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1.
The performance of an air sampler and a small gamma-ray spectrometer was tested in an unmanned aerial vehicle (UAV) able to carry payload with mass up to 0.5 kg. Operation of the sampler was investigated with the aid of radon progeny normally present in outdoor air. Detection limits for several transuranium nuclides in air are of the order of 0.3 Bq m?3 assuming 0.5 h sampling time and 1 h counting time in direct alpha spectrometry. Unshielded 137Cs and 60Co point sources at the ground level were used to test the CsI spectrometer. Detection limits are approximately 1 GBq or larger depending on the flying altitude.  相似文献   

2.
Radionuclide concentrations in wharf roaches inhabiting coastal areas of Honshu, Japan, were investigated in October 2011 and June 2012. Relative high concentrations of 110mAg (2.1–127 Bq kg-wet?1), 134Cs (2.6–61 Bq kg-wet?1), and 137Cs (3.5–92 Bq kg-wet?1) were detected in specimens from the eastern Honshu areas. Significantly lower 137Cs concentrations (0.7–1.6 Bq kg-wet?1) were detected in specimens from western and northern Honshu. The decay-corrected 137Cs concentration was significantly inversely correlated with the distance from the Fukushima Dai-ichi Nuclear Power Plant. Thus, wharf roach may serve as a good bioindicator for monitoring radioactive contamination of its habitats.  相似文献   

3.
The aim of this work was to determine 137Cs and 40K radioactivities in soil samples taken from the Babia Góra National Park (BPN) in south Poland. The cluster analysis (CA) and principal component analysis (PCA) were used to discuss the obtained data. 10 cm thick soil cores were collected from the BPN area. Each sample was divided into three sub-samples. The samples were dried, homogenized and packed in polyethylene containers. The radioactivities of 137Cs and 40K were measured by means of gamma spectrometry. It was found that 137Cs radioactivity in the whole 10 cm soil cores was in the range from 1,916 to 28,551 Bq m?2. The radioactivity of 40K varied from 1,642 to 25,654 Bq m?2. Using CA it was possible to diverse the soils taking into account soil types. By use of the PCA method, it was chosen three factors which are appropriate to characterize researched parameters.  相似文献   

4.
In 2002, an extensive study was performed in forest sites of Izmir. This first study results led on the one hand, to quantify of 137Cs and 40K concentration in mushrooms collected in the Izmir region and to a first evaluation of dose in people due to the ingestion of radionuclide-contaminated mushrooms. The mushroom concentration values varied over a wide range from below detection limit to 401 ± 4 Bq kg?1 (dry wt) for 137Cs. The 40K concentration values obtained for different species of mushrooms ranged from 588 ± 26 Bq kg?1 to 2024 ± 63 Bq kg?1 (dry wt). The annual effective dose values due to mushroom ingestion for 137Cs are lower than the ICRP-2007’s reference level value of 1 mSv for “existing” exposure situation. Inductively coupled plasma-mass spectrometry was used to measure many alkali–alkaline earth elements and heavy metals in mushroom samples. The relationships among the concentrations of 137Cs and the stable elements were presented and the occurrence of metals in mushrooms was evaluated.  相似文献   

5.
In this study, soil samples were collected at Canadian embassy in Tokyo (about 300 km from Fukushima) on 23 March and 23 May of 2011 for purposes of estimating concentrations of radionuclides in fallout, the total fallout inventory, the depth distribution of radionuclide of interest and the elevated ambient gamma dose-rate at this limited location. Some fission products and actinides were analyzed using gamma-ray spectrometry, alpha spectrometry and liquid scintillation counting. The elevated activity concentration levels of 131I, 132I, 134Cs, 137Cs, 136Cs, 132Te, 129mTe, 129Te, 140Ba and 140La were measured by the gamma-ray spectrometer in the first sample collected on 23 March. Two months after the accident, the 134Cs and 137Cs became only detectable nuclides. A mass relaxation depth of 3.0 g/cm2 was determined by the activities on the depth distribution of 137Cs in a soil core. The total fallout inventory was thus calculated as 225 kBq/m2 on March sampling date and 25 kBq/m2 on May sampling date. The ambient gamma dose-rates in the sampling area estimated by the fallout fission products inventory and 137Cs depth distribution ranged from 184 to 38 nGy/h. There was no detectable americium or plutonium in the soil samples by alpha spectrometry. Although 90Sr or 89Sr were detected supposedly as a result of this accident, it was less than the detection limit, which was about 0.4 Bq/kg in the soil samples.  相似文献   

6.
The Marshall Islands Program at the Lawrence Livermore National Laboratory has completed a series of radiological surveys at Bikini, Rongelap, Utrōk, and Enewetak Atolls in the Marshall Islands designed to take a representative sample of food supplies with emphasis on determining 137Cs activity concentrations in common food plants. Coconuts (Cocos nucifera L.) are the most common and abundant food plant, and provided a common sample type to characterize the level and variability of activity concentrations of 137Cs in plant foods collected from different islands and atolls. Other dominant food types included Pandanus (Pandanus spp.) and breadfruit (Actocarpus spp.). In general, the activity concentration of 137Cs in food plants was found to decrease significantly between the main residence islands on Bikini, Rongelap, Utrōk, and Enewetak Atolls. The mean activity concentration of 137Cs measured in drinking coconut meat and juice was 0.72 (95 % CI 0.68–0.77) and 0.34 (95 % CI 0.30–0.38) Bq g?1, respectively, on Bikini Island; 0.019 (95 % CI 0.017–0.021) and 0.027 (95 % CI 0.023–0.031) Bq g?1, respectively, on Rongelap Island; 0.010 (95 % CI 0.007–0.013) and 0.007 (95 % CI 0.004–0.009) Bq g?1, respectively, on Utrōk Island; and 0.002 (95 % CI 0.0013–0.0024) and 0.002 (95 % CI 0.001–0.0025) Bq g?1, respectively, on Enewetak Island. High levels of variability are reported across all islands. These results will be used to improve the accuracy and reliability of predictive dose assessments, help characterize levels of uncertainty and variability in activity concentrations of fallout radionuclides in plant foods, and allow atoll communities to make informed decisions about resettlement and possible options for cleanup and rehabilitation of islands and atolls.  相似文献   

7.
In this article, we present results obtained from a radiometric survey that was conducted in the Leepa Valley of Azad Jammu & Kashmir, Pakistan. The purpose of current study is to appraise the radioactivity levels and the associated health hazards due to the terrestrial radionuclide in soil and rock samples. In this regard, 16 soil and 17 rock samples were collected from different locations of the Leepa Valley. After processing the samples, activity concentrations of primordial (232Th, 226Ra and 40K) and anthropogenic (137Cs) radionuclides were determined using a P-type coaxial high purity germanium detector. From the results obtained the mean activity concentrations of radionuclides 226Ra, 232Th and 40K in the soil samples were found to be 31.25 ± 0.46, 44.1 ± 1.07 and 575 ± 8.89 Bq kg?1 respectively. Whilst, in rock samples 226Ra, 232Th and 40K mean activities were found as 28.46 ± 0.45, 48.63 ± 1.12 and 666.7 ± 9.39 Bq kg?1, respectively. The 137Cs concentration level in soil and rock samples is found to be 15.04 ± 0.29 and 5.7 ± 0.16 Bq kg?1, respectively. The average radium equivalent activity (R aeq) was found as 143.16 and 142.93 Bq kg?1 in soil and rock samples, respectively. These findings are less than the recommended safe value of 370 Bq kg?1 as given in OECD report (1979). The values of external (H ex) and internal hazard index (H in) are also less than unity. Mean value of absorbed dose rate was found as 69.78 nGy h?1 for the soil samples, which is in good agreement with the world wide average value (70 nGy h?1). Mean value of absorbed dose rate from rock samples was found as 70.01 nGy h?1. Mean values of the annual effective dose is also lower than the values reported for different other countries of the world.  相似文献   

8.
Impact of the TEPCO Fukushima-Daiichi NPP accident, FNPP1, to the North Pacific Ocean occurred through two pathways, namely direct release and atmospheric deposition to wide ocean surface. We collected more than 100 seawater samples in the North Pacific Ocean in April and May 2011 by seven commercial ships as VOS. Since the sample volume was 2 l each, we measured radiocaesium activity at Ogoya Underground Facility to obtain reliable activity. 137Cs was detected at all stations and 134Cs was detected at most of the stations in the North Pacific Ocean. The 137Cs activity ranged from around 1 to 1,000 Bq m?3 with activity ratios of 134Cs/137Cs close to 1 which is a signature of radiocaesium originated from the FNPP1 accident. At east of the International Date Line north of 40°N in the Pacific Ocean in April 2011, the 134Cs activity ranged from 2 to 12 Bq m?3.  相似文献   

9.
The March 2011 earthquake off the Japanese coast and subsequent tsunami that devastated the Fukushima Dai-Ichi nuclear power plant resulted in the largest accidental release of cesium 137 and 134 to the oceans. Seawater samples were collected in June 2011 from 30 to 600 km off the coast of Japan as part of initial mapping of the spread of contamination in the ocean. Cesium was extracted from unfiltered and filtered (<1.0 μm) seawater using an absorber based upon an organic polymer polyacrylonitrile (PAN) containing ammonium molybdophosphate (AMP) Sebesta and Stefula (J Radioanal Nucl Chem 140:15–21, 1990). The AMP-PAN resin can be counted directly using gamma spectroscopy for 134Cs and 137Cs. Stable 133Cs was added to evaluate extraction efficiency and quantified by ICP-MS. Our 5 mL AMP-PAN resin column was on average 95 % efficient in the removal of cesium from 20 L samples at an average flow rate of 35 mL min?1. Measured activities of 134Cs and 137Cs ranged from a few Bq m?3 to >300 Bq m?3. The extraction column can be adapted to different sample volumes and easily used in the field.  相似文献   

10.
131I, 137Cs and 134Cs were observed in environmental samples in Milano (40°N), Italy and Thessaloniki (45°N), Greece, soon after the nuclear accident in Fukushima, Japan. The radionuclide concentrations were determined and studied as a function of time. In Thessaloniki the 131I in air was observed for the first time on March 24, 2011. In Milano, the first evidence of Fukushima fallout has been confirmed with 131I and 137Cs measured in wet precipitation collected 2 days later. The maximum 131I activity concentration in air of 467 ± 25 μBq m?3, observed in Milano on April 3–4, 2011, was almost similar to the highest value of 497 ± 53 μBq m?3 observed in Thessaloniki. The 134Cs/137Cs activity ratio values in air were around 1 in both regions. Soil, grass and milk samples were contaminated with 131I and 137Cs at a low level. Finally, a dose assessment for these two areas showed clearly that the detected activities in all environmental samples were far below levels of concern.  相似文献   

11.
Concentrations of 238U, 232Th, 226Ra, 40K and 137Cs are measured in collected soil samples from various locations in the Thrace region of Turkey. The activity concentrations range from 12.82 to 101.75 Bq kg?1 d.w. (dry weight) for 238U, from 5.16 to 73.34 Bq kg?1 d.w. for 232Th, from 185.54 to 5399 Bq kg?1 d.w. for 40K and from 11.42 to 90.73 Bq kg?1 d.w. for 226Ra. In addition to naturally occurring radionuclides, 137Cs activity concentration is determined between 3.05 and 46.78 Bq kg?1 d.w. for soil samples. Determination of the radiological hazard is achieved through calculations of the external terrestrial gamma dose rate in air (nGy h?1) and annual effective dose rate (mSv year?1) and the results are compared with the similar works in different countries.  相似文献   

12.
Analyses of anthropogenic and natural gamma-ray emitters in the environment require high sensitive detector systems operating in coincidence-anticoincidence modes. Thanks to an excellent energy resolution and a high efficiency, large volume HPGe detectors have been widely used in low-level gamma-ray spectrometry. In the present paper we discuss the characteristics of single and coincidence (HPGe-NaI(Tl)) arrangements suitable for analysis of environmental samples containing cascade gamma-ray emitters (e.g., 60Co), positron emitters (e.g., 22Na) and single gamma-ray emitters (e.g., 137Cs). The detectors were placed in a large volume shields consisting of iron, lead and copper layers. The reduction of background for the single gamma-ray spectrometer is between 60 and 250, depending on the gamma-ray energy. As an improvement of the apparatus, low detection limits for analysis of 137Cs (0.3 Bq·kg−1) and 60Co (0.1 Bq·kg−1) in environmental samples, respectively, have been obtained.  相似文献   

13.
The deposition flux of 7Be was measured in the range from 0.4 to 5.2 Bq m?2 d?1, with a mean value of 2.6 Bq m?2 d?1, during the period of May 31, 2009?CMay 31, 2010 in the Three Gorges Reservoir region, China. The low annual deposition flux of 7Be was probably due to the adsorption of 7Be within high altitude clouds and the Qinling-Daba Mountain??s barrier and blocking effects on the cold air during winter months. There was a seasonal trend for 7Be deposition, showing a spring maximum and winter minimum, which may be attributed to the seasonal folding of tropopause in spring and little rainfall amount in winter. A strong positive correlation (R 2 = 0.67) between 7Be deposition flux and rainfall was observed. The depth distribution of 7Be in undisturbed purple soil profiles suggested that the nuclide was mainly distributed within the top 20.0 kg m?2 (~1.5 cm) of soil in depth and the maximum concentration occurred at a depth of 3.0 kg m?2 (~0.2 cm), then the concentration declined quickly and exponentially with depth. The seasonal inventories of 7Be in soils were consistent with the values calculated from the atmospheric fluxes, which shows a great potential for using 7Be as a tracer to assess soil redistribution in purple soil areas of China.  相似文献   

14.
The impact of the Fukushima nuclear accident in north–western Greece was assessed through an environmental monitoring programme activated by the Nuclear Physics Laboratory of the University of Ioannina. Measurements of 131I were carried out in atmospheric particulate, ovine milk and grass samples. In daily aerosol samplings, radioiodine was first detected on March 25–26, 2011 and reached maximum levels, up to 294 μBq m?3, between April 2 and April 4, 2011. In ovine milk samples, 131I concentrations ranged from 2.0 to 2.7 Bq L?1 between April 2 and April 6, 2011, while an average activity of 2.7 Bq kg?1 was measured in grass samples on April 4, 2011. The 134,137Cs isotopes were below detection limits in all samples and could only be determined in the air, by analysis of multiple daily filters. A maximum average activity concentration of 137Cs amounting to 24 μBq m?3 was measured during the period from April 5 to April 9, 2011, with the 134Cs/137Cs activity ratio being close to unity. Activity concentrations were consistent with measurements conducted in other parts of the country and were well below those reported in May 1986 after the Chernobyl accident. The committed effective dose to the whole body and to the thyroid gland from inhalation of 131I was estimated for the adult and infant population and was found to be of no concern for the public health.  相似文献   

15.
The extent of soil erosion in some Spanish semiarid regions has caused great concern regarding the sustainability of soil resources. Accelerated soil erosion, particularly in some Mediterranean areas, is likely to be one of the main environmental problems associated with climate change. Fallout 137Cs has been shown to provide a reliable basis for assessing soil erosion rates in different environments around the world. However, existing information concerning the spatial variation of 137Cs inventories at reference sites has identified a need for further investigation of the factors affecting their spatial variability in semiarid environments, where stony and skeletal soils are predominant. Reference sites at three locations in the central Ebro valley were selected to investigate the 137Cs content of several grain size fractions. Each site included both natural vegetated conditions and cultivated land and the three sites were characterized by different values of mean annual rainfall. The results obtained demonstrate the influence of lithology, land use and climate on the spatial variability of 137Cs inventories that increase from 1190, to 1500 and 1710 Bq·m?2 with increasing annual rainfall values from 300 to 500 mm at the study sites. The soils on marls at the Valareña site had the highest proportion of 137Cs in the coarse fractions of cultivated soils (12%) in comparison with soils developed on limestones at Loma Negra (5%), whereas no 137Cs content was found in the coarse fractions of soils on glacis-terrace materials at Peñaflor. The 137Cs reference inventories are higher in soils on marls and sands at cultivated locations at Valareña and Peñaflor, but have similar values in soils at cultivated and uncultivated locations on limestones at Loma Negra. Therefore, in absence of level undisturbed soils with natural vegetation cover, cultivated flat soils on hard rocks could provide reliable reference inventories.  相似文献   

16.
Radioactive concentrations of several artificial and natural radionuclides were determined in water and sediment samples collected from various locations in the NW Black Sea in December 1999. For water samples, 90Sr and 137Cs activity concentrations were of approximately 11 mBq/l and 26.3-41.2 mBq/l, respectively. The concentration of tritium ranged from 7 to 24 T.U. In sediment samples, maximum concentrations of 137Cs, 239+240Pu and 241Am were found of 128±6 Bq·kg-1, 1.8±0.1 Bq·kg-1 and 0.05±0.04 Bq·kg-1, respectively. For U and Th radionuclides, the concentrations ranged from 20-80 Bq·kg-1 and 30-50 Bq·kg-1, respectively. The results were consistent with those reported in earlier research for the Black Sea. This revised version was published online in July 2006 with corrections to the Cover Date.  相似文献   

17.
Determining radioactivity levels in foodstuffs is of great importance for the protection of human health. In addition, the literature includes few studies related to this subject in Turkey. In this study, gamma spectroscopic system was used in order to measure 226Ra, 232Th, 40K and 137Cs activity concentrations in vegetables and fruits produced in Elaz?? Region. The average activity concentrations in vegetables was calculated as 0.64 ± 0.26 Bq kg?1 for 226Ra, 0.65 ± 0.14 Bq kg?1 for 232Th, 13.98 ± 1.22 Bq kg?1 for 40K, and 0.54 ± 0.04 Bq kg?1 for 137Cs. The average activity concentrations in fruits were 1.52 ± 0.34, 0.98 ± 0.23, 18.66 ± 1.13 and 0.59 ± 0.16 Bq kg?1, respectively for 226Ra, 232Th, 40K and 137Cs. Total committed effective dose value was determined as 20 and 30.55 μSv y?1, respectively for vegetables and fruits. The findings were compared with previous data reported for Turkey and other regions of the world.  相似文献   

18.
The background distributions of 239+240Pu and 137Cs fallout in agricultural soil were investigated in Rokkasho where Japan's first commercial nuclear fuel reprocessing plant is now being constructed. The mean inventories of 239+240Pu and 137Cs in three fields with non-yam-cultivation history were 116 Bq·m−2 and 3.4 kBq·m−2, respectively. The mean atomic ratio of 240Pu/239Pu for all studied fields was 0.18±0.04, and was similar to that of global fallout. The 239+240Pu concentrations correlated very well with 137Cs (r = 0.97) in spite of heavy disturbance of the soil, and the activity ratio of 239+240Pu/137Cs was 0.037±0.007, which is a typical value for global fallout. These results showed that the nuclides had similar behavior in agricultural upland fields in Rokkasho. Since 210Pb is steadily deposited from the atmosphere to the land, this nuclide could be an index for the degree of disturbance of a field and of soil lost from the field. The ratio of excess 210Pb inventory in the soil to the equivalent inventory of atmospheric 210Pb deposition was 96%, and indicated that soil was not lost from the cultivated fields. This revised version was published online in July 2006 with corrections to the Cover Date.  相似文献   

19.
The method developed for cesium concentration from large freshwater samples was tested and adapted for analysis of cesium radionuclides in seawater. Concentration of dissolved forms of cesium in large seawater samples (about 100 L) was performed using composite absorbers AMP-PAN and KNiFC-PAN with ammonium molybdophosphate and potassium–nickel hexacyanoferrate(II) as active components, respectively, and polyacrylonitrile as a binding polymer. A specially designed chromatography column with bed volume (BV) 25 mL allowed fast flow rates of seawater (up to 1,200 BV h?1). The recovery yields were determined by ICP-MS analysis of stable cesium added to seawater sample. Both absorbers proved usability for cesium concentration from large seawater samples. KNiFC-PAN material was slightly more effective in cesium concentration from acidified seawater (recovery yield around 93 % for 700 BV h?1). This material showed similar efficiency in cesium concentration also from natural seawater. The activity concentrations of 137Cs determined in seawater from the central Pacific Ocean were 1.5 ± 0.1 and 1.4 ± 0.1 Bq m?3 for an offshore (January 2012) and a coastal (February 2012) locality, respectively, 134Cs activities were below detection limit (<0.2 Bq m?3).  相似文献   

20.
As a result of routine soil sampling to determine the 137Cs background activities country-wide in Venezuela, it was decided to further investigate El Mirador (Lookout) area at the base of the Sierra de Lema mountain range. In April 2003 (A), soil samples were collected at eight sites on and around the edge of the diabase outcrop to confirm that this area had anomalously high 137Cs activities. In July 2003 (B), not only soil samples were collected again, but also black mat, palm tree leaves and trunks, fruit bushes leaves and its fruit and fern leaves. The 137Cs content was measured by high resolution gamma-ray spectroscopy by a comparative method with reference materials. The 137Cs activity values range from 16.3 to 30.8 Bq·kg-1 in the soil samples collected in July 2003, 20.7–32.1 Bq·kg−1 for the black mat, 26.3–38.4 Bq·kg−1 for the palm leaves, 16.8–31.2 Bq·kg−1 for the palm trunks and 17.6–27.3 Bq·kg−1 for the fruit bush leaves, while, the 137Cs activity values for the whole fruit were between 23.4 and 30.7 Bq·kg−1; but, the value of the 137Cs activity in the center of the fruit (the edible part) was 51.6 Bq·kg−1, and the value of the 137Cs activity for the fern leaves was 51.8 Bq·kg−1. Thus, most of the 137Cs activity values determined in the soil, black mat and vegetation samples from El Mirador (Lookout) were considered anomalously high with respect to those found near the equator and in other areas of Venezuela. Only the center of the fruit from the Clusia grandiflora bushes and the fern leaves had high activity ratios, about a factor of three and could be considered as biomonitors that concentrate and retain the 137Cs. Finally, these anomalously high 137Cs activities have been attributed not only to the rich organic soils, as sinks, but also due to the affect of the cloud forests.  相似文献   

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