Evidence for deformation in <Superscript>113-116</Superscript>Cd isotopes

High-spin states in ^113-116Cd have been investigated with the fusion-fission reaction ²⁸Si +¹⁷⁶Yb at 145 > MeV. The experiment has been performed with the Eurogam2 array. New rotational bands based on two quasi-particle states have been observed for even-even cadmium isotopes. A new level scheme based on the 11/2⁻ isomeric state is proposed for ¹¹⁵Cd and the one of ¹¹³Cd has been extended to spin (31/2⁻). The decoupled bands identified in both odd-A nuclei are interpreted as being built upon a low-Ωh_11/2 quasi-neutron configuration. Microscopic Hartree-Fock + BCS calculations confirm the prolate deformation in this mass region especially for the odd cadmium isotopes. Received: 21 December 1999 / Revised version: 16 February 2000     

Shapes of the neutron-rich 88-94Kr nuclei

Neutron-rich, ^88-94Kr nuclei, populated in spontaneous fission of ²⁴⁸Cm, have been studied with EUROGAM 2, by measuring prompt γ-rays. Many new excited states in even-even Kr isotopes have been identified. For the first time spins and parities were determined experimentally in these nuclei. Our results indicate that the quadrupole deformation of Kr isotopes will appear only above N = 58, as observed in Sr and Zr nuclei. The newly found 3^- level at 1506.4 keV in ⁹⁰Kr suggests the exsistence of a new region of increased octupole correlations, probably associated with the ν(d _5/2 h _11/2) pair of Δl = Δj = 3 orbitals. Received: 18 September 2000 / Accepted: 18 October 2000     

On-line production of Rb and Cs isotopes from uranium carbide targets

A series of on-line mass separation experiments have been performed at the IRIS facility to measure the yield and release of Rb and Cs neutron-rich isotopes produced by fission reaction of ²³⁸U. A 1 GeV proton beam was used to bombard uranium carbide targets with the densities of 11 g/cm³ and 1.5 g/cm³ held at temperatures in the range (2000-2230) ^°C. The release curves of Rb and Cs long-lived isotopes were measured from both kinds of targets. The overall production efficiency was determined making use of experimentally measured cross-sections of that isotope production. Comparison of the experimental yields of Rb and Cs isotopes with the calculated ones after corrections for losses due to finite release times suggests that the diffusion is the dominating process reducing the efficiency for short-lived isotopes. When normalized to the same thickness, an enhancement for the high-density rod target of the measured isotope yields is observed when going far from stability. This is possibly explained by the reactions induced by secondary neutrons. A significant odd-even effect with higher yields of Cs even neutron isotopes has been observed, confirming a similar effect obtained in earlier experiments.     

First observation of 55, 56Zn

In an experiment at the SISSI/LISE3 facility of GANIL, the most proton-rich zinc isotopes ^55,56Zn have been observed for the first time. The experiment was performed using a high-intensity ⁵⁸Ni beam at 74.5 MeV/nucleon impinging on a nickel target. The identification of ^55,56Zn opens the way to ⁵⁴Zn, a good candidate for two-proton radioactivity according to theoretical predictions. Received: 31 October 2000 / Accepted: 9 November 2000     

Isotope shifts and hyperfine structure in calcium 4snp and 4snf F Rydberg states

Isotope shifts and hyperfine structure have been measured in 4snp ¹ P₁ and Rydberg states for all stable calcium isotopes and the radioisotope ⁴¹Ca using high-resolution laser spectroscopy. Triple-resonance excitation via Rydberg state was followed by photoionization with a CO₂ laser and mass selective ion detection. Isotope shifts for the even-mass isotopes have been analyzed to derive specific mass shift and field shift factors. The apparent isotope shifts for ⁴¹Ca and ⁴³Ca exhibit anomalous values that are n-dependent. This is interpreted in terms of hyperfine-induced fine-structure mixing, which becomes very pronounced when singlet-triplet fine-structure splitting is comparable to the hyperfine interaction energy. Measurements of fine-structure splittings for the predominant isotope ⁴⁰Ca have been used as input parameters for theoretical calculation of the perturbed hyperfine structure. Results obtained by diagonalizing the second-order hyperfine interaction matrices agree very well with experimentally observed spectra. These measurements allow the evaluation of highly selective and sensitive methods for the detection of the rare ⁴¹Ca isotope. Received 17 December 1999 and Received in final form 29 March 2000     

New states in heavy Cd isotopes and evidence for weakening of the N = 82 shell structure

A chemically selective laser ion source has been used in a β-decay study of heavy Ag isotopes into even-even Cd nuclides. Gamma-spectroscopic techniques in time-resolving event-by-event and multiscaling modes have permitted the identification of the first 2⁺ and 4⁺ levels in ¹²⁶Cd₇₈, ¹²⁸Cd₈₀, and tentatively the 2⁺ state in ¹³⁰Cd₈₂. From a comparison of these new states in ₄₈Cd with the E(2⁺) and E(4⁺)/E(2⁺) level systematics of ₄₆Pd and ₅₂Te isotopes and several recent model predictions, possible evidence for a weakening of the spherical N = 82 neutron-shell below double-magic ¹³²Sn is obtained. Received: 13 July 2000 / Accepted: 12 October 2000     

High-spin states in neutron-rich Dy isotopes populated in deep-inelastic reactions

High-spin states in neutron-rich Dy isotopes, populated in deep-inelastic processes produced by the interaction of 234 MeV ³⁷Cl ions with a ¹⁶⁰Gd target, have been studied using the highly sensitive EUROBALL IV gamma-ray detector array. The previously known level schemes for ^{159,160,161,162}Dy have been extended to significantly higher spin ( ? 30?) and the i _13/2 band crossing in ¹⁵⁹Dy has been observed for the first time. The experimental results are discussed within the framework of cranked shell model and projected shell model calculations with particular reference to the observed delayed band crossing in ¹⁶²Dy. Received: 20 October 2000 / Accepted: 16 January 2001     

Decay of the neutron-rich isotope 113Ru to 113Rh

The decay of neutron-rich isotope ¹¹³Ru obtained as on-line mass separated product of proton-induced fission has been investigated by γγ coincidence and spectrum multiscaling measurements. Decay schemes for both low- and high-spin isomers of ¹¹³Ru have been constructed. The level scheme of ¹¹³Rh is considerably extended. Systematics of the lowest-lying rhodium levels is smooth. The picture of shape coexistence established for neutron-rich Rh isotopes near-neutron midshell is confirmed with the observation of a K = 1/2 deformed band, with its 3/2⁺ state at 600 keV being the lowest-lying level and of probable 7/2⁺ and 5/2⁺ band members. A large fraction of β feeding is found to populate high-lying levels in ¹¹³Rh. The GT strength in ¹¹³Ru^m decay is significantly larger than for the decay of ¹¹³Ru_g and of lighter rhodium isotopes. Received: 18 January 2001 / Accepted: 14 January 2002     

High-accuracy mass determination of unstable cesium and barium isotopes

Direct mass measurements of short-lived Cs and Ba isotopes have been performed with the tandem Penning trap mass spectrometer ISOLTRAP installed at the on-line isotope separator ISOLDE at CERN. Typically, a mass resolving power of 600 000 and an accuracy of δm ≈ 13 keV have been obtained. The masses of ^123,124,126Ba and ^122mCs were measured for the first time. A least-squares adjustment has been performed and the experimental masses are compared with theoretical ones, particularly in the frame of a macroscopic-microscopic model.     

Isomeric states in proton-unbound 187, 189Bi isotopes

Prompt and delayed gamma-ray spectroscopy of very neutron-deficient bismuth isotopes ^{187, 189}Bi has been performed using the Recoil Decay Tagging (RTD) method. The isomeric i _13/2 states have been identified and their lifetimes have been measured. The systematics of these long-lived M2 isomers has been extended to the proton-unbound isotopes. The general behaviour of single-proton states is discussed within the systematics and interpreted within the shell-model framework. Received: 2 May 2002 / Accepted: 3 June 2002 / Published online: 19 November 2002 RID="a" ID="a"e-mail: wkorten@cea.fr RID="b" ID="b"Present address: GANIL, Caen, France. RID="c" ID="c"Present address: Radiation and Nuclear Safety Authority, P.O. Box 14, FIN-00881 Helsinki. Communicated by D. Schwalm     

Simplex s = ±i excitations in 141Xe

Excited levels in ¹⁴¹Xe, populated in spontaneous fission of ²⁴⁸Cm, were studied by means of prompt -ray spectroscopy, using the EUROGAMM2 array. Level scheme of ¹⁴¹Xe obtained in this work shows patterns characteristic of simplex symmetry with s=+i and s=-i bands present but low value of D₀ moment indicates that octupole correlations in Xe isotopes are systematically lower than in Ba nuclei. Received: 9 March 2000 / Accepted: 4 May 2000     

Yields of products from fast neutron-induced fission of 233U measured by means of an isotope separator on-line (ISOL) system

A comprehensive study has been carried out of the yield pattern of fission products formed in fast neutron-induced fission of ²³³U. The isotope separator on-line facility at Studsvik to the R2-0 nuclear reactor was used for rapid separation of the fission products. At a target temperature of 2250 ^°C fission products of the elements from zinc (Z = 30) to barium (Z = 56) are released, with the exception of yttrium, zirconium, niobium, molybdenum, technetium, ruthenium and rhodium. The individual isotopes are then available for study, implying that an almost complete mapping of the yield distribution can be made. In the analysis, the delay between production and measurement and the overall separator efficiency for three consecutive elements (the one under study and its parent and grand parent) are taken into account. Independent and/or cumulative yields have been obtained for 203 nuclear species, among them 59 isomeric states. Received: 19 April 2000 / Accepted: 19 June 2000     

High-spin states following multi-nucleon transfer

High-spin states in neutron-rich nuclei, populated following deep-inelastic multi-nucleon transfer, have been studied using the GAMMASPHERE array at the LBNL, USA. A ⁶⁴Ni beam at an energy ∼ 15% above the Coulomb barrier was incident upon a thick ²⁰⁸Pb target, leading to the population of more than 130 different nuclei. The strongest channels correspond to nuclei close to the projectile and target, although transfer of up to 50 nucleons has been observed. New high-spin states in neutron-rich ^60,62Fe and ^68,70,72Zn nuclei have been observed. Some limitations of this method of high-spin spectroscopy are discussed, including the apparent difficulty of populating odd-odd and odd-even isotopes via this type of reaction. The data have been searched for superdeformed (SD) states in the A = 190-200 region, but no evidence for their presence has been found. Received: 14 April 2000 / Accepted: 12 September 2000     

Studying the ω mass in-medium in γ + A →π0γ + X reactions

Simulations based on a coupled-channel transport model have been performed to analyze the feasibility to study the in-medium ω mass exploiting the process γ + A→π⁰γ + X for C, Ca and Nb nuclei. The distortions due to final-state interactions of the π⁰ and background contributions from the reaction γ + A→π⁰π⁰ + X are found to be small in the mass range of interest ( 0.6 < M _π0γ < 0.8 GeV). Furthermore, the effect of the detector resolution on the π⁰γ mass determination is discussed. Received: 5 December 2000 / Accepted: 18 May 2001     

Separation of laser-cooled 42Ca+ and 44Ca+ in a linear Paul trap

Rare calcium isotope ions, ⁴²Ca⁺ and ⁴⁴Ca⁺, were efficiently separated from a laser-cooled ionic cloud in a linear Paul trap which was loaded from an atomic source of a natural isotope mixture of calcium, in spite of their negligibly small abundances (0.647% and 2.086%, respectively) compared with that of ⁴⁰Ca (96.94%). Selective heating and cooling that arise from the isotope shifts were mainly used for the elimination of the isotopes; selective heating and cooling enable flexible separation when combined with other mechanisms such as the inherent mass selectivity of RF traps. Received: 7 July 2000 / Published online: 10 January 2001     

Physics with heavy neutron-rich RIBs at the HRIBF

The Holifield Radioactive Ion Beam Facility at Oak Ridge National Laboratory has recently produced the world's first post-accelerated beams of heavy neutron-rich nuclei. The first experiments with these beam are described, and the results discussed. B(E2;0⁺ → 2⁺) values for neutron-rich ^126,128Sn and ^132,134,136Te isotopes have been measured by Coulomb excitation in inverse kinematics. The results for ¹³²Te and ¹³⁴Te (N = 80, 82) show excellent agreement with systematics of lighter Te isotopes, but the B(E2) value for ¹³⁶Te (N = 84) is unexpectedly small. Single-neutron transfer reactions with a ¹³⁴Te beam on ^natBe and ¹³C targets at energies just above the Coulomb barrier have also been studied. Received: 21 March 2002 / Accepted: 16 May 2002 / Published online: 31 October 2002 RID="a" ID="a"e-mail: radford@mail.phy.ornl.gov     

The β-delayed one- and two-proton emission of 27S

In an experiment performed at the GANIL LISE3 facility, radioactive ²⁷S isotopes have been produced by projectile fragmentation of a 95 AMeV ³⁶Ar primary beam. After selection by means of the LISE3 separator, the isotope of interest was implanted in a silicon-detector telescope where its half-life ( T _1/2 = 15.5(15) ms) and its main decay branches were measured. Received: 19 October 2001 / Accepted: 5 December 2001     

On the search for a narrow penta-quark Z+-baryon in NN interactions

The possibility for an observation of a narrow penta-quark Z⁺-baryon in NN reactions is discussed. It is shown that the pp↦nΣ⁺ K ⁺ reaction at excess energies around 100 MeV above threshold provides optimal conditions for Z⁺-baryon detection by an analysis of the nK⁺ invariant mass spectrum, if the Z⁺ mass is located around 1.5 GeV involving a rather narrow width. Received: 24 May 2000 / Accepted: 3 August 2000     

Synthesis and decay properties of superheavy atoms in nuclear reactions induced by stable and radioactive ion beams

This talk consists of two parts. The first one presents the results of investigations performed in 1998-2000 in Dubna on the synthesis of superheavy nuclei in reactions induced by ⁴⁸Ca ions. The radioactive decay properties of the nuclei, indicating a considerable increase in the α-decay and spontaneous fission half-lives of the isotopes of elements 110-116 when approaching the closed neutron shell at N = 184, are given. In the second part the possible ways of advancing into the region of more neutron-rich nuclei, using stable and radioactive ion beams, are discussed. Since so far no intense radioactive ion beams are available, some experiments with stable beams are considered as a test for the suggested ideas. Received: 1 May 2001 / Accepted: 4 December 2001     

Mass Measurements of 114–124,130Xe with the ISOLTRAP Penning Trap Spectrometer

The masses of the xenon isotopes with 114≤A≤123 were directly measured for the first time. The experiments were carried out at the ISOLTRAP triple trap spectrometer at the on-line mass separator ISOLDE/CERN. A mass resolving power of the Penning trap spectrometer of m/Δm≈500 000 was chosen and an accuracy of δm≈12keV for all investigated Xe isotopes was achieved. An atomic mass evaluation was performed and the results of this adjustment are compared with theoretical predictions. The new results for the xenon isotopes and their effects on neighboring nuclides are discussed within the two-neutron separation energy picture. This revised version was published online in July 2006 with corrections to the Cover Date.