Antimagnons in ferrimagnets

Purely antiferromagnetic intrinsic oscillations of magnetic ions in a tetragonal ferrimagnet are considered. The magnetic ions occupy two double positions (forming four magnetic sublattices) so that the center of symmetry for each position is not a closed element. Not involving the total magnetization vector, the oscillations are not excited by the magnetic field; however, the oscillations can be excited by an alternating electric field or by a combination of a constant electric field and the alternating magnetic field of a certain frequency. This phenomenon is a dynamic manifestation of the magnetoelectric interaction. These oscillations, representing a new special type of spin waves (magnons), were called antimagnons. The intrinsic frequencies of antimagnons, as well as the corresponding susceptibilities, were determined. Quantitative estimates were obtained for a Mn₂Sb-based ferrimagnetic phase in both easy-axis and easy-plane orientation states.     

Propagating energy modes in the heisenberg chain: Just plain magnons

We show that the oscillations in the energy density observed in classical simulations on ferromagnetic chains are present in the antiferromagnet as well, and are not due to hydrodynamic “second magnon” modes, but arise from a singularity in the non interacting two spin wave density of states.Quantum occupation number effects change qualitatively the nature of the oscillations, producing a perfectly well defined mode at the spin wave frequency as T→0.     

Pulsed inductive microwave magnetometer response calculated for IrMn/FeNi bilayers

Micromagnetic simulations of a pulsed inductive microwave magnetometer (PIMM) experiment are performed using a well established model for exchange bias. The model (Interacting Grain Model) consists of ferromagnetic grains and antiferromagnetic grains with randomly distributed easy axes. A perfectly compensated interface between the ferromagnet and the antiferromagnet is assumed which leads to spin flop coupling. The antiferromagnetic layer is modelled as two totally antiparallel sublattices with a small intergrain exchange between each antiferromagnetic sublattice. Simulations of an experimental PIMM setup provide a shift of the minimum of the resonance frequency which is also observered experimentally.     

Low temperature thermodynamics of quantum spin chains

Low temperature thermodynamic quantities of quantum spin chains are obtained by combining the high temperature expansion and an argument based on the spin wave theory. The method is tested in the XY chain and applied to the Heisenberg chain for which low temperature specific heat and antiferromagnetic susceptibility are calculated.     

Dynamics of Random One-Dimensional ±J Systems

Finite chains of a two-state random Potts spin model with periodic boundary conditions are studied within Glauber dynamics. The spin exchange is assumed random with frustration between ferro and antiferromagnetic values (±J). Time-dependent fluctuations are induced by periodic temperature oscillations. Master type differential equations for spin correlation functions are solved within linear response theory. The spectrum of relaxation times are calculated at different temperatures. The ±J Potts glass chains undergo a zero temperature phase transition. The barriers against inversion of the spin chain take only two values; 0 and 2|J|. The temperature behaviour of specific heat is characterized by rounded peaks. The frequency dependence displays two plateaus for the real part of specific heat and two corresponding peaks for the imaginary part. The dynamic specific heat is not affected by the longest relaxing mode like susceptibility. The time separation of the modes is demonstrated by the Cole-Cole plots.     

Time-correlated soliton tunneling in charge and spin density waves

We consider a model in which an electric field induces quantum nucleation of kink-antikink pairs in a pinned charge or spin density wave. Pair nucleation events, prevented by Coulomb blockade below a pair creation threshold, become correlated in time above threshold. The model provides a natural explanation for the observed (i) small density wave polarization below threshold in NbSe (3), (ii) narrow band noise, (iii) coherent oscillations, and (iv) mode-locking at high drift frequencies.     

Spin wave propagation in the domain state of a random field magnet

Inelastic neutron scattering with high wave-vector resolution has characterized the propagation of transverse spin wave modes near the antiferromagnetic zone center in the metastable domain state of a random field Ising magnet. A well-defined, long wavelength excitation is observed despite the absence of long-range magnetic order. Direct comparisons with the spin wave dispersion in the long-range ordered antiferromagnetic state reveal no measurable effects from the domain structure. This result recalls analogous behavior in thermally disordered anisotropic spin chains but contrasts sharply with that of the phonon modes in relaxor ferroelectrics. Received 2 November 2002 / Received in final form 4 February 2003 Published online 11 April 2003 RID="a" ID="a"leheny@pha.jhu.edu     

Exchange bias and spin valve systems with Fe–Mn antiferromagnetic pinning layers, obtained by the thermo-ionic vacuum arc method

Exchange bias and spin valve systems with Fe–Mn antiferromagnetic layers of different Fe concentrations were obtained by the thermo-ionic vacuum arc method. The adherence of the multilayer system to the Si substrate depends on the Fe–Mn composition. The overall roughness depends on the growing order of the antiferromagnetic/ferromagnetic layers. Very low blocking temperatures for exchange bias were observed for the considered compositions of the Fe–Mn layer. The coercive forces of both the pinned and the free layers of spin valve structures can be considerably modified along a large set of samples simultaneously prepared.     

Dimensional crossover in alternating spin chains

The effect of antiferromagnetic interchain coupling in alternating spin chains is studied by means of spin wave (SW) theory and density matrix renormalization group (DMRG). Two limiting cases are investigated, the two-leg ladder and its two-dimensional (2D) generalization. For the 2D case, SW approximation predicts a smooth-dimensional crossover keeping the ground state ordered, whereas in the ladder case the DMRG results show a gapped ground state for any J>0. Furthermore, the behavior of the correlation functions closely resemble the uniform spin- ladder. However, for small J, the gap behaves quadratically as Δ0.6J². Similarly to uniform spin chains, it is conjectured an analogous spin gap behavior for an arbitrary number of mixed spin chains.     

Anomalous polarization characteristics of magnetic resonance in a quasi-one-dimensional CuGeO<Subscript>3</Subscript>: Co magnet

Doping of CuGeO₃ by 2% Co was found to cause a new magnetic resonance, which has anomalous polarization characteristics. In the Faraday geometry, where a microwave field B _ω is directed along certain crystallographic directions, this mode is suppressed, which indicates that the character of magnetic oscillations in this mode differs strongly from standard spin precession. This resonance coexists with the EPR on Cu²⁺ chains and is likely to be caused by an unknown collective mode of magnetic oscillations of an antiferromagnetic quantum S = 1/2 spin chain.     

Reduction in critical current density of current-induced magnetization switching

We have investigated the current-induced magnetization switching in an exchange-biased spin valve structure. By using an unpatterned antiferromagnetic layer to pin the fixed Co layer, we obtained a lower switching current density by a factor of 5 than a simple spin valve structure. For the application, it is important to know how to keep the spin polarization when the thicker layer is pinned by an antiferromagnet. The unpatterned pinned ferromagnetic lead can be a good solution for spin-transfer-torque-activated device. The effect of Cu buffer layer on the top of the thin Co and Ru buffer layer under the thick Co layer on the current-induced magnetization switching in cobalt-based trilayer spin valves was also investigated. The experimental results showed that the Ru buffer layer in combination with Cu buffer layer could induce a decrease in the critical switching current by 30%, and an increase in the absolute resistance change by 35%, which is caused by an improvement of a microstructure of a thicker Co polarizer.     

Gyroscopic dynamics of antiferromagnetic vortices in domain boundaries of yttrium orthoferrite

It is established experimentally that the magnetic field directed along the b axis has little effect on the velocities of antiferromagnetic vortices in the domain boundary (DB) of yttrium orthoferrite and fails to explain the presence of an appreciable gyroscopic force acting on these vortices. This force is induced by the dynamic canting of magnetic sublattices proportional to the DB velocity. Due to the canting, the velocities of antiferromagnetic vortices depend initially quadratically on the DB velocity, as was experimentally found in this work. The dynamics of antiferromagnetic vortices in the yttrium orthoferrite DBs is gyroscopic and quasi-relativistic, with the limiting velocity of 20 km/s equal to the velocity of spin waves at the linear portion of their dispersion curve.     

Macroscopic quantum coherence of the Neel vector in antiferromagnetic system without Kramers' degeneracy

At low temperatures the Neel vector in a small antiferromagnetic particle can possess quantum coherence between the classically degenerate minima. In some cases, the topological term in the magnetic action can lead to destructive interference between the symmetry-related trajectories for the half-integer excess spin antiferromagnetic particle. By studying a macroscopic quantum coherence problem of the Neel vector with biaxial crystal symmetry and a weak magnetic field applied along the hard axis, we find that the quenching of tunnel splitting could take place in the system without Kramers' degeneracy. Both the Wentzel-Kramers-Brillouin exponent and the pre-exponential factors are found exactly for the tunnel splitting. Results show that the tunnel splitting oscillates with the weak applied magnetic field for both the integer and half-integer excess spin antiferromagnetic particles, and vanishes at certain values of the field. All the calculations are performed based on the two sublattices model and the instanton method in spin-coherent-state path integral. Received: 24 July 1997 / Accepted: 30 September 1997     

Nonequilibrium Phase Transition in Spin-S Ising Ferromagnet Driven by Propagating and Standing Magnetic Field Wave

The dynamical response of spin-S(S=1, 3/2, 2, 3) Ising ferromagnet to the plane propagating wave, standing magnetic field wave and uniformly oscillating field with constant frequency are studied separately in two dimensions by extensive Monte Carlo simulation. Depending upon the strength of the magnetic field and the value of the spin state of the Ising spin lattice two different dynamical phases are observed. For a fixed value of S and the amplitude of the propagating magnetic field wave the system undergoes a dynamical phase transition from propagating phase to pinned phase as the temperature of the system is cooled down. Similarly in case with standing magnetic wave the system undergoes dynamical phase transition from high temperature phase where spins oscillate coherently in alternate bands of half wavelength of the standing magnetic wave to the low temperature pinned or spin frozen phase. For a fixed value of the amplitude of magnetic field oscillation the transition temperature is observed to decrease to a limiting value as the value of spin S is increased. The time averaged magnetisation over a full cycle of the magnetic field oscillation plays the role of the dynamic order parameter. A comprehensive phase boundary is drawn in the plane of magnetic field amplitude and dynamic transition temperature. It is found that the phase boundary shrinks inwards for high value of spin state S.Also in the low temperature(and high field) region the phase boundaries are closely spaced.     

Periodic density redistribution of parametrically excited spin waves in an antiferromagnet

A nonuniform distribution of the density of parametrically excited magnons is observed experimentally in an antiferromagnetic CsMnF₃ sample. The nonuniform distribution occurs at a high pumping power when oscillations of the high frequency susceptibility occur. These oscillations were observed earlier and their nature was not clear. It is found that during the increase of the absorbed power on the occurrence of the oscillation, the spin wave condenses near the middle of the sample. The condensation occurs as a result of a nonlinear shift of the magnon spectrum and is similar to self-focusing of light in nonlinear media. The electromagnetic radiation of parametrically excited spin waves is studied. It is found that the periodic redistribution of the density exerts an additional restrictive effect on the amplitude of the parametrically excited magnons.     

Spin glass and antiferromagnetism in Kondo-lattice disordered system

The competition between spin glass (SG), antiferromagnetism (AF) and Kondo effect is studied here in a model which consists of two Kondo sublattices with a Gaussian random interaction between spins in different sublattices with an antiferromagnetic mean J ₀ and standard deviation J. In the present approach there is no hopping of the conduction electrons between the sublattices and only spins in different sublattices can interact. The problem is formulated in the path integral formalism where the spin operators are expressed as bilinear combinations of Grassmann fields which can be solved at mean field level within the static approximation and the replica symmetry ansatz. The obtained phase diagram shows the sequence of phases SG, AF and Kondo state for increasing Kondo coupling. This sequence agrees qualitatively with experimental data of the Ce₂Au_1-x Co _x Si₃ compound.Received: 9 April 2003, Published online: 9 September 2003PACS: 05.50.+q Lattice theory and statistics; Ising problems - 64.60.Cn Order disorder transformations; statistical mechanics of model systems     

阻挫对准一维非对称子格反铁磁链自旋波激发的影响

子格对称性破缺使得s=1/2准一维海森伯自旋链具有三支自旋波激发谱(其中一支属于声学模，两支属于光学模). 计算表明：阻挫导致两支光学模能隙简并解除；阻挫引起声学模自旋波激发谱软化，但并不导致光学模激发谱软化；阻挫导致两支光学模激发谱中的一支明显下移，这意味着阻挫使光学模激发变得重要且容易实现；阻挫引起的自旋偏离对于属于不同子格的自旋是不同的；阻挫对于系统基态磁性长程序的削弱随着阻挫增强变得越来越明显. 通过与严格对角化方法和DMRG方法的数值结果比较，还分析了自旋波近似的合理性和不足之处. 关键词： 准一维反铁磁自旋系统 自旋波激发 光学模 能隙简并     

Excitation hierarchy of the quantum sine-gordon spin chain in a strong magnetic field

The magnetic excitation spectrum of copper pyrimidine dinitrate, a material containing S = 1 / 2 antiferromagnetic chains with alternating g tensor and the Dzyaloshinskii-Moriya interaction and exhibiting a field-induced spin gap, is probed using submillimeter wave electron spin resonance spectroscopy. Ten excitation modes are resolved in the low-temperature spectrum, and their frequency-field diagram is systematically studied in magnetic fields up to 25 T. The experimental data are sufficiently detailed to make a very accurate comparison with predictions based on the quantum sine-Gordon field theory. Signatures of three breather branches and a soliton, as well as those of several multiparticle excitation modes, are identified.     

Thermal conductivity evidence for a dx2-y2 pairing symmetry in the heavy-fermion CeIrIn5 superconductor

The phase diagram of the quasi-2D Ce(Ir,Rh)In5 system contains two distinct superconducting domes. By the thermal transport measurements in rotating magnetic fields H, we pinned down the superconducting gap structure of CeIrIn5 in the second dome, located distant from the first dome in proximity to an antiferromagnetic quantum critical point. Clear fourfold oscillation was observed when H is rotated within the ab plane, while no oscillation was observed within the bc plane. In sharp contrast to previous reports, our results are most consistent with dx2-y2 symmetry, implying that the superconductivity in the second phase is also mediated by antiferromagnetic spin fluctuations.     

Coupled catalytic oscillators: Beyond the mass-action law

We present Monte Carlo simulations of the reaction kinetics corresponding to two coupled catalytic oscillators in the case when oscillations result from the interplay between the reaction steps and adsorbate-induced surface restructuring. The model used is aimed to mimic oscillations on a single nm catalyst particle with two kinds of facets or on two catalyst particles on a support. Specifically, we treat the NO reduction by H(2) on a composite catalyst containing two catalytically active Pt(100) parts connected by an inactive link. The catalyst is represented by a rectangular fragment of a square lattice. The left- and right-hand parts of the lattice mimic Pt(100). With an appropriate choice of the model parameters, these sublattices play a role of catalytic oscillators. The central catalytically inactive sublattice is considered to be able only to adsorb NO reversibly and can be viewed as a Pt(111) facet or a support. The interplay of the reactions running on the catalytically active areas occurs via NO diffusion over the boundaries between the sublattices. Using this model, we show that the coupling of the catalytically active sublattices may synchronize nearly harmonic oscillations observed on these sublattices and also may result in the appearance of aperiodic partly synchronized oscillations. The spatio-temporal patterns corresponding to these regimes are nontrivial. In particular, the model predicts that, due to phase separation, the reaction may be accompanied by the formation of narrow NO-covered zones on the left and right sublattices near the boundaries between these sublattices and the central sublattice. Such patterns cannot be obtained by using the conventional mean-field reaction-diffusion equations based on the mass-action law. The experimental opportunities to observe the predicted phenomena are briefly discussed. (c) 2001 American Institute of Physics.