Lifetime vibrational interference during the NO 1s-1π* resonant excitation studied by the NO+(A 1Π → X 1Σ+) fluorescence

Dispersed fluorescence from fragments formed after the de-excitation of the 1s^-1π^* resonances of N^*O and NO^* has been measured in the spectral range of 118–142 nm. This range is dominated by lines of atomic nitrogen and oxygen fragments and by the bands in the NO⁺ ion which result from the participator Auger decay of the 1s^-1π^* resonances. Ab-initio calculations of the transition probabilities between vibrational levels during the reaction NO N^*O ⇒ NO were used to explain the observed intensity dependence for the fluorescence bands on the exciting-photon energy across the resonances and on both v^′ and v^′′ vibrational quantum numbers. The multiplet structure of the 1s^-1π^* resonance and lifetime vibrational interference explain the observed exciting-photon energy dependence of the fluorescence intensity. A strong spin-orbit coupling between singlet and triplet states of NO⁺ is proposed to reduce additional cascade population of the state via radiative transitions from the and states and to explain remaining differences between measured and calculated integral fluorescence intensities.     

Fine structure levels of Cl V and their lifetimes

We report a large scale configuration interaction calculation of Cl V by taking account of relativistic effect through the Breit-Pauli approximation. Excitation energies of the lowest 49 fine structure levels relative to the ground state are found to be in good agreement with the NIST recommended data. Oscillator strengths, line strengths and radiative rates for the optically allowed and intercombination transitions among these levels and life times for some relatively longer lived fine structure levels are also reported for this ion. We confirm the interesting result that the life times for the multiplets of and are of the order of microseconds.Received: 28 May 2003, Published online: 12 August 2003PACS: 32.10.Fn Fine and hyperfine structure - 32.70.Cs Oscillator strengths, lifetimes, transition moments - 95.30.Ky Atomic and molecular data, spectra, and spectral parameters (opacities, rotation constants, line identification, oscillator strengths, gf values, transition probabilities, etc.)     

Hyperfine quenching of the 4s4p <Superscript>3</Superscript>P<Subscript>0</Subscript> level in Zn-like ions

In this paper, we used the multiconfiguration Dirac-Fock method to compute with high precision the influence of the hyperfine interaction on the [Ar] P₀ level lifetime in Zn-like ions for stable and some quasi-stable isotopes of nonzero nuclear spin between Z=30 and Z=92. The influence of this interaction on the [Ar] P P₀ separation energy is also calculated for the same ions.     

New experimental limits on violations of the Pauli exclusion principle obtained with the Borexino Counting Test Facility

The Pauli exclusion principle (PEP) has been tested for nucleons (n,p) in and nuclei, using the results of background measurements with the prototype of the Borexino detector, the Counting Test Facility (CTF). The approach consisted of a search for , n, p and/or s emitted in a non-Paulian transition of 1P- shell nucleons to the filled 1S _1/2 shell in nuclei. Similarly, the Pauli-forbidden decay processes were searched for. Due to the extremely low background and the large mass (4.2 tons) of the CTF detector, the following most stringent up-to-date experimental bounds on PEP violating transitions of nucleons have been established: , , , , and , all at C.L.Received: 18 June 2004, Published online: 1 October 2004PACS: 11.30.-j, 24.80. + y, 23.20.-g, 27.20. + nG. Bellini: SpokesmanL. Cadonati: Now at Massachusetts Institute of Technology, NW17-161, 175 Albany St. Cambridge, MA 02139O. Dadoun: Marie Curie fellowship at LNGS Correspondence to: A. Derbin. On leave of absence from St. Petersburg Nuclear Physics Inst. - Gatchina, RussiaM. Deutsch: DeceasedR. Ford: No w at Sudbury Neutrino Observatory, INCO Creighton Mine, P.O.Box 159 Lively, Ontario, Canada, P3Y 1M3B. Freudiger: Marie Curie fellowship at LNGS. Now at Institute for Nuclear Physics, Forschungszentrum Karlsruhe, Postfach 3640, 76021 KarlsruheS. Gazzana: GLIMOSV.V. Kobychev: Now at Institute for Nuclear Research, Prospekt Nauki 47, MSP 03680, Kiev, UkraineG. Korga: On leave of absence from KFKI-RMKI, Konkoly Thege ut 29-33 H-1121 Budapest, HungaryC. Lendvai: Marie Curie fellowship at LNGSP. Lombardi: Detector installation managerA. Martemianov: DeceasedV. Muratova: On leave of absence from St. Petersburg Nuclear Physics Inst. - Gatchina, RussiaL. Niedermeier: Marie Curie fellowship at LNGSL. Papp: On leave of absence from KFKI-RMKI, Konkoly Thege ut 29-33 H-1121 Budapest, HungaryR.S. Raghavan: Present Address: Department of Physics, Virginia Polytechnic Institute and State University, Blacksburg VA 24061G. Ranucci: Project managerC. Salvo: Operational manager Correspondence to: O. SmirnovA. Sonnenschein: Center for Cosmological Physics, University of Chicago, 933 E.56^th St., Chicago, IL 60637     

Hyperfine structure and isotope shift study in singly ionized lead

Hyperfine structure and isotope shifts in five optical transitions: 424.5 nm ( – ), 537.2 nm ( – ), 554.5 nm ( – ), 560.9 nm ( – ) and 666.0 nm ( – ) of Pb  II have been measured. As a light source the discharge tube was used. The hyperfine structure measurements were performed using metallic isotope ²⁰⁷Pb. For isotope shifts measurements natural lead was used. The high resolution spectral apparatus consisted of a silver coated Fabry-Perot etalon and a grating spectrograph combined with a CCD camera used as a detector. In the analysis of the spectra a computer simulation technique was used. The hyperfine structure observations yielded the splitting constants A for seven levels of Pb II. The isotope shift studies enabled to separate the mass and the field shifts and to determine values of changes of the mean square nuclear charge radii.     

Flavour-independent h<Superscript>0</Superscript>A<Superscript>0</Superscript> search and two Higgs doublet model interpretation of neutral Higgs boson searches at LEP

Upper limits on the cross-section of the pair-production process , assuming 100 branching fraction to hadrons, are derived from a new search for the hadrons final state, independently of the hadronic flavour of the decay products. This study, combined with previously published searches for the neutral Higgs bosons h⁰ and A⁰, is used to constrain the Type II Two Higgs Doublet Model (2HDM(II)) with no CP violation in the Higgs sector and no additional non-Standard Model particles besides the five Higgs bosons. The analysis combines LEP1 and LEP2 data collected with the OPAL detector up to the highest available centre-of-mass energies. The searches are sensitive to the and decay modes of the Higgs bosons. A benchmark scan of the 2HDM(II) parameter space is performed. Large regions of the 2HDM(II) parameter space explored are excluded at the 95% CL in the ( and planes, using both direct neutral Higgs boson searches and indirect limits derived from Standard Model high precision measurements. The region GeV and GeV is excluded at 95 % CL, independently of and for selected values of which are representative of a complete -scan.Received: 28 July 2004, Revised: 4 January 2005, Published online: 3 March 2005     

Updated estimate of the muon magnetic momentusing revised results from <Emphasis Type="Italic">e</Emphasis><Superscript> + </Superscript><Emphasis Type="Italic">e</Emphasis><Superscript>-</Superscript>annihilation

A new evaluation of the hadronic vacuum polarization contribution to the muon magnetic moment is presented. We take into account the reanalysis of the low-energy e ⁺ e ^-annihilation cross section into hadrons by the CMD-2 Collaboration. The agreement between e ⁺ e ^-and spectral functions in the channel is found to be much improved. Nevertheless, significant discrepancies remain in the center-of-mass energy range between 0.85 and , so that we refrain from averaging the two data sets. The values found for the lowest-order hadronic vacuum polarization contributions are where the errors have been separated according to their sources: experimental, missing radiative corrections in e ⁺ e ^-data, and isospin breaking. The corresponding Standard Model predictions for the muon magnetic anomaly read where the errors account for the hadronic, light-by-light (LBL) scattering and electroweak contributions. The deviations from the measurement at BNL are found to be (1.9 ) and (0.7 ) for the e ⁺ e ^-- and -based estimates, respectively, where the second error is from the LBL contribution and the third one from the BNL measurement.Received: 7 September 2003, Published online: 30 October 2003     

Decay of metastable states in Nd II

The difficulty associated with an accurate determination of transition rates for forbidden lines in lowly ionized heavy elements is illustrated in the case of Nd II. We have investigated the radiative decay of the low-lying metastable levels in Nd⁺ including the two levels K_11/2 and I_13/2. In these two particular cases, using different theoretical approaches, we find that the decay is dominated by the M1 channels but that the E2 contributions are of the same order of magnitude. These levels have also been studied experimentally by lifetime measurements with the heavy ion storage ring CRYRING of Stockholm University. The difficulties encountered when performing such experiments are underlined and discussed.     

A precise measurement of the tau lifetime

The tau lepton lifetime has been measured with the events collected by the DELPHI detector at LEP in the years 1991-1995. Three different methods have been exploited, using both one-prong and three-prong decay channels. Two measurements have been made using events in which both taus decay to a single charged particle. Combining these measurements gave . A third measurement using taus which decayed to three charged particles yielded These were combined with previous DELPHI results to measure the tau lifetime, using the full LEP1 data sample, to be .Received: 12 November 2003, Revised: 1 June 2004, Published online: 20 July 2004     

Multijet production in neutral current deep inelastic scattering at HERA and determination of $\alpha_s$

Multijet production rates in neutral current deep inelastic scattering have been measured in the range of exchanged boson virtualities . The data were taken at the ep collider HERA with centre-of-mass energy using the ZEUS detector and correspond to an integrated luminosity of . Jets were identified in the Breit frame using the k_T cluster algorithm in the longitudinally invariant inclusive mode. Measurements of differential dijet and trijet cross sections are presented as functions of jet transverse energy ( ), pseudorapidity ( ) and Q² with and . Next-to-leading-order QCD calculations describe the data well. The value of the strong coupling constant , determined from the ratio of the trijet to dijet cross sections, is . Received: 1 April 2005, Revised: 28 June 2005, Published online: 30 August 2005     

Decelerated molecular beams for high-resolution spectroscopy

Ultimately, the resolution of any spectroscopic experiment is limited by the interaction time between the particles that are to be examined and the measuring device. The obtainable spectroscopic resolution in a molecular beam experiment can be considerably improved using samples of slow molecules, as produced, for example, in a Stark-decelerator. This is demonstrated here by measuring the inversion tunneling spectrum of using a pulsed molecular beam that has been decelerated to about 52 m/s. Hyperfine resolved inversion transitions in in the state (around 1.43 GHz) are induced in a microwave region, and molecules that have undergone the transition are subsequently detected using a UV-laser based ionization detection scheme. To increase the signal intensity, the decelerated molecular beam is both transversally and longitudinally focused into the laser detection region. The observed spectral width of individual hyperfine transitions in the fully resolved spectrum is about 1 kHz, and the standard deviation of the best fit is 62 Hz.Received: 7 September 2004, Published online: 23 November 2004PACS: 33.15.Pw Fine and hyperfine structure - 33.20.Bx Radio-frequency and microwave spectra - 33.40. + f Multiple resonances - 33.70.Jg Line and band widths, shapes, and shifts - 39.10. + j Atomic and molecular beam sources and techniques     

Search for chargino and neutralino productionat $\sqrt{s} = 192$-209 GeV at LEP

Approximately 438 pb^-1 of e ⁺ e^- data from the OPAL detector, taken with the LEP collider running at centre-of-mass energies of 192-209 GeV, are analyzed to search for evidence of chargino pair production, , or neutralino associated production, . Limits are set at the 95% confidence level on the product of the cross-section for the process and its branching ratios to topologies containing jets and missing energy, or jets with a lepton and missing energy, and on the product of the cross-section for and its branching ratio to jets. R-parity conservation is assumed throughout this paper. When these results are interpreted in the context of the Constrained Minimal Supersymmetric Standard Model, limits are also set on the masses of the and , and regions of the parameter space of the model are ruled out. Nearly model-independent limits are also set at the 95% confidence level on with the assumption that each chargino decays via a W boson, and on with the assumed to decay via a Z⁰.Received: 15 December 2003, Revised: 16 February 2004, Published online: 23 April 2004     

Measurement of charm fragmentation ratios and fractionsin photoproduction at HERA

The production of , D⁰, D ⁺ , D_s ⁺ and charm hadrons and their antiparticles in e p scattering at HERA was measured with the ZEUS detector using an integrated luminosity of . The measurement has been performed in the photoproduction regime with the exchanged-photon virtuality and for photon-proton centre-of-mass energies in the range . The charm hadrons were reconstructed in the range of transverse momentum and pseudorapidity . The production cross sections were used to determine the ratio of neutral and charged D-meson production rates, , the strangeness-suppression factor, , and the fraction of charged D mesons produced in a vector state, . The measured and values agree with those obtained in deep inelastic scattering and in e ⁺ e^- annihilations. The measured value is smaller than, but consistent with, the previous measurements. The fractions of c quarks hadronising as a particular charm hadron, , were derived in the given kinematic range. The measured open-charm fragmentation fractions are consistent with previous results, although the measured is smaller and is larger than those obtained in e ⁺ e^- annihilations. These results generally support the hypothesis that fragmentation proceeds independently of the hard sub-process. Received: 12 August 2005, Revised: 8 September 2005, Published online: 6 October 2005     

Two-step laser optogalvanic spectroscopy of the odd-parity Rydberg states of atomic mercury

We present new experimental data on the highly excited levels in mercury using the two-step laser excitation and optogalvanic detection technique in conjunction with a RF discharge cell. The 6s7s ³S₁ intermediate level has been accessed from the 6s6p ³P₂ metastable level that is collisionally populated in the mercury discharge in the presence of a buffer gas at a pressure of about 1 Torr. Two beams fromtwo different dye lasers pumped with a common excimer laser were passed through the discharge cell containing mercury vapors. The first laser was tuned to 6s7s ³S₁ level whereas the second laser was scanned covering the wavelength region between 544-458 nm. We have observed the 6snp ³P₀ ( ), 6snp ( ), 6snp ( ) and 6snp ) Rydberg series. The 6snp Rydberg series to such high n-value has been reported for the first time. The first ionization potential of mercury is determined from the 6snp Rydberg series as 84184.15 0.05 cm^-1. Some collisionally induced parity forbidden transitions have also been located that are identified as 6sns ( ) series.Received: 5 November 2003, Published online: 20 January 2004PACS: 31.50.-x Potential energy surfaces - 32.30.Jc Visible and ultraviolet spectra - 32.80.Rm Multiphoton ionization and excitation to highly excited states (e.g., Rydberg states)     

Search for anomalous weak dipole moments of the $\tau$ lepton

The anomalous weak dipole moments of the lepton are measured in a data sample collected by ALEPH from 1990 to 1995 corresponding to an integrated luminosity of 155 pb^-1. Tau leptons produced in the reaction at energies close to the mass are studied using their semileptonic decays to , , or . The real and imaginary components of both the anomalous weak magnetic dipole moment and the CP-violating anomalous weak electric dipole moment, , , and , are measured simultaneously by means of a likelihood fit built from the full differential cross section. No evidence of new physics is found. The following bounds are obtained (95% CL): , , , and .Received: 25 September 2002, Published online: 29 August 2003     

$ {\rm{V}}_2 {\rm{O}}_5^ + $ {\rm{V}}_2 {\rm{O}}_5^ + " border="0"> reaction with C2H4: theoretical considerations of experimental findings

Density functional calculations have been performed for the reactions towards ethylene considering atomic and molecular oxygen loss, oxygen transfer and association reactions. The oxygen transfer channel to ethylene is energetically favourable in contrast to the oxygen loss. This is in agreement with the experimental results [1] which show that does not lose atomic oxygen during the collision induced dissociation at thermal energies. A radical cation mechanism based on structure-reactivity relation of cluster is proposed to explain oxygen transfer channel indicating that this reaction is size selective.     

Di-jet production in photon-photon collisionsat $\sqrt{s_{\protect\bf\mathrm{ee}}}$ from 189 to 209 GeV

Di-jet production is studied in collisions of quasi-real photons at e ⁺ e^- centre-of-mass energies from 189 to 209 GeV at LEP. The data were collected with the OPAL detector. Jets are reconstructed using an inclusive -clustering algorithm for all cross-section measurements presented. A cone jet algorithm is used in addition to study the different structure of the jets resulting from either of the algorithms. The inclusive di-jet cross-section is measured as a function of the mean transverse energy of the two leading jets, and as a function of the estimated fraction of the photon momentum carried by the parton entering the hard sub-process, , for different regions of . Angular distributions in di-jet events are measured and used to demonstrate the dominance of quark and gluon initiated processes in different regions of phase space. Furthermore the inclusive di-jet cross-section as a function of and is presented, where is the jet pseudo-rapidity. Different regions of the - -space are explored to study and control the influence of an underlying event. The results are compared to next-to-leading order perturbative QCD calculations and to the predictions of the leading order Monte Carlo generator PYTHIA.Received: 20 December 2002, Published online: 17 October 2003     

Electron impact excitation of 2p and 3p states of hydrogen at intermediate energies

The recent theoretical work by Bartlett et al. [J. Phys. B 38, L95 (2005)] and the latest measurements on the reduced Stokes parameters , and for 54.4 eV electron impact excitation of the 2p state atomic hydrogen by Williams and Mikosza [J. Phys. B 39, 4113 (2006)] has motivated the present work. A coupled-channel-optical calculation with 9 and 12 atomic states supplemented with the continuum optical potentials for the stronger coupling channels has been performed. The calculated n = 2 and n = 3 differential cross sections and the reduced Stokes parameters are comparable with the state-of-the art calculations. There is closer agreement between the present calculations and the experimental measurements for the reduced Stokes parameters and in the n = 2p excitation at 54.4 eV. The present CCO calculations also display good accord with the limited experimental data for the reduced Stokes parameters in the n=3p excitation.     

Probing spin-orbit quenching in Cl (2P) + H2 via crossed molecular beam scattering

In our previous work we investigated electronically non-adiabatic effects in using crossed molecular beam scattering coupled with velocity mapped ion imaging. The prior experiments placed limits on the cross-section for electronically non-adiabatic spin-orbit excitation and electronically non-adiabatic spin-orbit quenching . In the present work, we investigate electronically non-adiabatic spin-orbit quenching for which is the required first step for the reaction of Cl^* to produce ground state HCl+H products. In these experiments we collide Cl (²P) with H₂ at a series of fixed collision energies using a crossed molecular beam machine with velocity mapped ion imaging detection. Through an analysis of our ion images, we determine the fraction of electronically adiabatic scattering in Cl^* +H₂, which allows us to place limits on the cross-section for electronically non-adiabatic scattering or quenching. We determine the following quenching cross-sections σ _quench(2.1 kcal/mol) = 26 ± 21 ?², σ _quench(4.0 kcal/mol) = 21 ± 49 ?², and σ _quench(5.6 kcal/mol) = 14 ± 41 ?².     

Studies of ion energy and yield from argon clusters heated by intense femtosecond laser pulses

Using time-of-flight spectrometry, the interaction of intense femtosecond laser pulses with argon clusters has been studied by measuring the energy and yield of emitted ions. With two different supersonic nozzles, the dependence of average ion energy on cluster size in a large range of has been measured. The experimental results indicate that when the cluster size , the average ion energy Coulomb explosion is the dominant expansion mechanism. Beyond this size, the average ion energy gets saturated gradually, the clusters exhibit a mixed Coulomb-hydrodynamic expansion behavior. We also find that with the increasing gas backing pressure, there is a maximum ion yield, the ion yield decreases as the gas backing pressure is further increased.