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1.
K.?Koyasu M.?Niemietz W.?Westh?user G.?Gantef?r 《The European Physical Journal D - Atomic, Molecular, Optical and Plasma Physics》2009,53(1):59-62
The decay path of an Ag8(O2)- cluster photoexcited by a 3.1 eV photon is elucidated using time-resolved photoelectron spectroscopy. Photoabsorption results
in the formation of an excited state giving rise to a peak in the photoelectron spectra with well-resolved vibrational finestructure.
With a lifetime of about 100 fs this bound state decays into an anti-bonding state which dissociates into O2 and Ag8- on a timescale of 10 ps. In the photoelectron spectra, this corresponds to a broad maximum shifting gradually towards higher
binding energy while the O2 and Ag8- separate. Finally, the spectrum of bare Ag8- appears. This process is unique to small clusters, because on metal surfaces excited state lifetimes are too short to allow
for direct dissociation. 相似文献
2.
E. Govea-Alcaide I. García-Fornaris P. Muné R. F. Jardim 《The European Physical Journal B - Condensed Matter and Complex Systems》2007,58(4):373-378
Measurements of the electrical resistivity as a function
of temperature, ρ(T), for different values of applied
magnetic field, Ba (0 ≤ Ba ≤ 50 mT), were performed in
polycrystalline samples of Bi1.65Pb0.35Sr2Ca2
Cu3O10+δ subjected to different uniaxial compacting
pressure (UCP). We have found appreciable differences in the grain
orientation between samples by using X-ray diffractometry. From
the X-ray diffraction patterns performed, in powder and pellet
samples, we have estimated the Lotgering factor along the (00l)
direction, F(00l). The results indicate that F(00l)
increases ~23% with increasing UCP suggesting that grains
of these samples are preferentially aligned along the c-axis,
which is parallel to the compacting direction. The resistive
transition of the samples have been interpreted in terms of the
thermally activated flux-creep model. In addition, the effective
intergranular pinning energy, U0, have been determined for
different applied magnetic field. The magnetic field dependence of
U0, for Ba > 8 mT, was found to follow a H- α
dependence with α = 0.5 for all samples. The analysis of the
experimental data strongly suggested that increasing UCP results
in appreciable changes in both the grain alignment and the grain
connectivity of the samples. We have successfully interpreted the
data by considering the existence of three different
superconducting levels within the samples: the superconducting
grains, the weak-links, and the superconducting clusters. 相似文献
3.
M. B. Das S. Karmakar 《The European Physical Journal D - Atomic, Molecular, Optical and Plasma Physics》2006,40(3):339-341
Lifetimes of eight levels belonging to the 5p46d configuration of
singly ionized xenon have been measured by high frequency deflection
technique with a delayed coincidence single photon counting arrangement. The
results have been compared with other experimental and theoretical values.
The lifetimes of the 6d 2F3/2 and 6d 4F3/2 levels have
been measured for the first time. 相似文献
4.
M. Bonura A. Agliolo Gallitto M. Li Vigni C. Ferdeghini C. Tarantini 《The European Physical Journal B - Condensed Matter and Complex Systems》2008,63(2):165-177
We report on the microwave surface resistance of two
polycrystalline Mg11 B2 samples; one consists of
pristine material, the other has been irradiated at very high neutron
fluence. It has already been reported that in the strongly irradiated
sample the two gaps merge into a single value. The mw surface resistance
has been measured in the linear regime as a function of the temperature and the DC magnetic
field, at increasing and decreasing fields. The results obtained in the
strongly irradiated sample are quite well justified in the framework of a
generalized Coffey and Clem model, in which we take into account the field
distribution inside the sample due to the critical state. The results
obtained in the pristine sample show several anomalies, especially at low
temperatures, which cannot be justified in the framework of standard
models for the fluxon dynamics. Only at temperatures near Tc and for
magnetic fields greater than 0.5Hc2(T) the experimental data can quantitatively be
accounted for by the Coffey and Clem model, provided that the
upper-critical-field anisotropy is taken into due account. 相似文献
5.
M. S. B. Darby T. C. May-Smith R. W. Eason 《Applied Physics A: Materials Science & Processing》2008,93(2):477-481
We have demonstrated pulsed laser deposition of Nd-doped gadolinium gallium garnet on Y3Al5O12 by the simultaneous ablation of two separate targets of Nd:Gd3Ga5O12 (GGG) and Ga2O3. Such an approach is of interest as a method of achieving stoichiometry control over films whilst the growth parameters are
kept constant and optimal for high quality crystal growth. We show here how the stoichiometry and resultant lattice parameter
of a film can be controlled by changing the relative deposition rates from the two targets. Films have been grown with enough
extra Ga to compensate for the deficiency that commonly occurs when depositing only from a GGG target. We have also grown
crystalline GGG films with an enriched Ga concentration, and this unconventional approach to film stoichiometry control may
have potential applications in the fabrication of films with advanced compositionally graded structures. 相似文献
6.
K. Araki T. Goto Y. Nemoto T. Yanagisawa B. Lüthi 《The European Physical Journal B - Condensed Matter and Complex Systems》2008,61(3):257-259
The temperature dependence of the elastic constants in
Tb3Ga5O12 was measured and analysed with a simple crystal
field model. The magneto-elastic coupling constants have been deduced from
this experiment. The coupling constant gΓ5, related to the
c44 mode, is anomalously large. These coupling constants are important
for the interpretation of the phonon Hall effect. 相似文献
7.
8.
B. Schmidt V. Yushankhai L. Siurakshina P. Thalmeier 《The European Physical Journal B - Condensed Matter and Complex Systems》2003,32(1):43-47
A pronounced Curie-like upturn of the magnetic susceptibility χ(
T
) of the quasi one-dimensional spin chain compound Ba2V3O9 has been found recently [#!kaul:02!#]. Frequently this is taken as a signature for a staggered field mechanism due to the
presence of g-factor anisotropy and Dzyaloshinskii-Moriya interaction. We calculate this contribution within a realistic structure of vanadium
3
d- and oxygen 2
p-orbitals and conclude that this mechanism is far too small to explain experimental results. We propose that the Curie term
is rather due to a segmentation of spin chains caused by broken magnetic bonds which leads to uncompensated S
= ? spins of segments with odd numbers of spins. Using the finite-temperature Lanczos method we calculate their effective moment
and show that ∼ 1% of broken magnetic bonds is sufficient to reproduce the anomalous low-T behavior of χ(
T
) in Ba2V3O9.
Received 19 December 2002 / Received in final form 29 January 2003 Published online 14 March 2003 相似文献
9.
X. D. Zhang M. L. Guo C. L. Liu L. A. Zhang W. Y. Zhang Y. Q. Ding Q. Wu X. Feng 《The European Physical Journal B - Condensed Matter and Complex Systems》2008,62(4):417-421
A first-principles study has been performed to evaluate the electronic and
optical properties of wurtzite Zn1-xMgxO. Substitutional doping is
considered with Mg concentrations of x = 0, 0.0625, 0.125, 0.1875 and 0.25,
respectively. Mg incorporation can induce band gap widening due to the
decrease of Zn 4s states. The imaginary part of the dielectric function shows
that the optical transition from band edge emission decreases slightly with
increasing Mg contents. The optical band gap also increases from 3.2 to 3.7
eV with increasing Mg contents from 0.0625 to 0.25. The calculated results
suggest that relatively high Mg concentration is necessary for effective
band gap engineering of wurtzite Zn1-xMgxO. 相似文献
10.
Z.-S. Liu 《Applied Physics A: Materials Science & Processing》2009,95(2):443-445
In a rare-earth antiferromagnet, two neighboring magnetic ions order spontaneously in opposite directions below the Néel temperature.
Especially when it is placed in an external magnetic field, the two magnetic ions react to the field in different ways, so
that they usually have different magnitudes and orientations below the magnetic transition temperature. Therefore, to describe
the magnetic structure of an antiferromagnet, the single-ion ferromagnetic-like model is inadequate. To solve this problem,
a two-ion model for rare-earth antiferromagnets is proposed and used in this work to investigate the magnetic properties of
DyNi2B2C. The magnetic susceptibility curves obtained with this model show good agreements with experimental data. 相似文献
11.
N. Coluccelli G. Galzerano L. Bonelli A. Toncelli A. Di Lieto M. Tonelli P. Laporta 《Applied physics. B, Lasers and optics》2008,92(4):519-523
We present a comparative analysis on the growth, the spectroscopic features, and the cw laser action of room-temperature Yb(5%):LiYF4 (YLF) and Yb(10%):KYF4 (KYF) crystals. Optical slope efficiencies of 33% and 52% have been demonstrated for Yb:YLF and Yb:KYF crystals, respectively.
A remarkable wide wavelength tunability from 1.01 to 1.07 μm has been obtained for both laser crystals. 相似文献
12.
S. Ramasubramanian M. Rajagoplan R. Thangavel J. Kumar 《The European Physical Journal B - Condensed Matter and Complex Systems》2009,69(2):265-268
Elastic and Thermodynamical properties of Ti1-xZrxC have been investigated using LAPW + lo within the density-functional theory with the generalized gradient approximation.
We have studied the stability of the alloy Ti1-xZrxC as a function of Zr composition in rocksalt (B1) structure by calculating the elastic constants C11, C12 and C44 using the tetragonal and trigonal distortions. Mechanical properties such as Poisson ratio, bulk, shear and Young’s modulii
of Ti1-xZrxC are calculated. The Debye temperature and hardness are also computed for the first time to our knowledge for Ti1-xZrxC in various compositions. 相似文献
13.
O.-H. Kwon H. Yoo D.-J. Jang 《The European Physical Journal D - Atomic, Molecular, Optical and Plasma Physics》2002,18(1):69-75
While the intercalation of C60 and the formation of C
60
-
in the supercages of NaX and NaY are confirmed by using 129Xe NMR and ESR, the photophysical properties of C60 and C
60
-
are characterized by monitoring transient reflectance spectra and kinetics, fluorescence kinetics, and diffuse reflectance
spectra. C
60
-
is considerably more abundant in NaY than in NaX. This difference is explained in terms of polarity difference between two
zeolites. Both C60 and C
60
-
have remarkably elongated excited-state lifetimes due to their collision-free environment in zeolitic nanocavities although
C
60
-
has much shorter lifetimes than C60. C
60
-
, in particular, shows intense absorption and emission due to its reduced symmetry in zeolites.
Received 13 July 2001 and Received in final form 8 October 2001 相似文献
14.
A.-S. Rüetschi D. Jaccard 《The European Physical Journal B - Condensed Matter and Complex Systems》2009,67(1):43-49
High pressure resistivity measurements of the organic compound (TMTTF)2BF4 have been performed in a newly developped Bridgman cell providing good pressure conditions on a wide pressure range. For
the first time in this compound a zero resistance superconducting state is observed between 3 and 4 GPa. At temperatures above
the superconducting transition, the resistivities of the two high quality samples show a different behavior. One sample, provides
indications for a magnetic quantum critical point at the maximum of Tc, whereas in the other antiferromagnetic spin-fluctuations are present above Tc. 相似文献
15.
Francis Leonard Deepak Alvaro Mayoral Miguel Jose Yacaman 《Applied Physics A: Materials Science & Processing》2009,96(4):861-867
The structural transformation of MoO3 nanobelts into MoS2 nanotubes using a simple sulfur source has been reported. This transformation has been extensively investigated using electron
microscopic and spectroscopic techniques including scanning electron microscopy (SEM), transmission electron microscopy (TEM),
high-resolution transmission electron microscopy (HRTEM), electron diffraction (ED), and energy-dispersive X-ray analysis
(SEM-EDAX and TEM-EDX). The method described in this report will serve as a generic route for the transformation of other
oxide nanostructures into the chalcogenide nanostructures. 相似文献
16.
C. Michail A. Toutountzis S. David N. Kalyvas I. Valais I. Kandarakis G. S. Panayiotakis 《Applied physics. B, Lasers and optics》2009,95(1):131-139
The aim of the present study was to measure the imaging transfer characteristics and the luminescence efficiency (XLE) of
a Lu2SiO5:Ce (LSO:Ce) powder scintillator for use in X-ray mammography detectors. An LSO:Ce powder scintillating screen, with a coating
thickness of 25 mg/cm2, was prepared in our laboratory. The imaging performance of the screen was assessed by experimental determination of the
modulation transfer function (MTF) and the detective quantum efficiency (DQE) as well as single index image quality parameters
such as noise equivalent pass band (Ne) and informational efficiency (n
I). A theoretical model, describing radiation and light transfer, was fitted to experimental MTF values in order to estimate
optical properties of the scintillator. Screen irradiation was performed under exposure conditions employed in mammographic
applications (27 kVp, 63 mAs). MTF was determined by the square wave response function (SWRF) method. Results showed that
LSO:Ce exhibits high MTF and DQE values, which are comparable to those of the commercially used Gd2O2S:Tb. Considering our image quality parameters and luminescence efficiency results as well as the fast response of the LSO:Ce
scintillator screen (40 ns), this material can be considered for use in X-ray mammographic detectors. 相似文献
17.
C.-X. Ji J. J. Yang A. K. Bengtson D. Morgan H. Xiang M. S. Rzchowski Y. A. Chang 《Applied Physics A: Materials Science & Processing》2009,97(1):73-77
The tunneling magnetoresistance of Co70Fe30/AlO
x
/Co70Fe30 magnetic tunnel junctions with epitaxial bottom electrode annealed at different temperatures was studied. The TMR was significantly
enhanced when the bottom electrodes were annealed at 300°C and above. The interface roughness, barrier width and height are
almost identical within the experimental uncertainty. However, high resolution reciprocal space mapping studies showed that
the lattice distortion of the epitaxial bottom electrodes from body centered cubic to body centered tetragonal had the same
trend as the TMR. The tetragonal lattice distortion is attributed to be the dominant factor for this spin polarization enhancement. 相似文献
18.
S. Kang Y.-M. Liu T.-Y. Shi 《The European Physical Journal B - Condensed Matter and Complex Systems》2008,63(1):37-42
The energy spectra of H2
+-like impurities confined in
finite spherical quantum dots have been calculated as a function
of the distance between nuclear with different sizes on the basis
of effective-mass approximation by linear variational method.
B-splines have been used as basis functions, which can easily
construct the trial wavefunctions with appropriate boundary and
cusp conditions. The quantitative analyses of the partial wave
weights for ground state and some low lying states have been done. 相似文献
19.
S. W. Tang L. L. Sun J. D. Feng H. Sun R. S. Wang Y. F. Chang 《The European Physical Journal D - Atomic, Molecular, Optical and Plasma Physics》2009,53(2):197-204
A systematic investigation of D3 C32 fullerene and its derivatives C32Xn (X = H and Cl) has been performed using B3LYP/6-31G(d) method based on the density functional theory. The geometry structures,
reaction energies, relative stabilities, and electronic properties have been studied. By investigating the possible C32Xn (X = H and Cl) molecules, C32H2 and C32Cl2 behave more thermodynamically accessible with respect to other derivatives. The frontier molecular orbitals and electronic
density of states calculations of C32X2 system indicate that H and Cl passivation have less contribution to the electronic structures, but significantly improve
the stability of D3 C32 fullerene. Finally, the 13C NMR chemical shifts of C32H2 and C32Cl2 have been simulated to provide helpful information for further experiment identification. 相似文献
20.
Syed B. Qadri Anthony Garzarella Terrence Wieting Dong Ho Wu Nadeemullah A. Mahadik 《Applied Physics A: Materials Science & Processing》2009,94(4):1011-1013
Sr0.75Ba0.25NbO3 (SBN-75) has the tungsten-bronze structure with a tetragonal unit cell and exhibits electro-optic properties that are important
for sensors. Due to its quaternary nature, its structural uniformity, integrity, and homogeneity become important for these
applications. In this paper, we present high-resolution X-ray diffraction studies of the crystalline quality and lattice parameter
variation across the surface of single crystals of SBN-75. Using rocking curves, topographs, and point-wise measurements of
lattice parameters, we show that these crystals have a high degree of crystalline quality and microscopic homogeneity for
any electro-optic application. 相似文献