共查询到18条相似文献,搜索用时 122 毫秒
1.
Pseudogap and Superconducting Gap in SmFeAs(O1-xFx) Superconductor from Photoemission Spectroscopy 下载免费PDF全文
刘海云 ;贾小文 ;张文涛 ;赵林 ;孟建桥 ;刘国东 ;董晓莉 ;吴刚 ;刘荣华 ;陈仙辉 ;任治安 ;衣纬 ;车广灿 ;陈根富 ;王楠林 ;王桂玲 ;周勇 ;朱镛 ;王晓阳 ;赵忠贤 ;许祖彦 ;陈创天 ;周兴江 《中国物理快报》2008,25(10):3761-3764
High resolution photoemission measurements are carried out on non-superconducting SmOFeAs paxent compound and superconducting SmFeAs(O1-xFx) (x = 0.12, and 0.15) compounds. The momentum-integrated spectra exhibit a clear Fermi cutoff that shows little leading-edge shift in the superconducting state. A robust feature at 13 meV is identified in all these samples. Spectral weight suppression near IF, F with decreasing temperature is observed in both undoped and doped samples that points to a possible existence of a pseudogap in these Fe-based compounds. 相似文献
2.
Angle-resolved photoemission spectroscopy (ARPES) has played an important role in determining the band structure and the superconducting gap structure of iron-based superconductors. In this paper, from the ARPES perspective, we briefly review the main results from our group in recent years on the iron-based superconductors and their parent compounds, and depict our current understanding on the antiferromagnetism and superconductivity in these materials. 相似文献
3.
Crystal structures and microstructural features, such as structural phase transitions, defect structures, and chemical and structural inhomogeneities, are known to have profound effects on the physical properties of superconducting materials. Recently, many studies on the structural properties of Fe-based high-Tc superconductors have been published. This review article will mainly focus on the typical microstructural features in samples that have been well characterized by physical measurements. (i) Certain common structural features are discussed, in particular, the crystal structural features for different superconducting families, the local structural distortions in the Fe2Pn2 (Pn = P, As, Sb) or FeeCh2 (Ch = S, Se, Te) blocks, and the structural transformations in the 122 system. (ii) In FeTe(Se) (11 family), the superconductivity, chemical and structural inhomogeneities are investigated and discussed in correlation with superconductivity. (iii) In the Ko.sFe1.6+xSe2 system, we focus on the typical compounds with emphasis on the Fe-vacancy order and phase separations. The microstructural features in other superconducting materials are also briefly discussed. 相似文献
4.
Based on structural and bonding features, a new classification scheme of superconductors is proposed to classify them into three classes: three-dimensional, two-dimensional and molecule-assembled superconductors. The 'sandwich model' for the high-Tc euprates is extended to a 'binary structure model': i.e., the crystal structure of most super- conductors can be partitioned into two parts, a superconducting active component and a supplementary component. Partially metallic covalent bonding is found to be a common feature in all superconducting active components, and the electron states of the atoms in the active components usually make a dominant contribution to the energy band near the Fermi surface. Possible directions to explore new superconductors are discussed based on the structural classification and the binary structure model. 相似文献
5.
《中国物理 B》2021,30(7):77403-077403
Discovery of a new superconductor with distinct crystal structure and chemistry often provides great opportunity for further expanding superconductor material base, and also leads to better understanding of superconductivity mechanisms. Here, we report the discovery of superconductivity in a new intermetallic oxide Hf_3Pt_ Ge_2O synthesized through a solid-state reaction. The Hf_3Pt_ Ge_2O crystallizes in a cubic structure(space group Fm-3 m) with a lattice constant of a = 1.241 nm, whose stoichiometry and atomic structure are determined by electron microscopy and x-ray diffraction techniques. The superconductivity at 4.1 K and type-II superconducting nature are evidenced by the electrical resistivity, magnetic susceptibility, and specific heat measurements. The intermetallic oxide Hf_3Pt_ Ge_2O system demonstrates an intriguing structural feature that foreign oxygen atoms can be accommodated in the interstitial sites of the ternary intermetallic framework. We also successfully synthesized a series of Hf_3Pt_ Ge_2O1+δ(-0.25 ≤δ≤ 0.5), and found theδ-dependent superconducting transition temperature Tc. The atomic structure and the electronic structure are also substantiated by first-principles calculations. Our results present an entirely new family of superconductors with distinct structural and chemical characteristics, and could attract research interest in further finding new superconductors and exploring novel physics pertaining to the 5 d-electron in these intermetallic compound systems. 相似文献
6.
Direct Microwave Synthesis of 11-Type Fe(Te,Se) Polycrystalline Superconductors with Enhanced Critical Current Density 下载免费PDF全文
We report a direct microwave synthesis method for the preparation of 11-type high quality Fe(Te,Se) polycrystalline superconductors. The bulk samples are rapidly synthesized under the microwave irradiation during several minutes, with a subsequent annealing process at 400℃. The samples exhibit a nearly single phase of the tetragonal PbO-type crystal structure with minor impurities. Morphology characterization shows high density, tight grain connectivity and large grain sizes around 100 μm with small cavities inside the sample. Resistivity and magnetization measurements both show similar superconducting transitions above 14 K. The magnetic hysteresis measurements display broad and symmetric loops without magnetic background, and a high critical current density J_c about 1.2 × 10~4 A/cm~2 at 2 K and 7 T is estimated by the Bean model. Compared with the solidstate reaction synthesized samples, these superconducting bulks from microwave-assisted synthesis are possibly free of the interstitial Fe due to smaller c-axis, higher T_c in magnetic transitions, better M–H loops without magnetic background and greatly enhanced J_c, and are promising as raw materials for the non-toxic Fe-based superconducting wires for large currents and high field applications. 相似文献
7.
Electronic and magnetic structures of iron selenide compounds Ce2O2FeSe2 (2212*) and BaFe2Se3 (123*) are studied by the first-principles calculations. We find that while all these compounds are composed of one-dimensional (1D) Fe chain (or ladder) structures, their electronic structures are not close to be quasi-lD. The magnetic exchange couplings between two nearest-neighbor (NN) chains in 2212* and between two NN two-leg-ladders in 123* are both antiferromagnetic (AFM), which is consistent with the presence of significant third NN AFM coupling, a common feature shared in other iron-chalcogenides, FeTe (11*) and KyFe2-xSe2 (122*). In magnetic ground states, each Fe chain of 2212* is ferromagnetic and each two-leg ladder of 123* form a block-AFM structure. We suggest that all magnetic structures in iron-selenide compounds can be unified into an extended J1-J2-J3 model. Spin-wave excitations of the model are calculated and can be tested by future experiments on these two systems. 相似文献
8.
Our recent scanning tunneling microscopy (STM) studies of the NaFelxCoxAs phase diagram over a wide range of dopings and temperatures are reviewed. Similar to the high-Tc cuprates, the iron-based superconductors lie in close proximity to a magnetically ordered phase. Therefore, it is widely believed that magnetic interactions or fluctuations play an important role in triggering their Cooper pairings. Among the key issues regarding the electronic phase diagram are the properties of the parent spin density wave (SDW) phase and the superconducting (SC) phase, as well as the interplay between them. The NaFe l-xCoxAs is an ideal system for resolving these issues due to its rich electronic phases and the charge-neutral cleaved surface. In our recent work, we directly observed the SDW gap in the parent state, and it exhibits unconventional features that are incompatible with the simple Fermi surface nesting picture. The optimally doped sample has a single SC gap, but in the underdoped regime we directly viewed the microscopic coexistence of the SDW and SC orders, which compete with each other. In the overdoped regime we observed a novel pseudogap-like feature that coexists with supercon- ductivity in the ground state, persists well into the normal state, and shows great spatial variations. The rich electronic structures across the phase diagram of NaFel_xCoxAs revealed here shed important new light for defining microscopic models of the iron-based superconductors. In particular, we argue that both the itinerant electrons and local moments should be considered on an equal footing in a realistic model. 相似文献
9.
A series of layered (Sr1-xKx)Fe2As2 compounds with nominal x = 0-0.40 are synthesized by solid state reaction method. Similar to other parent compounds of iron-based pnictide superconductors, pure SrFe2As2 shows a strong resistivity anomaly near 210 K, which was ascribed to the spin-density-wave instability. The anomaly temperature is much higher than those observed in LaOFeAs and BaFe2As2, the two prototype parent compounds with ZrCuSiAs- and ThCr2Si2-type structures. K-doping strongly suppresses this anomaly and induces superconductivity. Like in the case of K-doped BaFe2As2, sharp superconducting transitions at Tc ~ 38 K is observed. We perform the Hall coefficient measurement, and confirm that the dominant carriers are hole-type. The carrier density is enhanced by a factor of 3 in comparison to F-doped LaOFeAs superconductor. 相似文献
10.
《中国科学:物理学 力学 天文学(英文版)》2018,(12)
Muon spin relaxation/rotation(μSR) is a vital technique for probing the superconducting gap structure, pairing symmetry and time reversal symmetry breaking, enabling an understanding of the mechanisms behind the unconventional superconductivity of cuprates and Fe-based high-temperature superconductors, which remain a puzzle. Very recently double layered Fe-based superconductors having quasi-2 D crystal structures and Cr-based superconductors with a quasi-1D structure have drawn considerable attention. Here we present a brief review of the characteristics of a few selected Fe-and Cr-based superconducting materials and highlight some of the major outstanding problems, with an emphasis on the superconducting pairing symmetries of these materials. We focus on μSR studies of the newly discovered superconductors ACa_2Fe_4As_4F_2(A = K, Rb, and Cs), ThFeAsN, and A_2Cr_3As_3(A = K, Cs), which were used to determine the superconducting gap structures, the presence of spin fluctuations, and to search for time reversal symmetry breaking in the superconducting states. We also briefly discuss the results of μSR investigations of the superconductivity in hole and electron doped BaFe_2As_2. 相似文献
11.
A single band t-U-J1-J2 model is proposed as the minimum model to describe the superconductivity of the newly discovered iron-based superconductorsR(O1-xFx)FeAs and RO1-xFeAs (R=La, Ce, Sm, Pr, Nd, Gd). With the mean-field approach, it is found that the pairing occurs in the d-wave channel. In the likely parameter region of the real materials, by lowering temperature, the system enters firstly the dxy superconducting phase with D4h-symmetryand then enters the time-reversal-symmetry-broken dxy+idx2-y2 superconducting phase with C4h-symmetry. 相似文献
12.
Element Substitution Effect in Transition Metal Oxypnictide Re(O1-xFx)TAs (Re=rare earth, T=transition metal) 下载免费PDF全文
CHEN Gen-Fu LI Zheng WU Dan DONG Jing LI Gang HU Wan-Zheng ZHENGPing LUO Jian-Lin WANG Nan-Lin 《中国物理快报》2008,25(6):2235-2238
Different element substitution effects in transition metal oxypnictide Re(O1-xFx)TAs, with Re=La, Ce, Nd, Eu, Gd, Tm, T=Fe, Ni, Ru, are studied. Similarto the La- or Ce-based systems, we find that the pure NdOFeAs shows a strong resistivity anomaly near 145K, which is ascribed to the spin-density-wave instability. Electron doping by F increases Tc to about 50K. While in the case of Gd, Tc is reduced below 10K. The tetragonal ZrCuSiAs-type structure could not be formed for Eu or Tm substitution in our preparing process. For the Ni-based case, although both pure and F-doped LaONiAs are superconducting, no superconductivity is found when La is replaced by Ce in both the cases, instead a ferromagnetic ordering transition is likely to form at low temperature in the undoped sample. We also synthesize LaO1-xFxRuAs and CeO1-xFxRuAs compounds. The metallic behaviour is observed down to 4K. 相似文献
13.
M.R. Cimberle F. Canepa M. Ferretti A. Martinelli A.S. Siri C. Tarantini C. Ferdeghini 《Journal of magnetism and magnetic materials》2009,321(19):3024-3030
In this paper, the magnetic behavior of undoped and 15%F-doped SmFeAsO (Sm-1111) and LaFeAsO (La-1111) samples is presented and discussed. Magnetization measurements are not a simple tool to use for the characterization of the new family of Fe-based superconductors, because magnetic impurities can be easily formed during the preparation procedure and may affect the magnetic signal. In spite of this problem bulk magnetization measurements, properly treated, may give very useful information. In the undoped samples we gathered the main aspects of the physical behavior of the 1111 phase, i.e. the onset of the spin density wave (SDW), the antiferromagnetic ordering at the Sm sublattice and the susceptibility increase with increasing temperature above the SDW temperature, and, in addition, we were able to estimate the Pauli contribution to susceptibility and therein the Wilson ratio both for LaFeAsO and SmFeAsO compounds, and the amplitude of the jump at the SDW temperature. In the doped samples, while the presence of magnetic signals due to impurities is dominating in the normal state, the superconducting behavior may be clearly observed and studied. In particular, in the Sm-1111 superconducting sample the coexistence-competition between superconductivity and antiferromagnetic ordering of the Sm ions was clearly observed. 相似文献
14.
REN Zhi-An LU Wei YANG Jie YI Wei SHEN Xiao-Li LI Zheng-Cai CHE Guang-Can DONG Xiao-Li SUN Li-Ling ZHOU Fang ZHAO Zhong-Xian 《中国物理快报》2008,25(6):2215-2216
We report the superconductivity in iron-based oxyarsenide Sm[O1-xFx]FeAs, with the onset resistivity transition temperature at 55.0K and Meissner transition at 54.6K. This compound has the same crystal structure as LaOFeAs with shrunk crystal lattices, and becomes the superconductor with the highest critical temperature among all materials besides copper oxides up to now. 相似文献
15.
OU Hong-Wei ZHAO Jia-Feng ZHANG Yan SHEN Da-Wei ZHOU Bo YANGLe-Xian HE Cheng CHEN Fei XU Min WU Tao CHEN Xian-Hui CHEN Yan FENG Dong-Lai 《中国物理快报》2008,25(6):2225-2227
The electronic structure of the new superconductor SmO1-xFxFeAs (x=0.15) is studied by angle-integrated photoemission spectroscopy. Our data show a sharp feature very close to the Fermi energy, and a relative flat distribution of the density of states between 0.5eV and 3eV binding energy, which agrees well with the band structure calculations considering an antiferromagnetic ground state. No noticeable gap opening is observed at 12K below thesuperconducting transition temperature, indicating the existence of large ungapped regions in the Brillouin zone. 相似文献
16.
Hidenori Hiramatsu Toshio Kamiya Masahiro Hirano Hideo Hosono 《Physica C: Superconductivity and its Applications》2009,469(9-12):657-666
FeAs-based layered superconductors such as F-doped LaFeAsO have recently been investigated intensively because of their high superconducting transition temperatures. Epitaxial films of these compounds are important to examine their intrinsic materials properties as well as to transfer them to device applications. In this review, we first present our research route from transparent p-type oxides semiconductors to the Fe-based superconductors. Then we review growth of epitaxial thin films for the layered oxychalcogenides and oxypnictides. Reactive solid-phase epitaxy technique was inevitable to prepare epitaxial thin films of the oxychalcogenides and Zn-based oxypnictides. On the other hand, epitaxial thin films of Mn-based oxypnictides were grown by standard pulsed laser deposition. These techniques, however, did not grow epitaxial thin films for LaFeAsO. Thus, we developed a modified pulsed laser deposition process and succeeded in obtaining epitaxial thin films of FeAs-based superconductors, LaFeAsO and cobalt-doped SrFe2As2. 相似文献
17.
Klauss HH Luetkens H Klingeler R Hess C Litterst FJ Kraken M Korshunov MM Eremin I Drechsler SL Khasanov R Amato A Hamann-Borrero J Leps N Kondrat A Behr G Werner J Büchner B 《Physical review letters》2008,101(7):077005
We present a detailed study on the magnetic order in the undoped mother compound LaFeAsO of the recently discovered Fe-based superconductor LaFeAsO1-xFx. In particular, we present local probe measurements of the magnetic properties of LaFeAsO by means of 57Fe M?ssbauer spectroscopy and muon-spin relaxation in zero external field along with magnetization and resistivity studies. These experiments prove a commensurate static magnetic order with a strongly reduced ordered moment of 0.25(5)muB at the iron site below T(N)=138 K, well separated from a structural phase transition at T(S)=156 K. The temperature dependence of the sublattice magnetization is determined and compared to theory. Using a four-band spin density wave model both, the size of the order parameter and the quick saturation below T(N) are reproduced. 相似文献
18.
Electronic Structure and Optical Properties of La-Doped SrTiO3 and Sr2TiO4 by Density Function Theory 下载免费PDF全文
The effect of La doping on the electronic structure and optical properties of SrTiO3 and Sr2TiO4 is investigated by the first-principles calculation of plane wave ultrasoft pseudopotential based on the density function theory (DFT). The calculated results reveal that the electron doping in the case of Sr0.875La0.125TiO3 and Sr1.875La0.125TiO4 can be described within the rigid band model. The La3+ ions fully acts as electron donors in Sr0.875La0.125TiO3 and Sr1.875La0.125TiO4 systems and the Fermi level shifts further into the conduction bands (CBs) for Sr1.875La0.125TiO4 compared to Sr0.875La0.125TiO3. The two systems exhibit n-type degenerate semiconductor features. At the same time, the density of states (DOS) of the two systems shift towards low energies and the optical band gaps are broadened. The Sr1.875La0.125TiO4 is highly transparent with the transmittance about 90% in the visible range, which is larger than that of Sr0.875La0.125TiO3(85%). The wide band gap, small transition probability and weak absorption due to the low partial density of states (PDOS) of impurity in the Fermi level result in the optical transparency of the films... 相似文献