Nicole: New on-line orientation facility at ISOLDE/CERN

This paper presents off-line and on-line orientation results obtained with the new on line nuclear orientation device NICOLE in CERN. Magnetic moments of^187,185Pt ^g and¹⁸⁶Ir ^m , electric quadrupole moment ratios between Pt isotopes with mass number 185, 187 and 189, the spin of the 2 h isomer of¹⁸⁶Ir and a new decay scheme of¹⁸⁴Au involving a metastable state are established. The shape variation versus mass number of the Pt isotopes leads to sign change of the spectroscopic quadrupole moment between A=187 and 185.     

New developments and trends in NMR-ON

New developments and new trends in NMR-ON are presented, especially in the context of precise measurements of nuclear magnetic moments and electric quadrupole moments of short-lived nuclei far off stability with on-line nuclear orientation techniques. The main emphasis is put on the following items:

1. Quadrupole-interaction-resolved NMR-ON (QI-NMR-ON): It is shown that hcp-Co is an ideal matrix for precise measurements of electric quadrupole moments of radioactive nuclei in the region Hg, Au, Pt, Ir, Os. Recently, the first on-line experiment was performed successfully at NICOLE/ISOLDE-CERN and the very interesting quadrupole moment of¹⁸⁶Au could be determined precisely.
2. General problems with lattice location and NMR-ON line widths in long decay chains, such as “lattice-site conservation” by implantation of a suitable precursor.
3. β-decay-induced lattice site change. In the context of integral nuclear orientation measurements on nuclei far off stability, where the β-decay energies become large, lattice site changes may occur, which make the interpretation of γ-anisotropies measured by integral and even time-differential techniques difficult or even impossible. A pilot experiment is described, in which such a β-decay-induced lattice site change has been identified by a double-resonance NMR-ON measurement.

     

Studies of low-lying states of even-even Xe isotopes within the nucleon pair approximation

We study the relevance of nucleon pairs with higher spins, in addition to spin-zero and spin-two pairs (i.e., SD pairs), in low-lying states of even-even Xe nuclei. By including those higher-spin pairs in our configuration, we recalculate energy level schemes, electrical quadrupole moments, magnetic moments and electric quadrupole transition rates, for low-lying states of even-even ^128–142Xe nuclei. The agreement between our calculated results and the experimental data is substantially improved in comparison with previous studies.     

Nuclear moment determination by Mössbauer effect detection of low temperature nuclear orientation (No/Me)

Absorption Mössbauer spectra were measured on low temperature (6–21 mK) oriented nuclei. For magnetic orientation this method allows the determination of the sign of the parent state magnetic moment. The method enables the determination of the parent state quadrupole coupling even for a polycrystalline sample. Signs of ground state magnetic moments for¹⁹¹Pt and¹⁹³Os, and electric quadrupole moments for¹²⁵Te^m and¹²⁹Te are determined.     

Recent developments and new trends in NMR on oriented nuclei

Recent developments in nuclear magnetic resonance on oriented nuclei (NMR-ON) are reviewed with the following main topics: (i) Measurement of magnetic moments. In this context the resonance shift of NMR-ON resonances with an external magnetic field is discussed critically. (ii) Resonance techniques for the measurement of electric quadrupole moments. It is shown that — with hcp-Co as host matrix — the techniques QI-NMR-ON (quadrupole-interaction-resolved NMR-ON) and MAPON (modulated adiabatic passage on oriented nuclei) have a tremendous potential for the measurement of quadrupole moments of radioactive nuclei. Data are presented for medium (Zr, Nb) and heavy elements (Ir, Pt, Au, Hg). With results on the 11/2^– isomers in Au it is shown that MAPON yields highly precise quadrupole moments of states with half-lives of the order of seconds, for which no other technique with comparable precision exists up to now. In the case of⁹⁰Nb it is demonstrated that MAPON allows also the measurement of very small quadrupole moments with high precision. (iii) Electric field gradients in cubic Fe, fcc-Co and Ni. MAPON experiments show a strong magnetic-field dependence of the effective quadrupole interaction; the implications are discussed. (iv)-decay-induced lattice site change identified by a double-resonance NMR-ON measurement. The resulting change of the hyperfme interaction has severe consequences for the interpretation of time-integral and even time-differential nuclear orientation measurements on nuclei far off stability. (v) Spin-lattice relaxation for nuclei on non-substitutional lattice sites. Recent experiments support the global character of the spin-lattice relaxation, in contrast to the local character of the static magnetic hyperfine interaction. (vi) Magnetic-field dependence of the spin-lattice relaxation. Recent experiments with hcp-Co as host lattice strongly support the so-called enhancement factor model and disfavour the one-, two- or three-magnon processes postulated in the literature.     

Ground-state properties of neutron-deficient platinum isotopes

The hyperfine structure splitting and the isotope shift in the =266 nm transition of Pt isotopes within the mass range 183 A 198 have been determined by Resonance Ionization Mass Spectroscopy (RIMS) in combination with Pulsed-Laser Induced Desorption (PLID). The Pt isotopes were obtained at the on-line isotope separator ISOLDE-3/CERN as daugthers of the primarily produced Hg isotopes. Magnetic moments, quadrupole moments, and changes in the mean-square charge radii are deduced and compared with results of a particle-triaxial rotor model and mean field calculations. Good agreement with experimental data (including nuclear level schemes and transition probabilities) can only be obtained if triaxial shape is admitted. The calculations yield a smooth transition in the shape of odd-A Pt nuclei from a slightly deformed, nearly oblate¹⁹⁵Pt via triaxial^197-187Pt to a strongly deformed nearly prolate¹⁷⁷Pt.Dedicated to P. Armbruster on the occasion of his 60th birthday     

Optical polarization of neutron-rich sodium isotopes and β-NMR measurements of quadrupole moments

The nuclear quadrupole moments of neutron-rich sodium isotopes are being investigated with the help of in-beam polarization by optical pumping in combination with-NMR techniques. First measurements have yielded the quadrupole splittings of NMR signals in the lattice of LiNbO₃ for the isotopes²⁶Na,²⁷Na and²⁸Na. Interaction constants and ratios of the electric quadrupole moments are derived. In view of future experiments,-decay asymmetries for the sequence of isotopes up to theN=20 neutron shell closure,^26–31Na, have been measured.     

Measurement of electric quadrupole moments of neutron-rich nuclei14B and15B

The experimental study of nuclear moments of several neutron-rich nuclei, using the phenomenon of ejectile spin polarization in the projectile fragmentation reaction, is reported. The spin-polarized fragments¹⁴B and¹⁵B were produced in the fragmentation of¹⁸O projectiles on a Nb target at 64.7 MeV/u. They were implanted into a Mg single crystal, and the quadrupole momentsQ were determined by the-NMR method. The results, ¦Q(¹⁴B)¦ =29.84 ±0.75 mb and ¦Q(¹⁵B)¦=38.01 ±1.08 mb, are compared with theoretical models. Shell model calculations in a 0 model space, using effective charges commonly accepted in this mass region, predict values about 40% larger than the experimentalQ(¹⁵B). Agreement is obtained when a much smaller effective charge for neutrons is employed. The method was also applied to the measurement of the magnetic moments of¹⁷N and¹⁷B. The result reveals an important contribution of configurations with excess neutrons coupled to formJ =2⁺.     

Nuclear magnetic moment of 12 d 11/2− 131mXe

NMR-ON measurements were performed on^131mXe (I=11/2^–; T_1/2=12.0 d) in Fe, the sample being prepared by recoil implantation after the¹³⁰Te(,3n)^131mXe compound reaction at E=40 Mev. The hyperfine splitting _NB_HF/h¦, extrapolated to zero external magnetic field, was found to be 209.9(1) MHz. Taking B_HF=+1523(8) kG for the hyperfine field of XeFe, the magnetic moment of^131mXe is deduced to be (–)0.994(5) _N. As a byproduct, the zero-field hyperfine splitting of^129mXe (I=11/2^–; T_1/2=8.9d) in Fe was measured as 188.1(1) MHz, with which a magnetic moment of (–)0.891(5) _N is deduced for^129mXe.     

Nuclear moments around the Z=40 shell closure:91mY,95Zr and97Nb

Magnetic moments around the Z=40 shell closure have been established using nuclear magnetic resonance on oriented nuclei (NMR/ON) in iron. From the resonance frequencies we established |μ(⁹¹Y;9/2⁺)|=5.96(6)μ_N, |μ(⁹⁵Zr;5/2⁺)|= 1.103(23)μ_N, | μ(⁹⁷Nb;9/2⁺)| = 6.153(5)μ_N. From the electric quadrupole alignement of⁹⁵Zr+⁹⁵Nb in a Zr single crystal Q(⁹⁵Zr)=+0.29(5)b and Q(⁹⁵Nb)<0 have been derived. The results obtained are discussed using the Nilsson deformed single particle model. It is shown that for certain deformation regions, a measurement of the magnetic moment can give information on the nuclear quadrupole deformation. the NICOLE-ISOLDE Collaboration, CERN     

Pionic degrees of freedom in atomic nuclei and quasielastic knockout of pions by high-energy electrons

The microscopic mechanism of the identical bands in odd-odd nucleus ¹⁹⁴Tl and its neighbor odd-A nuclei ^193,195Tl is investigated using the particle-number-conserving (PNC) method for treating the cranked shell model with monopole and quadrupole pairing interactions. It is found that the blocking effect of the high-j intruder orbital plays an important role in the variation of moments of inertia (J⁽¹⁾ and J⁽²⁾) with rotational frequency for the superdeformed bands and identical bands. The variation of the occupation probability of each cranked orbital and the contributions to moment of inertia from each cranked orbital are presented.     

Rare-earth nuclei and the pseudo-SU(3) model

An extended version of the pseudo-SU(3) model is used to describe low-energy positive-parity states of three rare-earth nuclei in a full proton-neutron formalism. Along with other residual interactions, the Hamiltonian includes the pairing which induces mixing between different representations of SU(3). Excitation energies, B(E2) values, B(M1) values, quadrupole moments, andg _R factors of¹³⁶Xe,¹³⁸Ba, and²⁰⁴Hg are calculated in a truncation free environment and the results are compared with the experimental data and other theories.     

Giant quadrupole moment andproton halo discovered in8B

The nuclear quadrupole moment of⁸B(I =2⁺,T _1/2=769 ms) has been determined by use of a modified -NMR detection as |Q(⁸B)|=68.3±2.1 mb, which is twice the prediction of the Cohen-Kurath shell model calculation. The anomalous quadrupole moment which is carried mainly by the protons in the nucleus, has been accounted for by the proton halo effect.     

Dimension six corrections to the vector sector of AdS/QCD model

We study the effects of dimension six terms on the predictions of the holographic model for the vector meson form factors and determine the corrections to the electric radius, the magnetic and the quadrupole moments of the ρ  -meson. We show that the only dimension six terms which contribute nontrivially to the vector meson form factors are X²F²$X^2{F}^2$ and F³$F^3$. It appears that the effect from the former term is equivalent to the metric deformation and can change only masses, decay constants and charge radii of vector mesons, leaving the magnetic and the quadrupole moments intact. The latter term gives different contributions to the three form factors of the vector meson and changes the values of the magnetic and the quadrupole moments. The results suggest that the addition of the higher dimension terms improves the holographic model.     

Laser spectroscopy and the properties of light nuclei near the neutron drip line

The interesting nuclear structure phenomena observed in some light nuclei at the neutron drip line suggest the measurement of basic ground state properties such as spins, magnetic moments and electric quadrupole moments. Here it will be discussed what experiments are presently feasable using laser spectroscopy. For the outstanding example of a halo nucleus,¹¹Li, the development of a technique combining -asymmetry detected optical pumping in a fast beam with NMR spectroscopy has yielded pertinent results, the most recent of which is an experimental value of the nuclear quadrupole moment.     

High-spin isomers in W and Os nuclei; Competition betweenK-quantization and triaxiality

Results of a search for high-spin isomers in W and Os nuclei withN=104–107 are presented. Targets of⁴⁸Ca and^{48, 50}Ti are bombarded with a pulsed¹³⁶Xe beam, and delayed gamma-radiation is detected by an array of NaI- and Ge-detectors. Several new isomers, with spin values up to ～22h, are found in^178,180W and^{180, 182, 183}Os. Markedly different decay patterns and hindrance factors are found in the Os isotopes as compared to the expectations based on theK-selection rule valid for axially symmetric nuclei. The findings are ascribed to the onset of triaxial distortions.     

Control of the nuclear spin of the <Superscript>129</Superscript>Xe and <Superscript>131</Superscript>Xe isotopes in the spin-exchange interaction with <Superscript>87</Superscript>Rb atoms

Nuclear spin dynamics of the ¹²⁹Xe and ¹³¹Xe isotopes in an external magnetic field B ₀ is considered. Nuclear spin is pumped by the laser through ⁸⁷Rb, which transfers the electron spin to the ¹²⁹Xe and ¹³¹Xe nuclei in the spin-exchange interaction. The nuclear spin dynamics is controlled with a transverse magnetic field that causes nuclear magnetic resonance in both ¹²⁹Xe and ¹³¹Xe isotopes. Numerical calculations are performed to find conditions at which the transverse component of the nuclear spin in the established motion is of maximum and the slope angle relative to the vector of the constant magnetic field B ₀ is 45°. This regime is taken to be optimal for simulation of practical applications. It is also found that the pump of the nuclear spin of xenon is strongly attenuated when the rubidium polarization vector is turned to the plane perpendicular to the external magnetic field vector B ₀.     

Nuclear moments and charge radii of107–111in determined by laser spectroscopy

Collinear fast beam laser spectroscopy has been used to measure the hyperfine structure and isotope shift in the atomic 5s ² 5p ² P _3/2-5s ² 6s ² S _1/2 transition (λ=451 nm) of^107–111In. Secondary beams of neutron deficient indium isotopes were prepared at the GSI on-line mass separator following fusion evaporation reactions. Magnetic dipole moments and electric quadrupole moments have been determined. The isotope shifts are discussed in terms of the change of the mean square nuclear charge radii and compared with the droplet model predictions and the deformation values calculated from the quadrupole moments.