共查询到20条相似文献,搜索用时 683 毫秒
1.
E. Buixaderas S. Kamba J. Petzelt M. Savinov N.N. Kolpakova 《The European Physical Journal B - Condensed Matter and Complex Systems》2001,19(1):9-16
The infrared reflectivity of Cd2Nb2O7 single crystal was studied in the temperature interval of 10-540 K, together with complementary dielectric measurements.
A ferroelectric soft mode was revealed above the ferroelectric phase transition at T
c = 196 K coupled with a central-mode type dispersion in the near-millimetre range. This proves the mixed displacive and order-disorder
nature of the transition. Below T
c many new modes were detected due to lowering of the symmetry, especially below the previously suggested incommensurate transition
at 85 K. Discussion of the possible phase transitions based on symmetry considerations is presented with the conclusion that
the ferroelectric transition is proper with the F1u symmetry of the order parameter, whereas the intermediate ferroelastic transition is improper and triggered by the coupling
with the ferroelectric order parameter.
Received 17 July 2000 相似文献
2.
Th. Brückel D. Hupfeld J. Strempfer W. Caliebe K. Mattenberger A. Stunault N. Bernhoeft G.J. McIntyre 《The European Physical Journal B - Condensed Matter and Complex Systems》2001,19(4):475-490
We report on X-ray resonance exchange and neutron scattering of metallic GdS. At the LII and L III absorption edges of Gd, resonance enhancements of more than two orders of magnitude over the non-resonant magnetic scattering
are observed. Polarisation analysis proves that these enhancements are due to dipolar transitions from the 2p to the 5d states. The branching ratio between the LII and L III edges of 2.5 suggests a polarisation of the 5d electrons in the ground state. The antiferromagnetic order is of type II in the fcc lattice. Single crystal diffraction of
hot neutrons suggests that the spin direction lies within the (111) planes with a value for the sublattice magnetisation of
6.51(3) . The critical exponent for the sublattice magnetisation has a value of β = 0.38(2) in agreement with a pure Heisenberg model.
Above T
N, a sharp component persists in the critical diffuse scattering. Lattice distortions give indications for two additional low-temperature
phase transitions at about 49 K and 32 K. We argue that these transitions are not connected to spin reorientations and discuss
the possible influence of fourth-order exchange interactions.
Received 19 November 1999 and Received in final form 12 December 2000 相似文献
3.
L. Zhang W. Kleemann J. Dec R. Wang M. Itoh 《The European Physical Journal B - Condensed Matter and Complex Systems》2002,28(2):163-171
The dielectric permittivity ε′ - i
of SrTi 18O 3 (STO18) is studied under a dc electric field E as a function of the temperature, T. In ε′
vs.
T, a double-peak is found when 0 < E < 30 KV/m. While the peak at high-T is attributed to the smeared ferroelectric phase transition, the low-T one is induced by domain wall motion. The transverse Ising model including an external homogeneous and quenched random-fields
is successfully used to describe both the smeared phase transition and the domain wall response in the low-T domain state. The calculations are in good agreement with the experimental results.
Received 4 January 2002 / Received in final form 25 March 2002 Published online 19 July 2002 相似文献
4.
V.P. Dyakonov M.T. Borowiec A. Jedrzejczak M. Górska N.A. Doroshenko E. Zubov Yu. Bukhantsev T. Zayarnyuk H. Szymczak 《The European Physical Journal B - Condensed Matter and Complex Systems》2002,29(1):9-14
Magnetic phase transition in the CsDyW2O8 magnet has been studied by means of low temperature specific heat C
(
T
) measurements. The magnetic ordering temperature of the Dy3+ sublattice was established to be 1.34 K. The experimental results indicate on the antiferromagnetic character of interactions
between Dy3+ ions. The behavior of the C
(
T
) dependencies above and below T
N
is discussed in frames of different theoretical models. The measurements data on temperature and field dependencies of magnetization
are used to calculate the exchange and dipole-dipole interactions energy and to determine the possible magnetic structure
of the ground state.
Received 7 January 2002 / Received in final form 15 May 2002 Published online 7 September 2002 相似文献
5.
A new interpretation of light-induced magnetization changes of a magnetic semiconductor, manganese arsenide (MnAs), observed
by the authors of references [1,2], is proposed in this paper. Contrary to references [1,2], where the results of experiments
were interpreted as the observation of light-induced phase transition, here we propose a completely different approach. It
suggests that at least far from the vicinity of T
c, there are no real magnetization changes as in case of phase transition, but there are changes of the magnetic flux threading
the MnAs-sample. These changes are due to non-equilibrium light-induced diamagnetic moments of quasi-free electrons of narrow
d-subbands of the MnAs-conduction band. The other aspects of the experiments of [1,2] are also discussed and some similarity
between this effect and the orbital diamgnetism due to persistent currents in mesoscopic structures is emphasised.
Received 7 November 2000 相似文献
6.
W. Zhong W. Chen H.Y. Jiang X.S. Liu C.T. Au Y.W. Du 《The European Physical Journal B - Condensed Matter and Complex Systems》2002,30(3):331-337
Polycrystalline two-layered perovskite La2.5-xK0.5+xMn2O
7 + δ
(0 <
x
< 0.5) samples have been prepared by a modified sol-gel method and their magnetoresistance and magnetocaloric effects have been
studied. A large deviation between the metal-insulator (MI) transition temperature (T
ρ
) and the magnetic transition temperature (TC) is observed. Large magnetoresistance (MR) effects with Δρ/ρ
of ∼40% at 12 kOe are obtained in wide temperature ranges. The maximum of the magnetic entropy change peaks at its Curie temperature
(TC), far above its MI transition temperature (T
ρ
). The large magnetic entropy change (∼1.4 J/kg.K) is obtained in the sample La2.5-xK0.5+xMn2O
7 + δ
(x
= 0.35) upon 10 kOe applied magnetic field.
Received 2 May 2002 / Received in final form 1st October 2002 Published online 19 December 2002
RID="a"
ID="a"e-mail: wzhong@ufp.nju.edu.cn 相似文献
7.
V.Yu. Irkhin M.I. Katsnelson 《The European Physical Journal B - Condensed Matter and Complex Systems》2001,19(3):401-408
The longitudinal and transverse nuclear magnetic relaxation rates 1/T
1(T) and 1/T
2(T) are calculated for three- and two-dimensional (3D and 2D) metallic ferro- and antiferromagnets (FM and AFM) with localized
magnetic moments in the spin-wave temperature region. The contribution of the one-magnon decay processes is strongly enhanced
in comparison with the standard T-linear Korringa term, especially for the FM case. For the 3D AFM case this contribution diverges logarithmically, the divergence
being cut at the magnon gap ω due to magnetic anisotropy, and for the 2D AFM case as ω-1. The electron-magnon scattering processes yield T
2ln(T/ω) and T
2/ω1/2-terms in 1/T
1 for the 3D AFM and 2D FM cases, respectively. The two-magnon (“Raman”) contributions are investigated and demonstrated to
be large in the 2D FM case. Peculiarities of the isotropic 2D limit (where the correlation length is very large) are analyzed.
Received 29 November 1999 and Received in final form 6 June 2000 相似文献
8.
K. Prokes R.T. Gramsma Y. Janssen E. Brück K.H.J. Buschow F.R. de Boer 《The European Physical Journal B - Condensed Matter and Complex Systems》2000,16(3):429-434
Neutron-diffraction experiments reveal that ErFe6Ga6 forms in the tetragonal ThMn12-type of structure (space group I4/mmm). The Fe sublattice orders ferromagnetically below K. The Er moments order antiparallel to the Fe moments which, below about 250 K, leads to a decrease of the total magnetization.
The easy magnetization direction of ErFe6Ga6 is perpendicular to the c-axis in the whole temperature range. Refinement at 2 K shows that ErFe6Ga6 orders ferrimagnetically with Er moments of 8.5 (2) and Fe moments at the 8(j) site of 1.9 (1) and at the 8(f) site of 1.7 (1) , respectively. At room temperature, ErFe6Ga6 exhibits the same type of magnetic order, however with substantially lower Er moments of 1.0 (4) and Fe moments at the 8(f) site of 1.2 (2) . The Fe moments at the 8(j) site amount to 1.9 (5) /Fe.
Received 24 November 1999 and Received in final form 27 March 2000 相似文献
9.
O. Moze J.M. Cadogan Y. Janssen F.R. de Boer K.H.J. Buschow S.J. Kennedy 《The European Physical Journal B - Condensed Matter and Complex Systems》2001,23(1):29-36
The magnetic structure of RFe6Ga6 intermetallic compounds with R = Y, Ho have been determined by neutron powder diffraction, 57Fe M?ssbauer spectroscopy, AC susceptibility, TGA (Thermo-Gravimetric Analysis) and magnetization measurements. Both compounds
crystallize in the tetragonal ThMn12 structure (space group I4/mmm) with the magnetic structure of YFe6Ga6 consisting of a simple ferromagnetic alignment of Fe moments in the basal plane with a Curie temperature of 475(5) K. Gallium
atoms are found to fully occupy the 8i site, with Fe and Ga atoms equally distributed over the 8j site, whilst Fe atoms fully
occupy the 8f site. The average Fe moments are 1.68(10)
and 1.46(10)
at 15 and 293 K, respectively. The average room temperature Fe magnetic moments determined by neutron diffraction are in
overall agreement with the average Fe moment deduced from M?ssbauer spectroscopy and bulk magnetization measurements on this
compound. The magnetic anisotropy of the compound HoFe6Ga6 is also planar in the temperature range 6-290 K, with Ho magnetic moments of 9.28(20)
and 2.50(20)
at 6 K and 290 K, respectively, coupled anti-ferromagnetically to the Fe sublattice and a Curie temperature of 460(10) K.
The magneto-crystalline anisotropies of both compounds are comparable at low temperatures.
Received 8 March 2001 and Received in final form 18 June 2001 相似文献
10.
F. Honda A.V. Andreev V. Sechovský Y. Homma Y. Shiokawa 《The European Physical Journal B - Condensed Matter and Complex Systems》2002,30(3):313-318
Single crystals of U(Ni1-xPdx)2Si2 with x = 0.05, 0.09 and 0.135 have been grown. Magnetization and electrical resistivity measurements were performed in a wide range
of temperatures and magnetic fields in order to study stability of magnetic phases in the solid solutions between UNi2Si2 and UPd2Si2 with a special emphasis on the type of ground state. In UPd2Si2 the simple AFI-type antiferromagnetic structure of U moments is observed at low temperatures. UNi2Si2 adopts the uncompensated AF structure (UAF) with the + + - stacking of U moments along the c-axis and consequently this compound exhibits a spontaneous magnetization corresponding to 1/3 of the U moment. The substitution
of Pd for Ni leads to a rapid decay of the spontaneous magnetization. The evolution of magnetization and electrical resistivity
behavior with Pd doping is tentatively attributed to the coexistence of the AF-I and UAF phases in the ground state of U(Ni0.91Pd0.09)2Si2 and U(Ni0.865Pd0.135)2Si2. In this scenario, the volume fraction of the AF-I phase rapidly grows with Pd doping on account of the UAF. At lowest temperatures
an irreversible transition to the UAF phase is observed when a sufficiently high magnetic field is applied along the c-axis.
Received 28 March 2002 / Received in final form 8 August 2002 Published online 19 December 2002
RID="a"
ID="a"e-mail: sech@mag.mff.cuni.cz 相似文献
11.
A. Podlesnyak Th. Strässle A. Mirmelstein A. Pirogov R. Sadykov 《The European Physical Journal B - Condensed Matter and Complex Systems》2002,29(4):547-552
Neutron powder diffraction was employed to study the pressure effect on the magnetic transition in the pseudobinary Laves-phase
compound Er0.57Y0.43Co2 and to determine the magnetic moments of the Er- and Co-subsystems. Our studies reveal that the onset of long-range magnetic
order for both the localized 4
f (Er) and itinerant 3
d (Co) electron moments appears at about the same temperature at ambient pressure. The pressure effect on Tc is found to be negative and equal for both sublattices, namely
T
c
/
p
∼ - 0.4 K/kbar. The values of the magnetic moments of the Er and the Co ions are found
= 5.40±0.15μ
B
/atom,
= 0.50±0.07μ
B
/atom and 5.35±0.15μ
B
/atom, 0.37±0.09μ
B
/atom, for p
= 0 and 6 kbar, respectively. Our experimental results give evidence for short-range magnetic order formation at temperatures
already above Tc and for a coexistence short- and long-range order below Tc down to 4 K.
Received 20 December 2001 / Received in final form 12 June 2002 Published online 31 October 2002
RID="a"
ID="a"e-mail: andrew.podlesnyak@psi.ch 相似文献
12.
Hartmann L Gorbatschow W Hauwede J Kremer F 《The European physical journal. E, Soft matter》2002,8(2):145-154
The molecular dynamics in thin films (18 nm-137 nm) of isotactic poly(methyl methacrylate) (i-PMMA) of two molecular weights
embedded between aluminium electrodes are measured by means of dielectric spectroscopy in the frequency range from 50 mHz
to 10 MHz at temperatures between 273 K and 392 K. The observed dynamics is characterized by two relaxation processes: the
dynamic glass transition (α-relaxation) and a (local) secondary β-relaxation. While the latter does not depend on the dimensions
of the sample, the dynamic glass transition becomes faster (≤2 decades) with decreasing film thickness. This results in a
shift of the glass transition temperature T
g to lower values compared to the bulk. With decreasing film thickness a broadening of the relaxation time distribution and
a decrease of the dielectric strength is observed for the α-relaxation. This enables to deduce a model based on immobilized
boundary layers and on a region displaying a dynamics faster than in the bulk. Additionally, T
g was determined by temperature-dependent ellipsometric measurements of the thickness of films prepared on silica. These measurements
yield a gradual increase of T
g with decreasing film thickness. The findings concerning the different thickness dependences of T
g are explained by changes of the interaction between the polymer and the substrates. A quantitative analysis of the T
g shifts incorporates recently developed models to describe the glass transition in thin polymer films.
Received 12 August 2001 and Received in final form 16 November 2001 相似文献
13.
A.M. Balagurov V.Yu. Pomjakushin D.V. Sheptyakov V.L. Aksenov N.A. Babushkina L.M. Belova O.Yu. Gorbenko A.R. Kaul 《The European Physical Journal B - Condensed Matter and Complex Systems》2001,19(2):215-223
The atomic structure of (
La
1 - y
Pr
y
)
0.7
Ca
0.3
MnO
3
compound with 0.5≤
y
≤1 has been systematically studied by neutron powder diffraction in the temperature range from 15 to 293 K. For composition
with y
= 0.75, the structural analysis was performed on two samples, one containing the natural mixture of oxygen isotopes and the other
one 75% enriched by
18
O. The room temperature structural characteristics of the series, including cell volume, average Mn-O bond distance, and average
Mn-O-Mn bond angle, are the linear functions of the <
r
A
>. Temperature dependencies of these parameters are quite smooth, except for the point T
=
T
FM
, where a jump like changes occur. The isotope enriched samples have been found identical in crystal and magnetic structure
down to the temperature of transition of the sample with
16
O into the metallic ferromagnetic phase. It confirms that different transport and magnetic properties of the samples with
16
O and
18
O at low temperature are driven by the different oxygen atoms dynamics solely. Temperature dependencies of the CO and AFM diffraction
peak intensities and of the peak widths for compositions close to the metal-insulator boundary ( y
≈ 0.75) indicate the macroscopically phase separated AFM-dielectric + FM-metallic state below T
FM
.
Received 28 April 2000 相似文献
14.
D. Blaschke M.K. Volkov V.L. Yudichev 《The European Physical Journal A - Hadrons and Nuclei》2003,17(1):103-110
The phase diagram for quark matter is investigated within a simple Nambu-Jona-Lasinio model without vector correlations. It
is found that the phase structure in the temperature-density plane depends sensitively on the parametrization of the model.
We present two schemes of parametrization of the model where, within the first one, a first-order phase transition from a
phase with broken chiral symmetry to a color superconducting phase for temperatures below the triple point at T
t = 55 MeV occurs, whereas for the second one a second-order phase transition for temperatures below T
t = 7 MeV is found. In the latter case, there is also a coexistence phase of broken chiral symmetry with color superconductivity,
which is a new finding within this class of models. Possible consequences for the phenomenology of the QCD phase transition
at high baryon densities are discussed.
Received: 3 January 2003 / Accepted: 21 February 2003 / Published online: 24 April 2003 相似文献
15.
L. Martín-Carrón A. de Andrés 《The European Physical Journal B - Condensed Matter and Complex Systems》2001,22(1):11-16
We have studied the behavior of the Raman phonons of a stoichiometric LaMnO3 single crystal as a function of temperature in the range between 77 K and 900 K. We focus on the three main phonon peaks
of the Pbnm structure, related to the tilt, antisymmetric stretching (Jahn-Teller mode) and stretching modes of Mn-O octahedra.
The phonon frequencies show a strong softening that can be fit taking into account their renormalization because of three
phonon anharmonic effects in the pseudoharmonic approximation. Thermal expansion effects, in particular the variation of Mn-O
bond lengths with temperature, are not relevant above 300 K. On the contrary, phonon width behavior deviates from the three
phonon scattering processes well bellow T
c
. The correlation between the magnitude of the cooperative Jahn-Teller distortion, that disappears at 800 K, and the amplitude
of the Raman phonons in the orthorhombic phase is shown. Nevertheless, Pbnm phonons are still observable above this temperature.
Phonon width and intensity behavior around T
c
can be explained by local melting of the orbital order that begins quite below T
c
and by fluctuations of the regular Mn-O octahedra that correspond to dynamic Jahn-Teller distortions.
Received 25 January 2001 and Received in final form 14 March 2001 相似文献
16.
The lattice QCD studies indicate that the critical temperature T
c ≃ 260-280 MeV of the deconfinement phase transition in quenched QCD is considerably smaller than the lowest-lying glueball
mass m
G ≃ 1500-1700 MeV, i.e., T
c ≪ m
G. As a consequence of this large difference, the thermal excitation of the glueball in the confinement phase is strongly suppressed
by the statistical factor e
-mG/Tc ≃ 0.00207 even near T ≃ T
c. We consider its physical implication, and argue the abnormal feature of the deconfinement phase transition in quenched QCD
from the statistical viewpoint. To appreciate this, we demonstrate a statistical argument of the QCD phase transition using
the recent lattice QCD data. From the phenomenological relation between T
c and the glueball mass, the deconfinement transition is found to take place in quenched QCD before a reasonable amount of
glueballs is thermally excited. In this way, quenched QCD reveals a question “what is the trigger of the deconfinement phase
transition ?”
Received: 18 November 2002 / Accepted: 4 February 2003 / Published online: 29 April 2003 相似文献
17.
G. Li S.-J. Feng F. Liu Y. Yang R.-K. Zheng T. Qian X.-Y. Guo X.-G. Li 《The European Physical Journal B - Condensed Matter and Complex Systems》2003,32(1):5-11
The magnetic transport properties have been measured for La0.67-xYxCa0.33MnO3 ( 0 ⩽
x
⩽ 0.14) system. It was found that the transition temperature T
p
almost linearly moves to higher temperature as H increases. Electron spin resonance confirms that above T
p
, there exist ferromagnetic clusters. From the magnetic polaron point of view, the shift of T
p
vs. H was understood, and it was estimated that the size of the magnetic polaron is of 9.7 ∼ 15.4 ? which is consistent with the magnetic correlation length revealed by the small-angle neutron-scattering technique. The
transport properties at temperatures higher than T
p
conform to the variable-range hopping mechanism.
Received 27 August 2002 / Received in final form 2 December 2002 Published online 14 March 2003 相似文献
18.
N. Keller J. Mistrík Š. Višňovský D.S. Schmool Y. Dumont P. Renaudin M. Guyot R. Krishnan 《The European Physical Journal B - Condensed Matter and Complex Systems》2001,21(1):67-73
Orthoferrites present, as bulk materials, reorientation transitions of their magnetic moment alignment at temperatures depending
on the rare-earth (RE) ion. In particular, orthoferrites (REFeO3) with RE = Sm, Dy, present this transition at T
SRT = 443 K and 36 K, respectively. The spectra of the complex Kerr and Faraday angle have been measured on orthoferrite thin
films (RE = Sm, Dy, Y), which were prepared by pulsed laser deposition on amorphous quartz substrates. The obtained spectra
exhibit contributions of both surfaces and interfaces. Propagation effects of the polarized light in the magneto-optical medium
which is interpreted in terms of a simplified theoretical formalism, is also observed. For selected photon energies, temperature
dependent Faraday rotation measurements, , on orthoferrite thin films (RE = Sm, Dy, Y) have been performed. A quite different thermal variation compared to the bulk
magnetization has been observed. Curie temperatures are found to be close to the bulk values or slightly larger by 10 K to
20 K as in the case of DyFeO3 and YFeO3. For RE = Sm and Dy, increases with increasing temperature contrary to the saturation magnetization, passes through a maximum at about 460 K and
vanishes with a T
C of 647±18 K, 695 K for RE = Sm and Dy respectively.
Received 28 July 2000 相似文献
19.
L. Pareti M. Solzi F. Albertini A. Paoluzi 《The European Physical Journal B - Condensed Matter and Complex Systems》2003,32(3):303-307
We have studied the isothermal entropy change around a first-order structural transformation and in correspondence to the
second-order Curie transition in the ferromagnetic Heusler alloy Ni2.15Mn0.85Ga. The results have been compared with those obtained for the composition Ni2.19Mn0.81Ga, in which the martensitic structural transformation and the magnetic transition occur simultaneously. With a magnetic field
span from 0 to 1.6 T, the magnetic entropy change reaches the value of 20 J/kg K when transitions are co-occurring, while
5 J/kg K is found when the only structural transition occurs.
Received 27 September 2002 / Received in final form 17 February 2003 Published online 11 April 2003
RID="a"
ID="a"e-mail: solzi@fis.unipr.it 相似文献
20.
H. Kockar T. Meydan 《The European Physical Journal B - Condensed Matter and Complex Systems》2002,26(4):435-438
Compositions of Fe81B13.5Si3.5C2, Fe67Co18Si1B14 and Fe5.85Co72.15Mo2B15Si5 were deposited on to rigid and flexible substrates for the first time using a dc sputtering source as part of a novel Rotating
Cryostat (RC). The films sputtered on silicon and glass show only isotropic magnetisation, whereas those sputtered on a polyimide
(KaptonTM) substrate exhibited either isotropic or anisotropic magnetisation depending upon composition. Similar findings were obtained
for equivalent evaporated films.
Received 23 October 2001 and Received in final form 29 January 2002 相似文献