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1.
A remarkably narrow component was found in the angular correlation curve of photon pairs resulting from the annihilation of positrons in neutron-irradiated niobium containing voids. The gamma-ray energy spectrum obtained from a NaI(TI) detector did not give evidence of 3-γ annihilation. This suggests that in voids positrons exist in positronium states or in free states and decay primarily by 2-γ annihilation.  相似文献   

2.
A kinetic scheme of decay of positron and positronium states for the general case — a real ionic crystal with point lattice defects and a developed surface — is examined. The properties of positron and positronium states in the volume of the crystal, positron and positronium color centers, and surface positron and positronium states, are analyzed. It is shown that all the available experimental data qualitatively confirm the conclusion of an annihilation mechanism based on the postulated kinetic scheme of positron annihilation in real ionic crystals.Translated from Izvestiya Vysshikh Uchebnykh Zavedenii, Fizika, No. 9, pp. 50–55, September, 1977.  相似文献   

3.
The technique of positron annihilation experiments as applied to the study of Fermi surfaces in metals and alloys is briefly reviewed. The angular correlation of the two annihilation photons is directly related to the momentum distribution of the positron-electron system; breaks in this distribution reflect the size and shape of the Fermi surface. Recent two-dimensional angular correlation measurements designed to study the Fermi surface of Cu?Al and Cu?Zn alloys are presented, and are compared with theoretical predictions.  相似文献   

4.
It is shown that the existence of a metastable state in which positrons in metals are “self-trapped” by strong interaction with the lattice gives rise to an anomalous temperature dependence in positron annihilation properties. The “intermediate” temperature variation of the shape of the annihilation photon line discovered by MacKenzieet al. is well accounted for by this mechanism; alternative interpretations in terms of thermal expansion effects may be refuted. This result calls for considerable revision of some of the published monovacancy formation energies obtained from positron annihilation measurements. Approximate criteria for the existence and the metastability of a selftrapped state of positively charged particles in metals are given. It is found that metastable self-trapping may occur for positrons; hydrogen isotopes and positive muons should be self-trapped in configurations that are always stable relative to the Bloch-wave states of these particles.  相似文献   

5.
Taking into account the core electron enhancement factor the rare-gas core contribution to the angular correlation positron annihilation spectra and to the total annihilation rate in some simple and transition metals are calculated. It is shown that the valence high-momentum part of the Gaussian fraction is not negligible in simple metals. In 3d and 4d metals, the rare-gas core part of the total annihilation rate amounts from 9 to 37%. The results are expected to help in the correct interpretation of the positron annihilation data.  相似文献   

6.
Calculations are performed together with the summarization of published data on the measurement of positron annihilation rates in a number of simple substances. The information potential of different methods underlying positron annihilation spectroscopy is analyzed as applied to the study of condensed matter. The features of the mechanism of positron annihilation in metals are discussed. The possibility of investigating the electronic and defect structures of metals and alloys using the method of the time distribution of annihilation photons is considered.  相似文献   

7.
The relative contribution of 3d electrons to the momentum densities for positron annihilation in the iron series transition metals are calculated, using the atomic Hartree-Fock-Slater orbitals. A discussion is given of the observed systematics. The per electron contribution to the angular correlations is found to decrease with the filling up of the d shell. The high momentum components are found to be relatively enhanced in case of higher Z metals. The built in spin dependence of the electron HFS wavefunction is reflected in the calculated curves.  相似文献   

8.
金属中点缺陷的电子结构和缺陷谱   总被引:1,自引:0,他引:1       下载免费PDF全文
本文以胶体模型为基础,利用密度冷函理论和局域密度近似研究了过渡金属Cr,Fe,Ni和贵金属Cu中空位型缺陷、氢杂质、空位-杂质复合体的电子结构以及以正电子湮没寿命表征的缺陷谱。表明了用正电子湮没寿命谱研究金属点缺陷电子结构和缺陷尺度大小的可行性。 关键词:  相似文献   

9.
R M Singru 《Pramana》1974,2(6):299-303
The two photon pair momentum density and the angular correlation curves for positron annihilation radiation from copper have been obtained by a band structure calculation, employing Hubbard’s approximation scheme. A comparison of the calculated curve for the long slit geometry with the experimental results shows that the theory rather overestimates the contributions in the high momentum region. An angular correlation curve for a point slit geometry is also calculated.  相似文献   

10.
In this review we discuss the different aspects of positron annihilation in metals that involve the dynamics of positron motion before annihilation. The emphasis is on the theory, but also some experimental evidence is quoted. The topics covered are: slowing down and thermalization, effective mass, temperature dependence of positron vacancy trapping, positron channeling, and escape of low energy positrons from metal surfaces.  相似文献   

11.
A new method is proposed to deal with analysis of positron annihilation lifetime spectra which defy ordinary computer fitting. The method is particularly suited for investigations of defects in metals.  相似文献   

12.
The annihilation radiation of low energy positrons gives information on the electronic and defect structure of solids. There are three conventionally measurable quantities: the positron lifetime, the angular correlation of 2 annihilation radiation and the Doppler-broadened annihilation line shape. In the presence of lattice defects the annihilation characteristics show considerable changes. This is due to positron trapping at defects like vacancies and their agglomerates, voids, dislocations and grain boundaries. The concentration of defects can be deduced from the ratio of trapped and free positrons.The annihilation characteristics are different for different defect configurations. Positrons reveal vacancy agglomeration and the lifetime of trapped positrons gives estimates on the size of microvoids in the range of 2–10 Å. Various examples on the study of equilibrium and non-equilibrium defects, radiation damage and defect annealing are presented. Special emphasis is given to vacancy recovery and vacancy-impurity interactions in electron and neutron irradiated bcc transition metals like Fe, Mo, Nb, Ta.  相似文献   

13.
A new fit to the long-range angular correlation of annihilation radiation data of the sum of a parabola, so-called Ferrell function, and a Gaussian for noble and d-transition metals is presented. The three functions are considered to describe the positron annihilation with three different electron groups: nearly free, d-like and rare-gas core electrons, respectively.  相似文献   

14.
A brief survey of theoretical and experimental work that is devoted to studying the resonance absorption and scattering of gamma rays by nuclei and which was initiated at the Institute of Theoretical and Experimental Physics (ITEP, Moscow) in the 1950s and has been continued to date is given. Investigations of various versions of interaction in beta decay, magnetic-field-perturbed angular distributions of resonantly scattered gamma rays, the problem of the Mössbauer gamma resonance of long-lived isomeric states of nuclei, and the resonance scattering of annihilation photons by nuclei are described.  相似文献   

15.
A.S. Hamid 《哲学杂志》2013,93(34):4302-4310
The Fermi surface (FS) and spin-dependent momentum space density distribution of ferromagnetic Gd was studied via longitudinally polarised positrons. The measurements were performed using a 2D angular correlation of the annihilation radiation experiments with the reversal magnetic field direction parallel and anti-parallel to the polarisation direction of the positron. It was found that the minority-spin states were concentrated in the basal plane and majority-spin states were concentrated around the A, L and H points. The analysis confirmed that the main contributions to the FS of Gd were influenced by the mixing of both the 5d–6s and the 4f–5d hybrid bands. The general layout of this FS was observed as two hole-like surfaces running along the [ΓA] axis and one electron-like surface running along the [MK] direction. In general, the experimental results showed good agreement with earlier investigations.  相似文献   

16.
Potential energy curves for excited leptonic states of the helium-antihydrogen system are calculated within the Ritz variational approach. An explicitly correlated ansatz for the leptonic wave function is employed describing accurately the motion of the leptons (two electrons and positron) in the field of the helium nucleus and of the antiproton with an arbitrary orbital angular momentum projection Lambda onto the internuclear axis. Results for Lambda=0, 1, and 30 are presented. For quasibound states with large values of Lambda and rotational quantum numbers J>Lambda no annihilation and rearrangement decay channels occur; i.e., they are metastable.  相似文献   

17.
A point geometry angular correlation measurement of the annihilation radiation from an annealed single crystal of copper is presented. The results are compared with results for an unannealed sample and theoretical predictions obtained from a simple picture of the electronic wave-functions combined with two models for the positron wavefunction.  相似文献   

18.
In positron annihilation investigations of nonmetallic solids, the standard deviation of the gaussian component of the angular correlation curve is elucidated as material constant. It is related to the apparent radius of the chemical unit of the substance in question.  相似文献   

19.
Positron annihilation from a positron-anion bound state is considered. A critical analysis of the optical positron model is given, and a modification is suggested with the purpose of removing drawbacks of this model. A calculation of angular correlation curves and positron life time is carried out. In the calculation we explicitly account for repulsion forces between the positron and the nucleus, dominating at short distances. It is shown that the inner electron of the anion plays no significant role in the formation of the angular correlation curve, and does not affect the value of the positron lifetime. The model makes it possible to determine the effective anion charges and the value of the repulsion force between the positron and the nucleus from experimental angular correlation curve and positron lifetimes in ionic media. Specific analysis is carried out for the O2– ion.Translated from Izvestiya Vysshikh Uchebnykh Zavedenii, Fizika, No. 4, pp. 58–63, April, 1987.The authors are grateful to V. A. Kashcheev for performing numerical calculations.  相似文献   

20.
The effect of electron beam irradiation on the positron annihilation in KCl, KBr, NaCl single crystals was investigated. The narrowing of the angular correlation curves increases up to the saturation value with the absorbed radiation dose. The shape of the received narrow components differs from the narrow component measured in the additively colored samples. This phenomenon shows the considerable influence of the hole centres upon the positron annihilation in ionic crystals. Paper presented at 3rd Internat. Conf. Positron Annihilation, Otaniemi, Finland (August 1973).  相似文献   

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