Further Study of A-Related Quantum Interference of П-State Diatomic on Collision-Induced Rotational Energy Transfer

In our previous theoretical studies [Meng-Tao Sun, Yong-Qing Lee, and Feng-Cai Ma, Chem. Phys.Lett. 371 (2003) 342], we have reported the quantum interference on collision-induced rotational energy transfer on CO (A1П, v = 3) with inert gases, which originates from the difference between the two A-related collision potential energy surfaces. The interference angle, which measures the degree of coherence, is presented in this paper. Based on the time-dependent first order Born approximation, taking into account the anisotropic Lennard-Jones interaction potentials, the relation of the interference angle with the factors, including experimental temperature, partner, and rotational quantum number, are obtained. The changing tendencies with them are discussed. This theoretical model is important to understanding and performing this kind of experiment.     

The differential interference angle in collisional quantum interference on rotational energy transfer

Collisional quantum interference （CQI） in the intramolecular rotational energy transfer was observed in experiment by Sha and co-workers. The interference angle, which measuring the degree of the coherence, were measured in the experiment of the static cell. Based on the first Born approximation of time dependent perturbation theory, taking into accounts the anisotropic Lennard-Jones interaction potentials, this paper describes the theoretical model of CQI in intramolecular rotational energy transfer in an atom-diatom collision system. In the model, the differential interference angle for the experiment of the molecular beam is calculated, the changing tendencies of the differential interference angle with the impact parameter and collision partners are obtained. This theoretical model is important for understanding or performing this kind of experiments.     

Relationship Between Differential Interference Angle and Parameter of Experiment in Molecular Beam

Collisional quantum interference （CQI） was observed in the intramolecular rotational energy transfer in the experiment of the static cell, and the integral interference angles were measured. To observe more precise information, the experiment in the molecular beam should be taken,from which the relationship between the differential interference angle and the scattering angle can be obtained. In this paper, the theoretical model of CQI is described in an atom-diatom system in the condition of the molecular beam, based on the first-Born approximation of time-dependent perturbation theory, taking into accounts the long-range interaction potential. The method of observing and measuring correctly the differential interference angle is presented. The changing tendency of the differential interference angle with the impact parameter and relative velocity is discussed. The changing tendencies of the differential interference angle with the parameter of experiment in the molecular beam, including the impact parameter and the velocity are discussed. This theoretical model is important to understand or perform the experiment in the molecular beam.     

Collisional quantum interference on rotational energy transfer： physical interpretation of the differential interference angle

Collisional quantum interference （CQI） on the intramolecular rotational energy transfer is observed in an experiment with a static cell, and the integral interference angles are measured. To obtain more accurate information, an experiment with a molecular beam is carried out, and thereby the relationship between the differential interference angle and the scattering angle is obtained. Based on the first-Born approximation of time-dependent perturbation theory, the theoretical model of CQI is developed in an atom-diatom system in the condition of the molecular beam, with the long-range interaction potential taken into account. The method of measuring correctly the differential interference angle is presented. The tendencies of the differential interference angle changing with the impact parameter and rel- ative velocity are discussed. The theoretical model presented here is important for understanding or performing the experiment in the molecular beam.     

The differential interference angle of ^2∏[Case（a）] diatom on rotational energy transfer in NO（X^2∏） collision with He,Ne and Ar system

To study theoretically the relationship between the differential interference angle and the scattering angle in collisional quantum interference （CQI）, we have investigated the differential interference angle of the atom-diatomic [case（a）] molecule system in detail. For the 2∏ electronic state in Hund＇s case （a）, the degree of the differential interference is also discussed. The differential interference angles of NO（X^2∏） are calculated quantitatively for the rotational energy transfer in Hund＇s case （a） induced by collision with He, Ne and Ar atoms. The method to calculate the differential interference angle is presented. Several factors that affect the differential interference angle are investigated. Finally the variation of the differential interference angle with the impact parameter and relative velocity is discussed.     

Interference Angle on Quantum Rotational Energy Transfer in Na＋Na2 （A1 ∑u^＋,v=8-b^3∏0u,v=14） Molecular Collision System

In order to study the collisional quantum interference （CQI） on rotational energy transfer in atom-diatom system, we have studied the relation of the integral interference angle and differential interference angle in Naq-Na2 （A1 ∑u^＋,v=8-b^3∏0u,v=14） collision system. In this paper, based on the first-Born approximation of timedependent perturbation theory and taking into accounts the anisotropic effect of Lennard-Jones interaction potentials, we present a theoretical model of collisional quantum interference in intramolecular rotational energy transfer, and a relationship between differential and integral interference angles.     

Collisional Quantum Interference on Rotational Energy Transfer： Relation Between Integral Interference Angle and Rotational Quantum Number in Na2（A^1∑u^＋,ν=8～b^3∏0u,ν=14）-Na System

Collisional quantum interference （CQI） on rotational energy transfer was observed in Na2（A^1∑u^＋,ν=8～b^3∏0u,ν=14） system in collision with Na [Chem. Phys. Lett. 318 （2000） 107], and the degree of the interference was measured. The integral interference angle was obtaJned through theoretical calculation. We will research the factors that have effect on collisional quantum interference on rotational energy transfer in Na2（A^1∑u^＋,ν=8～b^3∏0u,ν=14）-Na system. Basing on the time-dependent first order Born approximation, and taking into account the anlsotroplc Lennard Jones interaction potentials and ＂straight-line＂ trajectory approximation, we obtain the factors that have effect on CQI in Na2-Na system, and obtain the relation between the integral interference angle and rotational quantum number.     

Surface Corrugation in Rotational and Diffractive Scattering of O2 from LiF （001）

A quantum dynamic calculation on a five-dimensional O2/LiF （001） model system is performed using the multi-configuration time-dependent Hartree method. The obtained results show that the mechanism of rotational and diffractive excitation in details： Comparison with the rotational excited state, the initially non-rotational state is seen to favor the inelastic scattering in the rotational excitation process. The surface corrugation can damp the quantum interferences and produce a greater amount of rotational inelastic scattering at the expense of the elastic process in the rotational excitation process. The diffraction process and the average energy transferred into the rotational and diffractive mode are also discussed.     

A b initio calculation of the growth of Te nanorods and Bi2Te3 nanoplatelets

In this paper the growth mechanism of a Te/Bi2Te3 novel structure is studied by ab-initio calculations. The results show that the growth of Te nanorods is determined by the adsorption energy of Te atoms on different crystalline Te surfaces. The adsorption energy of Te on the Te （001） surface is 3.29 eV, which is about 0.25 eV higher than that of Te on the Te （110）. This energy difference makes the preferential growth direction along the 〈 001 〉 direction. In addition, the higher surface energy of Bi2Te3 （110） and the lattice misfit between crystalline Bi2We3 and Te along 〈 001 〉 direction are considered to explain the growth of the Bi2Te3 nanoplatelets, in which Volmer-Weber model is used. The theoretical results are in agreement with experimental observation.     

Ionization Potentials and Quantum Defects of ls^2np^2p Rydberg States of Lithium Atom

Abstract In this work, ionization potentials and quantum effects of ls^2 np^2 P Rydberg states of lithium are calculated based on the calibrated quantum defect function. Energy levels and quantum defects for ls^2np^2P bound states and their adjacent continuum states are calculated with the R-matrix theory, and then the quantum defect function of the ls^2np （n ≥ 7） channel is obtained, which varies smoothly with the energy based on the quantum defect theory. The accurate quantum defect of the ls^2 7p^2P state derived from the experimental data is used to calibrate the original quantum defect function. The new function is used to calculate ionization potentials and quantum effects of ls^2np ^2P （n ≥ 7） Rydberg states. Present calculations are in agreement with recent experimental data in whole.     

光的干涉衍射综合实验仪

根据传统的光的干涉衍射实验装置存在的不足,研制出了光的干涉衍射综合实验仪．将光学元件放置在同一小型光学平台上,按照实验需要组合成相应仪器．该实验仪既可以用于光学演示实验,也可以作为光学专用的实验仪器。     

磁致伸缩系数的测量

为了避免非平衡电桥法测量磁致伸缩系数出现的漂移现象，本文提出了一种用光学干涉法间接测量磁致伸缩系数的实验方法。     

转动传能量子干涉效应:干涉角影响因素的研究

碰撞转动传能中存在量子干涉效应已经在静态池实验中被观测到,并且积分角也能被测量.利用分子束实验可得到转动传能更准确的信息,进而得到影响干涉角的的具体因素.文中利用一阶含时波恩近似和L-J相互作用势,建立了原子—双原子分子碰撞系统转动传能的量子干涉模型,描述了观察和测量微分干涉角的方法,得到了微分干涉角与碰撞半径和碰撞速度间的关系,同时也得到了积分干涉角和实验温度的关系.此理论模型对于理解和进行分子束实验是非常重要的.     

光场空间相干性的测量方法及比较

本文归纳了基于分波前干涉原理的具有代表性的干涉测量方法——杨氏双孔干涉法、逆波前杨氏干涉法和非冗余孔径阵列干涉测量法,以及基于分振幅干涉原理的干涉测量方法——自参考干涉测量法;介绍了各种测量方法的工作原理、实验配置;比较了4种测量方法的优缺点,并给出每种方法的最佳应用领域。本文结论可为根据对空间相干性测量的不同要求,选择合适的测量方法提供初步参考。     

多光束法布里-珀罗干涉实验的计算机模拟简

用计算机数值计算的方法,模拟了法布里-珀罗多光束干涉实验的光强分布,并与双光束等倾干涉条纹进行了比较,分析了薄膜反射率对法布里-珀罗干涉实验的波长分辨率影响。     

High sensitivity micro-displacement homodyne interferometry北大核心CSCD

Interferometry is widely used in nano-scale micro-topography measurement. In order to improve its accuracy and sensitivity, a high-sensitivity homodyne interferometry based on white light interference and laser secondary interference was proposed. A high-sensitivity homodyne interferometry system was designed, and the zero point of the laser secondary interference was used to locate the dark striation of white light interference, so that it could reach the maximum slope when optical path difference was zero. The signals of white light and laser were analyzed by using the wave principle and intensity formula of interference fringes, and a sensitivity calculation method based on the combination of white light and laser interference signal was proposed. The system and its sensitivity were simulated. Finally, the optical path was built, and the white light interference fringes were adjusted to the dark striations position, so as to locate the zero position of laser secondary interference and carry out the data acquisition. It is showed that the sensitivity of the measurement method is at least 1 832 times higher than that of the laser secondary interference, and the corresponding measurement uncertainty is only ±0.288 7 mV. The measurement system can effectively solve the problem of large amount of calculation in traditional interferometry, and has high sensitivity, stability and reliability. Copyright ©2022 Journal of Applied Optics. All rights reserved.     

基于点光源的迈克耳孙干涉实验条纹的机理分析

一般国内的大学物理和大学物理实验教材都只介绍干涉圆条纹和直线干涉条纹,用迈克耳孙干涉仪可以调制出椭圆和双曲线干涉条纹;但对条纹形成的理论推导很少涉及．本文根据点光源双光束干涉理论,分析基于点光源照明的迈克耳孙干涉实验中所产生的各种可能的干涉条纹：双曲线形干涉条纹、圆形干涉纹、椭圆形干涉纹及直线形干涉纹的形成条件．本文也对等倾干涉条纹、等厚干涉条纹与既非等倾也非等厚干涉条纹的机理进行分析和比较．通过对每一种干涉图样的解析分析和比较,旨在对迈克耳孙干涉实验有更全面和更深刻的了解．     

白光频谱干涉原理及其应用

本文详细讨论了白光频谱干涉的基本原理及其在微位移测量中的应用,并将其与传统白光干涉以及时域迈克尔逊干涉进行了比较,探讨了白光频谱干涉在大学物理理论与实验教学中的重要应用前景。     

多模液芯光纤干涉的实验研究

本文介绍了多模液芯光纤干涉的一些性质,干涉条纹的最大可见度条件.给出了干涉传感的二种测量结果.     

信息光学视角下菲涅耳双棱镜干涉的研究

菲涅耳双棱镜干涉在相衬成像和全息显微术中有重要应用。为了促进其应用,本文从信息光学角度研究双棱镜干涉,首先利用光场与脉冲响应函数之间的关系,理论导出了菲涅耳双棱镜干涉条纹强度公式,分析并讨论了狭缝缝宽及狭缝到双棱镜距离对菲涅耳双棱镜干涉条纹的影响,狭缝宽度大于0. 1 mm时,干涉条纹分辨率变差。接着给出了改变狭缝宽度(变化量为0. 08 mm)和改变狭缝到双棱镜的距离(从8 cm变化到12 cm)的实验结果,理论分析和实验结果一致。该结果有助于促进菲涅耳双棱镜干涉在相衬成像等领域的应用。