Isomeric state at 945.3 keV in237Np

A new isomeric state in²³⁷Np has been discovered at an excitation energy of (945.3±0.2) keV withT _1/2 =(711±40) ns. Six gamma-ray lines have been measured depopulating the isomeric state to known levels in²³⁷Np. The comparison of the measured absolute gamma-ray transition probabilities with empirical values yields as most probable spinI andK assignmentI=K=13/2 for this isomeric state. It is most likely a 1-proton-2-neutron quasiparticle state 13/2^?π5/2⁺ [642] +ν7/2^? [743] + ν 1/2⁺ [631]. However, a one-quasiparticle 11/2^? [505] configuration for the isomer cannot be excluded.     

Half-life measurements of intrinsic states in deformed odd-mass nuclei

The half-lives of the following intrinsic states in deformed odd-mass nuclei has been measured by delayed coincidences with a time-to-amplitude converter:

1. 5/2 5/2⁺[642] at 86.5 keV in¹⁵⁵Gd:T _1/2=6.7±0.3 ns, which results in the determination of theE1,ΔK=1 transition probability to the ground state 3/2 3/2^?[521] and first rotational state 5/2 3/2^?[521], yielding hindrance factors ofF _N ≈5.5 and ≈1.8 (F _W =3.1×10⁴ and 2.3×10⁴) respectively.
2. (3) 5/2 5/2^?[512] at 191.4 keV in¹⁶⁹Yb:T _1/2=3.35±0.15 ns and at 122.39 keV in¹⁷¹Yb:T _1/2=265±20 ns which results in the determination of the transition probabilities of theE1,ΔK=1 transitions to the ground states 7/2 7/2⁺[633], of theK-forbiddenM1 transitions to the 5/2 and 3/2 1/2^?[521] and of theE2 transitions to the 5/2, 3/2 and 1/2 1/2^?[521] states in both nuclei.

TheE1 transition probabilities are compared to the transitions between the same Nilsson states in¹⁷³Yb and¹⁷⁵Hf discussing the influence of the position of the Fermi surface — obtained from recent stripping and pick-up reactions — on these transition probabilities. Additional information on the decay scheme of¹⁷¹Lu→¹⁷¹Yb is obtained by delayed coincidence measurements. For testing the used time-to-amplitude converter the well known half-lives of the 482 keV level in¹⁸¹Ta (T _1/2=10.4±0.3 ns) and of the 279 keV level in²⁰³Tl (T _1/2=0.285 ±0.015 ns) were measured, in good agreement with other measurements.     

States of167Ho from the decay of neutron rich nuclide167Dy

Theβ ^?-decay of ₆₆ ¹⁶⁷ Dy produced through the fast neutron reaction¹⁷⁰Er(n, α)¹⁶⁷Dy has been investigated by using several kinds of detectors and a high-capacity two-parameter recording system. The half-life andβ ^?-decay energy of¹⁶⁷Dy were determined to beT _1/2 = 6.20 ± 0.08min andQ _β-=2.35±0.06, respectively. The observed level scheme of ₆₇ ¹⁶⁷ Ho (completely unknown previously) contains 12 states, among them a 6.0±0.1 μsM2 isomer at 259.3 keV. On the basis of theoretical and systematic considerations combined with multipole determinations, the following Nilsson model assignments are proposed for the lowest states of¹⁶⁷Ho: 0 keV (7?/2 [523]), 259.3 keV (3+/2[411]), 319.8 keV (5/2 3+/2[411]), 392.5 keV (1+/2[411]), 410.0 keV (3/2 1+/2[411]), 569.7 keV (3?/2{7?/2[523], 2⁺}). Theβ-decay proceeds mainly to the proposed gamma-vibrational state at 569.7 keV with an anomalously low logft value 5.4, indicating similarity between the microscopic structures of this state and the famous ¦K ₀?2¦ gamma vibration of¹⁶⁵Ho.     

Level structure of170Er observed in the decay of the 2.76 min170Ho

TheΒ ^?-decay of the longer-lived¹⁷⁰Ho isomer produced through the¹⁷⁰Er(n, p)¹⁷⁰Ho reaction has been investigated by using a versastile detector and coincidence equipment. The half-life andΒ ^?-decay energy were determined to beT _1/2=2.76±0.05 min andQ _β =3.85±0.15 MeV, respectively. In addition to the ground state band and some higher energy levels, the proposed level scheme of¹⁷⁰Er contains 11 states between 1.0 and 1.6 MeV (6 new ones), which are connected mutually by previously unknown low-energy transitions. Spin and/or parity assignments based mainly on coincidence data and multipolarity determinations are suggested for most of these states. By using systematic considerations and the nuclear projection model calculations several bands withK≧2 can be assigned tentatively. As a side result the half-life of¹⁶⁹Ho was determined to be 4.7 ±0.2 min.     

Decay of the first excited state at 13.3 keV in73Ge

Singles and coincidence measurements of the 13.3 keV transition of⁷³Ge are reported. The total andK conversion coefficients of this gamma-ray and the half-life of this level have been determined. The results are: α _T =1095±55; α _K =312±30;T _1/2=2.98±0.05 μs.     

Thex- (orΔ) transition in152Dy

A 53.3 keV E2 transition de-exciting the 60 ns isomer in¹⁵²Dy has been identified in γγ-coincidence measurements, which locates that isomer at E_x=5088 keV. The half life of the 11^? level at 3161 keV was measured to be T_1/2=4.3±0.9 ns.     

Der Zerfall des125m Xe,des127m Xe und des127g Xe

The decay of^125m Xe produced by the reaction¹²²Te(α, n)^125m Xe using a target enriched in¹²²Te (95.4%) and the decay of^127m Xe produced by the reaction¹²⁷J(d, 2n)^127m Xe have been investigated: ^125m Xe decays with a half-life ofT _1/2=(56±3) sec by ayy- cascade withE _γ1=(140.4 ±0.5) keV andE _γ2=(110.5 ±0.5) keV. The experimental conversion coefficients yield multipolarities ofE3 for the 140.4 keV isomeric transition and predominantlyM1 for the 110.5 keV-transition. ^127m Xe decays with a half-life ofT _1/2=(71±2) sec. The decay also proceeds by aγγ-cascade with an isomeric E3 transition ofE _γ1=(172.5±0.3) keV and a predominantlyM1 transition ofE _γ2=(124.6±0.3) keV. In the decay of^127g Xe an additional branching of the electron capture to a level at (618.1±0.3) keV was observed. The relative probability forK-captureP _K618/P_K375=0.40 ±0.07 yields a total transition energyQ _EC=(664 ±4)keV. A spin of 1/2⁺ was assigned to the ground state.     

A new isomer in205Po

A new isomer withT _1/2=58±2 ms has been observed in²⁰⁵Po. We propose the assignmentsI ^π = 19/2^? and an excitation energyE _x =1461 keV.     

Half-Life of the 37.1 keV level in121Sb

The half-life of the first excited state at 37.1 keV in¹²¹Sb has been measured using the technique of delayed coincidences with a time to amplitude converter. Scintillators with fast timing properties have been used in various combinations. From 17 independent measurements a result for the half-life ofT _1/2=(3.46±0.03) ns has been obtained and this is compared with previously published values.     

New isomers in83Br,85Rb,85Kr and86Kr

Using methods of in-beam spectroscopy in connection with 35 MeV⁷Li bombardment of⁸²Se targets four new isomers have been identified. They are observed in⁸³Br at 3070 keV (T_1/2=0.6±0.2 μs), in⁸⁵Rb at 2826 keV (T_1/2=12.5±0.6 ns), in⁸⁵Kr at 1991 keV (T_1/2=1.2+ _0.4 ^1.0 μs) and in⁸⁶Kr at 2250 keV (T_1/2=3.1±0.6 ns). Spin and parity 19/2^? have been assigned to the new isomer in⁸⁵Rb that is interpreted as the coupling of a p_3/2 proton to the g ₉ ^2/?2 two-neutron excitation of the N=48 neutron system. Using the TDPAD method an upper limit for the g-factor of ¦g¦≦0.17 has been estimated for this isomer. The same two-neutron excitation is also believed to be responsible for the new isomer in⁸³Br. The new isomers in⁸⁵Kr and⁸⁶Kr are interpreted as configurations containing the two-proton excitation (f ₅ ^2/?1 , p ₃ ^2/?1 ) where in the isomeric 17/2⁺ level of⁸⁵Kr an additional g_9/2 neutron hole is involved.     

Die Konversion des86mRb

^86mRb was produced by irradiation of natural Rb and Rb enriched in⁸⁷Rb (99.2%) with fast neutrons. The half-life ofT _1/2=(61.2±1.0) sec and the energy ofE _ρ=(556.03±0.25) keV were remeasured. The experimental conversion coefficients α_tot=0.0184±0.0015 andα _K =0.0158±0.0015 yield the multipolarity of E4 for the isomeric transition. The spin of 6^? was assigned to the isomeric state. It is proposed that the spin 6^? is formed by coupling ap _3/2-proton and ag _9/2-neutron according to Nordheim's “weak” rule.     

Investigation of the decay rate for71Ge in chemical compounds and calibration of the Mössbauer isomer shift of the 67 keV γ-transition of73Ge

Changes of the radioactive decay rate of⁷¹Ge (T _1/2=11.43 days) have been studied experimentally for⁷¹Ge in some compounds of bivalent and quadrivalent germanium. Relative changes Δλ/λ of the electron capture probability have been measured, and the chemical changes Δρ(0) of the electron density at the germanium nuclei have been determined from these measurements. Values for the Mössbauer isomer shift calibration constants for the 67 keV γ-transition of⁷³Ge have been estimated:C=δ/Δρ(0)=(0.061±0.020) mm·s^?1/a.u., Δ〈r ²〉=(21±7)·10^?3 fm², ΔR/R=(6.9±2.3)·10^?4.     

p-n Multiplets and band-like structures in106Ag

The half-life of a 3^? excited state in¹⁰⁶Ag was measured as T_1/2 (364.4 keV)=0.9±0.1 ns using the¹⁰³Rh(α, n)¹⁰⁶Ag reaction. The intramultiplet transition rate B(M1, 3^?→2^?) indicates that the configuration π(g_9/2)₀ ^?2π(p_1/2)^?1 vd_5/2 can be assigned. A low-lying 3⁺ isomer, as known in^108,110Ag, was not found in¹⁰⁶Ag, what is explained by the raising energy of the vd_3/2 shell with decreasing neutron number. For the 6^? bandhead of a rotational-like structure T_1/2 (765.2 keV)< 0.2 ns was derived in contradiction to an earlier prediction (200 ns). Indirect evidence for a negative sign of the magnetic moment of¹⁰⁵Ag (g.s.) is obtained.     

Die Lebensdauer des 23/2-Dreiteilchenniveaus des Hafnium 177 und sein Zerfall durchK-verbotene Gamma-Übergänge

An isomeric state of Hf¹⁷⁷ withT _1/2=(1,12±0,10)s was found by a fast chemical separation of the hafnium daughter from the 155d Lu^177m activity. We measured the same half-life by observing the delayedβ-γ-coincidences. A systematic investigation of the whole region 5s≧T _1/2≧10^?7s by the technique of delayed coincidences gave no further isomerism. We assign the observed half-life to the 23/2 three particle state of Hf¹⁷⁷ at 1315 keV and assume that the second hypothetical three particle state at 1337 keV does not exist. The 21/2 rotational state of theK=9/2 band is populated by a strongly converted 14,16 keVγ-transition from the isomeric state at 1315 keV. The 14,16 keVM _I andN _I conversion lines were observed by use of a double focusing magneticβ-spectrometer. The isomerism is caused by theK-selection rule. The retardation of the following threeγ-transitions by different degrees ofK-forbiddeness is discussed. The pulse height spectrum, measured by means of a Li-drifted Ge-detector, does not show the 36,52 keV-γ-transition which was previously assumed to populate the 1301keV-state. In addition to the knownγ-transitions we found a 40,9 keV-line. This is probably the transition between the 1301,1 keV and the 1260,3 keV-states.     

A retarded intramultipletM1 transition in214Bi

The half-life of the 53.2 keV level in²¹⁴Bi has been measured asT _1/2=0.52±0.15 ns, furtherT _1/2(295.2 keV and 351.9 keV levels)≦0.10 ns was estimated. TheB(M1,2^?→1^?) transition rates within theπh _9/2 vg _9/2 multiplet in^210,212,214Bi are found to decrease rapidly with increasing neutron number, reaching in²¹⁴Bi a value as low as those typical for intraband M1 transitions in deformed odd-odd nuclei.     

Innere Konversion der 161 keV- und 223 keV-Übergänge in133Cs

Using a Ge(Li)-Si (Li)-spectrometer the 161 keV and 223 keV transitions of¹³³Cs were investigated. TheK-conversion coefficients were deduced to beα _K =0.205±0.007 andK-conversion coefficients were deduced to beα _K =0.0743±0.0043, respectively. TheK/L ratio for the 161 keV transition is 4.72±0.37. From theK-conversion coefficients were deduced to beα _K -values,M1 penetration factors ofλ=8.6±3.4 andλ=7.8 _?2.8 ^3.0 were deduced which are inconsistent with known data from angular correlation experiments (λ=40±10 andλ=90±13). The penetration factor fromK/L-measurement for the 161 keV-transition isλ=52±19. A theoretical reinvestigation of the formulas used in the literature appears recommendable. Furthermore, theK/L ratio of the 1770 keV transition of²⁰⁷Pb was determined experimentally to be 5.52±0.54.     

Transition probabilities and the structure of some negative-parity states in126,130Xe and132Ba

The lifetimes of several negative-parity states in^126,130Xe and¹³²Ba have been determined by means of the generalized centroid-shift method. The reactions^124,128Te(α,2n) and¹²²Sn(¹³C, 3n) have been used. Following results were obtained:T _1/2(2758 keV)=1.3±0.2 ns in¹²⁶Xe,T _1/2(2060 keV)=0.20±0.10 ns,T _1/2(2104 keV)=0.50±0.10 ns,T _1/2(2376 keV)=0.30±0.10 ns andT _1/2(2973 keV)=4.6±0.4 ns in¹³⁰Xe as well asT _1/2(2120 keV)=0.40 _?0.10 ^+0.20 ns in¹³²Ba. A systematics of the B(E2; 7 _? ¹ ?5 ₁ ^? ) values in theN=76 nuclei is presented. Electric dipole and quadrupole transition rates are discussed in terms of octupole and quadrupole collectivity. The structure of the 5 ₁ ^? and 7 ₁ ^? states is considered. Nuclear reactions:^124,128Te(α, 2 _n ),E=26 MeV,¹²²Sn (¹³C, 3n),E=53 MeV; measuredE _γ I _γ , γ-r.f. DeducedT _1/2, B(σL) in^126,130Xe and¹³²Ba. Ge detectors. Generalized centroid-shift analysis.     

The electron capture decay of125I and145Pm

The productP _K ω _K of theK-capture probability and theK-fluorescence yieldω _K was measured in the EC decay of 17.7 y¹⁴⁵Pm and 60.14d¹²⁵I by means ofK x-ray-γ-ray coincidences with semiconductor detectors. Accepting a best value ofω _K =0.920 forZ=60 from the literature, values ofP _K =0.606±0.025 and 0.554±0.025 for decay of¹⁴⁵Pm to the 67.2 and 72.4 keV levels in¹⁴⁵Nd, respectively, were determined, from which the application of EC theory givesQ _EC=153±4 keV to the ground state. TheP _K ω _K ratio to the 67.2 and 72.4 keV levels also was determined independently to be 1.11±0.01, which serves as a good check on theγ-ray-gatedP _K values. Theγ-ray energies were determined more accurately to be 72.4±0.1 and 67.2±0.1 keV, together with a ratio of their relative intensities,I _72.4/I _67.2=3.35±0.09. In the decay of¹²⁵I, a value ofP _K ω _K =0.699±0.030 was measured, and by using an independent determination ofQ _EC=178±2 keV to the ground-state from the literature, a value ofP _K=0.801 is calculated from allowed EC theory, from whichω _K =0.873±0.017 atZ=52 is obtained. This value is in good agreement with theoretical values and with a value of 0.875±0.028 predicted by the best fit curve of Bambyneket al.     

Collective contributions to E1, ΔK=1 matrix elements in odd-odd deformed nuclei

The half-life of the 184.3 keV state in¹⁶⁵Dy has been remeasured asT _1/2=1.0±0.1 ns in order to deduce a reliable value for the transition matrix element of the depopulatingE l,ΔK=1 transition. Experimental E1,ΔK=1 transition matrix elements in odd-odd deformed nuclei are found to be systematically larger than similar values in adjacent odd-A isotones. This effect is supposed to be associated with higher-order vibrational admixtures coupled via RPC andp— n interaction mixings.