Fragment dependence of high energy γ-ray emission in the spontaneous fission of 252Cf

The high energy γ-ray emission accompanying the spontaneous fission of ²⁵²Cf has been measured in coincidence with individual fission fragments selected by discrete γ-ray transitions. The enhancement of the γ-ray emission probability in the energy range E_γ= 3–8 MeV has been observed for the fission fragments in the region of nearly symmetric mass splitting, confirming results reported in previous investigations. The γ-γ coincidence technique employed in the present work clearly demonstrate that the major contribution to this enhancement is caused by the fission channels where one fragment is near to the N= 82 or Z= 50 shell closures. The high energy γ-ray emission probability does not show any significant dependence on the number of neutrons emitted in the fission process, supporting the hypothesis that high energy γ-rays are mainly emitted from the fragments after the neutron evaporation. Received: 22 December 1998     

Decay of the very neutron-deficient isotope 131Pm

The decay of ¹³¹Pm has been investigated by means of γ-ray spectroscopy. The ¹³¹Pm nuclei were produced by fusion-evaporation reaction of ¹⁰⁶Cd(³²S,3p4n) at the beam energy of 170 MeV. A helium-jet technique and a tape transport system were used to collect the activities and transfer them to a detecting position for X and γ rays measurement. Two γ rays of 185.0 and 220.0 keV were unambiguously identified to follow the β⁺ decay of ¹³¹Pm by results of X-γ and γ–γ coincidence. A growth-decay feature of the decay curve for 87.8 keV γ-ray of ¹³¹Nd confirmed the production of ¹³¹Pm nuclei. The half-life of ¹³¹Pm was measured to be 6.3 ± 0.8 s. A partial decay scheme of ¹³¹Pm is proposed on the basis of X-γ and γ–γ coincidence data in this experiment and the known structure information deduced from in-beam experiments of the daughter nucleus ¹³¹Nd. Received: 11 January 1999 / Revised version: 20 May 1999     

Study of the Mo-Ba partition in 252Cf spontaneous fission

Measurements of fission fragment yields and neutron multiplicities have been carried out for the Mo-Ba fragment pairs in the spontaneous fission of ²⁵²Cf, using the γ-ray spectroscopy technique to analyze γ-γ-γ coincidence data. Prompt γ -ray multiplicities were also measured as a function of the number of neutrons emitted in the fission process leading to the Mo-Ba partition. We do not observe the enhancement in the yields of events with high neutron emission multiplicity (ν_n > 7) that has been associated to a second fission mode leading to the production of hyperdeformed Ba fragments, as reported in some earlier studies. The average γ-ray multiplicity is found to be rather weakly dependent on the number of neutrons emitted in the fission process. Received: 21 July 1999 / Revised version: 19 November 1999     

Decay of 1.643 h <Superscript>95</Superscript>Ru and its daughter's level structure

The decay of ⁹⁵Ru has been investigated by means of γ-ray spectroscopy. The ⁹⁵Ru nuclei were produced by the reaction ⁹²Mo( α, n) ⁹⁵Ru at a beam energy of 17MeV. High-purity Ge detectors have been used singly and in coincidence to study γ-rays in the decay of ⁹⁵Ru to ⁹⁵Tc. 132 γ-rays are reported, among them, energies and intensities for 127 transitions have been determined. A decay scheme of ⁹⁵Ru with 31 levels is proposed which accommodates 127 of these transitions. Spins and parities for three new levels are proposed from calculated log ft values, measured γ-ray branching ratios, and in-beam experiment results of the daughter nucleus ⁹⁵Tc. Combining with the high-spin states observed by in-beam γ-ray spectroscopy of previous decay works, the structure of the excited states of ⁹⁵Tc is discussed in the framework of the projected shell model.     

Study of the N = 50 major shell effect toward 78Ni at PARRNe⋆

The γ-ray de-excitations following the β-decay of ⁸³Ga and the β-n decay of ⁸⁴Ga have been studied. The radioactive species were produced using the PARRNe on-line mass-separator installed at the IPN Orsay Tandem accelerator. Two γ-lines were attributed to ⁸³Ge with the aid of β-γ and γ-γ coincidences. The Z identification of the γ-lines was provided by time analysis of a buid-up/decay cycle. The excited levels of ⁸³Ge can be explained by the coupling of the single neutron state ν2d _5/2 to the first 2⁺ excitation of the ⁸²Ge core.     

Bimodal fission in binary and ternary spontaneous fission of 252Cf

The hot bimodal fission of ²⁵²Cf is reexamined with new high-statistics data. We constructed a γ-γ-γ coincidence cube for binary fission and LCP-gated γ-γ matrix for ternary fission. By identifying the secondary fission fragments from their γ-ray transitions, we measured the yields for various fission splits. The normal neutron yield distribution is found to be Gaussian for Xe-Ru. However, the binary fission split of Ba-Mo is found to exhibit a bimodal neutron distribution with the “hot mode” corresponding to ≈3.1% of the total yield. In α ternary fission, the first measurements of yields for specific fission splits are presented. The Te-α-Ru and Xe-α-Mo neutron yields fit well with a single mode, but the Ba-α-Zr split shows evidence for an enhanced hot mode with an intensity of ≈13.8% of the normal mode. The text was submitted by the authors in English.     

Radioactive decay of 217Pa

The radioactive decay of ²¹⁷Pa was investigated by means of α-γ-spectroscopy. Fine structure in the ground-state α-decay was established. Ambiguities in the fine structure of the α-decay of the previously known isomeric state could be clarified by α-γ-coincidence measurements. A previously unknown α-transition of E _α = (8306 ± 5) keV was detected and identified by means of delayed α-α- and α-γ-γ-coincidence measurements. A second isomeric state decaying by α-emission was not observed. The quality of the previously reported data of the α-decay fine structure of ²¹⁷Th was improved. Received: 29 April 2002 / Accepted: 17 June 2002 / Published online: 19 November 2002 RID="a" ID="a"e-mail: f.p.hessberger@gsi.de Communicated by J. ?yst?     

Decay of 83Sr and level structure of 83Rb

The excited states of the ⁸³Rb nucleus were investigated in radioactive decay of ⁸³Sr. The level scheme was established and for a number of levels spin-parity assignments are suggested on the basis of log ft values and γ-branching ratios. Combining with the high-spin states observed by the in-beam γ-ray spectroscopy of a previous decay work, the structure of the excited states of ⁸³Rb is discussed in the framework of the projected shell model. Received: 17 November 1999 / Accepted: 11 December 2000     

The new isotope 270110 and its decay products 266Hs and 262Sg

The even-even nucleus ²⁷⁰110 was synthesized using the reaction ⁶⁴Ni + ²⁰⁷Pb. A total of eight α-decay chains was measured during an irradiation time of seven days. Decay data were obtained for the ground-state and a high-spin K isomer. The new nuclei ²⁶⁶Hs and ²⁶²Sg were identified as daughter products after α-decay. Spontaneous fission of ²⁶²Sg terminates the decay chain. The measured data are in agreement with calculations using the macroscopic-microscopic model and with self-consistent HFB calculations with Skyrme-Sly4 interaction. Received: 27 November 2000 / Accepted: 16 January 2001     

Intruder bands in 113Sn

Abstact: The level structure of ¹¹³Sn has been investigated. The data were obtained by in-beam γ-ray spectroscopy using the reaction ¹⁰⁰Mo(¹⁸O,5n)¹¹³Sn at 70 MeV performed at the OSIRIS gamma array in the Institut für Kernphysik FN Tandem accelerator. We report in this short note the observation of two intruder type rotational bands in this nucleus. Received: 28 April 1998     

In-beam study of 145Tb

The high-spin states of ¹⁴⁵Tb have been studied in the ¹¹⁸Sn(³²S, 1p4n) reaction at ³²S energies from 161 to 175 MeV using techniques of in-beam γ-ray spectroscopy. Measurements of γ-ray excitation functions and γ-γ-t coincidences were performed with 12 BGO(AC)HPGe detectors. Based on the measured results of γ-γ coincidences, γ-ray anisotropies and DCO ratios, a level scheme for ¹⁴⁵Tb was established for the first time. The observed excited states show typical irregular pattern in a spherical nucleus, and the low-lying levels have been interpreted qualitatively with a particle-core coupling. Received: 21 September 2001 / Accepted: 9 November 2001     

New states and γ-transitions in 209Bi observed in the (3He, d*γγ)-subcoulomb-reaction

High-spin states in ¹⁴³Pm have been investigated via the ¹²⁸Te(¹⁹F,4nγ)¹⁴³Pm reaction using techniques of in-beam γ-spectroscopy. γ-ray singles, γ-γ coincidences, γ-ray anisotropies and DCO ratios have been measured. Based on these measurements, the level scheme of ¹⁴³Pm has been extended up to an excitation energy of 10535.4 keV, including 48 new γ-rays deexciting 28 new levels. The yrast levels in ¹⁴³Pm can be understood qualitatively in the framework of a weak-coupling model. Received: 10 July 2000 / Accepted: 12 October 2000     

Beta Decay of 111Tc to 111Ru

The β-decay of the very neutron-rich ¹¹¹Tc nucleus has been observed. A partial decay scheme of ¹¹¹Ru is presented, complementing the high-spin levels earlier reported in spontaneous fission work. Received: 15 January 1998     

Angular momenta of fission fragments in the α-accompanied fission of 252Cf

For the first time, average angular momenta of the ternary fission fragments ^{100, 102}Zr, ¹⁰⁶Mo, ^{144, 146}Ba and ^{138, 140, 142}Xe from the α-accompanied fission of ²⁵²Cf were obtained from relative intensities of prompt γ-ray transitions with the use of the statistical model calculation. Average values of the angular momenta were compared with the corresponding values for the same fission fragments from the binary fission of ²⁵²Cf. Results indicate the presence of a decreasing trend in the average values of angular momenta induced in ternary fission fragments compared to the same binary fission fragments. On the average, the total angular momentum extracted for ternary fission fragments is ∼1.4 ℏ lower than in binary fission. Consequently, results indicate that the mechanism of the ternary α-particles emission may directly effect an induction of angular momenta of fission fragments, and possible scenarios of such mechanisms are discussed. Further, the dependence of the angular momenta of ¹⁰⁶Mo and ¹⁴⁰Xe on the number of emitted neutrons from correlated pairs of primary fragments was obtained also showing a decreasing dependence of average angular momenta with increasing number of emitted neutrons. Consequences are briefly discussed.     

Measuring high-energy γ-ray emission accompanying the spontaneous fission of <Superscript>252</Superscript>Cf nuclei

The probability of high-energy γ-ray emission accompanying the spontaneous fission of ²⁵²Cf nuclei in the energy range of 5–60 MeV was measured experimentally. The γ rays were detected by a BGO detector with a size of ∅7.6 × 7.6 cm in coincidence with neutrons detected by an organic polystyrene-based scintillator with a size of ∅6.0 × 2.0 cm. To reject events associated with the cosmic background, we propose an original method that combines rapid digitizing of the pulse shape and the time-of-flight method.     

Band structures in 108In

High spin states in ¹⁰⁸In have been established upto ∼ 8 MeV in excitation energy and to a tentative spin of (23⁻). The data were obtained by in-beam γ-ray spectroscopy using the reaction ⁹³Nb(¹⁹F, p3n)¹⁰⁸In at a beam energy of 86 MeV. Four sequences of dipole bands and a normal rotational band of E2 γ-transitions have been placed in the level scheme. Received: 16 June 1998     

Study of analogue states in52Cr through proton capture by51V

γ-Ray yield function has been studied for the proton capture by vanadium in the proton energy range 720–1300 keV. Isobaric analogues of low lying states in⁵²V have been identified. At two resonances theγ-decay andγ-ray angular distributions have been obtained and the branching ratios and the multipole mixing ratios have been deduced. The analogue-antianalogue M1 transition in⁵²Cr is found to be strongly hindered as in other f_7/2 nuclei. TheQ-value obtained for this reaction is (10500±2.8) keV and the Coulomb displacement energy is (8.06±0.01) MeV. An upper limit of 2 meV has been obtained for theα- decay strength of the 11.395 MeV state in⁵²Cr.     

Shape co-existence and structural evolution of the yrast band in 157Yb

The high-spin states of ¹⁵⁷Yb have been studied via the ¹⁴⁴Sm(¹⁶O, 3n) reaction at ¹⁶O energy of 90 MeV using techniques of in-beam γ-ray spectroscopy. Measurement of γ-γ-t coincidences was performed with 11 BGO(AC)HPGe detectors. Based on the measured results of γ-γ coincidences, γ-ray anisotropies and DCO ratios, the level scheme for ¹⁵⁷Yb was established. The shape co-existence and structural evolution of the νi _13/2 band with increasing angular momentum in ¹⁵⁷Yb have been discussed. The systematics of the νi _13/2 bands in the N = 87 odd-A isotones have been compared. Received: 7 January 2002 / Accepted: 10 April 2002     

Mechanisms for the appearance of prescission γ-rays and their related T-odd asymmetries

Conditions for the appearance and observation of prescission γ-rays emitted by a fissioning nucleus before its separation into fission fragments were investigated within the quantum theory of fission. It was demonstrated that these conditions can be fulfilled in the γ-decay of giant electric isovector dipole resonances in a fissioning nucleus that become excited due to the nonadiabaticity of the collective deformation motion of the nucleus at the final stages of its prefission evolution. Angular and energy distributions of prescission γ-rays emitted by unpolarized fissioning nuclei were analyzed. Characteristics of T-odd asymmetries in angular distributions of prescission γ-rays were investigated for fission of unpolarized target nuclei induced by polarized cold neutrons, and these correlations were shown to be similar in nature to the T-odd ROT correlations earlier found for α-particles emitted in ternary nuclear fission.     

High-spin levels in 147Tb

The high-spin states of ¹⁴⁷Tb have been studied with regard to their spins. The data were obtained by in-beam γ-ray spectroscopy using the reaction ¹²⁰Sn(³¹P,4n)¹⁴⁷Tb at 152 MeV performed at the Osiris spectrometer in Berlin. We obtained multipole mixing ratios for 60 transitions, and level spins up to 67/2ħ are introduced. Received: 30 March 1998