有限温度下二维Heisenberg铁磁系统的横向声频支声子激发

在二维正方Heisenberg铁磁系统的基础上建立了磁振子-声子相互作用模型.利用Matsubara格林函数理论研究了系统的横向声频支声子激发，计算了布里渊区的主要对称点线上的横向声频支声子色散曲线，发现在第一布里渊区的Σ线上，小波矢区(Γ附近k_xa＜0.2)横向声频支声子有硬化现象，但是在软化区(0.25＜k_xa＜0.7)有横向声频支声子有软化现象，在M附近(0.75＜k_xa)横向声频支声子有硬化现象.在Δ线上没有发生横向声频支声子有软化与硬化现象.在Z线上小波失区(X附近k_xa＜0.65)横向声频支声子有软化现象，但是在M附近横向声频支声子有硬化现象.并且又讨论了各项参数对横向声频支声子激发的影响，发现磁振子-声子耦合与自旋波劲度常数对横向声频支声子软化起很大的作用. 关键词： 磁振子-声子相互作用 横向声频支声子软化 Matsubara格林函数理论 铁磁系统     

有限温度下二维Heisenberg铁磁系统的声子衰减

在二维正方Heisenberg铁磁系统的基础上建立了磁振子-声子相互作用模型. 利用松原格林函数理论研究了系统的声子衰减，计算了布里渊区的主要对称点线上的声子衰减曲线. 发现在第一布里渊区，在Δ线上，横向声频支声子无衰减，在Z线上，纵向声频支声子无衰减；横向声频支声子衰减比纵向声频支声子衰减至少大一个数量级，并讨论了各项参数的变化对横向声频支声子衰减与纵向声频支声子衰减的影响. 根据声子衰减与声子寿命的关系，声子衰减与声子态密度的关系，可以讨论横向声频支声子与纵向声频支声子的寿命与态密度. 关键词： 磁振子-声子相互作用 横向声频支声子衰减 纵向声频支声子衰减 声子寿命     

Effect of magnon-phonon interaction on phonon damping of two-dimensional Heisenberg ferromagnetic system at finite temperature

A magnon-phonon interaction model is developed on the basis of a two-dimensional square Heisenberg ferromagnetic system. By using Matsubara Green function theory we studied the transverse and longitudinal acoustic phonon dampings and calculated the transverse and longitudinal acoustic phonon damping curves on the main symmetric point and line in the first Brillouin zone. It is found that on the line Δ there is no damping for transverse acoustic phonon and on the line Z there is no damping for longitudinal acoustic phonon. In the first Brillouin zone the damping of transverse acoustic phonons is at least one order larger than that of longitudinal acoustic phonons. The influences of various parameters on transverse and longitudinal acoustic phonon dampings are discussed and the lifetime and the density of state of transverse and longitudinal acoustic phonons are explored as well according to the relation of the phonon damping and its lifetime and the relation of the phonon damping and its density of state.     

高压下有序晶态合金Fe3Pt的低能声子不稳定性及磁性反常

有序晶态Fe₃Pt因瓦合金处于一种特殊的磁临界状态, 这种磁临界状态下体系的晶格动力学稳定性对压力极为敏感. 基于密度泛函理论的第一性原理的投影缀加平面波方法研究了不同晶态合金的Fe₃Pt的焓和磁性随压力的变化规律, 结果表明, 在压力小于18.54 GPa下, P4/mbm结构是热力学稳定的相. Pm3m结构、I4/mmm结构、DO₂₂结构的Fe₃Pt在铁磁性坍塌临界压力附近体系的总磁矩急剧下降并具有振荡现象, 且I4/mmm结构和DO₂₂结构的Fe₃Pt 在临界压力附近出现了Fe1原子磁矩反转现象. 在43 GPa下, DO₂₂结构的Fe₃Pt出现了亚铁磁微观磁特性突然增强且伴随着体积突然增大的现象. 在高压下, 对Pm3m结构Fe₃Pt的晶格动力学计算表明, 压力小于26.95 GPa的铁磁态下体系的自发磁化诱导了体系横向声学支声子软化, 表明体系中存在很强的自发体积磁致伸缩. 特别是在铁磁性坍塌临界压力41.9 GPa至磁性完全消失的57.25 GPa压力区间, 晶格动力学稳定性对压力更加敏感. 压力大于57.25 GPa时, 压力诱导了体系声子谱的稳定.     

光频支声子对二维Heisenberg铁磁系统磁激发的影响

在二维复式正方Heisenberg铁磁系统的基础上建立了磁振子-声子相互作用模型. 利用松原格林函数理论研究了系统的磁激发，计算了布里渊区的主要对称点线上的磁振子色散曲线，比较了光频支声子与声频支声子对系统磁激发的影响以及各项参数的变化对磁振子软化的影响. 发现光频支声子-磁振子耦合对磁振子软化起主要作用，尤其是纵向光频支声子对磁振子软化起更大的作用，并且非磁性离子的光频支声子对磁振子软化的作用比磁性离子的光频支声子对磁振子软化的作用更显著.     

Softening behavior of acoustic phonon mode in ZnO nanoparticles: the effect of impurities and particle size variation with temperature

Decay dynamics of the acoustic phonon mode in ZnO nanoparticles, synthesized using the wet chemical technique, is investigated. It is well established that optic phonon modes in a semiconductor favor an anharmonic decay dynamics; in contrast, acoustic modes evidence a rather complex decay behavior, manifesting their dependence on other parameters such as particle size, impurity species, etc. At lower temperatures (T < 500 K), the anharmonic decay process, caused by the weakening of the bond strength, is responsible for the observed decrease in the acoustic mode wavenumbers. However, particle growth due to the coalescence sintering process is prominent at higher temperatures (>600 K) and governs the softening behavior of the acoustic phonon mode towards the Rayleigh line. On the other hand, the precursor species and reaction byproducts on the surface of ZnO nanoparticles induce an anomalous softening behavior in the decay dynamics at specific temperatures by damping the acoustic phonon mode. Copyright © 2011 John Wiley & Sons, Ltd.     

金刚石氮-空位色心的原子自旋声子耦合机理

金刚石氮-空位色心结构因在量子精密测量领域的高灵敏度优势而备受关注.本文引入耦合声子场对氮-空位色心原子自旋进行共振调控,以提高氮-空位色心的自旋跃迁效率.首先,基于波函数和晶格的点阵位移矢量关系,分析了声子与晶格能量交互作用,研究了基于声子共振调控的氮-空位色心的自旋跃迁机理,建立了基于应变诱导的能量转移声子-自旋交互耦合激发模型.其次,基于氮-空位色心晶格振动理论,引入满足布洛赫定理的系数矩阵,建立了不同轴向氮-空位色心第一布里渊区特征区域的声子谱模型.同时,基于德拜模型,考虑热膨胀效应,解析该声子共振系统的声子热平衡性质,并对其比热模型进行研究.最后,基于分子动力学仿真软件CASTEP和密度泛函理论进行第一性原理研究,构建了声子模式下不同轴向氮-空位色心的结构优化模型,并分析了其结构特性、声子特性和热力学特性.研究结果表明,系统声子模式的演化依赖于氮-空位的占位,声子模式强化伴随着热力学熵的降低.含氮-空位色心金刚石的共价键较纯净无缺陷金刚石更弱,热力学性质更不稳定.含氮-空位色心金刚石的声子主共振频段处于THz量级,次共振频率约为[800,1200]MHz.根据次共振频段设计叉指宽度为1.5μm的声表面波共振机构,其中心频率约为930 MHz.在该声子共振调控参数条件下,声子共振调控方法可有效增大氮-空位色心的自旋跃迁概率,实现氮-空位色心原子自旋操控效率的提高.     

Far-infrared laser spectroscopy of phonon difference band absorption in TlCl

Far-infrared laser radiation is used to study the lattice absorption of a TlCl crystal over a large temperature range. We found a strong absorption band caused by phonon difference processes where longitudinal and transverse acoustic phonons with wave vectors at the Brillouin zone boundary are involved.     

Phonon dispersion on Ag(100) surface:A modified analytic embedded atom method study

Within the harmonic approximation, the analytic expression of the dynamical matrix is derived based on the modified analytic embedded atom method(MAEAM) and the dynamics theory of surface lattice. The surface phonon dispersions along three major symmetry directionsΓˉXˉ, Γˉ Mˉ, and Xˉ Mˉ are calculated for the clean Ag(100) surface by using our derived formulas. We then discuss the polarization and localization of surface modes at points Xˉ and Mˉ by plotting the squared polarization vectors as a function of the layer index. The phonon frequencies of the surface modes calculated by MAEAM are compared with the available experimental and other theoretical data. It is found that the present results are generally in agreement with the referenced experimental or theoretical results, with a maximum deviation of 10.4%. The agreement shows that the modified analytic embedded atom method is a reasonable many-body potential model to quickly describe the surface lattice vibration. It also lays a significant foundation for studying the surface lattice vibration in other metals.     

高压下γ'-Fe4N晶态合金的声子稳定性与磁性

利用基于密度泛函理论的第一性原理研究了高压下有序晶态γ’-Fe₄N合金的晶格动力学稳定性与磁性. 对比没有考虑磁性的γ’-Fe₄N的声子谱, 得出压力小于1 GPa时, 自发磁化诱导了铁磁相γ’-Fe₄N基态晶格动力学稳定. 压力在1.03-31.5 GPa时, Σ线上的点(0.37, 0.37, 0)、对称点X和M 上相继出现了声子谱软化现象. 压力在31.5-60.8 GPa时, 压致效应与自发磁化对诸原子的作用达到了稳定平衡, 表现出了声子谱稳定. 压力大于61.3 GPa时, 随着压力的增大压力诱导体系动力学不稳定性越强. 通过软模相变理论对于γ’-Fe₄N, 在10 GPa下的声学支声子的M点处软化现象的处理, 发现了动力学稳定的高压新相P2/m-Fe₄N. 压力小于1 GPa时高压新相P2/m-Fe₄N 是热力学稳定的相, 且磁矩与γ’-Fe₄N的磁矩几乎相同. 2.9-19 GPa时, P2/m相的焓比γ’相的焓小, 基态结构更稳定. 大于20 GPa时, 两相磁矩几乎相同.     

Fermi-Pasta-Ulam β 格点链系统能量载流子研究

Fermi-Pasta-Ulam (FPU) β格点链中能量输运的载流子是孤子还是声子一直存在较多的争议. 本文通过单脉冲方法, 明确了一个能量波包在该格点链系统中从声子波包转变成为孤子波包的条件, 即波包能量达到一定阈值. 基于纯四次势链的声子真空效应, 构造了由FPU-β链与纯四次势链构成的双段链系统. 通过对比研究双段链系统和单段FPU-β链中的热流, 发现低温下声子是FPU-β链中能量的主要载流子, 而随着温度的升高孤子逐步取代声子成为能量的主要载流子. 关键词： Fermi-Pasta-Ulam格点链 声子 孤子 热传导     

Anomalous phonon wind effect on the lateral exciton migration in ultrathin quantum well CdTe/ZnTe

The effect of nonequilibrium acoustic phonon flux on the photoluminescence of an ultrathin quantum well CdTe/ZnTe upon its quasi-resonant excitation by a He-Ne laser was studied. It is found that the phonon flux generated by an external source affects the quantum well luminescence bandshape even at small lasing power and large (up to 1 cm) distance between the phonon generation zone and the quasi-resonant luminescence excitation zone. It is assumed that the phonon flux stimulates exciton in-plane (lateral) migration in the quantum well through the tunneling between the local potential minima accompanied by induced phonon emission.     

Effects of contact shape on ballistic phonon transport in semiconductor nanowires

We study the effects of contact shape on ballistic phonon transport in semiconductor nanowires at low temperatures using an approximative scalar model of continuum elasticity. Five different contacts connected to two semiconductor nanowires with different transverse widths are discussed. Numerical results show that the contact shape acts as an ‘acoustic impedance adaptor’, playing a crucial role on the ballistic phonon transmission and thermal conductance. The phonon coupling in the contacts with certain length facilitates ballistic phonon transmission compared to the abrupt interface, in which the phonon scattering is the strongest. It is found that the more the contact is abrupt, the smaller the thermal conductance is. The catenoidal contact rather than the abrupt interface is also the competitive candidate to obtain bigger thermal conductance. These results indicate that choosing an appropriate contact shape is one of the most critical factors to accurately measure the thermal conductance with a very high precision and reliability in different temperature ranges at low temperatures.     

A method to calculate the thermal conductivity of HMX under high pressure

A method based on Debye theory is developed to calculate the thermal conductivity of octahydro-1,3,5,7-tetranitro-1,3,5,7-tetrazocine (HMX). The phonon–phonon interaction model is built up for solid HMX. The phonon lifetime formula is derived by the phonon–phonon scattering mechanism, and the thermal conductivity tensor is derived by the phonon dispersion model. The thermal conductivities of α/β/δ-HMX are calculated in the temperature range 0–700?K and pressure range of 0–10?GPa. The phonon softening process of HMX is investigated. We have proven that the Debye frequency and thermal conductivity tend to 0 at the phonon softening point. A physical picture of the phonon–phonon interaction, phonon lifetime and phonon softening is built up.     

含半圆弧形腔的量子波导中声学声子输运和热导特性

采用散射矩阵方法,研究了在应力自由和硬壁两种典型的边界条件下含半圆弧形腔的量子波导中声学声子输运和热导性质.结果表明在两种边界条件下声子透射谱和热导有着不同的特征.在应力自由边界条件下,能观察到普适的量子化热导现象,当结构为一理想的量子线时,在低温区域有一个量子化平台出现,而当半圆弧形结构存在时,非均匀横向宽度引发的弹性散射使得量子化平台被破坏;在硬壁边界条件下,不可能观察到量子化热导现象,热导随温度的增加单调上升;计算结果表明还可以通过调节半圆弧形结构的半径来调控声子的输运概率和热导. 关键词： 声学声子输运 热导 量子体系     

Influence of atomic order on TA1[110] phonon softening [4] and displacive phase transition in Fe72Pt28 Invar alloys

The acoustic phonon dispersions of two Invar crystals , one ordered with the () structure, the other disordered fcc, have been investigated between 3.4 K and 470 K by inelastic and elastic neutron scattering. For the ordered crystal, pronounced softening of the whole phonon branch is observed on cooling below the Curie temperature. Particularly strong phonon softening at the M-point zone boundary of the structure leads to a displacive, antiferrodistortive phase transition at low temperatures. For the disordered crystal, much weaker softening of the phonons is observed and restricted to the region near the Brillouin zone center, where increasing elastic scattering with decreasing temperature indicates the growth of local tetragonal strain. This strain is considered as a typical precursor of the transformation to bct martensite. Specific heat measurements, performed at low temperatures on both crystals confirm the neutron scattering results and reveal considerable enhancement of the low energy phonon density of states in the ordered crystal. Received 18 January 1999     

Numerical studies on the boundary entanglement in an optomechanical phonon laser system

In our previous work (Meng et al 2020 Phys. Rev. A 101 023838), we discover the phenomenon that the quantum entanglement on the driving threshold line remains a constant in a three-mode optomechanical phonon laser system. In this paper, to find the conditions under which the constant boundary entanglement shows up, we explicitly study how this boundary entanglement depends on various parameters through numerical integrations. The results show that the necessary and sufficient condition is a resonant frequency match between the optical frequency difference and the mechanical vibrational frequency, and this constant value is proportional to the multiplication of the square of the optomechanical coupling strength and the resonant driving threshold power.     

二维圆盘颗粒体系声学行为的数值研究

数值测量了卸载过程中二维单分散圆盘颗粒系统的横波、纵波声速、声衰减系数、非线性系数随压强的变化以及声衰减系数随频率的变化.结果表明,二维(2D)圆盘颗粒体系的横波、纵波声速均随压强呈分段幂律标度:当压强P10~(-4)时,横波、纵波声速随压强的增大而减小;当P10~(-4)时,有v_t~P~(0.202),v_l~P~(0.338).进一步得到其剪切模量和体积模量的比值G/B也随压强呈幂律标度,G/B~P~(-0.502),暗示在低压强下,与三维(3D)球形颗粒体系类似,2D圆盘颗粒体系也处于L玻璃态.水平激励和垂直激励下2D圆盘颗粒系统的衰减系数随频率变化也呈现分段行为:当频率f0.05时,衰减系数不随f变化;当f0.05时,横波纵波的衰减系数α~f;当f0.35时,横波衰减系数α_T~f~2,纵波衰减系数α_L~f~(1.5).此外,竖直水平激励下的2D圆盘颗粒系统的非线性系数和衰减系数随压强也呈现与声速类似的分段规律:当P10~(-4)时,横波非线性系数β_T~P~(-0.230),其余都不随压强变化.当P10~(-4)时,两者均随压强增大呈幂律减小:β_T~P~(-0.703),β_L~P~(-0.684),α_T~P~(-0.099),α_L~P~(-0.105).进而得到2D圆盘颗粒系统中散射相关的特征长度?~*随压强呈幂律标度,当P10~(-4)时,?~*~P~(-0.595);当P10~(-4)时,?~*~P~(0.236).     

Coherent acoustic phonon oscillations in semiconductor multiple quantum wells with piezoelectric fields

Large coherent acoustic phonon oscillations were demonstrated using InGaN/GaN multiple quantum wells with piezoelectric fields. With UV femtosecond pulse excitation, photogenerated carriers screened the piezoelectric field and initiated the displacive coherent phonon oscillations. The specific phonon frequency was selected by the coupling between the periodic carrier distribution and the corresponding acoustic phonon mode. The induced acoustic phonon oscillation resulted in piezoelectric field modulation and then caused absorption variation through the quantum confined Franz-Keldysh effect. The wave vector uncertainty due to the finite sample width was found to determine the observed dephasing time.     

Raman phonon anomalies in Sr(Fe1-xCox)2As2

Phonon anomalies have been reported in iron-pnictide superconductors indicating a diverse interplay between different orders in the materials.Here,we report Raman scattering measurements on Sr(Fe_1-xCo_x)₂As₂(x=0 and x=0.04)single crystals in the B;symmetry with respect to a 1 Fe unit cell.Upon cooling,we observe a larger split(13 cm;)of Eg Raman phonon modes pertaining to in-plane Fe and As displacements as the crystals undergo the tetragonal-toorthorhombic structural phase transition,although a considerable split(9 cm;)has been reported in BaFe_1-xCo_x)₂As₂.Furthermore,the splitting of E;phonon modes is strongly reduced upon doping.We perform an order-parameter analysis revealing a similar doping dependence of E;phonon splitting as reported in other compounds of the 122 family,indicating these phonon anomalies widely exist in 122 iron-based superconductors and might share the same mechanisms.