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 共查询到17条相似文献,搜索用时 93 毫秒
1.
采用位置灵敏探测和散射离子 反冲离子飞行时间技术测量了强相互作用区F2 + 和F3 + 离子与Ne原子碰撞中的转移电离截面与单电子俘获截面之比 .与Fq+ He实验结果进行了比较 ,并进行了定性讨论. The ratios of the cross-section of the transfer ionization to the single electron capture of Neon induced by F 2+ and F 3+ ions are measured by means of the time-of-flight technologie. In the present energy range, the transfer ionization C1I1 of neon can be considered as a two-step process, in which one electron is captured by projectile and another one is directly ionized, and the transfer ionization C1I2 process should be considered as a subsequent rearrangement of neon following...  相似文献   

2.
介绍了对于Na+ 离子和Rb(5s ,5p)原子碰撞中态选择单电子俘获微分截面的理论计算,并与实验数据进行比较,实验结果是离子与在磁光学阱中用激光冷却的碱金属靶原子碰撞而测量到的;还对高能量质子引起的He原子的转移电离进行了理论研究,在Shakeoff模型的基础上 ,分析解释了转移电离截面与单电子俘获截面的比值 ,并与最新实验结果作了比较. We report a theoretical study of state-selective differential single-electron capture cross sections between Na + and Rb(5s, 5p) atoms. The experimental data have been obtained with laser cooled target in a magnetic optical trap. We also report a theoretical study of transfer ionization of He by protons at high collision energies and analyze the transfer ionization cross section with respect to single electron capture cross section in terms of a shakeoff model.  相似文献   

3.
In this paper a projectile ions recoil ions coincidence technique is employed to investigate the target ionization and projectile charge state changing processes in the collision of 0.22-6.35 MeV Cq^+ (q = 1 - 4) ions with argon atoms. The partial cross section ratios of the double, triple, quadruplicate ionization to the single ionization (or the single capture) of argon associated with single electron loss (or single electron capture) by the projectile are measured and compared with the previous experimental results. In the present experiment, it is observed that the ratios of ionization cross sections R associated with single loss and single capture depend strongly on the projectile charge state and vary significantly with different reaction channels as impact energy increases. In addition, this paper gets empirical scaling laws for the ionization cross section ratios R corresponding to the projectile single loss and finds that the ratios of the double ionization to the single ionization associated with single electron capture remain constant in the present energy range.  相似文献   

4.
主要揭示了不同电离机制对高电荷态离子单电离和多重电离的贡献 ,包括直接电离 (一步过程 )、激发 自电离 (两步过程 )以及内壳Auger过程 ,研究了高电荷态镨离子的电子碰撞电离. Electron-impact ionization of ions is one of the most fundamental processes in every kind of plasma. Especially in high-temperature plasmas-whether in laboratory (nuclear fusion) or in astrophysics (atmosphere of stars)-atoms become ionized into multiply-charged ions by electron impact. The main purpose of our investigations is to unravel the contributions from different ionization mechanisms-like direct ionization (one-step process), excitation-autoionization (two-step process) and...  相似文献   

5.
在Monte Carlo方法模拟keV电子碰撞薄膜/厚衬底靶过程中,输入材料数据中采用的内壳层电离截面数据不同,得到的反映膜厚及村底对电离截面测量结果影响的修正因子值也有差别。讨论了Monte Carlo模拟得到的修正因子值受输入材料数据中内壳层电离截面影响的程度,并完成了入射keV电子在法拉第筒中逃逸率的估算工作。 The sensitivity of the correction factor, which describes the combined effect of finite film thickness and the thick substrate in the measurement of atomic inner-shell ionization cross-sections by low-energy electron impact, to the adopted ionization cross-sections in the Monte Carlo simulation is discussed. Moreover, the electron escape ratio from the Faraday cup in our experiment is also obtained by Monte Carlo method.  相似文献   

6.
王菲  芶秉聪 《中国物理 B》2008,17(4):1227-1230
This paper uses the two-centre atomic orbital close-coupling method to study the ionization and the single electron capture in collision of highly charged Ar^16+ ions with He atoms in the velocity range of 1.2-1.9 a.u.. The relative importance of single ionization (SI) to single capture (SC) is explored. The comparison between the calculation and experimental data shows that the SI/SC cross section ratios from this work are in good agreement with experimental data. The total single electron ionization cross sections and the total single electron capture cross sections are also given for this collision. The investigation of the partial electron capture cross section shows a general tendency of capture to larger n and l with increasing velocity from 1.2 to 1.9 a.u..  相似文献   

7.
在ECPSSR理论的基础上, 利用OBKN近似描述电子俘获过程, 得到了包括电子俘获过程贡献的ECPSSR理论, 编写了相应的计算程序。 采用该程序计算了不同电荷态离子与多种靶原子碰撞的电子俘获截面和相应的X 射线产生截面, 将计算得到的包含电子俘获过程贡献的X 射线产生截面与实验结果进行了比较。 对于具有满K壳层的入射离子碰撞, X 射线产生截面与入射离子电荷态基本无关; 对于以直接电离为主导的碰撞过程, 计算得到的X 射线产生截面与实验数据符合得很好; 对于全裸和单K空穴入射离子的碰撞, 计算高估了X 射线产生截面。 Based on the ECPSSR theory, the contribution of the electron capture is described by the OBKN theory. The cross sections of electron capture and X ray production for the collision of different charge state projectiles with various targets are calculated, and compared with the available experimental data. It is found that the obtained X ray production cross sections are almost independent of the projectile charge states for projectiles without a K vacancy. For the collision processes of direct ionization, the present calculated results agree well with the experimental data. The calculations overestimate the X ray production cross sections for the projectiles with full and a K vacancy.  相似文献   

8.
The study of multi-electron process has been a very active area of atomic physics research. The simultaneous electron emission and electron transfer is one of the most interesting two-electron processes in the study Of ionatom collisions, In last decade much experimental and theoretical attention has been devoted to the process, named transfer ionization (TI). This process is normally considered as the successive process of the single electron capture and the ionization of the second or more target electrons. The studies of transfer ionization are motivated by the understanding of the role of the electron correlation in ion-atom collisions which is of great interest in basic atomic physics and may provide important information for the applications both in astrophysics and fusion plasmas researches. Different authors have investigated the transfer ionization process by measuring the angular distribution of the emitted electrons. Up to now, the systematic study of the transfer ionization and the dependences of these processes on the collision parameters for the low energy ion-atom collisions are still rarely reported in the literatures.  相似文献   

9.
Strong-field tunneling ionization is the first step for a broad class of phenomena in intense laser-atom/molecule interactions. Accurate information about the electron wave packet from strong-field tunneling ionization of atoms and molecules is of essential importance for understanding various tunneling ionization triggered processes. Here, we survey the property of the electron wave packet in tunneling ionization of molecules with a method based on strong-field photoelectron holography. By solving the time-dependent Schr ¨odinger equation, it is shown that the holographic interference in the photoelectron momentum distribution exhibits the asymmetric behavior with respect to the laser polarization direction, when the molecule is aligned with a nonzero angle to the linearly polarized laser field. We demonstrate that this asymmetry is due to the nonzero initial transverse displacement of the electron wave packet at tunneling. By analyzing the holographic interference, this transverse displacement for the launching of electron wave packet tunneling from the molecules is accurately retrieved. This displacement is directly related to the electron density distribution in molecules, and thus our work developed a novel concept for probing electronic structure in molecules.  相似文献   

10.
Photoelectron momentum distribution in strong-field ionization has a variety of structures that reveal the complicated dynamics of this process. Recently, we identified a low-energy interference structure in the case of a super-intense extreme ultraviolet(XUV) laser pulse and attributed it to the laser-induced electron Fresnel diffraction. This structure is determined by the laser-induced electron displacement [Geng et al. Phys. Rev. A104(2021) L021102]. In the present work, we find that the Fre...  相似文献   

11.
采用位置灵敏探测和散射离子-反冲离子飞行时间测量技术,测量了氧离子与氖和氦原子碰撞过程中转移电离截面与单电子俘获截面之比.通过比较发现测量结果与文献结果的趋势一致,并对测量结果进行了讨论.  相似文献   

12.
介绍了使用位置灵敏技术和飞行时间方法研究中低能低电荷态离子-原子碰撞过程中转移电离与单电子俘获过程.对于确定的入射离子电荷态,通过理论分析及与实验数据对比给出了转移电离与单电子俘获截面比RTS随着入射离子速度VP的变化规律和转移电离过程中电离的电子主要来自靶原子的最外亚壳层. 关键词: 转移电离 逃离半径 电离半径 俘获半径  相似文献   

13.
The most common secondary-ionization mechanism in positive ion matrix-assisted laser desorption/ionization (MALDI) involves a proton transfer reaction to ionize the analyte. Peptides and proteins are molecules that have basic (and acidic) sites that make them susceptible to proton transfer. However, non-polar, aprotic compounds that lack basic sites are more difficult to protonate, and creating charged forms of this type of analyte can pose a problem when conventional MALDI matrices are employed. In this case, forming a radical molecular ion through electron transfer is a viable alternative, and certain matrices may facilitate the process. In this work, we investigate the performance of a newly developed electron-transfer secondary reaction matrix: 9,10-diphenylanthracene (9,10-DPA). The use of 9,10-DPA as matrix for MALDI analysis has been tested using several model compounds. It appears to promote ionization through electron transfer in a highly efficient manner as compared to other potential matrices. Thermodynamic aspects of the observed electron transfers in secondary-ionization reactions were also considered, as was the possibility for kinetically controlled/endothermic, electron-transfer reactions in the MALDI plume. Copyright ? 2012 John Wiley & Sons, Ltd.  相似文献   

14.
Summary The fluid theory is applied to study the axisymmetrical steady-state magnetically confined electron clouds sustained by ionization or emission. These electron clouds can be obtained by means of low-pressure Penning discharge, thermoelectronic emission, ion beam ionization, etc. In the electron clouds the property of motion of electrons can be described by the fluid equations: the continuity equation, the momentum equation, the energy equation, the heat transfer equation and the electrostatic field equation. These equations are used to discuss the equilibrium between supplement and escape of electrons in the clouds and the distributions of the physical quantities of some long electron clouds. The authors of this paper have agreed to not receive the proofs for correction. The work is supported by National Natural Science Foundation of China.  相似文献   

15.
The shakeoff theory of Aberg [Phys. Rev. A 2, 1726 (1970)] is revisited. With the sudden approximation, we calculate the shakeoff probability when one of the electrons in He is ejected with a finite velocity. This theory is used to examine ratios of cross sections for double to single photoionization and transfer ionization to single electron capture. It is also shown that the momentum distribution of the shakeoff electron provides a means to measure the correlation of the ground state wave function directly.  相似文献   

16.
The ratios of the multiple ionization cross-section to those of the single ionization of neon are measured for 2.0-8.0 MeV and ( q = 2-5) ions bombardment. By means of the coincidence beween the charge state-selected scattered projectiles and recoil ions the contribution of the electron capture is separated from the total multiple ionization. A theoretical method is proposed to exclude the Auger transitions from the considered multiple ionization processes in the present work. The (q / v) dependence of the obtained ratios of the “pure” direct multiple ionization to those of the single ionization is discussed. The electronic structure dependence of the electron transition occurring in ion-neon collisions is studied and discussed for the symmetrical collision systems - and -. Received: 4 June 1998 / Received in final form: 24 August 1998  相似文献   

17.
吕瑛  陈熙萌  曹柱荣  吴卫东 《物理学报》2010,59(6):3892-3896
基于入射离子双俘获后势能沉积与双电离靶离子势能的比值定义了势能参数Ω,研究了低能高电荷态离子(q=4,5,6,7)与He原子碰撞系统中双俘获和转移电离反应道的选择规律.研究发现,在Ω坐标下,双俘获和转移电离存在截面反转效应,Ω1.0时双俘获为双电子转移过程主反应道,Ω≥1.0时转移电离成为双电子转移过程主反应道.  相似文献   

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