Cross sections of the reactions16O(γ,x)13 N and16O (γ,x)11 C,and Yield of12C (γ, t) up to 55 MeV

Yield curves of the reactions¹⁶O (γ, x)¹¹C,¹⁶O (γ, x)¹³N and¹²C(γ, t) have been measured relative to¹²C(γ, n)¹¹C with bremsstrahlung. The cross section σ[¹⁶O(γ, x)¹¹C] has a shape similar to σ[¹⁶O(γ, t)] and shows a broad maximum near 38 MeV. Differences between σ[¹⁶O(γ, x)¹³ N] and σ[¹⁶O(γ, t)] point to a reaction mechanism via quadrupole absorption in¹⁶O. The yield of¹²C(γ, t) exceeds the¹⁶O(γ,t) yield by a factor of two.     

Die Spektren der Neutronen aus den Reaktionen C12(γ,n)C11 und O16(γ,n)O15

The (γ, n)-reactions on carbon and oxygen were studied using the 30,5 MeV brems-strahlung beam of the Heidelberg betatron. The photoneutrons were detected via the recoil protons in a stilbene scintillator. The pulse height spectrum of scintillations produced in the stilbene crystal by the recoil protons is analyzed to yield the incident neutron energy distribution. Theγ-ray and electron background was strongly reduced through pulse shape discrimination. To test the apparatus the spectrum of the neutrons from a Po-α-Be source was measured. The energy spectrum of the photo-neutrons from O¹⁶ shows clearly two peaks at excitation energies of 22,4 and 24,4 MeV also seen in the photo-proton spectra. The energy distribution of the neutrons from C¹² (γ, n) too contains indication of structure already known from the proton spectra from C¹² (γ, p). The derived cross sections of C¹² (γ, n ₀) and O¹⁶ (γ, n ₀) coincide as well in their shape as in their absolute magnitude with the corresponding (γ, p ₀)-cross sections. In both C¹² (γ, n) and O¹⁶ (γ, n)-reaction the neutrons seem to leave the final nucleus mainly in its ground state.     

Astrophysical <Emphasis Type="Italic">S</Emphasis>-factor of T(<Superscript>4</Superscript>He, γ)<Superscript>7</Superscript>Li reaction at <Emphasis Type="Italic">E</Emphasis><Subscript>cm</Subscript> = 15.7 keV

The astrophysical S-factor of the reaction T(⁴He, γ)⁷Li is measured for the first time at the center of mass energy E _cm = 15.7 keV, lower than the energy range of the Standard Big Bang Nucleosynthesis (SBBN) model. The experiment is performed on a Hall pulsed accelerator (TPU, Tomsk). An acceleration pulse length of 10 μs allows one to suppress the background of cosmic radiation and the ambient medium by five orders of magnitude. A beam intensity of ~ 5 × 10^{14 4}He⁺ ions per pulse allows one to measure an extremely low reaction yield. The yield of γ-quanta with the energies E _γ ⁰ = 2483.7 keV and E _γ ¹ = 2006.1 keV is registered by NaI(Tl) detectors with the efficiency ε = 0.331 ± 0.026. A method for direct measurement of the background from the chain of reactions T(⁴He, ⁴He)T→T(T, 2n)X→(n, γ) and/or (n, n′γ) which ends by neutron activation of materials surrounding the target is proposed and implemented in this study. The value of the astrophysical S-factor of the reaction T(⁴He, γ)⁷Li S _αt (E _cm = 15.7 keV) = 0.091 ± 0.032 keV b provides the choice from the set of experimental data for the astrophysical S _αt -factor in favor of experimental data [4] with S _αt (E _cm = 0) = 0.1067 ± 0.0064 keV b.     

A proposed direct measurement of cross section at Gamow window for key reaction ~(19)F( p,α)~(16)O in Asymptotic Giant Branch stars with a planned accelerator in CJPL

In 2014, the National Natural Science Foundation of China(NSFC) approved the Jinping Underground Nuclear Astrophysics laboratory(JUNA) project, which aims at direct cross-section measurements of four key stellar nuclear reactions right down to the Gamow windows. In order to solve the observed fluorine overabundances in Asymptotic Giant Branch(AGB) stars, measuring the key ~(19)F( p,α)~(16)O reaction at effective burning energies(i.e., at Gamow window) is established as one of the scientific research sub-projects. The present paper describes this sub-project in details, including motivation, status, experimental setup, yield and background estimation, aboveground test, as well as other relevant reactions.     

Reliability of the data on the cross sections of the partial photoneutron reaction for <Superscript>63,65</Superscript>Cu and <Superscript>80</Superscript>Se nuclei

The cross sections of partial photoneutron reactions are evaluated for the ^63,65Cu and ⁸⁰Se isotopes. The cross sections are free of systematic uncertainties from shortcomings of the experimental methods for neutron multiplicity sorting based on measurements of neutron energy used in experiments with quasimonoenergetic annihilation photon beams. An experimental-theoretical method is used to evaluate cross sections σ^eval(γ, in)= F_i^theor σ^exp(γ, xn), where ratios F_i^theor = σ^theor(γ, in)/σ^theor(γ, xn) = σ^theor(γ, in)/σ^theor[(γ, 1n) + 2(γ, 2n) + …] are calculated using a combined model of photonuclear reactions, and σ^exp(γ, xn) is the experimental cross section of the neutron yield reaction free from neutron multiplicity sorting problems. The cross sections are evaluated for reactions (γ, 1n) and (γ, 2n) for the ^63,65Cu and ⁸⁰Se isotopes, and for the total photoneutron reaction σ(γ, Sn) = σ[(γ, 1n) + (γ, 2n) + …]. It is shown that noticeable deviations of the experimental cross sections from the evaluated values result from the unreliable sorting of neutrons between the channels with multiplicities 1 and 2.     

Investigation of the reaction mechanism for the four-particle photodisintegration of a carbon nucleus

The four-particle photodisintegration of a carbon nucleus in the reactions ¹²C(γ, p)³H2α and ¹²C(γ, n)³H2α is investigated by a method that employs a diffusion chamber in a magnetic field. It is shown that these reactions proceed according a sequential-type scheme: excited states of ¹¹B and ¹¹C nuclei decay to weakly excited states of ⁸Be, ⁷Li, and ⁷Be nuclei. It is concluded that nucleons are knocked out from the s shell. In the excitation curve for the 2α system in the reaction ¹²C(γ, p)³H2α, a resonance is found between the maxima corresponding to the ground and the first excited state of the ⁸Be nucleus, and this resonance is identified as a ghost anomaly. The branching fractions of the decay modes are determined. The angular distributions of nucleons in the reaction c.m. frame are measured. The energy dependence of the asymmetry coefficient for the angular distributions is obtained. A fast increase in this coefficient is observed in the energy range 38–40 MeV. It is concluded that the asymmetry coefficient depends on the excitation energy of the final nucleus in the region of intermediate photon energies.     

Study of background processes with the formation of neutrons in nuclear reactions in the energy range of 26–32 kev

The nature of background processes accompanying astrophysical nuclear reactions induced by hydrogen, helium, and neon ions in deuterated targets with small cross sections has been studied in calculations and experiments. The experiments have been performed at a Hall pulsed plasma accelerator in the ion energy range of 26–32 keV. The yield of background neutrons and γ-quanta with energies below 4 MeV in the proton-induced D(p, γ)³He reaction is primarily due to the presence of a natural impurity of gaseous deuterium in gaseous hydrogen and the chain of D(D, ³He)n → (n, γ) or (n, n'γ) reactions. A small contribution comes from the chain of D(¹H, ¹H)D → D(D, ³He)n → (n, γ) or (n, n'γ) reactions. It has been shown that background neutrons and γ-quanta from the D(4He, γ)6Li reaction are entirely due to the chain of D(⁴He, ⁴He)D → D(D, ³He)n → (n, γ) or (n, n'γ) reactions. It has been shown that the yield of neutrons and γ-ray photons detected at the interaction of neon ions with deuterated targets is also entirely due to the chain of elastic- scattering reactions of neon ions on deuterons in the target and to subsequent inelastic processes of interaction of deuterons accelerated at elastic scattering with other deuterons of the target. The main contribution to the yields of background neutrons and γ-quanta comes from doubly charged neon ions. The main conclusion is that the explanation of the yield of neutrons and γ-quanta at the interaction of hydrogen, helium, and neon ions with deuterated targets does not require “exotic” theoretical models.     

Einige seltene Kernphotoreaktionen an C,O und Si

The nuclide Be⁷ was produced by irradiating graphite and water with bremsstrahlung from the Darmstadt 60 MeV linear accelerator. Yield curves and approximate cross-sections are presented up to 57 MeV. Integrated cross-sections at 57 MeV are 6,0 MeV mbarn for C¹²(γ, x) Be⁷ and about 0,7 MeV mbarn for O¹⁶(γ, x) Be⁷. At 51,4 MeV maximum bremsstrahlung energy the yield of Si³⁰(γ, 2p Mg²⁸) is 1,6% of the C¹² (γ, n) C¹¹ yield, and about 3,8 times as much Na²⁴ as Mg²⁸ is produced in a natural silicon target.     

Die Energieverteilung der Neutronen aus einer Po-α-Be-Quelle

The neutrons from a Po-α-Be source were detected via the recoil protons in a stilbene scintillator. The pulse height spectrum of the scintillations produced in the stilbene crystal by the recoil protons is analysed to yield the incident neutron energy distribution. Theγ-ray background was eliminated through pulse shape discrimination. Separately the spectrum of neutrons coincident withγ-rays, i.e. of neutrons from the Be⁹(α,n)C^12* reaction, has been determined. The resulting spectra are compared to previous measurements. The structure of the spectra is not compatible with an isotropic angular distribution of the neutrons relative to theα-direction. Furthermore it could be shown that the fraction of reactions leading to the 7,65 MeV state of C¹² is only about 10^?3.     

Physical criteria for the reliability of data on the photodisintegration of the <Superscript>89</Superscript>Y nucleus

Experimental photonuclear reaction cross sections obtained in experiments using quasimonoenergetic annihilation, monoenergetic tagged photons, and bremsstrahlung γ-radiation are analyzed using physical criteria for the reliability of data on the ⁸⁹Y nucleus. It is found that the reliability of data on the cross sections of partial reactions (γ, 1n) and (γ, 2n), obtained by means of photoneutron multiplicity sorting, is highly doubtful. Reliable cross sections of reactions (γ, 1n) and (γ, 2n) are obtained using the experimental–theoretical method (ETM) for evaluating using both experimental cross sections of neutron yield reaction σ^exp(γ, xn) that are free of neutron multiplicity problems, and theoretically calculated F _i ^theor ratios of the cross sections of definite (i) partial reactions to cross section σ^theor(γ, xn). It is shown that the evaluated cross sections differ noticeably from the experimental data.     

Cross sections of the photoneutron reaction for <Superscript>141</Superscript>Pr and <Superscript>186</Superscript>W nuclei,estimated from physical criteria of data reliability

Using objective physical criteria for data reliability, cross sections of partial photoneutron reactions (γ, 1n), (γ, 2n) and (γ, 3n) that are free of the shortcomings of neutron multiplicity sorting methods used on beams of quasimonoenergetic annihilation photons are obtained for ¹⁴¹Pr and ¹⁸⁶W nuclei. Evaluation is performed using the experimental–theoretical method (ETM), based on the experimental cross section of neutron yield reaction σ^exp(γ, xn) = σ^exp(γ, 1n) + 2 σ^exp(γ, 2ⁿ) + 3 σexp(γ, 3n) + … and ratios F _i ^theor= σ^theor(γ, in)/σ^theor(γ, xn) calculated within the combined model (CM) of photonuclear reactions, which stipulates that σ^eval(γ, in) = F _i ^theor σ^exp(γ, xn). It is found that for ¹⁴¹Pr and ¹⁸⁶W, ratios F ^exp _i do not contradict the data reliability criteria only at energies up to ~21 and ~22 MeV, respectively. At the same time, there are notable discrepancies between F _i ^theor and F ^exp _i, and thus between the evaluated and experimental cross sections of reactions. It is shown that the discrepancies between the evaluated and experimental cross sections are due to the assumed unreliable experimental distribution of neutrons in the channels with multiplicities 1, 2, and 3.     

Zum Kernphotoeffekt am Ar40 und Ar38

Liquid Argon was irradiated with bremsstrahlung from 18 to 31 MeV endpoint energy in steps of 2 MeV. The yields of the reactions Ar⁴⁰(γ, n)+(γ, p) and Ar³⁸(γ, n) were measured by detecting the 269a and the 35d rest activity with a low-level-counter. Cross section curves for the (γ, n)-processes could be found from the yield values, and they allowed together withσ _N, σ(γ, p) andσ(γ, np) a determination ofσ(γ, 2n) and σ_γabs for Ar⁴⁰. The integrated cross section forσ(γ, n) from threshold to 33 MeV yields (200±40) MeVmb for Ar⁴⁰ and (210±40) MeVmb for Ar³⁸, the corresponding value for σ_γabs being (450±60) MeVmb for Ar⁴⁰.     

Zur (γ,p)- und (γ,np)-Reaktion am Argon 40

Argon gas has been irradiated with 34 MeV bremsstrahlung. The yields of the reactions A⁴⁰(γ, p) Cl³⁹ and A⁴⁰ (γ, np) Cl³³ were determined relative to C¹²(γ, n) by β-counting. The resulting upper limits for the cross sections integrated to 28 MeV are 160 MeVmbarns for (γ, p), and 35 MeV mbarns for (γ, np). This does not confirm the anomalously high A⁴⁰ (γ, p)-cross section reported in the literature.     

Untersuchungen über die Energieabhängigkeit von Kernreaktionen mit Neutronen im Energiebereich zwischen 12 und 19 MeV

Continuing earlier investigations we studied the energy dependence of the cross sections of the following nuclear reactions produced by neutrons in the energy range from 12 to 19 MeV: P³¹(n, 2n)P³², P³¹(n,α)Al²⁸, Cu⁶⁵(n, 2n)Cu⁶⁴, Cu⁶⁵(n, p)Ni⁶⁵, Zn⁶⁴(n, 2n)Zn⁶³, Zn⁶⁴(n, p)Cu⁶⁴, V⁵¹(n, p)Ti⁵¹, Br⁷⁹(n, α)As⁷⁶, O¹⁶(n, α)C¹³. The results were compared with cross sections calculated according to the statistical theory, considering the competition ofγ-ray emission and particle (predominantly neutron) emission from the excited residual nucleus.     

Parametric study of radiofrequency helium discharge under atmospheric pressure

The parameters of radiofrequency helium discharge under atmospheric pressure were studied by electrical and optical measurements using high voltage probe, current probe and optical emission spectroscopy. Two discharge modes α and γ were observed within certain limits. During α to γ mode transition, a decrease in voltage (280–168 V), current (2.05–1.61 A) and phase angle (76^°–56^°) occurred. The discharge parameters such as resistance, reactance, sheath thickness, electron density, excitation temperature and gas temperature were assessed by electrical measurements using equivalent circuit model and optical emission spectroscopy. In α mode, the discharge current increased from 1.17 to 2.05 A, electron density increased from 0.19 × 10¹² to 0.47 × 10¹² cm^?3 while sheath thickness decreased from 0.40 to 0.25 mm. The excitation temperatures in the α and γ modes were 3266 and 4500 K respectively, evaluated by Boltzmann’s plot method. The estimated gas temperature increased from 335 K in the α mode to 485 K in the γ mode, suggesting that the radiofrequency atmospheric pressure helium discharge can be used for surface treatment applications.     

Messung der Zirkularpolarisation der 478 keV-Gammaquanten aus der Reaktion Li6(d,p)Li7 mit 2 MeV-Deuteronen

The circular polarizationP _γ of 478 keVγ quanta from the reaction Li⁶(d, pγ) Li⁷ with 2 MeV deuterons was measured by forward Compton scattering from magnetized iron. The protons were observed at 25° lab angle. The fast neutron background in theγ detector was suppressed by pulse shape discrimination. The resultP _γ=+ 0.022 ± 0.17 with the Basel sign convention confines the ratio of the reduced widthsΘ _± for the capture of the neutron withj=1±1/2 to the regions ?2.36≦Θ ₊/Θ _?≦?0.74 or ?0.06≦Θ ₊/Θ _?≦+0.61.     

Relativmessung integrierter Wirkungsquerschnitte für den Kernphotoeffekt: Die Reaktion O16(γ, n)O15

Li₂CO₃ and Na₂C₄H₈O₈ have been irradiated by 34 MeV bremsstrahlung. The yield of the induced O¹⁵ activity has been measured relative to the yield of the C¹²(γ, n)C¹¹ resp. Cu⁶³(γ, n)Cu⁶² reaction by detecting the annihilation quanta. Additional yield measurements with the bremsstrahlung beam attenuated by 18 mm of lead were made to determine the ratio of the integrated cross sections for the reactions O¹⁶(γ, n)O¹⁵ and C¹²(γ, n)C¹¹ resp. Cu⁶³(γ, n)Cu⁶². Using the cross section ofBarber et al. for C¹²(γ, n)C¹¹, the cross section integrated up to 33 MeV for O¹⁶(γ, n)O¹⁵ was obtained to 61±7 MeVmb.     

Transient bi-fractional diffusion: space-time coupling inducing the coexistence of two fractional diffusions

Anomalous diffusion is researched within the framework of the coupled continuous time random walk model, in which the space-time coupling is considered through the correlated function g(t) ~ t ^γ , 0 ≤ γ< 2, and the probability density function ω(t) of a particle’s transition time t follows a power law for large t: ω(t) ~ t ^{? (1 + α)},1 <α< 2. The bi-fractional generalized master equation is derived analytically which can be applied to describe the transient bi-fractional diffusion phenomenon which is induced by the space-time coupling and the asymptotic behavior of ω(t). Numerical results show that for the transient bi-fractional diffusion, there is a transition from one fractional diffusion to another one in the diffusive process.     

Isomeric ratios of (γ,p) and (γ,α) reactions on <Superscript>117<Emphasis Type="Italic">m,g</Emphasis></Superscript>In

The isomeric ratios of the (γ,p) and (γ,α) reactions on ^117m,g In have been measured. The ratios Y _m /Y _g was found to be 1.18(9) and 0.23(9), respectively, at a boundary energy of 22 MeV. The statistical character of the reactions under such conditions is shown.     

Excitation of <Superscript>109</Superscript>Pd and <Superscript>112</Superscript>In nuclear isomers in (γ, <Emphasis Type="Italic">n</Emphasis>) reactions

Dependence of isomeric ratios on maximum photon energy in the reactions ¹¹⁰Pd(γ, n)^{109m, g} Pd and ¹¹³In(γ, n)^{112m, g} In is studied in the energy region of bremsstrahlung 9–18 MeV with the step ΔE = 0.5 MeV. Cross sections of population of the metastable state for ¹⁰⁹Pd and ¹¹²In in (γ, n) reactions were first obtained in the energy region under study. The obtained results are compared with the results of the calculation in the framework of the cascade-evaporation model.