有机铬富勒烯衍生物的激发态与光限幅特性

应用倍频ｎｓ／ｐｓＮｄ：ＹＡＧ脉冲激光系统,在波长为５３２ｎｍ,脉冲宽度为２１ｐｓ的条件下,研究了新型有机铬富勒烯衍生物的激发态吸收与光限幅特性,其光限幅特性优于富勒烯甲苯溶液;并应用单重态激发态吸收理论对实验结果进行了分析,实验结果与理论结果基本一致。     

新型富勒烯衍生物的光限幅研究

应用倍频Ｎｄ∶ＹＡＧ脉冲激光，在波长为５３２ｎｍ、脉冲宽度分别为８ｎｓ和２３ｐｓ的条件下，研究了新型富勒氮烯乙酰氨衍生物（Ｎ－ａｃｅｔａｍｉｄｅ１，２－ｄｉｈｙｄｒｏ－１，２－ａｚａ－ｆｕｌｅｒｅｎｅ［６０］）的反饱和吸收与光限幅特性。实验结果表明，同脉宽为纳秒的激发脉冲相比，富勒烯乙酰氨衍生物对脉宽为皮秒的脉冲限幅效果比较好。     

C_（60）／PMMA的单重态激发态吸收光限幅研究

研究了Ｃ６０／ＰＭＭＡ对波长５３２ｎｍ，脉冲宽度为２１ｐｓ的脉冲激光的限幅特性，并应用三能级模型进行了理论模拟。结果表明光限幅起源于单重态激发态吸收     

C60／PMMA的单重态激光发态吸收光限幅研究

研究了Ｃ６０／ＰＭＭＡ对波长５３２ｎｍ，脉冲宽度为２１ｐｓ的脉冲激光的限幅特性，并应用三能级模型进行了理论模拟。结果表明光限幅起源于单重态发态吸收。     

PDATS对ps脉冲的光限幅效应

应用脉宽为２１ｐｓ脉冲，波长为５３２ｎｍ的激光脉冲研究了新型光限幅材料５－（２－硫甲基－４－甲基－５－嘧啶基）－２，４－戊二炔－１醇的对甲苯磺酸酯的光限幅效应，其优点是限幅幅值和限幅阈值低，分别为Ｅｃ＝１８０ｍＪ／ｃｍ＾２，Ｅｔｈ＝１５０ｍＪ／ｃｍ＾２；可见了光透射率高。     

受激布里渊散射对纳秒激光脉冲光限幅规律

 研究了受激布里渊散射对纳秒激光脉冲的光限幅效应。针对四氯化碳介质研究了受激布里渊散射对2ns激光脉冲的光限幅和稳定输出能量的特性,给出了光限幅特性及输出能量与光限幅介质的结构参数之间的关系。对于输入能量波动范围在 13%的激光脉冲,实验获得输出能量波动范围为 7%,与理论分析的结果基本符合。     

新型金属团簇化合物的光限幅特性研究

应用倍频 Nd:YAG脉冲激光 ,在波长为 5 32 nm、脉冲宽度为 8ns的条件下 ,研究了金属团簇化合物WOS3Cu3I(2 - Me Py) 3的光限幅特性。其光限福特性优于富勒烯。Z- Scan研究结果表明 :该团簇具有自聚焦特性 ,其光限幅起源于激发态吸收     

抽运能量对受激布里渊散射光限幅特性的影响

采用布里渊噪声起源模型,数值模拟了受激布里渊散射介质CCl4对波长1064nm的Nd：YAG纳秒激光脉冲的传输特性及光限幅特性。入射抽运脉冲能量较低时,非线性介质对纳秒激光脉冲呈光学透明。入射抽运脉冲能量高于受激布里渊散射产生阈值后,透射脉冲峰值受限,脉宽压缩,能量趋于饱和,说明该光学系统同时具有光功率限幅和能量限幅的光限幅特性。利用理论模型模拟了如下光限幅参量：透射脉冲峰值功率、透射能量、能量透射率、脉宽压缩率依赖抽运光能量的变化关系。相应的理论模拟计算结果由实验进行验证,实验结果与理论模拟相符合。     

萘酞菁铅化合物的光限幅特性研究

应用调Q倍频ns/ps Nd：YAG脉冲激光,在波长为532nm,脉冲宽度为8ns,重复频率为1Hz的条件下,研究了溶于二甲基亚砜(DMSO)中的萘酞菁铅溶液的反饱和吸收和光限幅特性。实验表明,萘酞菁铅具有良好的光限幅特性,它的有效激发态吸收截面与基态吸收截面的比值约为15．21,大于萘酞菁铜。研究结果表明,萘酞菁铅的光限幅特性优于C60,激发态吸收是其主要的光限幅机理。实验结果证实了重原子效应可以通过增强系际跃迁而使三重态的反饱和吸收增强,从而提高光限幅的能力。     

甲基红掺杂碳纳米管悬浮液的光限幅特性研究

利用实验的方法研究了甲基红掺杂碳纳米管悬浮液对波长为532 nm激光的光限幅效应.分析了样品厚度和入射激光重复频率对光限幅特性的影响,并与纯碳纳米管悬浮液的光限幅特性进行了比较.实验结果表明,对于线性透过率为60%（500 nm）的碳纳米管悬浮液,掺入甲基红后其沉淀速度明显减慢,限幅阈值由250 μJ降低为200 μJ;对于2和5 mm 厚度的样品,掺杂甲基红使碳纳米管悬浮液的箝位输出激光脉冲能量分别由45和20 μJ降低为35和9 μJ. 关键词： 非线性光学 光限幅效应 甲基红 染料掺杂碳纳米管悬浮液     

Study on the optical limiting properties of the mixed liquid of carbon black suspensions and green tea solution by multi-pulse laser

The optical limiting properties of the mixed liquid of carbon black suspensions (CBS) and green tea solution were studied by using an 8 ns laser pulse at 532\,nm. The optical limiting effects of the CBS and mixed liquid have been compared between 5 and 10\,Hz repetition frequencies with nanosecond laser pulse. The experimental results indicate that the optical limiting threshold of the sample with the incidence laser at 10\,Hz repetition frequency is lower than at 5\,Hz repetition frequency. The possible reasons for the influence of the repetition frequency on the samples are discussed. And by observing the optical radiant distributions when the laser pulse passing through different samples, a possible mechanism for the observed effects is suggested. At the same time, the result shows that the optical limiting of CBS is the dominant factor to optical limiting of the mixed liquid.     

受激布里渊散射光限幅输出波形控制研究

数值模拟了种子场诱导受激布里渊散射光限幅过程的限幅输出波形特性.得到利用种子场控制限幅脉冲波形的规律：选取种子场脉冲宽度为抽运脉冲宽度的五倍，抽运脉冲相对于种子脉冲的延迟时间控制在与抽运脉冲宽度相当时，限幅输出波形最佳.限幅输出波形同时受抽运光功率影响，随抽运能量的增加，限幅脉冲功率不断下降，直至趋于0. 关键词： 受激布里渊散射 限幅输出波形 注入种子     

Pulse duration and wavelength effects on the optical limiting behavior of carbon nanotube suspensions

We investigate pulse duration and wavelength effects on the optical limiting behavior of single-wall carbon nanotubes suspended either in chloroform or in water. The principal optical limiting effect in carbon nanotube suspensions is nonlinear scattering that is due to heat transfer from particles to solvent, leading to solvent-bubble formation and to sublimation of carbon nanotubes. We report on nonlinear transmittance measurements for pulse durations ranging from 3 to 100 ns and for wavelengths from 430 to 1064 nm. The dependence of optical limiting behavior on pulse duration and wavelength is analyzed and discussed in terms of nonlinear mechanisms.     

MoS2纳微薄膜激光非线性透射的调控研究

超短飞秒脉冲激光(脉冲时间<40 fs)有独特的热效应机理, 但尚无针对其设计的光限幅保护膜. 本文采用易于产业化的离散-旋涂法制备了MoS₂纳微薄膜(厚度150–200 nm). 光限幅测试结果表明, 针对超短脉冲激光, 此纳微薄膜在低光强下增透, 高光强下减透(光限幅); 且能通过改变入射波长, 调控其光限幅阈值, 可用于聚光太阳能电池的效率增强和损伤保护.利用此方法, 对已商用的砷化镓太阳能电池进行涂膜, 发现转换效率降低<3%, 但损伤阈值提高>50%.     

Time-resolved analysis of nonlinear optical limiting for laser synthesized carbon nanoparticles

Nonlinear optical limiting materials have attracted much research interest in recent years. Carbon nanoparticles suspended in liquids show a strong nonlinear optical limiting function. It is important to investigate the nonlinear optical limiting process of carbon nanoparticles for further improving their nonlinear optical limiting performance. In this study, carbon nanoparticles were prepared by laser ablation of a carbon target in tetrahydrofuran (THF). Optical limiting properties of the samples were studied with 532-nm laser light, which is in the most sensitive wavelength band for human eyes. The shape of the laser pulse plays an important role for initializing the nonlinear optical limiting effect. Time-resolved analysis of laser pulses discovered 3 fluence stages of optical limiting. Theoretical simulation indicates that the optical limiting is initialized by a near-field optical enhancement effect.     

线阵CCD用于长距离衍射准直测量

本文介绍了在半导体激光光纤与位相板相结合的准直情况下,利用线阵ＣＣＤ探测器测量大型工件形位误差遇到的光强变化而引起测量误差的问题,并对用线阵ＣＣＤ进行衍射信号测量的原理和特点作了分析。根据ＣＣＤ的工作原理和特性,提出了利用自动控制ＣＣＤ积分时间的方法,使ＣＣＤ输出的信号峰值保持恒定,提高了系统的测量精度。     

基于富勒烯纳米结构材料光限幅特性研究

应用倍频Nd:YAG脉冲激光,在波长为532nm,脉宽8ns,重复频率10Hz的条件下,研究了新型基于富勒烯纳米结构材料(C₆₀-bpy-Au)的光限幅特性.实验结果表明,其限幅特性较C₆₀有所提高,初步分析了光限幅和溶剂效应.     

Time-dependent thermal lensing and Kerr nonlinearity in CS2 with CO2-laser radiation

We report on optical limiting and z-scan in CS₂ as a function of the pulse duration of 10 µm TEA CO₂-laser radiation. We present a comprehensive and simple model for the shape of a laser pulse transmitted through this limiting device. For the first time, we propose the use of an optical limiting device for beam shaping.