Prospects for production of ultracold $\mathsf{X^{1}\Sigma^{ + }}$ RbCs molecules

Recently, we have reported photoassociation of laser-cooled Rb and Cs atoms, decay of the RbCs photoassociation resonances to high levels of the state, and reexcitation to vibronic levels of the state [Kerman et al. , Phys. Rev. Lett. 92, 033004; 153001 (2004)]. Considering the reexcitation spectrum, we report here a preliminary analysis of perturbations in the c state by high levels of the and low levels of the state. Mixing with the B state provides the singlet character needed to stimulate decay to v = 0 of the ground state. We conclude that an experimental procedure that involves photoassociation of laser-cooled atoms, radiative decay, and stimulated Raman transfer to the ground electronic state is a feasible method for producing translationally, rotationally, vibrationally and electronically cold RbCs molecules. Electronic supplementary material to this article is available at and is accessible for authorized users. Received: 1 September 2004, Published online: 23 November 2004 PACS: 33.80.Ps Optical cooling of molecules; trapping - 34.50.Gb Electronic excitation and ionization of molecules; intermediate molecular states (including lifetimes, state mixing, etc.) - 33.20.Kf Visible spectra - 34.20.-b Interatomic and intermolecular potentials and forces, potential energy surfaces for collisions - 33.15.Pw Fine and hyperfine structure A supplementary table (Tab. I) is only available in electronic form at http: //www.eurphysj.org     

Spectroscopic studies of NaCs for the ground state asymptote of Na + Cs pairs

The ground state X of NaCs was studied by laser induced fluorescence Fourier-transform spectroscopy. An accurate potential energy curve was derived from more than 5000 transitions. This potential reproduces the experimental observations within their uncertainties of cm^-1 and covers about 99.97% of the potential well depth. Few vibrational levels of the shallow state a below the atomic ground state asymptote were observed. The identification is mainly done by the observed and quantitatively interpreted molecular hyperfine structure applying atomic parameters of the ground states of Na and Cs. An estimated potential curve for a is reported which can be used together with that of X for coupled channel calculations of cold collisions between Na and Cs. An example is given. Electronic supplementary material to this article is available at and is accessible for authorized users. Received: 10 September 2004, Published online: 23 November 2004 PACS: 31.50.Bc Potential energy surfaces for ground electronic states - 33.20.Kf Visible spectra - 33.20.Vq Vibration-rotation analysis - 33.50.Dq Fluorescence and phosphorescence spectra Supplementary tables (Tabs. I-III) are only available in electronic form at http: //www.eurphysj.org     

Structures of the f 0(980), a 0(980) mesons and the strong coupling constants g_{f_0 K^+ K^-} , g_{a_0 K^+ K^-} with light-cone QCD sum rules

Making the assumption of explicit isospin violation arising from f ₀(980)-a ₀(980) mixing, we take the point of view that the scalar mesons f ₀(980) and a ₀(980) have both strange and non-strange quark-antiquark components and evaluate the strong coupling constants within the framework of the light-cone QCD sum rules approach. The large strong scalar-KK couplings through both the and components , , and will support the hadronic dressing mechanism; furthermore, in spite of the constituent structure differences between the f ₀(980) and a ₀(980) mesons, the strange components have larger strong coupling constants with the K ⁺ K ^- state than the corresponding non-strange ones, and . From the existing controversial values, we cannot reach a general consensus on the strong coupling constants and the mixing angles.Received: 9 January 2004, Revised: 23 July 2004, Published online: 2 September 2004     

New gauge bosons from the littlest Higgs modeland the process $e^{ + }e^{-}\rightarrow t\bar{t}$

In the context of the littlest Higgs (LH) model, we study the process . We find that the new gauge bosons Z _H and B _H can produce significant correction effects on this process, which can be further enhanced by suitably polarized beams. In most of the parameter space preferred by the electroweak precision data, the absolute value of the relative correction parameter is larger than 5 %. As long as and the absolute value of the relative correction parameter is larger than . With reasonable values of the parameters of the LH model, the possible signals of the new gauge bosons B _H and Z _H can be detected via the process in the future LC experiments with the CM energy . B _H exchange and Z _H exchange can generate significantly corrections to the forward-backward asymmetry only in a small part of the parameter space.Received: 29 October 2004, Revised: 29 November 2004, Published online: 15 February 2005     

Lifetime vibrational interference during the NO 1s-1π* resonant excitation studied by the NO+(A 1Π → X 1Σ+) fluorescence

Dispersed fluorescence from fragments formed after the de-excitation of the 1s^-1π^* resonances of N^*O and NO^* has been measured in the spectral range of 118–142 nm. This range is dominated by lines of atomic nitrogen and oxygen fragments and by the bands in the NO⁺ ion which result from the participator Auger decay of the 1s^-1π^* resonances. Ab-initio calculations of the transition probabilities between vibrational levels during the reaction NO N^*O ⇒ NO were used to explain the observed intensity dependence for the fluorescence bands on the exciting-photon energy across the resonances and on both v^′ and v^′′ vibrational quantum numbers. The multiplet structure of the 1s^-1π^* resonance and lifetime vibrational interference explain the observed exciting-photon energy dependence of the fluorescence intensity. A strong spin-orbit coupling between singlet and triplet states of NO⁺ is proposed to reduce additional cascade population of the state via radiative transitions from the and states and to explain remaining differences between measured and calculated integral fluorescence intensities.     

Investigation of highly excited states of calcium by three-photon ionization

The three-photon ionization in Ca from S₀ ground state is studied. The two-photon process is a near -- resonance process with one of the following bound states: 4s4d ¹D₂, 4p P₂, 4s6s ¹S₀, 4 D₂ and 4 S₀ while the third photon reach either directly the continuum or one of the autoionizing states. The succession of bound states as well as the transitions above the ionization limit are discussed. The dynamics of the multiphoton excitation processes is also discussed and radiative decay of 4 S₀ Ca state with two-photon excitation as well as (the measured) decay times of the Ca autoionizing states using the proper line profiles for different quantum numbers has been determined.Received: 29 September 2003, Published online: 18 May 2004PACS: 32.70.-n Intensities and shapes of atomic spectral lines - 32.70.Cs Oscillator strengths, lifetimes, transition moments - 32.80.Fb Photoionization of atoms and ions - 32.80.Rm Multiphoton ionization and excitation to highly excited states (e.g., Rydberg states)     

Studies of ion energy and yield from argon clusters heated by intense femtosecond laser pulses

Using time-of-flight spectrometry, the interaction of intense femtosecond laser pulses with argon clusters has been studied by measuring the energy and yield of emitted ions. With two different supersonic nozzles, the dependence of average ion energy on cluster size in a large range of has been measured. The experimental results indicate that when the cluster size , the average ion energy Coulomb explosion is the dominant expansion mechanism. Beyond this size, the average ion energy gets saturated gradually, the clusters exhibit a mixed Coulomb-hydrodynamic expansion behavior. We also find that with the increasing gas backing pressure, there is a maximum ion yield, the ion yield decreases as the gas backing pressure is further increased.     

Influence of the growth method upon the phase transition of RbCdCl $\mathsf{_{3}}$

Structural properties of two RbCdCl₃ samples grown either from the melt or from aqueous solution are studied via X-ray diffraction over a closed temperature cycle between 20 C and 300 C. During cooling step (300 C), the crystal grown from the melt undergoes a phase transition at 110 C that drives it from the cubic structure into a tetragonal structure that still persists at 20 C. It undergoes exactly the reverse phase transition at the same temperature during the heating ( C) step that immediately follows. The other crystal grows from aqueous solution at 20 C in an orthorhombic structure (i.e. not tetragonal as that of the crystal grown from the melt and cooled down to this temperature). During the heating ( C) step, it undergoes a direct orthorhombic-cubic phase transition at 240 C (without passing through the tetragonal phase) whereas, during subsequent cooling (300 C), it does not exhibit the corresponding reverse phase transition but rather exhibits exactly the same cubic-tetragonal phase transition at 110 C as the crystal grown from the melt. However, for both crystals, this tetragonal phase observed at room temperature is unstable and slowly converts into an orthorhombic phase over the course of time. Complementary Differential Scanning Calorimetry (D.S.C.) and Thermo Gravimetric Analysis (T.G.A.) measurements have been carried out over the range ( ) C in order to interpret diffraction experiments.Received: 19 May 2004, Published online: 30 September 2004PACS: 61.10.Nz X-ray diffraction - 64.70.Kb Solid-solid transitions - 65.40.Ba Heat capacity     

Optical manipulation of long-range interactions at the 3s + 3p asymptote of $\mathsf{Na_2}$

We investigate the influence of a laser field, which is near-resonant to the atomic sodium 3²P_1/2 3²D_3/2 transition, on the last bound levels of the A state in Na₂. In a molecular beam experiment level shifts up to 100 MHz and light induced line broadenings were observed using an optical double resonance excitation scheme. Moreover, the coupling laser can reduce the number of bound levels of the A state by one or more units, which effectively means that in the picture of a collision of a 3²S_1/2 and a 3²P_1/2-atom the scattering phase is altered by more than . The observed effects are interpreted as light induced couplings of the A state, which correlates to the 3s _1/2 + 3p _1/2 asymptote, to the and states at the 3s _1/2 + 3d _3/2 asymptote. We performed multi-channel calculations, applying the mapped Fourier grid method, which reproduce our experimentally observed level shifts well.Received: 7 October 2003, Published online: 21 November 2003PACS:   34.50.Rk Laser-modified scattering and reactions - 33.80.-b Photon interactions with molecules - 42.62.Fi Laser spectroscopy     

High resolution multiphoton ionization and dissociation of acetone via $\mathsf{3s\leftarrow n}$ Rydberg transitions

Measurements of multiphoton ionization and dissociation of acetone are reported in the wavelength range 582.60-585.80 nm at photon energy resolution of 0.3 cm^-1. To our knowledge there are not available results of (3 + 2) REMPI on acetone at 0.01 nm in this region. The experiments were performed using an Nd: YAG-OPO (optical parametric oscillator) laser system coupled to time-of-flight mass spectrometer. The ion yield and the single ion channel are presented. The high-resolution three-photon resonance multiphoton spectrum of the acetone Rydberg transition is also reported. The experimental results show three dissociation channels of the acetone ion, leading to the products: (CH₃CO ⁺ ), (CH₃ ⁺ ) and (COH ⁺ ); the channel CH₃COCH ₃CO ⁺ + CH₃ being the most favored. The acetone and acetyl ions are observed in all wavelength range investigated. In addition, we have measured the origin of the and transitions, and vibrational bands of the 3s state.Received: 21 March 2004, Published online: 11 May 2004PACS: 33.80.Rv Multiphoton ionization and excitation to highly excited states (e.g., Rydberg states) - 33.15.Ta Mass spectra - 33.80.Gj Diffuse spectra; predissociation, photodissociation     

Absolute resonance strengths in the $^{6,7}Li(\alpha, \gamma)^{10,11}B$ reactions

The absolute strengths of the keV resonance in the reaction and of the keV resonance in the reaction have been measured to meV and meV, respectively, in good agreement with previous values. These resonances can be used to measure the absolute acceptance of the recoil separator ERNA to a precision of about 10%.Received: 12 December 2003, Revised: 10 February 2004, Published online: 3 August 2004PACS: 24.30.-v Resonance reactions - 25.40.Lw Radiative capture - 26.20. + f Hydrostatic stellar nucleosynthesis     

Search for a narrow charmed baryonic state decaying to $D^{\ast \pm} p^\mp$in ep collisions at HERA

A resonance search has been made in the invariant-mass spectrum with the ZEUS detector at HERA using an integrated luminosity of . The decay channels and (and the corresponding antiparticle decays) were used to identify mesons. No resonance structure was observed in the mass spectrum from more than 60 000 reconstructed mesons. The results are not compatible with a report of the H1 Collaboration of a charmed pentaquark, .Received: 14 September 2004, Revised: 29 September 2004, Published online: 9 November 2004     

Two-step laser optogalvanic spectroscopy of the odd-parity Rydberg states of atomic mercury

We present new experimental data on the highly excited levels in mercury using the two-step laser excitation and optogalvanic detection technique in conjunction with a RF discharge cell. The 6s7s ³S₁ intermediate level has been accessed from the 6s6p ³P₂ metastable level that is collisionally populated in the mercury discharge in the presence of a buffer gas at a pressure of about 1 Torr. Two beams fromtwo different dye lasers pumped with a common excimer laser were passed through the discharge cell containing mercury vapors. The first laser was tuned to 6s7s ³S₁ level whereas the second laser was scanned covering the wavelength region between 544-458 nm. We have observed the 6snp ³P₀ ( ), 6snp ( ), 6snp ( ) and 6snp ) Rydberg series. The 6snp Rydberg series to such high n-value has been reported for the first time. The first ionization potential of mercury is determined from the 6snp Rydberg series as 84184.15 0.05 cm^-1. Some collisionally induced parity forbidden transitions have also been located that are identified as 6sns ( ) series.Received: 5 November 2003, Published online: 20 January 2004PACS: 31.50.-x Potential energy surfaces - 32.30.Jc Visible and ultraviolet spectra - 32.80.Rm Multiphoton ionization and excitation to highly excited states (e.g., Rydberg states)     

Study of Z pair production and anomalous couplingsin e + e- collisions at $\sqrt{s}$ between 190 GeV and 209 GeV

A study of Z-boson pair production in e ⁺ e^- annihilation at center-of-mass energies between 190 GeV and 209 GeV is reported. Final states containing only leptons, ( and ), quark and lepton pairs, ( , ) and only hadrons ( ) are considered. In all states with at least one Z boson decaying hadronically, lifetime, lepton and event-shape tags are used to separate pairs from final states. Limits on anomalous ZZ and ZZZ couplings are derived from the measured cross sections and from event kinematics using an optimal observable method. Limits on low scale gravity with large extra dimensions are derived from the cross sections and their dependence on polar angle.Received: 14 July 2003, Published online: 18 December 2003     

Accurate asymptotic ground state potential curves of Cs$\mathsf{_2}$ from two-colour photoassociation

Over 100 high lying level energies of the lowest electronic states and in Cs₂ are determined in a -like scheme two-colour photoassociation spectroscopy. The results are analyzed with a coupled channel model using an asymptotic approach, based on nodal lines. From this analysis we determine the long range dispersion coefficient C₆ to 6846.2 15.6 a.u. We also obtain the first experimental determination of the amplitude of the asymptotic exchange term.Received: 4 November 2003, Published online: 20 January 2004PACS: 34.20.-b Interatomic and intermolecular potentials and forces, potential energy surfaces for collisions - 32.80.Pj Optical cooling of atoms; trapping - 03.65.Ge Solutions of wave equations: bound states     

CP asymmetry in $B \rightarrow \phi K_{S}$ in a general two-Higgs-doublet model with fourth-generation quarks

We discuss the time-dependent CP asymmetry of the decay in an extension of the standard model with both a two Higgs doublet and additional fourth-generation quarks. We show that, although the standard model with a two Higgs doublet and the standard model with fourth-generation quarks alone are not likely to largely change the effective from the decay , the model with both an additional Higgs doublet and fourth-generation quarks can easily account for the possible large negative value of without conflicting with other experimental constraints. In this model, additional large CP violating effects may arise from the flavor-changing Yukawa interactions between neutral Higgs bosons and the heavy fourth-generation down type quark, which can modify the QCD penguin contributions. With the constraints obtained from processes such as and , this model can lead to an effective as large as - 0.4 in the CP asymmetry of .Received: 25 March 2004, Revised: 20 April 2004, Published online: 18 June 2004     

The rare annihilation decays $\bar{B}^0_{s,d} \to J/\psi\gamma$

We investigate the physics potential of the annihilation decays in the standard model and beyond. In a naive factorization approach, the branching ratios are estimated to be and . In the framework of QCD factorization, we compute the non-factorizable corrections and get , . Future measurements of these decays would be useful for testing the factorization frameworks. The smallness of these decays in the SM makes them sensitive probes of new physics. As an example, we will consider the possible admixture of the (V + A) charge current to the standard (V-A) current. This admixture will give a significant contribution to the decays.Received: 29 August 2003, Revised: 17 January 2004, Published online: 19 March 2004Corresponding author: Y.D. Yang     

Multiple ionization effects on L X-ray intensity ratios in Hf,Ta, Re,Ir, Pt,Au and Pb due to proton bombardment at energies 1-5 MeV

The L X-ray intensity ratios in the elements Hf, Ta, Re, Ir, Pt, Au and Pb due to proton bombardment at energies from 1 to 5 MeV are measured and compared with the ECPSSR theoretical intensity ratios. The L /L _l intensity ratios obtained in the present work are in good agreement with theoretical values while the L /L and L /L intensity ratios are consistently lower than the theoretical values. This deviation may be explained in terms of multiple ionization effects in M, N and O shells.Received: 27 March 2004, Published online: 6 July 2004PACS: 32.80.Hd Auger effect and inner-shell excitation or ionization - 32.30.Rj X-ray spectra - 41.75.-i Charged-particle beams - 41.75.Ak Positive-ion beams     

Search for chargino and neutralino productionat $\sqrt{s} = 192$-209 GeV at LEP

Approximately 438 pb^-1 of e ⁺ e^- data from the OPAL detector, taken with the LEP collider running at centre-of-mass energies of 192-209 GeV, are analyzed to search for evidence of chargino pair production, , or neutralino associated production, . Limits are set at the 95% confidence level on the product of the cross-section for the process and its branching ratios to topologies containing jets and missing energy, or jets with a lepton and missing energy, and on the product of the cross-section for and its branching ratio to jets. R-parity conservation is assumed throughout this paper. When these results are interpreted in the context of the Constrained Minimal Supersymmetric Standard Model, limits are also set on the masses of the and , and regions of the parameter space of the model are ruled out. Nearly model-independent limits are also set at the 95% confidence level on with the assumption that each chargino decays via a W boson, and on with the assumed to decay via a Z⁰.Received: 15 December 2003, Revised: 16 February 2004, Published online: 23 April 2004