Measurement of the extraordinary refractive index dispersion in the MIR for Mg:Nd:LiNbO3 crystals by the use of quasi-phase-matching in a random 1D domain structure

We present a method of measurement of the extraordinary refractive index dispersion in MIR for periodically and aperiodically poled nonlinear crystals with unknown or uncertain periods. The method is based on the spontaneous parametric down-conversion and is useful for the crystals with domain structure formed directly in the process of growth by Czochralski technique. As an example we measure the extraordinary refractive index of in-growth poled 2 mol% Mg and 1 mol% Nd doped congruent lithium niobate and present the corresponding Sellmeier equation in the range of 0.4–3.6 μm.     

Modeling and Characterization of Border Domain Effects in Periodically Poled Lithium Niobate Crystals Grown by the Off-center Czochralski Technique

We report on the optical characterization of periodically poled lithium niobate crystals grown through the Czochralski off-center technique. The optical diffraction technique pointed out that refractive index changes occur at the border domain. Their effect on the second harmonic generation is therefore investigated by numerical analysis in order to predict the conversion efficiency of the grown crystals.     

Phasematching properties of congruent MgO-doped and undoped periodically poled LiNbO<Subscript>3</Subscript> for optical parametric oscillation with ultrafast excitation at 1 µm

A detailed theoretical analysis of the optical properties of periodically poled crystals of lithium niobate for optical parametric oscillation with excitation at 1 μm is presented. Crystals of congruent lithium niobate with and without MgO-doping are considered. The choice of materials, their basic optical properties, quasi-phasematching and wavelength tuning ranges, as well as dispersive effects are discussed. These results provide a useful roadmap for the construction of optical parametric oscillators and generators operating in the ultrashort pulse regime with excitation at 1 μm.     

周期性极化铌酸锂晶体中半非共线型宽带光学参变放大理论研究

基于周期性极化铌酸锂晶体(PPLN)的准相位匹配光参变放大过程,通过倾斜周期极化铌酸锂晶体中极化域(极化光栅)一定角度,实现了介于共线匹配方式和非共线匹配方式之间的一种半非共线型准相位匹配方式,并以该匹配方式下的各光矢量几何关系得出相位匹配曲线,找到在特定抽运光和信号光波长下能获得宽带增益放大的周期极化长度。并研究其极化倾斜角度与温度特性。模拟计算表明,在合适的角度与温度条件下,该方式可以532 nm抽运光抽运的信号光在800 nm和1064 nm处均获得宽带光参变放大。     

Absorption measurement of a 50-mm-Long periodically poled lithium niobate optical parametric oscillator pumped at 1064 nm by a Nd: YAG laser

We measured the absorption of different periodically poled lithium niobate crystals when different wavelength beams come through them. The choice of a periodically poled lithium niobate crystal is utilized by a singly resonant oscillator to efficiently generate 3800-nm light when it is pumped by a 1064-nm laser and to generate the 2600-nm signal, and, then, injection seeded at 1550 nm. The temperature-tuning curve and idler output power of the chosen crystal are measured.     

Direct third harmonic generation due to quadratic cascaded processes in periodically poled crystals

We report the first, according to our knowledge, experiment for direct third harmonic (TH) generation in periodically poled quadratic crystals. TH radiation of a diode array pumped and acousto-optically Q-switched Nd:YVO₄ laser is generated in a 25 mm long periodically poled lithium niobate (PPLN) crystal of period 7.0 μm. A theoretical model is developed that explains the experimental results. It predicts that the efficient phase-matched direct TH generation in periodically poled structures with duty factor 0.5 requires even order quasi-phase matching. In contrast to the similar experiments in bulk birefringence crystals, where direct phase matched TH signal is the sum of the contribution of both intrinsic and cascaded cubic nonlinearities, in periodically poled quadratic crystals only cascaded cubic nonlinearity contributes to the direct phase-matched TH signal.     

Periodic poling of magnesium-oxide-doped stoichiometric lithium niobate grown by the top-seeded solution method

Magnesium-oxide-doped stoichiometric lithium niobate has been produced using the technique of top-seeded solution growth from a lithium-rich melt. Optical tests, performed with a combination of argon-ion laser lines, have confirmed a previously published result (at 532 nm) that this material has superior resistance to photorefractive damage. This material has been shown, for the first time, to be amenable to periodic poling. Optical parametric oscillator tests have shown that this material maintains the advantages of periodically poled, congruent, un-doped lithium niobate while showing no evidence of photorefractive damage under typical operating conditions. Operating wavelengths as a function of quasi-phase-matching period and temperature have been measured for the optical parametric oscillator, providing useful new information about refractive-index dispersion in this material. This work establishes periodically poled, magnesium-oxide-doped stoichiometric lithium niobate as a viable material for nonlinear optics. Received: 28 June 2000 / Revised version: 12 September 2000 / Published online: 7 February 2001     

Discrete spatial solitons formed in periodically poled lithium niobate by electro-optical effect

We report the numerical observation of discrete spatial solitons in a periodically poled lithium niobate waveguide array by applying an electrical field through electro-optical effect. We show that discrete spatial soliton can be controlled by applied voltage in the periodically poled lithium niobate.     

Efficient parametric conversion from 1.06 to 3.8 μm by an aperiodically poled cascaded lithium niobate

We experimentally demonstrated an efficient optical parametric oscillator (OPO) with high parametric conversion from 1.0645 to 3.8?μm. An aperiodically poled magnesium oxide doped lithium niobate wafer was designed and fabricated as the nonlinear crystal of the OPO. A linearly polarized acousto-optic Q-switched Nd:YVO4 laser was used as the pump source. High pump-to-idler conversion efficiency of 18.5% was achieved with a slope efficiency of up to 21.5%. When compared with a periodically poled channel fabricated on the same wafer, under the condition of output coupler optimized for the periodically poled lithium niobate based OPO, an improvement of slope efficiency by 28.3% from 15.2% to 19.5% and total efficiency by 12.5% from 13.6% to 15.3% under the highest pump power of 11?W was realized for the pump-to-idler conversion.     

Spectral phase correlation of coded femtosecond pulses by second-harmonic generation in thick nonlinear crystals

We demonstrate a novel all-optical scheme for measuring the correlation of spectrally phase-coded ultrashort optical waveforms that uses second-harmonic generation (SHG) in long, periodically poled lithium niobate crystals. The SHG yield can be controlled over a range of ~30 dB, depending on the correlation of the applied phase codes. Such a spectral phase correlator has applications for ultrashort-pulse optical code-division multiple-access networking and could serve as a nonlinear optical but classical analog for certain schemes for coherent quantum control of multiphoton processes.     

Frequency doubling of femtosecond erbium-fiber soliton lasers in periodically poled lithium niobate

We report efficient frequency doubling of passively mode-locked femtosecond erbium-fiber lasers. Quasi-phase-matched second-harmonic generation in periodically poled lithium niobate is used to generate 8.1 mW of 190-fs (FWHM), 90-pJ pulses at 777 nm with a conversion efficiency greater than can be obtained with existing birefringently phase-matched nonlinear materials. A dispersion-compensation-free soliton oscillator generating transform-limited 230-fs (FWHM) pulses at 1554 nm is used as a pump laser.     

Dispersion of the dielectric function real part for Mg:LiNbO3 crystals at terahertz frequencies

We study dispersion of the dielectric function real part ε′ in the terahertz-frequency range for bulk and periodically poled congruent LiNbO₃ and Mg:LiNbO₃ crystals. The concentration of Mg in Mg:LiNbO₃ samples was close to 5 mol%, which is the photorefractive threshold. Approximate expressions for extraordinary polariton dispersion dependence were obtained in the range 0.5–6.5 THz. The influence of Mg-dopant on the optical properties of crystals in the terahertz range is revealed. Changes of the defect structure of lithium niobate crystals are discussed.     

Bidirectional, synchronously pumped, ring optical parametric oscillator

We report the operation of a bidirectional femtosecond pulsed ring optical parametric oscillator based on periodically poled lithium niobate, pumped alternately with nonsimultaneous pulses from a Ti:sapphire mode-locked laser. A beat note between the two counterpropagating beams attests to a gyro response without dead band. The sensitivity of the device to differential phase changes is demonstrated by measurement of the nonlinear index of lithium niobate.     

Diffusion-bonded stacks of periodically poled lithium niobate

We constructed diffusion-bonded stacks of periodically poled lithium niobate (PPLN). Such crystals combine the advantages of planar processing used to make PPLN wafers with the power-handling capability of large apertures. We demonstrated an optical parametric oscillator that uses a 3-mm-thick diffusion-bonded stack consisting of three 1-mm-thick PPLN crystals.     

Observation of quadratic spatial solitons in periodically poled lithium niobate

We report what are to our knowledge the first observation and characterization of quadratic spatial solitons in periodically poled lithium niobate (PPLN). Using a Nd:YAG (1064-nm) source, we observed self-trapped solitary-wave propagation over more than six diffraction lengths as a result of the cascaded quadratic nonlinear process. Low-threshold operation (5-kW peak power) was measured for the quasi-phase-matched PPLN structure designed for frequency doubling.     

Electrode geometries for periodic poling of ferroelectric materials

We have realized novel electrode configurations for efficient periodic poling of ferroelectric crystals by applying a simple patterning method based on laser-induced material ablation. The new geometries were theoretically investigated and compared with conventional configurations. A systematic optimization of the patterning according to the ablated profile led to high-quality quasi-phase-matched structures in lithium niobate with a grating period of 20 mum . The periodically poled samples were characterized by use of third-order second-harmonic generation of a Nd:YAG laser.     

Experimental demonstration of super quasi-phase matching in nonlinear photonic crystal

We have demonstrated super quasi-phase matching (QPM) in a super periodically poled lithium niobate (PPLN), which is composed of multiple ordinary PPLN cells. When super QPM is achieved, the slight phase mismatch in each PPLN cell can be further compensated for, and the relevant second harmonic generation is facilitated greatly. This mechanism provides an insightful means to relieve the limitation imposed by sample fabrication inaccuracy and will open up a promising avenue toward highly efficient nonlinear interactions.     

Lateral patterning of nonlinear frequency conversion with transversely varying quasi-phase-matching gratings

We demonstrate control of the nonlinear conversion across a beam profile by using periodically poled lithium niobate with a laterally nonuniform quasi-phase-matching grating. As a representative experiment, generation of a flat-top second-harmonic beam is demonstrated.     

Holographic recording with reduced intermodulation noise in periodically poled lithium niobate

We show that the use of periodically poled lithium niobate doped with Fe and Y ensures a considerable improvement in the quality of reconstructed images compared with the use of single-domain crystals. This improvement is due to inhibition of intermodulation noise and elimination of optical damage.     

Photorefractive response of bulk periodically poled LiNbO3:Y:Fe at high and low spatial frequencies

Polydomain periodically poled samples of iron-doped lithium niobate allow for phase grating recording with the diffraction efficiency close to that ensured by a single-domain sample with identical thickness. At the same time the optical damage induced by a finite transverse size light beam is considerably reduced in the periodically poled sample as compared with single-domain material.