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1.
The resistivity of the heavy-doped La1/3Ca2/3MnO3 (LCMO) is simulated using a random resistor network model, based on a phase separation scenario. The simulated results agree well with the reported experimental data, showing a transition from a charge-disordered (CDO) state embedded with a few ferromagnetic (FM) metallic clusters to a charge-ordered (CO) state, corresponding to the transition from a high-temperature paramagnetic (PM) insulating state to a low-temperature antiferromagnetic (AF) insulating state. Furthermore, we find that the number of AF/CO clusters increases with decreasing temperature, and the clusters start to connect to each other around 250K, which causes percolating in the system. The results further verify that phase separation plays a crucial role in the electrical conductivity of LCMO.  相似文献   

2.
The measurement of low-field susceptibility X as a function of temperature T for La2/3Ca1/3MnO3 shows a significant downturn in 1/X(T) above the Curie temperature Tc, a behaviour generally observed in perovskite manganites. Such a downturn is argued to be due to the segregation of ferromagnetic clusters with larger spins in the paramagnetic matrix. Based on this consideration, a phenomenological expression for X(T) is proposed,in which the total susceptibility is assumed to be a sum of two susceptibilities arising from magnetic entities in the PM background and the FM clusters with T-dependent effective spins, respectively. The result is in good agreement with the experimental data obtained in La2/3Ca1/3MnO3.  相似文献   

3.
郑琳  周敏  赵建军  成昭华  张向群  邢茹  张雪峰  鲁毅 《中国物理 B》2011,20(8):87501-087501
The magnetic and electrical properties of nonmagnetic Ga +3 ion substitution for Mn site are investigated in the bilayer manganite La 1.2 Sr 1.8 Mn 2 O 7.When the Mn is substituted by Ga,the ferromagnetic property obviously weakens,the magnetic transition temperature decreases and a spin-glass behaviour occurs at low temperature.Meanwhile,doping causes the resistivity to dramatically increase,the metal-insulator transition temperature to disappear,and a greater magneto-resistance effect to occur at low temperature.These effects result from the fact that Ga substitution dilutes the magnetic active Mn-O-Mn network and weakens the double exchange interaction,and further suppresses ferromagnetic ordering and metallic conduction.  相似文献   

4.
谢燕武  王登京  沈保根  孙继荣 《中国物理》2007,16(10):3120-3124
A junction composed of ultrathin La0.9Ca0.1MnO3+δ (LCMO) film and 1 wt.% Nb-doped SrTiO3 was fabricated and its magnetoresistance (MR) was studied and compared with LCMO film. It was found that the resistance of the junction has a similar dependence on magnetic field as that of the LCMO film: the curvature of R-H curves is upward above Curie temperature (Tc) and downward below TC. These behaviours strongly suggest that the rotation of ferromagnetic clusters in manganite also causes MR in the corresponding junction. This MR can be qualitatively understood by the change of the width of the barrier induced by the rotation of ferromagnetic clusters. These results suggest a possibility to obtain junctions with large low-field MR.  相似文献   

5.
The Bogoliubov de Gennes equation is applied to the study of coherence effects in the ferromagnetic superconductor/insulator/normal metal/insulator/ferromagnetic/superconductor (FS/I/N/I/FS) junction. We calculated the Josephson current in FS/I/N/I/FS as a function of exchange field in ferromagnetic superconductor, temperature, and normal metal thickness. It is found that the Josephson critical current in FS/I/N/I/FS exhibits oscillations as a function of the length of normal metal. The exchange field always suppresses the Josephson critical current Ip for a parallel configuration of the magnetic moments of two ferromagnetic superconductor (FS) electrodes. In the antiparallel configuration, the Josephson critical current IAv at the minimum values of oscillation increases with the exchange field for strong barrier strength and at low temperatures.  相似文献   

6.
侯兆阳  刘让苏  田泽安  王晋国 《中国物理 B》2011,20(6):66102-066102
A larger-scale Mg70Zn30 alloy system including 100000 atoms has been simulated by using the molecular dynamics method to investigate the icosahedral medium-range order (IMRO) formed in the Mg70Zn30 metallic glass. It is found that the simulated pair distribution function of Mg70Zn30 metallic glass is in good agreement with the experimental results. The glass transition temperature Tg is near 450 K under the cooling rate of 1×1012 K/s. The icosahedral local structures play a critical role in the formation of metallic glass, and they are the dominant local configurations in the Mg70Zn30 metallic glass. The IMRO in the Mg70Zn30 metallic glass is characterized by certain types of extended icosahedral clusters combined by intercross-sharing atoms in the form of chains or dendrites. The size distributions of these IMRO clusters present a magic number sequence of 19, 23, 25, 27, 29, 31, 33, 35, 37, 39,. . . , and the magic clusters can be classified into three types according to their compactness. The IMRO clusters grow rapidly in a low-dimensional way with cooling, but this growth is limited near Tg.  相似文献   

7.
First-principles calculations have been performed for the study of the electronic band structure and ferromagnetic properties of double perovskite Ca2CrSbO6. The density of states, total energy, spin magnetic moment, and charge density were calculated and analyzed in details. It is found that Ca2CrSbO6 has a stable ferromagnetic ground state and the spin magnetic moment per molecule is about 2.99#B. The chromium contributes the most in the total magnetic moments. The results indicate that Ca2CrSbO6 is half-metallic.  相似文献   

8.
We numerically investigate the thermal entanglements of spins (1/2, 1) and spins (1/2, 1/2) in the three-mixed (1/2, 1, 1/2) anisotropic Heisenberg XXZ spin system on a simple triangular cell under an inhomogeneous magnetic field. We show that the external magnetic field induces strong plateau formation in the pairwise thermal entanglement for fixed parame-ters of the Hamiltonian in the cases of ferromagnetic and antiferromagnetic interactions. We also .observe an unexpected critical point at finite temperature in the thermal entanglement of spins (1/2, 1) for the antiferromagnetic case, while the entanglement of spins (1/2, 1) in the ferromagnetic case and the entanglement of spins (1/2, 1/2) in both ferromagnetic and antiferromagnetic cases almost decay exponentially to zero with increasing temperature. The critical point in the en-tanglement of spins (1/2, 1) in the antiferromagnetic case may be a signature of the quantum phase transition at finite temperature.  相似文献   

9.
We present the microscopic origin of the ferromagnetism of Feo.25TaS2 and its finite-temperature magnetic properties.The band structures of Feo.25TaS2 are first obtained by the first-principles calculations and it is found that both conventional and Dirac carriers coexist in metallic Feo.25TaS2-Accordingly,considering the spin-orbit coupling of Fe 3d ion,we derive an effective Ruderman-Kittle-Kasuya-Yosida-type Hamiltonian between Fe spins in the presence of both the conventional parabolic-dispersion and the Dirac linear-dispersion carriers,which contains a Heisenberg-like,an Ising-like and an XY-like term.In addition,we obtain the ferromagnetic Curie temperature Tc by using the cluster self-consistent Held method.Our results could address not only the high ferromagnetic Curie temperature but also the large magnetic anisotropy in Fex TaS2.  相似文献   

10.
The Stokes-Einstein(SE) relation has been considered as one of the hallmarks of dynamics in liquids. It describes that the diffusion constant D is proportional to(τ/T)~(–1), where τ is the structural relaxation time and T is the temperature. In many glassforming liquids, the breakdown of SE relation often occurred when the dynamics of the liquids becomes glassy, and its origin is still debated among many scientists. Using molecular dynamics simulations and support-vector machine method, it is found that the scaling between diffusion and relaxation fails when the total population of solid-like clusters shrinks at the maximal rate with decreasing temperature, which implies a dramatic unification of clusters into an extensive dominant one occurs at the time of breakdown of the SE relation. Our data leads to an interpretation that the SE violation in metallic glass-forming liquids can be attributed to a specific change in the atomic structures.  相似文献   

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