Nuclear spins and magnetic moments of some neutron-deficient rubidium isotopes

The nuclear spins and magnetic moments of some neutron-deficient rubidium isotopes have been measured by atomic-beam magnetic resonance techniques at the ISOLDE facility, CERN. The following results have been obtained: ⁷⁷Rb, $\text{I =}\text{3}\text{2}\text{, μ}{}_{\mathrm{I}}\text{= 0.652(7)}\text{n.m.}$; ⁷⁸Rb, I = 0; ^78mRb,I = 4, μ_I = 2.56(3)(rmn.m.); $\text{(su79)}\text{Rb}\text{, I =}\text{5}\text{2}\text{, ifμ}{}_{\mathrm{I}}\text{= 3.364(4)}\text{n.m.}\text{,}\text{and}{}^{\mathrm{<mtext>84</mtext><mtext>m</mtext>}}\text{Rb}\text{, I = 6}$.The data on the The data on the light rubidium isotopes gives evidence for deformed nuclear shapes     

On spontaneous fission of neutron-deficient isotopes of elements 103, 105 and 107

Experiments are described on the determination of the spontaneous fission probability for the isotopes of elements 103, 105 and 107 produced by bombarding Tl, Pb and Bi targets with ⁵⁰Ti, ⁵¹V, ⁵⁴Cr, ⁵⁵Mn and ⁵⁸Fe ions. The upper limit of the spontaneous fission probability is established to be 2% for the isotopes ^{252, 253}103. A new isotope of element 105 with mass number $\text{257(T}{}_{\mathrm{<mtext>1</mtext><mtext>2</mtext>}}\text{= 5}\text{s}\text{)}$ has been produced. In bombardment of ²⁰⁹Bi with ⁵⁴Cr ions a new spontaneous fission activity with $\text{T}{}_{\mathrm{<mtext>1</mtext><mtext>2</mtext>}}\text{≈ 1–2}\text{ms}$ has been observed. The experimental data permit identification of this activity as the isotope of the new element 107 with mass number 261, which mainly undergoes α-decay (≈ 80%) resulting in the formation of the isotope ²⁵⁷105. The values of the partial α-decay and spontaneous fission half-lives of the isotopes ²⁵⁷105 and ²⁶¹107 are compared with the systematics of the properties of transfermium nuclei.     

Nuclear structure studies in the Te isotopes: The Te(d, p)Te reaction

The reaction ¹²⁵Te(d, p)¹²⁶Te has been studied at a bombarding energy of 7.5 MeV in order to get information about the ¹²⁶Te nuclear level scheme. Forty-two levels were observed below an excitation energy of 5.1 MeV. The angular distributions of 25 of the emitted proton groups were compared with DWBA calculations to determine the angular momentum of the captured neutrons. Contributions from more than one l_n value were observed for two of the transitions. Transition strengths were extracted and compared to pairing-theory calculations.     

Decoupled bands in odd-mass mercury isotopes

The schemes of the low-lying high-spin states in mercury isotopes with A = 195, 197, and 199 have been studied by γ-ray spectroscopy following (α, xn) reactions on separated platinum targets. Two bands have been excited in each Hg nucleus, one with positive parity based on the isomeric i$\text{13}\text{2}$. state and one, probably with negative parity, starting at spin $\text{case21}\text{2}$. The positive-parity states are interpreted with the rotation-aligned coupling scheme as decoupled bands; this implies oblate deformation in these three Hg isotopes. The negative-parity states are discussed as a decoupled i$\text{13}\text{2}$ neutron state coupled to the 5^?, 7^?, 9^?,…states, recently discovered in doubly even mercury isotopes.     

Collective bands in even mass Sn isotopes

Positive parity bands in ^{112, 114, 116, 118}Sn have been excited up to levels with spin and parity J^π = 12⁺ using Cd(α, 2nγ)Sn reactions. The experiments consisted of γ-ray excitation function, γ-γ coincidence, lifetime, γ-ray angular distribution, γ-ray linear polarization and conversion electron measurements. The observed bands show strong resemblances with ground-state bands of transitional nuclei in this mass region. It is pointed out that the J^π = 0⁺ band-heads originate from 2p-2h excitations in the Z = 50 proton shell. The excitation energies of the band-heads are calculated by means of the macroscopic-microscopic renormalization method. Pair correlations between the 2h and 2p configurations are included separately in a phenomenological way by taking into account the pairing energies of the Cd and Te ground states with respect to the Sn ground state.     

Alpha decay of neutron-deficient isotopes of tungsten

Three neutron-deficient isotopes of tungsten have been produced by the reactions of ²⁴Mg on targets of ¹⁴⁷Sm and ¹⁴⁴Sm. They are ¹⁶⁴W, E_α = 5.153 MeV, $\text{T}{}_{\mathrm{<mtext>1</mtext><mtext>2</mtext>}}\text{= 6.3 s}$; ¹⁶³W, E_α = 5.385 MeV, $\text{T}{}_{\mathrm{<mtext>1</mtext><mtext>2</mtext>}}\text{= 2.5}\text{s}$; and ¹⁶²W, E_α = 5.53 MeV, $\text{T}{}_{\mathrm{<mtext>1</mtext><mtext>2</mtext>}}\text{< 0.25}\text{s}$.     

Spectroscopy of 166W and 167W and alignment effects in very neutron-deficient tungsten nuclei

High-spin states in ¹⁶⁶W and ¹⁶⁷W were populated by the reactions ¹⁴²Nd(²⁸Si,4n)¹⁶⁶W, ¹⁴²Nd(²⁸Si,3n)¹⁶⁷W and ¹⁴⁷Sm(²⁴Mg,4n)¹⁶⁷W. From the γ-decay the yrast band and a side band (with assumed negative parity) were identified to high spins. There is evidence for a second side band in ¹⁶⁷W. The observed backbend of the yrast sequences and band-crossing anomalies in the side bands are discussed in conjunction with cranked-shell-model calculations. A systematic comparison is made between the yrast bands of ^166,167,168W in order to understand the structure of the second backbend in ¹⁶⁸W.     

Elastic neutron transfer in the scattering of Si isotopes

Angular distributions of the elastic scattering of ²⁸Si on ²⁹Si and ³⁰Si have been measured for incident beam energies at E = 65 and 70 MeV with a time-of-flight spectrometer for heavy ions. At 70 MeV the neutron transfer ³⁰Si(²⁸Si, ²⁹Si)²⁹Si was observed in addition to the elastic channel. The pronounced oscillations in the elastic scattering distributions are interpreted as being due to an elastic transfer of neutrons between the colliding nuclei during the scattering process. This assumption is in accordance with some general features of the data and allows for the extraction of spectroscopic factors of the transferred neutrons.     

(p,t) strengths in the Ga isotopes

The (p, t) reaction on the two stable Ga isotopes has been performed at 25 MeV, with 11 keV energy resolution. Levels up to 3.5 MeV in ⁶⁷Ga and 4.3 MeV in ⁶⁹Ga were measured. Differences observed between the distribution of the L = 2 (p, t) strength and the distribution of the B(E2)↑ strength may be explained by a mixed character of the $\text{7}\text{2}{}_2$^? level wave function. The distribution of the L = 0 strength indicates that the striking change in the ground-state structure shown between N = 40 and 42 already begins, although weakly, between N = 38 and 40.     

High-spin states in 24Mg and upper limits for particle spectroscopy of high spins by heavy-ion compound reactions

High-spin states in ²⁴Mg have been investigated by the reaction ¹⁰B(¹⁶O, d)²⁴Mg up to $\text{E}{}^1\text{≈ 24}\text{MeV}$. High-spin states with $\text{I ≧ 9}$ have been identified at $\text{E}{}^1\text{= 19.20, 20.26, 20.8, 21.6, 23.1,}\text{and}\text{23.5}\text{MeV}$. The 10⁺ yrast state in ²⁴Mg is probably located at 20.26 MeV. The upper limits with respect to spin and excitation energy of the applicability of heavy-ion compound reactions for particle spectroscopy of high-spin states are discussed. The main limitations result from the increasing continuum and from a decrease of the high-spin selectivity when the final spins approach the critical angular momentum for compound-nucleus formation. It will be shown that the difficulty in the analysis of the experiments arising from the decreasing probability of finding isolated yrast states at high excitation energies, i.e. from the increasing level density, can be overcome in such experiments. The decrease in the high-spin selectivity of the total cross section is compensated for spins up to J_max by the fact that the shape of the angular distributions depends on the final spin for states with I ～ J_max. This is caused by the decreasing alignment of the final nucleus with decreasing values of |I ? J_max| and can be used for high-spin spectroscopy.     

Nuclear moments of the neutron-deficient thallium isotopes

The nuclear moments of the neutron-deficient^187,188Tl isotopes were determined by measuring the hyperfine structure splittings of the λ=535 nm line in neutral thallium. An optical efficiency of 2×10⁻⁴ photons per radioactive ion was achieved using collinear fast beam laser spectroscopy with a large solid angle fiber optical array detector. Most of the moments can be interpreted fairly well in the single particle model.     

Single-particle states at very high spin in the light dysprosium isotopes

High-spin states in ^150–152Dy have been investigated. Gamma-gamma coincidences in all three isotopes have been studied with Compton-suppressed Ge(Li) detectors. For ¹⁵¹Dy, lifetimes of the high-spin states have been measured by the recoil-distance technique. The spin and parity assignments, transition rates, and level systematics support the interpretation of the observed states as proton particle-hole excitations coupled to aligned valence neutron configurations. Shell-model calculations, based on effective interactions and a ¹⁴⁶Gd core, quantitatively reproduce the observed level patterns, and the predicted transition rates qualitatively agree with the observed values.     

Nuclear reaction studies of 168Tm

The intrinsic structure of ¹⁶⁸Tm has been studied using the (³He, d) and (α, t) proton stripping reactions as well as the (d, t) and (³He, α) neutron pick-up reactions. The beams of 24 MeV ³He particles, 25 MeV α-particles and 12 MeV deuterons were obtained from the McMaster tandem Van de Graaff accelerator. The reaction products were analyzed with an Enge-type magnetic spectrograph and detected with photographic emulsions. The spectra have been interpreted in terms of the coupling of an odd proton and an odd neutron, each moving independently in a spheroidal potential, which gives rise to intrinsic two-quasiparticle states with $\text{K = ¦Ω}{}_1\text{±Ω}{}_2\text{¦}$. The identification of the intrinsic states was made by comparing the experimental cross-section patterns with those predicted with the aid of Coriolis coupling and distorted-wave Born approximation (DWBA) calculations. Rotational bands superimposed on the K^π = 3⁺ and $\text{K}{}^{\mathrm{\pi }}\text{= 4}{}^{\mathrm{+}}\text{, {}\text{7}\text{2}{}^{\mathrm{+}}\text{[633]}{}_{\mathrm{n}}\text{±}\text{1}\text{2}{}^{\mathrm{+}}\text{[411]}{}_{\mathrm{p}}\text{}}$ configurations, the first of which is the ground state, ha been observed in the spectra of all four reactions. New assignments have been made for configurations resulting from coupling the $\text{1}\text{2}$^? [541], $\text{7}\text{2}$⁺ [404], $\text{5}\text{4}$⁺ [402] and $\text{1}\text{2}$^? [530] p to the $\text{7}\text{2}$⁺ [633] neutron state. The neutron pick-up measurements confirmed the earlier assignments based on (d, t) reaction studies and suggested tentative assignments for the {$\text{1}\text{2}$⁺ [400]_n±$\text{1}\text{2}$⁺ [411]_p} and {$\text{3}\text{2}$⁺ [402]_n±$\text{1}\text{2}$⁺ [411]_p}     

Nuclear shape transition in neutron-deficient gold isotopes

On-line resonance ionization mass spectrometry has been applied to determine the isotope shift and hyperfine structure of^185–189Au and tne I=11/2 isomer of¹⁸⁹Au in the 6s²S_1/2 6p²P_1/2=268 nm) transition. The Au atoms were obtained as daughters of mass-separated Hg isotopes produced at the ISOLDE facility at CERN, ionized by a three-step resonant photoionization process, detected and mass-selected by time of flight. A drastic change of the nuclear charge radius was observed between¹⁸⁷Au and¹⁸⁶Au, which is interpreted as an onset of strong deformation of ₂ 0.25 in¹⁸⁶Au and¹⁸⁵Au.This work has been supported by the Bundesministerium für Forschung und Technologie. One of us, J. Wood was supported in part by the U.S. Department of Energy, Contract DE-AS05-80 ER 10599.     

The reaction 36S(p, γ)37Cl: (II). Lifetimes,spins and parities of 37Cl levels

Analysis of the γ-ray angular distributions measured at 16 ³⁶S(p, γ)³⁷Cl resonances yields the spins and/or parities of 21 bound states of ³⁷Cl in addition to the resonance spins. Among the latter are four $\text{J =}\text{1}\text{2}$ resonances. For several other bound states the possible spins have been restricted. Multipolarity mixing ratios have been deduced from the same data. Lifetimes (or lifetime limits) of 29 bound states have been deduced from DSA measurements.This extensive experimental information allows a comparison with the results of a shell-model calculation for both the even- and odd-parity states of ³⁷Cl. In this calculation either zero, one or two particles are promoted from the 2s_{$\text{1}\text{2}$} or 1d_{$\text{3}\text{2}$} to the 1f_{$\text{7}\text{2}$} or 2p_{$\text{3}\text{2}$} subshells. Up to an excitation energy of about 5 MeV a one-to-one correspondence is found between experimental and calculated levels.     

Excitation functions for radioactive isotopes produced by proton bombardment of Cu and Al in the energy range of 16 to 70 MeV

Excitation functions for ^52,54,56Mn, ⁵⁹Fe, ^{55,56,57,58,60}Co, ^56,57Ni, ^60,61,64Cu and ^62,63,65Zn in copper and for ⁷Be and ^22,24Na in aluminium were measured with protons in the energy range of 16 to 70 MeV. The stacked foil technique was applied using aluminium as degrader material. The results are compared with published data and, for the (p, xn) reactions, with calculated excitation functions.     

Nuclear charge radii from X-ray transitions in muonic atoms of carbon,nitrogen and oxygen

Energies of muonic X-rays of the K-series of carbon, nitrogen and oxygen have been measured with an accuracy of about 15 eV. Root mean square radii of the nuclear charge distributions were deduced. The results 2.49±0.05 fm for carbon, 2.55±0.03 fm for nitrogen and 2.71 ±0.02 fm for oxygen are in good agreement at comparable accuracy with recent electron scattering data.     

Elastic 3He scattering from even Ar isotopes and backward-angle anomalies in the systematics of elastic 3He scattering

Angular distributions have been measured for ³He elastic scattering from ^{36, 38, 40}Ar at 26.5 MeV and from ³⁶Ar and ⁴⁰Ca at energies between 24.5 and 28 MeV. This scattering clearly shows features of “anomalous” backward-angle scattering, which is discussed in the systematics of ³He scattering from heavier target nuclei. The data for “anomalous” scattering can be described by optical potentials which show features significantly different from those of “normal” scattering. These features are smaller radius parameters for the real optical potential and a strongly reduced volume integral for the imaginary potential.     

Nuclear Radiation Detected Optical Pumping of neutron-deficient Hg isotopes

The extension of the Nuclear Radiation Detected Optical Pumping method to mass-separated samples of isotopes far off stability is presented for a series of light Hg isotopes produced at the ISOLDE facility at CERN. The isotope under investigation is transferred by an automatic transfer system into the optical pumping apparatus. Zeeman scanning of an isotopically pure Hg spectral lamp is used to reach energetic coincidence with the hyperfine structure components of the 6s ^{2 1} S ₀6s6p ³P₁,λ=2,537 Å resonance line of the investigated isotope and the Hg lamp. The orientation built up by optical pumping is monitored via the asymmetry or anisotropy of the nuclear radiation. Nuclear spins, magnetic moments, electric quadrupole moments and the isotope shifts are obtained for¹⁸¹Hg-¹⁹¹Hg using theβ asymmetry as detector. The extension of the method using theγ anisotropy is discussed and test measurements on¹⁹³Hg are presented. This paper describes the experimental procedure, results, and discussion are given in a following publication.