Cross-relaxation and spectral broadening of gain for Nd/Cr:YAG ceramic lasers with white-light pump source under high-temperature operation

Spectral broadening of the fluorescence of a Nd/Cr:YAG ceramic at the 1064 nm lasing wavelength was observed, and the amplification properties at a high temperature were investigated by considering cross-relaxation. These ceramics are promising for use as a solid-laser material pumped with solar or lamp light. It has been found that whenever the temperature of a laser medium is high and a spectral shift occurs, a high small-signal gain remains owing to the broad spectral band and the cross-relaxation. This optical property is remarkably different from that of a Nd:YAG laser. For a conventional Nd:YAG laser, the bandwidth at 1064 nm is 0.45 nm, and a reduction in small-signal gain occurs at a temperature of 373 K because the spectral peak shift is 0.005 nm/K. However, for the Nd/Cr:YAG ceramic, the bandwidths are 1.2 and 1.9 nm in the case of 0.1% Cr ion doping and 3% Cr ion doping, respectively, owing to the existence of excited Cr ions and the shortening of the effective Nd ion coherence time. It is prospected that the laser medium can be used at a high temperature of 600 K.     

Two-pass amplification of CW laser by Nd/Cr:YAG ceramic Active mirror under lamp light pumping

The concept of an Active mirror with transparent Nd/Cr:YAG ceramics is proposed. A new ceramic material pumped by an arc-metal-halide lamp has been experimentally implemented. CW-laser light generated in a 1064 nm Nd:YAG micro-tip oscillator was amplified by an Active mirror made of Nd/Cr:YAG ceramic and pumped by CW arc-lamp light. The saturation power density of the Nd/Cr:YAG ceramic was lower than that of Nd:YAG because the stimulated-cross-section and lifetime were effectively enhanced by the sensitization of Cr ions. The maximum output laser power while keeping spatial beam quality was up to 3 W with an input lamp power of 9 W; the resulting optical-optical conversion efficiency of 33% was close to the theoretical prediction of nearly 50%.     

Laser pulses amplified by Nd/Cr:YAG ceramic amplifier using lamp and solar light sources

Laser pulses generated in a laser oscillator were amplified by Nd/Cr:YAG ceramic amplifiers. The saturation of output-laser energy was experimentally observed. We found that the stimulated emission cross-section of Nd/Cr:YAG ceramics was effectively increased and the saturation fluence was effectively reduced to 0.1 J/cm² due to the energy transfer between excited Cr and Nd ions. The output-laser energy we calculated was compared with the experimental ones and the extractable stored energy in the Nd/Cr:YAG ceramics was evaluated. This laser material is suitable for high-repetition-rate operations because of the high laser gain with low pumping intensity and low effective saturation fluence.     

High repetition rate laser pulses amplified by Nd/Cr:YAG ceramic amplifier under CW arc-lamp-light pumping

Laser pulses with high repetitive rate generated from a Q-switch microchip Nd:YAG oscillator were amplified by Active mirror composed of Nd/Cr:YAG ceramic pumped by CW arc-lamp. The laser pulses were amplified, and saturation of averaged output laser power was observed. Repetitive ratio of injected laser pulses was changed from 20 to 100 kHz. Averaged output laser power and gain were measured, and gain coefficient and power-extraction efficiency were evaluated. Output laser power was calculated and compared to experimentally measured one, and the calculated results are consistent with the experimental ones. For amplification of laser pulses with high repetitive ratio, this laser material can realize very high laser gain with low pumping power density and high optical-optical conversion efficiency under CW-lamp-light pumping.     

Disk-type Nd/Cr:YAG ceramic lasers pumped by arc-metal-halide-lamp

We observed the lasing of highly sensitized Nd/Cr:YAG ceramic disks that use artificial solar radiation pumping. The disk material can be used for high power multi-stage amplifiers pumped by lamplight or sunlight because of its scalability and ability to handle high power densities. A maximum output power of 86 mW was experimentally obtained, and this value correlated well with the calculated results. A small signal gain of 1.9 was obtained, and the estimated stored energy was 0.6 J/cm³, which is three or four times higher than that from a Nd:YAG medium.     

Laser-diode pumped self-Q-switched microchip lasers

Optical properties of Cr,Yb:YAG, Cr,Nd:YAG crystals, and composite Yb:YAG/Cr:YAG ceramics self-Q-switched solid-state laser materials are presented. The merits of these self-Q-switched laser materials are given and the potentials of such lasers can be chosen by the applications. Cr,Yb:YAG and composite Yb:YAG/Cr:YAG ceramics self-Q-switched laser are conducted. Although several tens of kW peak power can be obtained with a monolithic microchip Cr,Yb:YAG laser, the experimental results show that the performance of this laser is limited by the absorption of Cr⁴⁺ ions at a pump wavelength of 940 nm and strong fluorescence quenching at high Cr concentration. Composite Yb:YAG/Cr:YAG ceramics are more suitable to realize high pulse energy and peak power (up to MW level) with optimized lasing and Q-switching parts. In addition, the instabilities induced by the multi-longitudinal mode competition in Cr,Nd:YAG and Cr,Yb:YAG microchip lasers are addressed. The different gain bandwidths of Yb:YAG and Nd:YAG play an important role in the instability of the output laser pulse trains. Stable laser pulses from the Cr,Yb:YAG microchip laser were obtained due to the antiphase dynamics. For the Cr,Nd:YAG microchip laser, the instability caused by the multi-longitudinal mode competition is an intrinsic property. Different transverse patterns were observed in Cr,Nd:YAG microchip lasers when a pump beam with larger diameter was used. Saturated inversion population distribution inside the gain medium plays an important role in the transverse pattern formation. Different transverse patterns were reconstructed by combining different sets of the Hermite-Gaussian modes.     

Optical characteristics of Cr and Nd codoped Y3Al5O12 ceramics

The optical characteristics of Cr³⁺ and Nd³⁺ codoped Y₃Al₅O₁₂ (YAG) ceramics are measured. These measurements are done using two pumping sources, a 808 nm laser diode (LD) and a Xe short-arc lamp, to simulate solar radiation. The specimens used are 0.1%Cr³⁺/1.0%Nd³⁺ and 3.0%Cr³⁺/1.0%Nd³⁺ (atomic%) codoped YAG ceramics. A Nd:YAG crystal doped with 1.0%Nd³⁺ is used as a reference. The saturation intensities of the Cr/Nd:YAG ceramics pumped by the LD are the same as that of the Nd:YAG crystal, while they are higher when they are pumped by the Xe lamp. The saturation intensities are for the 0.1% Cr-doped ceramic and for the 3.0%Cr-doped ceramic. The small signal gains of the 0.1%Cr-doped and 3.0%Cr-doped ceramics are measured and found to be 1.8 times and 7.0 times higher than that of Nd:YAG for the same intensity of solar pumping, respectively. The quantum efficiency of energy transfer from Cr³⁺ to Nd³⁺ is estimated to be 0.88±0.09 for the 0.1%Cr-doped ceramic and 0.67±0.08 for the 3.0%Cr-doped ceramic.     

678 nm RTP electro-optical Q-switched ceramic laser

The RTP electro-optical Q-switched ceramic laser at the wavelength of 678 nm with narrow pulse width is studied. We used the laser diode arrays side-pumped Nd:YAG ceramic crystal with 1.1 at% Nd doping and dimensions of Φ3 mm × 50 mm, designed folding cavity parameters, and discussed the variation of the beam radius in the ceramic crystal and frequency doubling crystal with the thermal focal length of ceramic crystal or KTP crystal. By using double RTP crystals as electro-optic Q-switch and KTP crystal type II phase matching for intracavity frequency-doubling, a narrow pulse width electro-optical Q-switched Nd:YAG ceramic laser was obtained. The output energy of 0.9 mJ and the pulse width of 41.6 ns at 678 nm are obtained at the repetition rate of 1000 Hz and pumped power of 144 W. The results formed the basis for the further development of the high power and high efficiency ceramic red laser.     

A kilowatt level diode-side-pumped QCW Nd:YAG ceramic laser

We demonstrate a kilowatt level Quasi-continuous-wave (QCW) diode-side-pumped Nd:YAG ceramic laser at 1064 nm. The laser system adopts a master oscillator power amplifier scheme (MOPA). The master oscillator contains two diode-pumped laser modules. Under the pump power of 2000 W, an output power of 686 W was obtained. After amplified by an identical ceramic laser module, a maximum output power of 1020 W was obtained under a total incident pump power of 3433 W, corresponding to an optical-optical conversion efficiency of 29.7%. At the maximal output power, the repetition frequency was measured to be 1 kHz and the pulse width was 114 μs. To the best of our knowledge, this is the first time to realize QCW side-pumped Nd:YAG ceramic laser system with output power above 1 kW.     

Dual-polarization electro-optical Q-switched ceramic laser

A dual-polarization electro-optical Q-switched Nd:YAG ceramic laser was studied. By selecting the appropriate size of calcite crystals, the dual-polarization Q-switched pulse was achieved by characteristics of calcite crystal. Experimental results show that compared with the traditional single-polarization electro-optical Q-switched laser, insertion loss is reduced, dynamic to static ratio is greatly improved, thermally induced birefringence of electro-optical Q-switched Nd:YAG ceramic laser is effective compensated. The output power of 19 W and the pulse width of 13 ns are obtained at the repetition rate of 1 kHz and pumped power of 144 W. The dynamic to static ratio is 71%. The results formed the basis for the further development of the high power and high efficiency ceramic red laser.     

Experiments of all-optical switching due to cross-phase modulation in fiber grating coupler by lock-in amp. detection scheme

We report results of experiments examining cross-phase modulation effect on fiber grating coupler (FGC). All-optical switching are observed in both cases of high pump pulses emitted from high-power Nd:YAG laser and mode-locked EDF laser. Based on coherent detection using a lock-in amplifier, the red-shift of the Bragg wavelength for a FGC was estimated to be 0.04-0.06 nm/1.5-1.7 kW peak power of EDF pump light at 1.55 μm. To avoid mixture of pump pulse and signal light at 1.55 μm, we have also performed the experiment using high power Nd:YAG laser as a pump power. For a Nd:YAG laser, the red-shift of Bragg wavelength is estimated to be 0.06 nm at maximum pump power of 2.1 kW. A simple model for the proposed detection scheme is given and the resultant red-shift is analyzed numerically.     

Efficient tunable Yb:YAG ceramic laser

A high-power efficient ceramic Yb:YAG laser was demonstrated at a room temperature of 20 °C with an Yb concentration of 9.8 at.%, a gain medium of 1 mm, a pumping power of 13.8 W, an output coupler of T = 10%, and a cavity length of 20 mm. A 6.8 W cw output power was obtained with a slope efficiency of 72%. The ceramic Yb:YAG laser exhibited a continuous tunability in the spectral range of 63.5 nm from 1020.1 to 1083.6 nm for T = 1% at a maximum output power of 1.6 W. To the best of our knowledge, this is the first study of the tunability of ceramic Yb:YAG lasers, except crystal Yb:YAG studies.     

Passive Q-switching of Pulsed and CW Nd: YAG Lasers with Cr~(4 ): YAG

Ｐａｓｓｉｖｅ　Ｑ－ｓｗｉｔｃｈｉｎｇ　ｏｆ　Ｐｕｌｓｅｄ　ａｎｄ　ＣＷ　Ｎｄ：ＹＡＧ　Ｌａｓｅｒｓ　ｗｉｔｈ　Ｃｒ￣（４＋）：ＹＡＧＰａｓｓｉｖｅＱ－ｓｗｉｔｃｈｉｎｇｏｆＰｕｌｓｅｄａｎｄＣＷＮｄ：ＹＡＧＬａｓｅｒｓｗｉｔｈＣｒ￣（４＋）：ＹＡＧ...     

Laser properties of yag: Nd,Cr, Ce

Summary Transient absorption of a long lifetime ( 20 s) of YAG: Nd is typical of pure material. It is the main reason of thermal deformation of the laser rods accompanied with power decreases at higher CW input. It may be prevented by an admixture of Fe, Ti or Cr. Using a small admixture ( 10^–3 wt.%) of Ti or Cr the energy transfer among Nd ions and the gain coefficient may be increased. Cr in a higher concentration absorbs the pumping light and serves as earlier described coactivator (sensitizer) only. Fe impurity fully prevents any increase of the gain of YAG: Nd containing Ti or Cr and causes slow but irreversible degradation of the active parameters. Ce favourably modifies properties of YAG: Nd, Cr. YAG: Nd, Cr, Ce free of iron impurity is advisable active material for powerfull CW lasers.     

Luminescence properties of highly Cr co-doped Nd:YAG powder produced by sol-gel method

We examined luminescence properties of highly chromium co-doped Nd:YAG powders fabricated by the sol-gel method. Though the maximum luminescence intensity of Cr:YAG was at 3.0 mol% of Cr³⁺ concentration, we found that the enhancement effect on Nd:YAG by co-doping Cr³⁺ was continued until 6.0 mol% of Cr³⁺ concentration. This phenomenon is well-explained by a simple energy transfer model derived from the rate equations between Cr³⁺ and Nd³⁺. The enhancement of sensitization for Nd³⁺ activator by high co-doped Cr³⁺ is very effective for making a miniaturized or thin film-type solar laser.     

Compact low threshold Cr:YAG passively Q-switched intracavity optical parametric oscillator

We report a compact KTP-based intracavity optical parametric oscillator (IOPO) driven by a diode-end-pumped passively Q-switched Nd:YVO₄/Cr:YAG laser. For the first time, we take the thermal lens effect of the Cr:YAG into consideration and discuss its impact on the signal output. Diode pump threshold as low as 0.52 W has been achieved, which is the lowest result reported to date. At the incident diode pump power of 4 W, we obtained the maximum signal average and peak power of 358 mW and 12.5 kW, respectively, corresponding to a diode-to-signal conversion efficiency of 9%. Moreover, cavity-dumping characteristic and pulse transforming process from 1064 to 1573 nm are qualitatively analyzed.     

Side-pumped continuous-wave Cr:Nd:YAG ceramic solar laser

To clarify the advantages of Cr:Nd:YAG ceramics rods in solar-pumped lasers, a fused silica light guide with rectangular cross-section is coupled to a compound V-shaped cavity within which a 7 mm diameter 0.1 at.% Cr:1.0 at.% Nd:YAG ceramic rod is uniformly pumped. The highly concentrated solar radiation at the focal spot of a 2 m diameter stationary parabolic mirror is transformed into a uniform pump radiation by the light guide. Efficient pump light absorption is achieved by pumping uniformly the ceramic rod within the V-shaped cavity. Optimum pumping parameters and solar laser output powers are found through ZEMAX^© non-sequential ray-tracing and LASCAD^© laser cavity analysis codes. 33.6 W continuous-wave laser power is measured, corresponding to 1.32 times enhancement over our previous results with a 4 mm diameter Nd:YAG single-crystal rod. High slope efficiency of 2.6 % is also registered. The solar laser output performances of both the ceramic and the single-crystal rods are finally compared, revealing the relative advantage of the Cr:Nd:YAG rod in conversion efficiency. Low scattering coefficient of 0.0018 cm^?1 is deduced for the ceramic rod. Heat load is considered as a key factor affecting the ceramic laser output performance.     

108 W Nd: YAG ceramic laser with birefringence compensation resonator

The quartz rotator's effective birefringence compensation for ceramic Nd:YAG rods has been first demonstrated. Furthermore, a high output power continuous-wave laser is presented based on an optimized resonator made up of four Nd:YAG ceramic rods. By an appropriate design of the resonator, an output power of 108 W at 1064 nm is obtained. The corresponding optical-to-optical conversion efficiency is 16.8% and the slope efficiency is 28.1%. Meanwhile, the numerical analysis for output power is detailed.     

Direct numerical simulation of quasi-three-level passive Q-switched laser

The Runge-Kutta method is used to solve numerically the rate equations of quasi-three-level passive Q-switched laser directly without any approximate treatment of these differential equations. The 946 nm self-Q-switched Cr,Nd:YAG laser is chosen for example to describe the details. The time-dependence of intra-cavity photon density is obtained and its detailed real-time changing process is reproduced in numerical solution. The curves of laser output parameters such as average output power, pulse width, repetition rate, pulse energy and peak power changing with different cavity conditions such as pump power, output coupler reflectivity, Cr,Nd:YAG crystal length, Nd³⁺ ion and Cr⁴⁺ ion concentrations are simulated according to direct numerical solution rather than analytical expressions. This direct numerical simulation method can be widely used to describe and optimize the quasi-three-level passive Q-switched laser theoretically.     

Nd:YAG split-disk laser amplifier for 10 J output energy

A prototype split-disk amplifier consisted of four Nd:YAG ceramics and single crystals was demonstrated with a 3.7 cm square clear aperture. A single-pass small-signal gain of 2.0 and a total stored energy of 11.1 J in the eight YAG disks were obtained. The maximum output energy of 10.4 J with the YAG disk amplifier was achieved in a single-shot operation. A near-field pattern of 31 mm × 31 mm square with super Gaussian shape was measured.