太赫兹波段石墨烯等离子体的增益特性

基于麦克斯韦方程组和物质本构方程对石墨烯表面等离子体进行了研究.从理论上探索了石墨烯表面等离子体激元在太赫兹波段的增益特性曲线,并且讨论了石墨烯表面等离子体增益与石墨烯中载流子浓度、石墨烯所处温度以及载流子动量弛豫时间的关系.研究结果表明:在太赫兹波段增益峰值随着石墨烯载流子浓度的增加而发生蓝移,并且在所讨论的温度范围内,由于增益峰所对应的频率都大于1 THz,因此温度的变化对增益峰值以及相应频率的影响不大,即在不同的温度下,相同载流子浓度所对应的增益曲线上峰值的位置和强度几乎相同;增益与石墨烯载流子动量弛豫时间相关,随着载流子动量弛豫时间的增加,使得激发态激励的电子增加,从而导致石墨烯表面等离子体增益变得更大,但这种动量弛豫时间的增加却因弛豫时间对受激辐射频率影响较小而并未对增益峰值位置产生影响.     

Picosecond buildup and relaxation of intense stimulated emission in GaAs

In support of the idea developed previously based on circumstantial evidence, we have found that stimulated emission emerges in GaAs and its intensity increases with a picosecond delay relative to the front of powerful picosecond optical pumping that produced a dense electron-hole plasma. The emission intensity relaxes with decreasing pumping with a characteristic time of ～10 ps. We have derived the dependences of the delay time, the relaxation time, and the duration of the picosecond emission pulse on its photon energy. The estimates based on the fact that the relaxation of emission is determined by electron-hole plasma cooling correspond to the measured relaxation time.     

光抽运信号的理论分析

在原子辐射跃迁原理的基础上,依据光磁共振实验的基本实验现象建立简化模型,给出光抽运过程中跃迁速率方程,理论计算了光抽运信号光强随外场变化关系以及粒子跃迁弛豫时间随外场的变化关系,理论计算结果与实验符合.     

基于振动弛豫理论提高光抽运太赫兹激光器输出功率的研究

以半经典密度矩阵理论和分子振动弛豫理论为基础,研究添加适当比例缓冲气体与适当减小波导芯径对光抽运太赫兹激光器输出光强的影响.计算结果表明,加入适当比例缓冲气体或适当减小波导的芯径均能提高太赫兹激光的输出光强;同时优化两个参数能进一步提高抽运激光能量转化为太赫兹激光能量的效率,延长工作腔中的有效激活区,延缓抽运饱和效应的出现,提高太赫兹激光输出光强.该研究对提高光抽运太赫兹激光器的能量转化效率、提高光抽运太赫兹激光器的输出功率及实现光抽运太赫兹激光器的小型化有重要的指导意义.     

Thermodynamic properties of saturated semiconductors

The thermodynamic properties of a direct gap semiconducting system, under high intensity optical pumping are studied. The strong electromagnetic field of the pumping beam must have a frequency larger than the band gap. A Bose condensation of electron-hole pairs of zero momentum is found as the temperature goes to zero. This condensation persits even when the finite wavevector of the pump is taken into account.     

Theoretical study of relaxation oscillation in triply resonant OPOs

The relaxation oscillation in triply resonant optical parametric oscillators (TROs) is studied theoretically. With constant pumping, the intensity noise spectra of the signal wave consist of a zero frequency and a relaxation oscillation frequency. An accurate relation between the relaxation oscillation frequency and the pump power is obtained. The square of the inherent relaxation oscillation frequency in TROs is linear in the square root of the pump power under high-power pumping. Also, the decay rate varies rapidly with low-power pumping and slowly with high-power pumping. Significantly, when there is a relaxation oscillation in the pumping, the undulation of the signal photon density in TROs also contains the relaxation oscillation frequency of the pumping besides its inherent noise. When those two frequencies are close, a resonance will appear, which should be avoided in practice. PACS 42.65.Yj; 42.65.Sf; 42.60.Rn     

ZnS/CdSe量子点中线性和三阶非线性光吸收系数研究

在有效质量近似下,利用量子力学的密度矩阵理论,采用无限深势阱模型,从理论上研究了ZnS/CdSe柱型核壳结构量子点中线性和三阶非线性光吸收系数。导出了柱型量子点中线性和三阶非线性光学吸收系数的解析表达式,分析了该系统在不同条件下线性和三阶非线性光吸收系数与入射光频率之间的关系。改变系统的参数,该系统的光吸收系数呈规律性变化。计算结果表明:弛豫时间τ、入射光强I和壳半径R2对系统的吸收系数α有很大的影响,从而为实验上研究核壳结构量子点的非线性光学效应提供了必要的理论依据。     

Temperature relaxation and energy loss of hot carriers in graphene

The temperature relaxation and energy loss of hot Dirac fermions are investigated theoretically in graphene with carrier–optical phonon scattering. The time evolutions of temperature and energy loss for hot Dirac fermions in graphene are calculated self-consistently. It shows that the carrier–optical phonon coupling results in the energy relaxation of hot carriers excited by an electric field, and the relaxation time for temperature is about 0.5–1 ps and the corresponding energy loss is about 10–25 nW per carrier for typically doped graphene samples with a carrier density range of 1–5×10¹² cm^?2. Moreover, we analyze the dependence of temperature and energy relaxation on initial hot carrier temperature, lattice temperature and carrier density in detail.     

Spin relaxation in single-layer and bilayer graphene

We investigate spin relaxation in graphene spin valves and observe strongly contrasting behavior for single-layer graphene (SLG) and bilayer graphene (BLG). In SLG, the spin lifetime (τ(s)) varies linearly with the momentum scattering time (τ(p)) as carrier concentration is varied, indicating the dominance of Elliot-Yafet (EY) spin relaxation at low temperatures. In BLG, τ(s) and τ(p) exhibit an inverse dependence, which indicates the dominance of Dyakonov-Perel spin relaxation at low temperatures. The different behavior is due to enhanced screening and/or reduced surface sensitivity of BLG, which greatly reduces the impurity-induced EY spin relaxation.     

On the possibilities of sub-Doppler atomic spectroscopy in multilayer gas cells

Possibilities of high-resolution spectroscopy of atoms (or molecules) for optical pumping and probing with the use of a proposed cell with a series of plane-parallel thin gas layers between spatially separated regions of this cell are theoretically studied. It is shown that efficient velocity selection of optically pumped atoms is possible in view of their characteristic transit and collisional relaxation in such a cell, which leads to the formation of narrow sub-Doppler resonances in absorption of a probe monochromatic wave. The resolution of this spectroscopic method is analyzed in the cases of stationary and definite nonstationary optical pumping of atoms by broadband radiation for different geometrical parameters of these cells and pumping intensity. The proposed multilayer gas cell is a compact analog of a large number of parallel atomic (molecular) beams and can be the basis for new high-precision and compact optical frequency standards.     

Post-transient relaxation in graphene after an intense laser pulse

High intensity laser pulses were recently shown to induce a population inverted transient state in graphene [T. Li, et al., Phys. Rev. Lett. 108, 167401 (2012)]. Using a combination of hydrodynamic arguments and a kinetic theory we determine the post-transient state relaxation of hot, dense, population inverted electrons towards equilibrium. The cooling rate and charge-imbalance relaxation rate are determined from the Boltzmann-equation including electron-phonon scattering. We show that the relaxation of the population inversion, driven by inter-band scattering processes, is much slower that the relaxation of the electron temperature, which is determined by intra-band scattering processes. This insight may be of relevance for the application of graphene as an optical gain medium.     

等离激元增强的石墨烯光吸收

石墨烯中等离激元具有特殊的光电性质,其和入射光的强烈耦合可以引起光吸收的增强.本文基于时域有限差分法和多体自洽场理论研究了等离激元对处于光学谐振腔中的石墨烯光吸收的影响.由于石墨烯中等离激元与入射光动量和能量不匹配而不能直接相互作用,因此石墨烯上施加了金属光栅结构.研究发现光栅结构能够对入射光进行动量补偿并且能够引起其下石墨烯中的电场强度产生很大程度增强,从而导致在该石墨烯结构中太赫兹等离激元和入射光发生强烈耦合而产生太赫兹等离极化激元,同时引起石墨烯光吸收的增强.希望本文能够加深对石墨烯光电特性的理解以及可以为基于石墨烯的太赫兹光电装置提供一定的理论依据.     

简并四波混频信号的饱和效应

本文由光学Bloch方程和密度矩阵方程出发,研究了二能级系统共振型简并四波混频(DFWM)的饱和效应,给出了DFWM信号强度与泵浦光强度的函数关系.饱和泵浦光强的大小取决于纵向弛豫时间T1和横向弛豫时T2.对理论结果与相应实验进行了比较,表明二者符合得很好.     

On the Sub-Doppler Spectroscopy of Optically Excited Atoms in a Thin Gas Cell

This work continues a theoretical investigation of the capabilities of the well-known method based on using a monochromatic probe light beam in combination with optical pumping of atoms (molecules) of a rarefied-gas medium by a broadband radiation in a thin cell the diameter of which is much larger than its internal thickness. In contrast to calculations carried out in the previous publications on this method of spectroscopy, here, we consider the case of arbitrary values of pump intensity and thickness of a cylindrical gas cell. Thus, all the possible mechanisms and specificities of velocity selection of atoms in optically excited levels caused by transit-time relaxation of such atoms in gas cells of this kind are analyzed. Within the framework of this approach, sub-Doppler absorption resonances of the probe light beam corresponding to quantum transitions from the upper level excited by optical pumping are investigated. The obtained results can be used in high-resolution spectroscopy of atoms (molecules), as well as for laser-frequency stabilization to established narrow spectral resonances.     

Selective excitation of multipolar surface plasmon in a graphene-coated dielectric particle by Laguerre Gaussian beam

Localized surface plasmonic resonance has attracted extensive attention since it allows for great enhancement of local field intensity on the nanoparticle surface. In this paper, we make a systematic study on the excitation of localized surface plasmons of a graphene coated dielectric particle. Theoretical results show that both the intensity and frequency of the plasmonic resonant peak can be tuned effectively through modifying the graphene layer. Furthermore, high order localized surface plasmons could be excited and tuned selectively by the Laguerre Gaussian beam, which is induced by the optical angular orbital momentum transfer through the mutual interaction between the particle and the helical wavefront.Moreover, the profiles of the multipolar localized surface plasmons are illustrated in detail. The study provides rich potential applications in the plasmonic devices and the wavefront engineering nano-optics.     

Nonequilibrium states of the soft mode anharmonic phonons

A theory of the nonequilibrium state of the soft mode optical phonons in ferroelectrics exposed to the pumping electromagnetic field has been developed. The self-consistent field equation, which determines the phase transition temperature shift and the dielectric permeability change due to a deviation of the system from the equilibrium state is derived. A two-temperature model describing the energy transport in the presence of pumping is suggested. Analytic solutions of this model both for evolving in time and for stationary states are obtained. Spatial oscillations of the soft mode temperature are predicted for the observation time approximately equal to the energy relaxation time. It is shown that nonlinear effects can be a reason of forming of the bottleneck in the energy relaxation process. An exactly solvable model of a breather: the breather with the one-site non-linearity has been constructed and investigated.     

Generation of picosecond optical pulses from single heterostructure GaAs diode laser and their emission characteristics

Emission characteristics of a single heterostructure GaAs diode laser are reported using a simple driver circuit. It provides a single picosecond time duration optical pulse, a pulse train or a broad optical pulse depending on the amplitude and time duration of the electrical pump pulse. Results show that relaxation oscillation frequency depends on the amplitude of pumping current pulse as well as on some inherent property of diode laser, which seems to be the level of impurity in lasing medium. Variation of relaxation oscillation frequency with amplitude of current pulse shows only the qualitative agreement with the reported theoretical predictions.     

紧聚焦飞秒脉冲与石英玻璃相互作用过程中的电子动量弛豫时间研究

本文通过数值模拟(3+1)维扩展的广义非线性薛定谔方程,研究了紧聚焦飞秒激光脉冲在诱导石英玻璃的非线性电离过程中电子动量弛豫时间对于该电离过程的影响.计算结果证明电子动量弛豫时间会直接影响入射脉冲在焦点区域所形成的峰值场强、自由电子态密度和能流等参量的分布态势,因此在与实验结果相比较后发现适合于相互作用过程的电子动量弛豫时间的理论值约为1.27 fs.进一步的研究表明,电子动量弛豫时间与逆韧致吸收效应、雪崩电离的概率、等离子体密度、等离子体的自散焦效果以及间接引起的焦平面位置的移动都有着密切的联系.当前的研究结果表明电子动量弛豫时间在飞秒激光脉冲与物质相互作用的过程中发挥着重要作用.     

Tunable dual-band terahertz graphene absorber with guided mode resonances

A tunable dual-band terahertz absorber is designed and investigated. The unit cell of the proposed absorber consists of a graphene monolayer on a guided-mode resonant filter. The graphene absorber presents > 40% absorption at two resonance frequencies, which is attributed to the guided mode resonances with different mode numbers. The electric field intensity distribution is analyzed to disclose the physical mechanism of such a dual-band absorption effect. Furthermore,the influence of optical properties of graphene, including Fermi level and relaxation time, on the absorption spectra are investigated. Finally, the influence of geometric parameters on the absorption spectrum is studied, which will provide useful guidance for the fabrication of this absorber. We believe that the results may be useful for developing the next-generation graphene-based optoelectronic devices.     

Ultrafast nonlinear optical response and high density excitation effects of the stacking fault exciton in BiI3

On the exciton states localized at a two-dimensional stacking fault interface in a layered crystal BiI₃, some nonlinear optical phenomena clearly appear reflecting large transition probability. The optical Stark shift and other high density exciton effect on the energy-shift and the spectral broadening are observed with clear separation under intense laser pumping by time-resolved measurements. The optical Stark shift is analyzed based on the dressed exciton model. The ultrafast optical response faster than 3 ps for the pump-laser field is confirmed on the Stark shift. Degenerate four-wave-mixing signals show fairly long dephasing time of 40 ps in this system. The dephasing probability depends linearly on the pump-laser intensity in the same manner as that of the spectral line-broadening reflecting the relaxation process. The dephasing mechanisms are understood by the exciton scattering at high density in parallel with the spectral changes. The blue-shift due to the high density excitons are discussed on the basis of exciton-exciton interaction in connection with a phase-space filling theory in two-dimensional systems.