Study of quasi-phase matching wavelength acceptance bandwidth for periodically poled LiNbO3 crystal-based difference-frequency generation

The temperature tuning characteristics of quasi-phase matching (QPM) wavelength acceptance bandwidth in a uniform periodically poled lithium niobate (PPLN) based on difference-frequency generation (DFG) are studied theoretically and experimentally. This paper proposes a PPLN device consisting of several segments of different temperatures to obtain a more desirable performance for the QPM-DFG. The result shows that through the tuning of temperature, the bandwidth can be changed considerably and the method was proved suitable and accurate to calculate QPM wavelength acceptance bandwidth of DFG in a uniform PPLN crystal for temperatures between room temperature and 180 °C and mid-infrared (mid-IR) wavelengths ranging from 2.8 to 4.8 μm.     

Optimization of optical parametric chirped pulse amplification with different pump wavelengths

Optical parametric chirped pulse amplification with different pump wavelengths was investigated using LBO crystal, at signal central wavelength of 800 nm. According to our theoretical simulation, when pump wavelength is 492.5 nm, there is a maximal gain bandwidth of 190 nm centered at 805 nm in optimal noncollinear angle using LBO. Presently, pump wavelength of 492.5 nm can be obtained from second harmonic generation of a Yb:Sr₅(PO₄)₃F laser. The broad gain bandwidth can completely support ∼6 fs with a spectral centre of seed pulse at 800 nm. The deviation from optimal noncollinear angle can be compensated by accurately tuning crystal angle for phase matching. The gain spectrum with pump wavelength of 492.5 nm is much better than those with pump wavelengths of 400, 526.5 and 532 nm, at signal centre of 800 nm.     

Broadband four-wave optical parametric amplification in bulk isotropic media in the ultraviolet

We report on four-wave optical parametric amplification of the ultrashort ultraviolet light pulses in bulk fused silica and CaF₂. Exact phase-matching in these isotropic media is achieved by means of non-collinear interaction with cylindrical beam focusing. Four-wave optical parametric amplifier efficiently operates in the UV spectral range with 1-ps laser pulses, delivering amplified signal energy exceeding 50 μJ using millijoule pump pulses in the visible (527 nm). Results of scanning of the parametric gain profile suggest that broad amplification bandwidth as wide as ∼20 nm (at FWHM) under these experimental settings is achieved, which might support amplification of sub-10-fs ultraviolet pulses with central wavelength around 330 nm. It is also shown experimentally and verified theoretically that the parametric gain profile exposes a distinct inhomogeneity and its bandwidth notably broadens due to effects of self- and cross-phase modulation imposed by the intense pump beam.     

A 9.5-W 82-MHz-repetition-rate picosecond optical parametric generator with cw diode laser injection seeding

We report on an injection-seeded 9.5-W 82-MHz-repetition-rate picosecond optical parametric generator (OPG) based on a 55 mm long crystal of periodically poled lithium niobate (PPLN) with a quasi-phase-matching (QPM) grating period of 29.75 μm. The OPG is excited by a continuously diode pumped mode-locked picosecond Nd:YVO₄ oscillator-amplifier system. The laser system generates 7 ps pulses with a repetition rate of 82.3 MHz and an average power of 24 W. Without injection-seeding the total average output power of the OPG is 8.9 W, which corresponds to an internal conversion efficiency of 50%. The wavelengths of the signal and idler waves were tuned in the range 1.57–1.64 μm and 3.03–3.3 μm, respectively, by changing the crystal temperature from 150 °C to 250 °C. Injection seeding of the OPG at 1.58 μm with 4 mW of single frequency continuous-wave radiation of a distributed-feedback (DFB) diode laser increases the OPG output to 9.5 W (53% conversion efficiency). The injection seeding increases the pulse duration and reduces the spectral bandwidth. When pumped by 10 W of 1.06 μm laser radiation, the duration of the signal pulses increased from 3.6 ps to 5.5 ps while the spectral bandwidth is reduced from 4.5 nm to 0.85 nm. Seeding thus improved the time-bandwidth product from 1.98 to a value of 0.56, much closer to the Fourier limit. Received: 29 April 2002 / Published online: 8 August 2002     

Widely tunable difference frequency generation around 3.4 μm using index dispersion property of PPLN

In this paper, the wide difference frequency generation (DFG) tuning characteristics around 3.4 μm are investigated by using the index dispersion property of PPLN. With a ytterbium doped fiber laser (YDFL) and an erbium doped fiber laser (EDFL) as the fundamental light sources, our simulation results show that the quasi-phase matching (QPM) wavelength acceptance bandwidth (BW) for the pump is much larger than that for the signal. Although the positions of the broadened QPM pump bands vary with the poling period and the signal wavelength, the corresponding idler tuning ranges center around 3.4 μm. With a signal wavelength of 1.57 μm, an idler tuning range of greater than 170 nm is experimentally obtained in the 30 uniform grating PPLN. When the signal wavelength and the poling period are respectively changed to 1.55 and 29.50 μm, wide DFG tuning operations around 3.4 μm are also achieved with the crystal temperature adjusted to adapt the change.     

Narrow-band terahertz wave generation and detection in one periodically poled lithium niobate crystal

In this article, we present studies on therahertz (THz) wave generation and frequency up-conversion in a periodically poled lithium niobate (PPLN) crystal. A frequency at 1.37 THz was generated as femtosecond pump pulses passed through a PPLN crystal with grating periods of 30 μm. The pump-induced THz wave interacts with the probe wave in the crystal by frequency mixing. The frequency up-converted THz wave is easily detected by a normal photodiode. A new scheme for generation and detection of THz wave in one non-linear crystal was proposed.     

3.5-μm high-resolution gas sensing employing a LiNbO3 QPM-DFG waveguide module

Diode laser technology coupled with a wavelength-conversion unit to produce mid-infrared narrow bandwidth laser light applicable to trace-gas detection and with the potential for high-resolution spectroscopy is described. Quasi-phase-matched difference-frequency generation (QPM-DFG) in a compact and fibre-coupled periodically poled lithium niobate (PPLN) waveguide module mixing 1063 and 1525-nm radiations has been adopted for generating 34 μW of 3.5-μm wavelength laser light. Optical detection methods, including sensitive wavelength modulation spectroscopy and a rapid wavelength chirp technique, have been employed with a single-pass cell to investigate methane and formaldehyde absorption profiles around 2855 cm⁻¹, as proof of principle experiments for high sensitivity and resolution spectroscopy on atmospherically important molecules.     

High efficiency and high energy parametric wavelength conversion using a large aperture periodically poled MgO:LiNbO3

We have demonstrated an efficient high energy 2 μm laser generation with a 36 mm long large aperture 5 mol% MgO-doped periodically poled LiNbO₃ (PPMgLN) nonlinear optical crystal. A high power Q-switched Nd:YAG laser (1.064 μm) was used to pump the quasi-phase matched (QPM) optical parametric oscillator (OPO). A total output energy of 186 mJ with 58% slope efficiency was obtained in two separate beams at 2 μm.     

Continuous-tunable 4.144-4.851 μm twin-MgO:PPLN cascaded optical parametric generator pumped by a 1.342 μm Nd:GdVO4 laser

An all-solid-state mid-infrared optical parametric generator with wide tunability by using multi-grating periodically poled 5 mol.-% MgO-doped lithium niobate (MgO:PPLN) is reported. The pump source is a diode-pumped Q-switched Nd:GdVO₄ laser operated at 1.342 μm with pulse width of 150 ns and repetition rate of 50 kHz. To extend the interaction length, two identical multi-grating MgO:PPLN crystals have been cascaded in the OPG system. When the incident pump average power is 10 W, the obtained maximum idler output power is 340 mW at 4.144 μm. Compared with only using one multi-grating MgO:PPLN crystal, the obtained idler output power increases by 20.1%. 4.144-4.851 μm continuous-tunable idler output is obtained with six grating periods from 29 to 31.5 μm and temperature from 40 to 200 °C. To our knowledge, this is the first time to use 1.342 μm laser as the pump source of OPG.     

Compact, 220-ps visible laser employing single-pass, cascaded frequency conversion in monolithic periodically poled lithium niobate

We report the first demonstration to our knowledge of 220-ps visible laser generation from passively Q-switched-laser pumped periodically poled lithium niobate (PPLN) in a single-pass, cascaded frequency-conversion process. The monolithic PPLN consists of a 1-cm section for frequency doubling the 1064-nm Nd:YAG pump laser to a 532-nm laser and a subsequent 4-cm section for generating the visible laser in a 532-nm-pumped optical parametric generation (OPG) process. In generating the 622.3-nm OPG signal wavelength we measured a 3.0-microJ/pulse pump threshold at the 1064-nm wavelength, 16% overall efficiency, and 35% slope efficiency at two times threshold. At 10(-6) pump duty cycle and 20-mW average power in the visible, photorefractive damage was not observed at the phase-matching temperature of 40.3 degrees C.     

Low-threshold mid-infrared optical parametric oscillation in periodically poled LiNbO3 synchronously pumped by a Ti:sapphire laser

We report the generation of tunable high-repetition-rate optical pulses in the mid-infrared using synchronously pumped parametric oscillation in periodically poled LiNbO₃ (PPLN). Using a Kerr-lens-mode-locked Ti:sapphire laser as the pump source and a PPLN crystal incorporating grating periods of 21.0–22.4 μm, we have achieved wavelength conversion in the -–4 6μm spectral range in the mid-infrared. The use of a semi-monolithic cavity design and hemispherical focusing has permitted pulse generation in the strong idler absorption region of PPLN, resulting in a simple, compact, all-solid-state configuration with a pump power threshold as low as 17 mW and mid-infrared idler powers of up to 64 mW at 9% extraction efficiency. Signal output powers of up to 280 mW at 35% extraction efficiency are available over the -–1.004 1.140μm spectral range at 80.5 MHz and pulse repetition rates at harmonics of the fundamental frequency up to 322 MHz have also been obtained. Received: 5 December 2000 / Revised version: 23 January 2001 / Published online: 27 April 2001     

Experimental observation of tunable wavelength down- and up-conversions of ultra-short pulses in a periodically poled LiNbO3 waveguide

All-optical tunable wavelength conversion of ps-pulses is proposed and experimentally demonstrated by use of cascaded sum- and difference frequency generation (cSFG/DFG) in a periodically poled LiNbO₃ (PPLN) waveguide. The amplified spontaneous emission (ASE) noise is effectively suppressed by employing two tunable filters. As a result, tunable wavelength down- and up-conversions are simultaneously observed. The temporal evolutions of the signal, pump, control and idler waves propagating along the PPLN waveguide are simulated. From the temporal waveforms and optical spectra in the simulations, it is interesting to find that continuous wave (CW) pump and control are evolved into optical pulses during the cSFG/DFG nonlinear interactions. Moreover, some new sidebands in the output pump spectrum are observed both in the simulations and experiments.     

Scattering-Enhanced Femtosecond Optical Parametric Generation

Scattering-enhanced femtosecond optical parametric generation （OPG） has been observed and studied in detail, which may decrease the pump threshold of OPGs dramatically and may make OPGs reliable. The experimental demonstration in a LiNbO3 crystal shows that strong enough OPG can be obtained at pump intensity of only about 30GW/cm2 which is well below the crystal damage threshold Either a synchronized pulsed laser or a cw laser has been used as the scattering source, of which the wavelength, spectral shape and irradiating angle are not strictly required.     

PPLN-based all-optical 40 Gbit/s ODB/AMI/FSK wavelength conversion and FSK logic NOT gate

We propose and demonstrate all-optical wavelength conversion for optical duobinary (ODB), alternate-mark inversion (AMI), and frequency-shift keying (FSK) signals and a logic NOT gate for a FSK signal based on cascaded second-harmonic generation and difference-frequency generation (cSHG/DFG) in a periodically poled lithium niobate (PPLN) waveguide. ODB/AMI/FSK are generated from the demodulation of differential phase-shift keying (DPSK) using one-bit-delay fiber delay interferometer (FDI). PPLN-based 40 Gbit/s ODB/AMI/FSK wavelength conversion and FSK logic NOT gate are simultaneously implemented in the experiment.     

Bandwidth enhancement and response flattening of cascaded sum- and difference-frequency generation-based wavelength conversion

We investigate bandwidth enhancement and response flattening of wavelength conversion based on cascaded sum-frequency generation and difference-frequency generation (SFG/DFG) in quasi-phase-matched periodically poled lithium niobate waveguides by use of two pump lights. Analysis shows that the conversion properties deeply depend on the pump settings. The bandwidth is efficiently enhanced by augmenting the pump wavelength difference. The critical bandwidth corresponding to the response fluctuation of 1 dB in a 3-cm-long waveguide reaches 80-90 nm, which is enough to cover the entire conventional-band and long-wavelength-band. The cascaded SFG/DFG bandwidth is about 24% broader than that of the cascaded second-harmonic generation and difference-frequency generation-based configuration with the same waveguide length. However, the response fluctuation is also enhanced together with the bandwidth enhancement. The method of pump detuning is presented to flatten the response fluctuation. The fluctuation is reduced by more than 1 dB and it can be further reduced by increasing the pump detuning value with a little efficiency penalty.     

Widely tunable, high-repetition-rate, dual signal-wave optical parametric oscillator by using two periodically poled crystals

This paper reports on a high-repetition-rate dual signal-wave (DSW) optical parametric oscillator (OPO) operating at the 1.5 μm band with tunable wavelength intervals from 2.5 nm to 69.1 nm. Two periodically poled crystals, a periodically poled lithium niobate (PPLN) with multiple gratings and a single grating MgO-doped PPLN (PPMgOLN), are cascaded in the same OPO cavity to generate dual signal-waves by using quasi-phase-matched (QPM) technique. The pump source was a Q-switched diode-pumped Nd:YVO₄ laser operating at 50 kHz. At an incident pump power of 3 W, an average output power of 169.6 mW at 1489.2 nm and 1558.3 nm has been achieved.     

Theoretical and experimental investigations of the Mid-IR DFG tuning property based on fiber laser fundamental lights

The tuning properties for the mid-IR DFG laser based on uniform grating PPLN have been investigated with tunable YDFL and EDFL fundamental lights. Our results show that, for a fixed crystal temperature, the idler tunable range is less than 10 nm when the EDFL is tuned. Although the pump may be allowed to be tuned in its two QPM acceptance bands, the idler tunable range is still narrow for a fixed temperature. By optimizing the crystal temperature, however, the two pump QPM acceptance bands may be overlapped to form one broadband QPM band, which may be used to increase the idler tunable range to 175 nm near 3.4 μm region. The positions of the single signal and the two separate pump QPM acceptance bands can be continuously moved by adjusting the temperature, which may also be used for enhancing the idler tuning range. By tuning the EDFL while adjusting the temperature, a whole combined idler tuning range between 2.98 and 3.78 μm was experimentally obtained with three fixed pump wavelengths of 1.05, 1.08 and 1.11 μm. By tuning the YDFL in the two separate QPM acceptance bands, a tuning range of 690 nm has been demonstrated with only one fixed signal wavelength of 1.58 μm.     

Spectroscopic diagnostics of chemical processes: applications of tunable optical parametric oscillators

Optical parametric oscillator (OPO) and amplifier (OPA) devices are useful for spectroscopic sensing of chemical processes in laboratory, industrial, and environmental settings. This is particularly true of nanosecond-pulsed, continuously tunable OPO/OPA systems, for which we survey a variety of instrumental strategies, together with actual spectroscopic measurements. The relative merits of OPO wavelength control by intracavity gratings and by injection seeding are considered. A major innovation comprises an OPO with a ring cavity based on periodically poled lithium niobate (PPLN) and injection-seeded by a single-mode tunable diode laser (TDL). Active cavity control by an ‘intensity dip’ method yields an optical bandwidth ≤0.005 cm^-1 (150 MHz), which compares favourably with the performance of advanced grating-tuned OPO/OPA systems. A novel adaptation of this TDL-seeded PPLN OPO employs a compact, inexpensive multimode pump laser, with which it is still possible to obtain continuously tunable single-mode signal output. Cavity ringdown (CRD) spectroscopy also figures prominently, with infrared (IR) CRD spectra from both grating-scanned and TDL-seeded OPOs reported. Finally, a tunable ultraviolet (UV) source, combining a TDL-seeded passive-cavity OPO and a sum-frequency generation stage, is developed for measurements of time-resolved IR-UV double resonance spectra of acetylene and UV laser-induced fluorescence spectra of nitric oxide. Received: 28 March 2000 / Published online: 13 September 2000     

Low-threshold mid-IR MgO:PPLN optical parametric generation with high reflectivity mirror for signal wavelength

A low-threshold middle-infrared(mid-IR) MgO:PPLN optical parametric generation(OPG)pumped by a laser diode(LDl end-pumped Z-type Nd:YLF laser at 1047 nm is realized with high reflectivity(HR) mirror for signal.At repetition rate of 10 kHz,the OPG threshold of 50μJ has been achieved with HR mirror for signal.Compared with the threshold without mirror,the threshold decreases by 17%.Using HR mirror for pump at output side of crystal,the threshold of 40μJ is achieved.The 2.7-4.1μm continuous tunable output is produced with seven grating periods from 28.5 to 31.5μm and temperatures from 30 to 200℃.When the incident average pump power is 3 W.the OPG idler output power is 0.46 W at 3.26 μm,which corresponds to optical-to-optical conversion efficiency up to 15.3%.     

Tunable, high-power, narrow-band picosecond IR radiation by optical parametric amplification in KTP

We report on an optical parametric amplifier (OPA) based on two potassium titanyl phosphate (KTP) crystals in a walk-off compensating geometry. An Nd:YLF regenerative amplifier at a 1-kHz repetition rate serves as the pump source. The seed beam is delivered by a synchronously pumped frequency-stabilized optical parametric oscillator (OPO) based on periodically poled lithium niobate (PPLN). At pump intensities of about 7 GW/cm² large amplification factors of more than 10⁴ were achieved, resulting in pulse energies of more than 450 μJ and 350 μJ for the signal and idler pulses, respectively, at a 1-kHz repetition rate. In the saturation regime the time–bandwidth product increases from two to three times the Fourier limit, with a pulse duration of 105 ps and a bandwidth of 12.7 GHz at the highest intensities employed. Received: 2 November 2001 / Published online: 14 March 2002