Cross relaxation of12B in single-crystal aluminium

The dipole-dipole interaction of extremely diluted probe nuclei with their surrounding host nuclei gives rise to mutual flip-flop processes of the nuclear spins. As energy has to be conserved in this so-called cross-relaxation (CR) process a transfer of polarization from the probes to the host nuclei occurs only at certain values of the inductionB leading to resonance-like dips in the probe's polarization. For the system¹²B in single-crystal aluminium CR spectra were measured forB=7...400 mT andT=310...410 K at various crystal orientations relative toB. All the spectra could be well explained by a theoretical calculation assuming the octahedral interstitial site for¹²B.     

Complete and incomplete fusion studies in7Li and16O induced reactions on51V by measurement of excitation functions and recoil ranges

Excitation function and mean projected recoil ranges of nuclei produced in the⁷Li and¹⁶O induced reactions on⁵¹V target were measured by conventional stacked foil and thick-target thick-recoil-catcher technique for bombarding energiesE ≤ 50.0 MeV for⁷Li ions andE ≃ 60.0-96.0 MeV for the¹⁶O ions. The measured recoil ranges are converted to momentum transfer. The momentum transfer information was used to get clues about some aspects of the interaction such as complete and incomplete fusion reaction mechanism which correspond to full and reduced momentum transfer respectively. The measured excitation functions are compared with the calculation based on the statistical model which describes only equilibrium decay of the compound nucleus using the CASCADE code. The comparison of the CASCADE code with the measured excitation functions for the residue radioisotopes⁵¹Cr and⁵⁴Mn for the⁷Li +⁵¹V system indicates the reaction mechanisms is complete fusion of⁷Li with the target nucleus⁵¹V. Similarly the comparison of the CASCADE code with the measured excitation functions of the residue radioisotopes for the system¹⁶O +⁵¹ V indicates that the four reaction mechanisms (i) complete fusion of¹⁶O, (ii) incomplete fusion of¹²C, (iii) incomplete fusion of⁸Be and (iv) incomplete fusion of⁴He respectively with the target might be contributing to reaction cross sections.     

Polarization in the quasielastic scattering of 1-GeV/c protons on light nuclei

Polarization measurements in the A(p, 2p)B reactions on ⁶Li, ⁷Li, and ²⁸Si nuclei at a proton-beam energy of 1 GeV were performed in a kinematically complete experiment. By using a two-arm magnetic spectrometer, two secondary protons were recorded in coincidence at asymmetric scattering angles of θ₁=15°?26° and θ₂=58.6° for residual-nucleus momenta in the range K _B=0–150 MeV/c. Either arm of the spectrometer was equipped with polarimeters based on proportional chambers. The data coming from this experiment are analyzed within the distorted-wave impulse approximation. It is shown that the polarization of recoil protons formed at angle θ₂ in the interaction featuring a proton from the P shell of the ⁷Li nucleus can be described under the assumption of an effective intranuclear-proton polarization by using the single-particle shell-model wave function of the nucleus. Our data on the polarizations of the two protons from the reaction (p, 2p) on a ²⁸Si nucleus also suggest the effective polarization of the protons in the D shell of the ²⁸Si nucleus. It is found that, for high recoil-nucleus momenta of K _B≥90 MeV/c, the effective polarization of the protons in the P shell of the ⁶Li nucleus—this polarization was discovered in studying the polarization of recoil protons in the reaction ⁶Li(p, 2p)⁵He—cannot be described within the shell model assuming LS coupling. As might have been expected, the polarization of recoil protons knocked out from the S shells of the ⁶Li and ⁷Li nuclei comply well with the predictions obtained in the impulse approximation with allowance for the depolarization effect alone.     

Investigation of the external-magnetic-field dependence of polarization transfer in a 8Li-6Li disordered nuclear system

Random walks in disorderedmedia are studied by considering the example of the delocalization of nuclear polarization in an ensemble of ⁸Li beta-active nuclei produced in (n, γ) reactions induced by polarized thermal neutrons in LiF single crystals. The process is initiated by magnetic dipole-dipole interactions. It consists in polarization transfer from a primarily polarized ⁸Li nucleus to the closest (stable) ⁶Li nuclei and in subsequent polarizationmigration over 6Li nuclei, the return of the polarization in question to the ⁸Li nucleus being possible. In order to obtain information about the polarization of ⁸Li nuclei, the asymmetry of beta radiation from them was measured with respect to the external magnetic field H ₀. The process was studied until it reached the diffusion asymptotic regime. The concentration of ⁶Li was varied between 3% and 10%, while the field strength H ₀ was changed from 200 to 1200 G. It is shown that microscopic theory is in satisfactory agreement with the experimental results obtained in the way outlined above. A comparison with the investigation of the mathematically allied process of the Förster electricdipole transfer of localized excitons is performed.     

Quadrupole interaction of8Li and9Li in LiNbO3 and the quadrupole moment of9Li

The quadrupole interaction of nuclear spin polarized⁸Li (I=2) and⁹Li (I=3/2) in LiNbO₃ has been studied at room temperature. The polarization was achieved by optical pumping of a fast atomic beam with circularly polarized laser light. The atoms were implanted into a hexagonal LiNbO₃ single crystal and the quadrupole splitting ofβ-NMR spectra was measured. A ratio of ¦Q(⁹Li)/Q(⁸Li)¦=0.88(4) for the nuclear quadrupole moments was deduced, yielding a new value of ¦Q(⁹Li)¦=25.3 (9) mb for the quadrupole moment of⁹Li.     

Preservation of nuclear spin polarization of 12B in superfluid helium

Beams of unstable nuclei, ⁸Li and spin-polarized ¹²B, were introduced into superfluid helium and “snowballs”, aggregates of helium atoms surrounding the singly charged impurity ions, were formed through electrostriction. β-rays from the unstable nuclei encapsulated in the snowballs were detected after the snowballs were transported under an electrostatic field. It was found that approximately 20 % of the implanted ions formed snowballs. The spin polarization of ¹²B in snowballs was measured by β-NMR method. The first decisive evidence was obtained that the polarization was maintained throughout the lifetime of ¹²B (τ = 29 ms). The snowballs can be versatile environments for spectroscopic studies of unstable nuclei     

Spin exchange polarization and measurement of the hyperfine splitting of short-lived8Li

Free⁸Li (T _1/2=0.84 sec) atoms were polarized by spin exchange with optically pumped rubidium vapour. The⁸Li nuclei were produced by the reaction⁷Li(d, p)⁸Li in a thin LiF target. They recoiled into helium which was used as a buffer gas for optical pumping as well. Nuclear polarization up to 2% was detected by β-decay asymmetry. Rf transitions between hfs levels of the atomic ground state yielded the hfs separation ΔW=382.543(7) MHz. The nuclear spin assignmentI=2 was confirmed.     

Hartree-Fock cluster investigations of electronic structure and nuclear quadrupole interaction in the superionic conductor Li3N

The nuclear quadrupole interactions for⁷Li and¹⁴N nuclei are studied for lithium nitride crystal using the Hartree-Fock cluster procedure to obtain the electronic structure. The influence of the Madelung potential due to the ions outside the cluster was incorporated in a first-principle manner. Our results for the quadrupole coupling constants will be compared with experimental data and the results of a recent band calculation.     

β-NMR and nuclear spin diffusion in a spatially disordered subsystem

The results of theoretical and experimental investigations of delocalization of nuclear polarization in spatially disordered media are presented. The experiment is based on the measurement of a depolarization of β-active ⁸Li impurity nuclei (β-nuclei) in the spatially disordered subsystem of ⁸Li-⁶Li nuclei in LiF single crystals. The process is determined by the dipole-dipole interaction in this subsystem and by its dipole interactions with nuclei of the ⁷Li¹⁹F matrix. It is effective in a wide range of external magnetic fields H ₀ = 200–3000 G owing to proximity of g-factors. The kinetics of a depolarization of β-nuclei at the ⁶Li concentration c = 0.15–10.06% in fields H ₀ = 200 and 1210 G is investigated. A satisfactory explanation of the results is based on the numerical-analytical simulation of the process.     

Element 107

A new and transparent method for the analysis of recoil distance Doppler shift data is presented, which we call thedifferentialdecay curve method (DDCM). The DDCM can be used for singles as well as for coincidence plunger data and systematic errors can be discovered with it much easier than in the conventional analysis. In addition we propose a modification of the normal plunger which we call the differential plunger. With the differential plunger in principle it is possible to determine lifetimes from quantities measured at only one target to stopper distance. The DDCM was tested with lifetime data for¹²⁰Xe and¹²⁸Ba.     

Nuclear orientation measurements of the magnetic dipole moments of the 11/2− Isomeric states in129Xe,131Xe and133Xe

The low-temperature nuclear orientation technique was used to measure the magnetic moments of¹²⁹ mXe,¹³¹ mXe and¹³³ mXe implanted in iron by isotope separator. The magnitudes of the magnetic dipole moments, extracted from the gamma-ray anisotropy measurements areμ=?0.80(10)μ _N for^129m Xe,μ=?0.80(10)μ _N for¹³¹Xe andμ=?0.87(12)% for¹³³Xe. The results for these 11/2^? isomers agree with theoretical calculations by the spin polarization procedure using wave functions from the pairing-plus-quadrupole model.     

Emission of X-ray continua by bombardment of thick Al,Si and Ti targets with protons and14N ions

Using thick targets the continuous X-ray spectra arising in the collision systems Al+p (0.5–7 MeV), Si+p (0.6–6 MeV), Si+¹⁴N (6 MeV, 14 MeV), Ti+p(1 MeV) and Ti+¹⁴N (14 MeV) were measured by means of a Si(Li) detector. Total yields were derived and compared with numerical results of calculations for secondary electron and nuclear bremsstrahlung. For Si and Ti the continuous spectra from one and the same target bombarded with protons and¹⁴N ions of equal velocity were investigated. Drastic deviations from theZ ₁ ² scaling have been found. They could be attributed to contributions of MO radiation originating by recoil of target atoms. The influence of characteristic line profiles on the measured spectra is also discussed.     

One-nucleon spectroscopy of light nuclei

The capabilities and limitations of the conventional many-particle shell model and modern potential cluster models are discussed. New revaluated and more accurate calculations of one-nucleon spectroscopic characteristics of the light nuclei of 1p shell are presented. In many-particle shell model for nuclei with A = 7, 9, 11, 13, and 15 nucleon partial widths of highly excited states with the isotopic spin T = 3/2 were calculated both for “allowed” and “forbidden” transitions. One-nucleon spectroscopic factors were calculated in threebody multicluster models of ⁶Li{αnp}, ⁸Li{αtn}, and ⁹Be{ααn} nuclei. For isobar-analogue nuclei ⁷Li and ⁷Be, the spectroscopic proton S _p and neutron S _n factors for transitions to the ground and excited states of corresponding residue nuclei of the triplet ⁶Li-⁶He-⁶Be were calculated in the framework of binary potential αtand ατ models. Integral, differential and polarization characteristics of photonuclear processes ⁷Li(γ, n ₀)⁶Li, ⁶He(p, γ_{0 + 1})⁷Li, ⁷Li(γ, p ₀)⁶He, and ⁹Be(γ, p _{0 + 1})⁸Li were calculated in this approach.     

Kinetics of the polarization transfer in spatially disordered spin systems: Depolarization of impurity beta-active nuclei

We performed theoretical and experimental studies of the delocalization of the nuclear polarization of impurity beta-active nuclei ⁸Li in the spatially disordered system of ⁶Li nuclei in LiF single crystals. The process is controlled by the dipole-dipole interaction of nuclear magnetic moments with other nuclei (⁷Li, ¹⁹F) in the crystal. It is effective in a wide range of magnetic fields H ₀ = 150–3000 G as a result of a unique proximity of the g-factors of ⁸Li and ⁶Li nuclei: (g(⁸Li) − g(⁶Li))/g(⁶Li) = 0.0057. The kinetics of the ⁸Li depolarization is measured for an ⁶Li concentration of 0.15%–10.06% and in the field H ₀ of 200, 692 and 1210 G. A satisfactory explanation of the results is obtained on the basis of a numerical-analytical simulation of the process.     

Nuclear spin dependence of polarization enhancement by multi-tilted foils studied by short-lived beta-emitters8B and12B

In order to study the basic mechanism of polarization enhancement realized by the multitilted foil technique, nuclear polarization of short-lived beta-emitter⁸B(T_1/2=769 ms,I =2⁺) was induced. Utilizing up to ten tilted foils, the polarization enhancement was measured as a function of the foil numbers. The observed enhancement for⁸B was combined with the previous results for¹²B(I =1⁺,T _1/2=20 ms) which has the same atomic configurations but different nuclear spin. Analyzing these results in the framework of the classical vector model, the essential features of the enhancement depending on the nuclear spin was disclosed.     

The Formation of Lithiated Ti-Doped α-Fe2O3 Nanocrystalline Particles by Mechanical Milling of Ti-Doped Lithium Spinel Ferrite

Perturbed Angular Correlation method has been used to study the hyperfine magnetic field in the Heusler alloy Pd₂MnSb(Sn). Ion implantation of the recoil ¹¹¹In nuclei following heavy ion nuclear reactions ¹⁰⁸Pd(⁷Li, 4n)¹¹¹In and ¹⁰⁸Pd(⁶Li, 3n)¹¹¹In has been used to great advantage in the present case resulting in large implantation efficiency. Only a few hours of irradiation time with moderate beam current of the order of 400–500 nA resulted in sufficient implanted ¹¹¹In activity on the sample for good quality measurements. The hyperfine field was measured at ¹¹¹Cd probe nuclei substituting Mn and Sb(Sn) sites as a function of temperature. The fraction of ¹¹¹Cd nuclei occupying Mn atom sites was found to increases with the annealing of sample at higher temperatures.     

Hyperfine interactions of polarized β-emitting12B and12N in Si,Ge, and GaP

Using a nuclear reaction, the polarized short-lived -emitters¹²B and¹²N were implanted into Si, Ge, and GaP crystals. Hyperfine fields were studied via both NMR techniques and an external magnetic holding field H_ext on-off techniques in an H_ext range 0–8 kG and a temperature range 100–1000 K. No significant NMR signal was observed between 2 and 30 MHz for¹²N in Si and Ge despite maintenance of 60% polarization at T100 K and H_ext>4 kG, whereas for¹²B in Si at T>800 K almost full polarization was found at the Larmor frequency.     

Theoretical study of deuteron polarization in γ+d → π0+d

The state of polarization of the recoil deuteron in γ+d → π⁰+d on unpolarized and target polarized deuterons is analyzed in detail. A new set of statistical tensors is introduced to describe non-oriented systems, such as the recoil deuteron in γ+d → π⁰+d, and their relationships to the vector and tensor polarization parameters are established. The new statistical tensors reduce, in the case of oriented systems, to Fano's statistical tensors. Numerical results are computed using two different deuteron models for polarized photon asymmetry, polarized target asymmetry and the vector and tensor polarizations of the recoil deuteron, and these are presented at various c.m. pion production angles at different energies in the region of the first π-N resonance. The study of these parameters is suggested as a promising source of information on isoscalar pion photoproduction amplitudes.     

Reaction cross section measurements of the neutron-rich isotopes8,9,11Li at 80 MeV/nucleon

Total interaction cross sections have been measured for⁸Li on C and Pb targets, for⁹Li on C, Al, Cu, Sn and Pb targets as well as for¹¹Li on C, Sn and Pb targets. For each beam, we also used a plastic scintillator as target. The measurements with the scintillator targets are used to extract reduced nuclear radii of the lithium isotopes. These radii are then used for the calculation of the nuclear part of the total cross section for the other targets. The total electromagnetic-dissociation (EMD) cross sections have been deduced and are compared to different models. A strong target-charge-dependent EMD cross section is measured for¹¹Li reaching 2.96 _–0.82 ^+0.84 b for the Pb target. In the⁹Li case, a large EMD cross section for high-Z targets has been observed which amounts to 0.75 ± 0.45 b for the Pb target. The EMD cross sections of both,⁹Li and¹¹Li, may be understood by the giantdipole-resonance model.This work forms part of the PhD Thesis of B. Blank