Few-cycle pulse compression through cascade of bulk media and hollow-core fiber

We experimentally demonstrated a new few-cycle pulse compression technique through the cascade of bulk media and hollow-core fiber (HCF) and this compression system has been intensively studied. The pulses with the duration of ∼5 fs and the energy of 0.33 mJ near 800 nm have been generated by compressing the ∼40 fs input pulse from a commercial laser system. In principle, this technique allows compression of pulses with duration of picoseconds to a few cycles (sub-7 fs) and the output can be above 1 mJ.     

Above-threshold ionization at the few-cycle limit

Photoelectron spectra measured for rare-gas atoms ionized with intense few-cycle laser pulses are presented. Several aspects of the few-cycle regime are discussed. In particular, the persistence of the plateaulike structure of spectra for high electron energies is shown. In contrast, a resonancelike feature at similar electron energies is suppressed as compared with longer laser pulses. Differences in the behavior of different species and implications for the electron-ion scattering cross section are pointed out.     

Time-domain differentiation of terahertz pulses

We report on the time-domain differentiation of light waves by metallic transmission gratings. Time-resolved terahertz experiments show that the first time derivative of an arbitrary waveform can be achieved by use of gratings of subwavelength period. The results are in accord with classical diffraction theory and may permit novel applications for tailoring few-cycle light pulses and ultrahigh-frequency optoelectronics.     

Carrier-envelope phase effects on high-harmonic generation driven by mid-infrared laser field

The influence of the carrier-envelope phase on high-harmonic generation is investigated, both experimentally and theoretically, for three different interaction gas media, driven by mid-infrared, few-cycle and CEP-stabiUzed laser pulses. Different patterns of harmonic spectra with varying CEP for the three interaction gas media are observed. Furthermore, in comparing our experiment results to the previous works driven by near-infrared laser pulses, different phenomena are found. Through numerical simulation, we find that for the two different kinds of driving fields, i.e. mid-infrared and near-infrared laser pulses, different kinds of electron trajectories contribute to the generation of high harmonics.     

少周期激光脉冲与气体作用产生的离化电流和THz波辐射

本文通过理论和数值模拟,研究少周期激光脉冲电离气体原子产生的离化电流 以及相应的THz波辐射.研究表明,少周期激光脉冲离化气体后能产生较大的离化电流, 因而可以产生较强的THz辐射.不同的少周期激光脉冲相位导致电离出的 电子初始速度和电离起始时刻不同,从而产生的离化电流有所不同, 辐射的THz波随激光脉冲的相位成周期性变化.该理论得到一维PIC数值模拟的验证. 对于给定的激光脉冲相位,离化电流和THz辐射振幅并没有随入射激光振幅的增加而单调增加, 而是存在一些极值点.与均匀分布气体相比,当气体分布具有一定梯度时, 辐射表现相似的规律,但频谱会发生一定的变化.     

Broadband Terahertz Wave Generation from Monolayer Graphene Driven by Few-Cycle Laser Pulse

We theoretically investigate the characteristics of terahertz(THz) radiation from monolayer graphene exposed to normal incident few-cycle laser pulses, by numerically solving the extended semiconductor Bloch equations. Our simulations show that the THz spectra in low frequency regions are highly dependent on the carrier envelope phase(CEP) of driving laser pulses. Using an optimal CEP of few-cycle laser pulses, we can obtain broadband strong THz waves, due to the symmetry breaking of the laser-graphene system. Our results also show that the strength of the THz spectra depend on both the intensity and central wavelength of the laser pulses. The intensity dependence of the THz wave can be described by the excitation rate of graphene, while wavelength dependence can be traced back to the band velocity and the population of graphene. We find that a near single-cycle THz pulse can be obtained from graphene driven by a mid-infrared laser pulse.     

Numerical modeling of generation of few-cycle pulses in a mode-locked laser

We have performed numerical simulation of a laser generating few-cycle pulses in the regime of coherent mode locking. It is shown that such a laser can support generation of pulses with a duration close to the reciprocal of the main laser transition frequency of the gain medium in a wide range of laser parameters.     

Controlling the carrier-envelope phase of ultrashort light pulses with optical parametric amplifiers

The phase link between signal, idler, and pump waves in a parametric interaction allows generation of an idler pulse with a phase independent of that of the input pulse. We suggest the use of a white-light seeded optical parametric amplifier as a self-stabilized source of few-cycle pulses, in which the phase of the electric field is exactly reproduced in each laser shot.     

Generation of high-energy few-cycle laser pulses by using the ionization-induced self-compression effect

A mechanism behind the ionization-induced self-compression effect for ultrashort laser pulses propagating in gas-filled capillaries is proposed. It is shown that as a result of excitation of the nonlinear-plasma waveguide laser pulses producing gas ionization can be self-compressed to few-cycle duration. This effect is used for high-energy laser pulses and its scalability to J-level energies is demonstrated.     

飞秒激光脉冲在正色散固体材料中的自压缩

实验研究了正色散固体介质中的激光脉冲自压缩现象,证明了无需任何外加色散补偿情况下，固体透明介质中的自聚焦传输过程可使高功率飞秒激光脉冲实现时域脉冲压缩，并详细研究了输出脉冲的时域和频域特性随入射脉冲强度的演化规律.实验结果表明脉冲自压缩量随入射脉冲强度的增加呈递增趋势，然而当入射光强增大到足以引起超连续谱及锥形辐射产生时，脉冲时域形状会发生分裂.此外还发现发散光束入射情况下同样可以观察到脉冲自压缩现象. 关键词： 超短激光脉冲 脉冲压缩 非线性传输     

Self-compression of 1.8-μm pulses in gas-filled hollow-core fibers

We numerically study the self-compression of the optical pulses centered at 1.8-μm in a hollow-core fiber(HCF) filled with argon. It is found that the pulse can be self-compressed to 2 optical cycles when the input pulse energy is 0.2-m J and the gas pressure is 500-mbar(1 bar = 10~5 Pa). Inducing a proper positive chirp into the input pulse can lead to a shorter temporal duration after self-compression. These results will benefit the generation of energetic few-cycle mid-infrared pulses.     

利用三色组合脉冲激光获得孤立阿秒脉冲发射

孤立阿秒脉冲因可以跟踪和控制原子及分子内电子的运动过程而备受关注.本文从理论上开展了氦原子在3束飞秒脉冲激光组合场辐照下产生的高次谐波和阿秒脉冲辐射的研究.组合激光场由16 fs/1600 nm,15 fs/1100 nm和5.3 fs/800 nm的钛宝石脉冲构成.与前两束脉冲合成的双色场产生谐波谱相比,附加钛宝石脉冲的三色场产生的高次谐波发射谱呈现出高转换效率及宽带超连续特性,超连续谱范围覆盖从230—690次谐波,傅里叶变换后实现了128 as高强度孤立短脉冲的产生.该结果归因于合成的三色场呈现出高功率及少周期的中红外飞秒脉冲激光特性,可以有效控制原子电离以及复合发生在中红外飞秒脉冲的一个有效光学周期内.     

Accurate retrieval of structural information from laser-induced photoelectron and high-order harmonic spectra by few-cycle laser pulses

By analyzing accurate theoretical results from solving the time-dependent Schr?dinger equation of atoms in few-cycle laser pulses, we established the general conclusion that laser-generated high-energy electron momentum spectra and high-order harmonic spectra can be used to extract accurate differential elastic scattering and photo-recombination cross sections of the target ion with free electrons, respectively. Since both electron scattering and photoionization (the inverse of photo-recombination) are the conventional means for interrogating the structure of atoms and molecules, this result implies that existing few-cycle infrared lasers can be implemented for ultrafast imaging of transient molecules with temporal resolution of a few femtoseconds.     

Optical pulse compression of ultrashort laser pulses in a multi-hollow-core fiber

By numerical simulations and analysis, we proposed a fiber with multi-hollow-core structure for optical pulse compression of high energy ultrashort laser pulses. In this scheme, different parts of a high-energy flat-top pulse are coupled into different hollow cores of such fiber and each of the cores functions as an independent traditional hollow-core fiber compressor. After the multi-hollow-core fiber, the output beams are collimated and compressed to few-cycle level. Then they can be focused to ultra-high intensity. This method can easily be scaled to compressing pulses of large beam size with high energy without limit in principle.     

基于固体薄片超连续飞秒光源驱动的高次谐波产生实验

本文报道了采用基于熔石英薄片超连续的少周期飞秒光源驱动高次谐波产生的实验研究.实验中通过将重复频率1kHz的飞秒钛宝石激光放大器所输出的能量0.8mJ、脉宽30fs的脉冲聚焦到7片0.1mm厚的熔融石英片中,得到了覆盖带宽大于倍频程的展宽光谱.利用啁啾镜补偿色散后,经瞬态光栅频率分辨光学开关法测得脉宽为6.3fs,对应约2.3个光学周期.利用压缩后的激光脉冲聚焦作用于惰性气体,并通过调节尖劈插入量改变脉宽,分别测得了分立以及连续的高次谐波截止区信号,结果与6.3fs的脉冲宽度相符合.     

Field-free molecular alignment and its application

Field-free molecular alignment can be achieved by nonadiabatic rotational excitation of molecules with strong femtosecond laser pulses. We experimentally and theoretically demonstrate that the degree of alignment can be improved with multi-pulse excitation. An approach is proposed to tune the frequency of few-cycle pulses using field-free alignment of molecules.     

Intensity-dependent asymmetric photoionization in few-cycle laser pulses

The asymmetric photoionization of atoms irradiated by intense, few-cycle laser pulses is studied numerically. The results show that the pulse intensity affects the asymmetric photoionization in three aspects. First, at higher intensities, the asymmetry becomes distinctive for few-cycle pulses of longer durations. Second, as the laser intensity increases, the maximal asymmetry first decreases then increases after it has reached a minimal value. Last, the value of the carrier-envelope phase corresponding to the maximal asymmetry varies with the pulse intensity. This study reveals that the increasing of pulse intensity is helpful for observing the asymmetric photoionization.     

Generation of few-cycle laser pulses by coherent synthesis based on a femtosecond Yb-doped fiber laser amplification system

We demonstrate a coherent synthesis system based on femtosecond Yb-doped fiber laser technology. The output pulse of the amplification system is divided into two replicas and seeded into photonic crystal fibers of two parallel branches for nonlinear pulse compression. Because of the different nonlinear dynamics in the photonic crystal fibers, the compressed pulses show different spectra, which can be spliced to form a broad coherent spectrum. The integrated timing jitter between the pulses of two branches is less than one tenth of an optical cycle.By coherently synthesizing pulses from these two branches, 8 fs few-cycle pulses are produced.     

Ultrashort-pulse wave-front autocorrelation

Combined spatially resolved collinear autocorrelation and Shack-Hartmann wave-front sensing of femtosecond laser pulses is demonstrated for the first time to our knowledge. The beam is divided into multiple nondiffracting subbeams by thin-film micro-optical arrays. With hybrid refractive-reflective silica/silver microaxicons, wave-front autocorrelation is performed in oblique-angle reflection. Simultaneous two-dimensional detection of local temporal structure and wave-front tilt of propagating few-cycle wave packets is demonstrated.     

Enhanced transmission and reflection of few-cycle pulses by a single slit

We show that a physical mechanism responsible for the enhanced transmission and reflection of ultrashort (few-cycle) pulses by a single subwavelength slit in a thick metallic film is the Fabry-Perot-like resonant excitation of stationary, quasistationary, and nonstationary waves inside the slit, which leads to the field enhancement inside and around the slit. The mechanism is universal for any pulse-scatter system, which supports the stationary resonances. We point out that there is a pulse duration limit below which the slit does not support the intraslit resonance.