longitudinal Josephson plasma modes, while the oscillator strength of the peak is found to be smaller than that calculated using the Josephson-coupled multilayer model. The difference is explained by assuming that only a few junctions at the disordered (La,Sr)(2)O(2-delta) block layer take part in the plasma oscillation with omega(pI(')) = 27 cm(-1).     

Low-temperature relaxation in spin glasses

We analyze the mechanism governing the long-time, low-temperature relaxation of the thermoremanent magnetization (σ_TRM) in metallic spin glasses. Ideas of quantum tunneling and “screening” of the local magnetic moments are employed to explain the existence of a hierarchy of relaxation times. This results in a time decay which is described by anenhanced power law: $$\sigma _{TRM} = \sigma _0 \exp - A[\ln (\omega t)]^y = \sigma _0 (\omega t)^{ - A[\ln (\omega t)]y - 1} $$ withy≧1. A crossover is predicted below which most parameters become temperature-independent.     

Electronic transitions on UHV-cleaved Si (111) adsorbed with oxygen

The electron energy loss spectra have been measured of oxygen-adsorbed Si (111) surfaces at the primary energies of 10–200 eV. The observed peaks are at the loss energies of 2.9, 3.6, 4.8, 5.7, 6.9, 8.2, 9.6, 12.0, and 13.0 eV. All the peaks are attributed to the one-electronic transitions related to the adsorbed oxygen, except for the 9.6 eV peak which could possibly be due to the relaxed surface plasmon excitation. It is shown that the “splitting” of surface plasmon reported by Ibach and Rowe does not exist.     

Nonlinear excitation of surface plasmon polaritons by four-wave mixing

We demonstrate nonlinear excitation of surface plasmons on a gold film by optical four-wave mixing. Two excitation beams of frequencies omega(1) and omega(2) are used in a modified Kretschmann configuration to induce a nonlinear polarization at a frequency of omega(4wm)=2omega(1)-omega(2), which gives rise to surface plasmon excitation at a frequency of omega(4wm). We observe a characteristic plasmon dip at the Kretschmann angle and explain its origin in terms of destructive interference. Despite a nonvanishing bulk response, surface plasmon excitation by four-wave mixing is dominated by a nonlinear surface polarization. To interpret and validate our results, we provide a comparison with second-harmonic generation.     

Observation of self-similar behavior of the 3D, nonlinear Rayleigh-Taylor instability

The Rayleigh-Taylor unstable growth of laser-seeded, 3D broadband perturbations was experimentally measured in the laser-accelerated, planar plastic foils. The first experimental observation showing the self-similar behavior of the bubble size and amplitude distributions under ablative conditions is presented. In the nonlinear regime, the modulation sigma(rms) grows as alpha(sigma)gt(2), where g is the foil acceleration, t is the time, and alpha(sigma) is constant. The number of bubbles evolves as N(t) alpha(omegat sq.rt(9) + C)(-4) and the average size evolves as (t) alpha omega(2)gt(2), where C is a constant and omega = 0.83 +/- 0.1 is the measured scaled bubble-merging rate.     

ab plane ac conductivity in the cuprates: pseudogap effects below Tc

Building on our understanding of the superfluid density rho(s)(T), we show how the pseudogap enters the in-plane optical conductivity sigma(omega,T) for temperatures T相似文献   

Theory of inelastic scattering from magnetic impurities

We use the numerical renormalization group method to calculate the single-particle matrix elements T of the many-body T matrix of the conduction electrons scattered by a magnetic impurity at T=0 temperature. Since T determines both the total and the elastic, spin-diagonal scattering cross sections, we are able to compute the full energy, spin, and magnetic field dependence of the inelastic scattering cross section sigma(inel)(omega). We find an almost linear frequency dependence of sigma(inel)(omega) below the Kondo temperature T(K), which crosses over to a omega(2) behavior only at extremely low energies. Our method can be generalized to other quantum impurity models.     

Interference effect in combined elastic and inelastic scattering of an energetic electron reflected from a disordered medium with generation of a surface plasmon

Quantum interference in combined elastic and inelastic scattering of an energetic electron with excitation of a surface plasmon leads to a change in the shape of the corresponding peak in the electron-energyloss spectrum. The plasmon generation is suppressed near the frequency \({{\omega _p } \mathord{\left/ {\vphantom {{\omega _p } {\sqrt 2 }}} \right. \kern-\nulldelimiterspace} {\sqrt 2 }}\). The suppression increases with increasing surface-plasmon wave length, because the interference of the energetic-electron scattering processes differing in the sequential order of elastic and inelastic scattering becomes progressively more destructive. The decrease in the height of the surface-plasmon peak in the electron-energy-loss spectrum leads to a non-dissipative broadening in this peak. Quantum interference also causes a specific feature to occur in the azimuthangle dependence of the spectral intensity as the electron energy loss increases in the immediate vicinity of the surface-plasmon peak.     

Classical properties of low-dimensional conductors: giant capacitance and non-ohmic potential drop

The electrical field arising around an inhomogeneous conductor when an electrical current passes through it is not screened, as distinct from 3D conductors, in low-dimensional conductors. As a result, the electrical field depends on the global distribution of the conductivity sigma(x) rather than on the local value of it, inhomogeneities of sigma(x) produce giant capacitances C(omega) that show frequency dependence at relatively low omega, and electrical fields develop in vast regions around the inhomogeneities of sigma(x). A theory of these phenomena is presented for 2D conductors.