Mathematical modeling of hybrid CO2 laser

A Teller–Landau six-temperature model describing the dynamic emission of single-mode TEA CO₂ laser has been adapted. This model has been also used to describe the mechanism of obtaining relatively high-power output pulses from hybrid TE-TEA or CW-TEA CO₂ laser consisting of high- and low-pressure sections. The suggested mathematical model allows to investigate the mechanism which limits the TEA oscillation to single longitudinal mode (SLM) due to the narrow gain bandwidth of low-pressure section, and also to study the effect of the laser input parameters on the smooth output laser pulse parameters. In addition, numerical solutions of non-linear rate equation system of the suggested model are quantitatively discussed. The solutions describe the radiation field intensity, the population inversion, and the energy transfer processes. The calculated values of maximum peak power, total energy in pulse, pulse width, etc. are in a very good agreement with the observed experimental values.     

Injection locked single mode operation of a tea CO2 laser with high energy extraction

Generation of reproducible smooth pulses from longitudinal mode control of a TEA CO₂ laser by signal injection from a cw CO₂ laser is reported and the operating conditions investigated for several new geometries. Applied to unstable resonators, the efficient and spectrally pure, high power output obtains has important application in the area of optical pumping.     

CO2 laser assisted removal of UO2 and ThO2 particulates from metal surface

Pulsed laser assisted removal of uranium dioxide and thorium dioxide particulates from stainless steel surface have been studied using a TEA CO₂ laser. Decontamination efficiency is measured as a function of laser fluence and number of pulses. Threshold fluence for the removal of UO₂ particulates has been found to be lower than that required for the removal ThO₂ particulates. Usage of a ZnSe substrate, that is transparent to the laser wavelength used here, enabled us to decouple the cleaning effect arising out of absorption in the particulates from that in the substrate and has contributed towards understanding the mechanism responsible for cleaning. The experimental observations are also corroborated by simple theoretical calculations.     

Review of theoretical gain-optimization studies in 10.6µm CO2-N2 gasdynamic lasers

A comprehensive theoretical analysis of optimization of gain in CO₂-N₂ gasdynamic laser employing wedge or conical or hyperbolic nozzles with either H₂O or He as the catalyst is presented. After a review of previous work, the usual governing equations for the steady inviscid quasi-one-dimensional flow in a supersonic nozzle of a gasdynamic laser are used to obtain similar solutions for the various flow quantities, which variables are subsequently used to optimize the small-signal gain on theP(20) line of the (001) → (100) transition of CO₂ at wavelength 10.6μm. The corresponding optimum values like reservoir pressure and temperature and nozzle area ratio also have been predicted and presented in the form of graphs. The analysis predicts that employing of 2D-wedge nozzle results in higher gain values and the CO₂-N₂-H₂O gasdynamic laser employing 2D-wedge nozzle is operationally the best laser system for which the optimum value as high as 3.1 m⁻¹ gain can be obtained.     

Injection seeding for single-mode operation in an optically pumped high-power D2O laser

Spectrally narrow, pulsed outputs consisting of almost a single mode have been obtained from an optically-pumped high-power (200kW) D₂O laser by adopting the injection seeding method, where single-mode radiation (seed pulse) from a low-power, compact D₂O laser has been injected into the main D₂O laser. Spectrally narrow outputs with high power having spectral widths as narrow as 5 MHz have been obtained, when the seed pulses with frequency tuned to one longitudinal mode of the main D₂O laser have been injected at a time sufficiently before the lasing of the main laser took place. The experimental results have been compared with those of numerical simulation modified to include the injection field with varying injection times.     

A sequential discharge TEA CO2 laser with high repetition rate and high output power

In this paper, a novel excitation method named as sequential discharge is realized in a two-module TEA CO₂ laser by using a special rotating spark gap. It is demonstrated that the repetition rate and the output power of a laser can be multiplied through this method. For the two-module TEA CO₂ laser in the experiment, the repetition rate is 300 Hz and the average power is 356 W when each module discharges; the repetition rate is 600 Hz and the average power is 713 W when the two modules discharge sequentially.     

Design and operation characteristics of a high power transverse flow pulser sustained cw CO2 laser

A transverse flow, transverse discharge cw CO₂ laser in which de discharge is sustained by employing high repetition rate high voltage pulses has been developed. Pulser sustained discharge through electrodes of innovative design provided uniform excitation at electrical input power densities more than 10 W/cc. Laser output power more than 2.5 kW was obtained in a laser gas mixture consisting of 0.5 mbar of CO₂, 16 mbar of N₂ and 38.5 mbar of He. Design details and operational characteristics of this laser are presented.     

Tunable te-CO2 laser-pumped formaldehyde far-infrared lasers: Offsets, assignment, and superfluorescence

Sixty and three absorption transitions in D₂CO and H₂CO, respectively, have produced a number of far infrared laser lines when they are pumped by an etalon-tuned TE-CO₂ laser. Almost all the absorption transitions pumped previously by a free runing TE-CO₂ laser have been efficiently pumped by the etalon tuned CO₂ laser and found to have offset within ±500 MHz from the line-center of the relevant CO₂ pump lines. 22 (1) absorption and 63 (4) emission lines of D₂CO (H₂CO) are assigned. Some of these lines have generated superfluorescence. In paticular, the D₂CO 319-m line pumped by CO₂-9P(32) delivered an output energy of approximately one half that of the well-known D₂O 66-m. It is shown that a large electric dipole moment and an appreciable amount of fractional population in the lower level of the pump transition of this line are responsible to the superfluorescence.     

A sensitive arc detection technique for reliable operation of high repetition rate TEA CO2 laser

A simple and sensitive technique, which utilizes the sensing of both the discharge current and the visible light emission from the discharge, has been developed to detect the arc formation during the operation of a high repetition rate TEA CO₂ laser. It is shown that the optical detection in the visible spectral region is more sensitive than that it is in the UV region and hence can be used more effectively to monitor the onset of arc formation, while the current signal is useful in the strong arc formation regime. We demonstrate that the trigger signals generated by both the methods can be employed for reliable protection of the laser system from catastrophic damage due to deleterious arc formation.     

Remote detection of sulfur dioxide by means of a CO2 laser

The possibility of remote detection of SO₂ in the 9-μm region of the spectrum by means of a TEA CO₂ laser was theoretically and experimentally investigated with regard to the real state of the atmosphere and the contribution of background concentrations of H₂O, CO₂ and NH₃ to absorption. For sounding along short paths (2L=2 km), the method of detection of small concentrations of SO₂ (at the MPC level) with the use of the lines of the CO₂-molecule regular transitions (00^o1–02^o0 band) has been devised and experimentally tested. It is shown that in sounding along longer paths (2L=6 km), a noticeable increase in sensitivity can be achieved by the generation lines of the CO₂-molecule sequential 00^o2–02^o1 band. B. I. Stepanov Institute of Physics of the National Academy of Sciences of Belarus, 70, F. Skorina Ave., Minsk, 220072, Belarus. Translated from Zhurnal Prikladnoi Spektroskopii, Vol. 65, No. 4, pp. 508–515, July–August, 1998.     

Third harmonic generation of CO2 laser radiation in AgGaSe2 crystal

Generation of third harmonic of CO₂ laser radiation has been obtained in a type-II, ϑ=57° cut 9 mm thick AgGaSe₂ crystal for the first time by sum-frequency-mixing of the fundamental with its second harmonic, the latter being obtained using another type-I, ϑ=55° cut 11 mm thick AgGaSe₂ crystal. The energy conversion efficiencies obtained for second harmonic and third harmonic generations are 6.3% and 2.4% respectively with the input fundamental pump power density of 5.9 MW/cm² only. The wavelength of the fundamental CO₂ laser radiation used for the generation of harmonics is 10.6 μm, P(20) line. A compact TEA CO₂ laser source has been built in the laboratory.     

Design and experimental characterisation of a DC-excited CW/repetitively pulsed sealed off CO2 laser

This paper reports the design procedure and experimental study of a sealed off CO₂ laser. Simple algorithms for threshold and steady state excitation voltage calculation, resonator design and its temperature dependent operation are presented. The sealed off CO₂ laser was operated both in CW and pulsed modes and found stable both thermodynamically and optically. Frequency limits for pulsed operation regarding maximum and minimum output energy ranges are determined. Different aspects of CO₂ laser studied include threshold excitation voltages, temperature dependent efficiency, optical power saturation limitations, pulsed and steady state discharge currents for optimum gases mixture combinations. The laser has successfully been constructed, operated and tested for different applications within the limits of its maximum output power of 14 W.     

Repetitive operation of a helium-free mini TEA CO2 laser

A helium-free mini TEA CO₂ laser has been operated at a repetition rate of 100 Hz wherein the gas re-circulatory loop consisting of heat exchanger and catalytic converter, mandatory for conventional repetitive operation of such lasers, have been totally dispensed with. The laser utilized inexpensive molecular gases alone that were simply flown out transversely through the inter-electrode region by an open gas flow system. The active medium was energized by making use of a spiker-sustainer excitation scheme. At this repetition rate, the laser produced an average power of 3.50 W.     

A 3 kW average power tunable TEA CO2 laser

A high average power line-tunable TEA CO₂ laser is described. Average output power up to 3 kW is achieved at repetition rate of 180 Hz. The maximum output power is almost equal among the four spectrum bands of CO₂ laser (the P and R branches of 00°1–10°0 and 00°1–02°0 transition bands). Several special technologies including rotating spark gap switching, PCB (printed circuit board) preionization and zeroth-order grating coupling are employed.     

Optically pumped submillimeter laser lines from CD2Cl2 using a large tunability CW CO2 laser

Twenty-five new laser lines have been obtained in the wavelength region from 155 to 830 μm by optically pumping the CD₂Cl₂ (deuterated dichloromethane) molecule with a CW CO₂ laser having a tunability range of 300 MHz. The wavelength, polarization relative to that of CO₂ pumping radiation, and offset relative to the CO₂ center frequency were determined for all of the new lines and some other already known laser emissions. For all of them we give also the relative intensity and the optimum pressure of operation. Permanent address: Depto de Física e Química da FEIS — UNESP 15.378-000 Ilha Solteira-SP, Brazil     

Mathematical modeling of tunable TEA CO2 lasers

A mathematical model, based on the Landau–Teller equations of six-temperature model for the CO₂–N₂–He–CO system, to describe the process of dynamic emission in tunable TEA CO₂ lasers is introduced. In this model, the Landau–Teller equations are rewritten with regard to fine longitudinal mode frequencies in the laser resonator. These revised equations can be utilized to estimate the laser output spectra as well as other laser output pulse parameters. Examples are given to show the modeling results of non-tunable, grating tuned or injection-locking TEA CO₂ lasers.     

The structure of multi-electrode-pair pulse laser and discharge pulse time selection

Applying multi-electrode-pair pulse TEA CO₂ laser to one optical resonance cavity will have several advantages over traditional method, including higher gain, shorter pulse discharge time interval, and in particular, continuous adjustable time interval of multi-pulse laser output can be achieved without high vacuum condition. To improve laser's working stabilization, we proposed new approaches to optimize laser structure design and discharge pulse time interval selection.     

Short single-mode CO2 laser pulse generation by pulsed Q-switching

A simple method for the generation of short, single-mode CO₂ laser pulses produced by applying two voltage gates (of amplitude 3U_λ/4 and U_λ/4) to an electro-optic Q-switch placed in a three-mirror cavity is proposed. Single, single-mode, well-synchronizable pulses of 3 ns duration and of 3 mJ energy have been experimentally achieved from a TEA CO₂ laser with an intracavity Pockels cell with 3 ns switching time. Using a numerical simulation it is shown that with shorter switching time (≈1 ns) the method enables one to obtain, from such a laser, a single, megawatt pulse of 1 ns duration.     

Numerical modeling of a fast-axial-flow CW–CO2 laser

A four-temperature model has been applied on a fast axial flow, longitudinal discharge CO₂ laser. Using Runge–Kutta method, a set of differential equations of the model is numericaly solved. These equations describe the operation of the laser with certain ratio 1:3:6 of the mixture CO₂:N₂: He and average output power of 550 W.The temporal behaviour of the output power and photon density was obtained. The effects of kinetic temperature, coupled mirror reflectivity, gas flow speed, and cavity loss on the output power were studied.Calculated output power was compared with its measured value taken from experiment and a good agreement was observed.     

Time-resolved spatial structure of TEA CO2 laser pulses

The evolution of the intensity profile of TEA CO₂ laser pulses along the pulse length is investigated both analytically and experimentally. A simple scalar model of the pulse amplitude is introduced, which gives the loaded-cavity modes as a linear combination of bidimensional Hermite-Gauss functions. According to this model a number of equations are derived which link the time-varying spatial structure of the pulse to its time-resolved second-order intensity moments, namely, the beam width and the M² parameter.