Penetration effects in111Cd

Penetration effects in the conversion process of the 7/2⁺→5/2⁺, 171 keV and 5/2⁺→1/2⁺, 245 keV transitions in¹¹¹Cd have been investigated. The decay of¹¹¹In has been studied to deduce the relative intensity of theK-conversion lines I_K(171)/I_K(245) and the ratioI _K(245)/I _L+M... (245). The values obtained for the penetration parameters of the two transitions are 0≦λ(171)≦2.3 and ?0.4≦λ ₁(245)≦1.9.     

Innere Konversion der 161 keV- und 223 keV-Übergänge in133Cs

Using a Ge(Li)-Si (Li)-spectrometer the 161 keV and 223 keV transitions of¹³³Cs were investigated. TheK-conversion coefficients were deduced to beα _K =0.205±0.007 andK-conversion coefficients were deduced to beα _K =0.0743±0.0043, respectively. TheK/L ratio for the 161 keV transition is 4.72±0.37. From theK-conversion coefficients were deduced to beα _K -values,M1 penetration factors ofλ=8.6±3.4 andλ=7.8 _?2.8 ^3.0 were deduced which are inconsistent with known data from angular correlation experiments (λ=40±10 andλ=90±13). The penetration factor fromK/L-measurement for the 161 keV-transition isλ=52±19. A theoretical reinvestigation of the formulas used in the literature appears recommendable. Furthermore, theK/L ratio of the 1770 keV transition of²⁰⁷Pb was determined experimentally to be 5.52±0.54.     

High resolution studies of transitions in the decay chain146Gd to146Eu to146Sm

Transitions in¹⁴⁶Eu and¹⁴⁶Sm were studied using a double-focussing beta-ray spectrometer and a Ge(Li) detector. Internal conversion and gamma-ray intensities were determined. The internal conversion spectrum of the three 155, 115 and 116 keV cascading transitions in¹⁴⁶Eu was studied for all subshells.K-,L- andM-subshell ratios were determined andE2/M1 mixing ratios were deduced for these three transitions. Intensities from theN- andO+P-shells were determined and compared to theoretical calculations. All internal conversion intensities were found to be in agreement with theoretical data for pureM1 character with smallE2 admixtures for all the three transitions. Selected parts of the internal conversion spectrum of the transitions in¹⁴⁶Sm were restudied at 0.06% momentum resolution. This study was mainly concentrated on four transition doublets feeding and deexciting the close lying levels at 1,380 and 1,381 keV. A new transition with 702.20 keV energy was detected in the 702–703 keV transition group. Internal conversion coefficients were deduced using reported gamma-ray intensities. Multipole characters of the transitions were deduced and used as a basis for a discussion of the spins and parities of the lower lying excited states of¹⁴⁶Sm.     

Search for a 11/2−→3/2+ M 4 transition in141Sm

The electromagnetic decay of the 11/2^{? 141m} Sm is investigated. Internal conversion electron and X-ray-conversion electron coincidence measurements indicate that the state undergoesβ ⁺ and electron capture decay with 99.69% strength and the remaining 0.31% goes to a 174.2±0.3 keVM4 transition. TheK/L conversion electron intensity ratio for the transition is measured to be 1.7±0.4. The energy of the 11/2^? is established at 175.8±0.3 keV above the 1/2⁺ ground state in¹⁴¹Sm. Systematics of theM4 transitions in theN=79 and 81 isotones are discussed.     

Internal conversion at the higher shells in the decay of113* In (100 min)

The ratios of the conversion coefficients at the higher shells and subshells were measured in the 391,7 keV isomeric transition of¹¹³In. On the basis of a computer analysis of theL subshell conversion lines it can be stated that the transition has anM4 character and the most probable value of theE5 admixture is zero. TheL/M andM/N conversion ratios show a good agreement with the recent calculations of Hager and Seltzer and Dragounet al.     

The odd-parity level at 687.59 keV in236U

The spin-parity of the 687.59 keV level in²³⁶U populated in the decay of²³⁶Np is determined to be 2^? in disagreement with recent 1^? assignments from reaction data, but in accordance with previous radioactive²³⁶Np decay studies. The 687 keV ground state transition is shown to have a pureM2 character. The 642 keV 2^?→2⁺ transition hasE1:M2:E3 mixing ratios of 64∶30∶6. The half-life of the 2^? state is 3.78 ± 0.09 ns. The hindrance factor of the E1-part fits an E1 transition withΔK=2, theM2-part has the same transition rate as the M2 transitions in the neighbouring²³⁷Np nucleus and the E3-part is enhanced by two orders of magnitude relative to the Weisskopf estimate. The data are compared to analogous transitions in the rare earth region.     

Penetration effects in the internal conversion process of the 204 keV transition in205Tl

Penetration effects have been detected in²⁰⁵Tl by measuring theK, L and (M+N+...) internal conversion coefficients of the 204 keV, 3/2⁺→l/2⁺ transition. From the resulting values α _K =0.29±0.04, α _L =0.132±0.006 and α _M+N+...=0.0397±0.0034 the penetration parameter and the mixing ratio have been deduced to be λ=13.1±2.7 andδ ²=1.40±0.46, respectively.     

Nuclear structure effect on internal conversion ofl-forbidden transitions in139La,141Pr and203Tl

Accurate experimental internal conversion data have been used to study the effect of nuclear penetration in the case of thel-forbidden transitions in¹³⁹La (165.8 keV),¹⁴¹Pr (145.4 keV) and²⁰³Tl (279.2 keV). The nuclear penetration parameterλ and theE2/M 1 mixing ratioδ ² have been deduced by graphical analysis. Following results were obtained:λ=2.8±1.3,δ ² =(8.4 _?8.4 ^+14.0 )·10^?4 for¹³⁹La,λ=1.2±0.6,δ ²=(4.8±0.5)·10^?3 for¹⁴¹Pr, andλ=6.4±1.1,δ ²=1.36±0.12 for²⁰³Tl.     

The effectiveg s factor for the odd proton153Sm nucleus determined by the internal conversion processes

TheK/L ₃,L ₁/L ₃,L ₁/L ₂ andL ₂/L ₃ conversion ratios for the 103 keV transition in¹⁵³Sm were measured by means of a high-resolution π√2 electron spectrometer. The values of theM1 conversion penetration parameter λ=5.0 _?0.7 ^+0.6 and the mixing ratio δ²=0.144±0.006 are deduced. By comparing the experimental penetration parameter with the value obtained from Nilsson model calculations the effective spin gyromagnetic ratio is found to be $$g_s^{eff} = \left( {3.7\begin{array}{*{20}c} { + 0.4} \\ { - 0.5} \\ \end{array} } \right)\mu _n .$$      

Relative internal conversion electron intensities of the 113 keV transition in177Hf

The intensities of the internal conversion lines of the 113 keVM1 +E2 transition in¹⁷⁷Hf have been measured. From comparison with theoretical conversion coefficients the transition has been found to be (95.2 ± 0.5)%E2 corresponding to ¦δ¦=4.5 ± 0.3. The theoreticalL _I andM _I conversion coefficients used in the comparison have been increased by 5% according to the result that for pureE2 transitions in the deformed region theL _I/L _II,L _I/L _III,M _I/M _II, andM _I/M _III theoretical ratios are too low (～5%). Moreover, the present result indicates that theL _II/L _III andM _II/M _III ratios obtained from the tabulations by Hager and Seltzer and from the computer program by Pauli are too high (1–2%).     

Determination of theL-shell conversion coefficient for the 26 keV Mössbauer transition in161Dy

TheL-shell conversion coefficient of the 26 keV Mössbauer transition in¹⁶¹Dy has been determined to be α_L=2.4 _?0.2 ^+0.3 by coincidence techniques using high resolution Ge(Li) and Si(Li) detectors. With theoretical values for theM- andN-shells the total conversion coefficient is calculated to be α_tot=2.9 _?0.2 ^+0.3 .     

In-beam spectroscopy of thek π=0− bands in230–236U

TheK ^π=0^? bands in even uranium nuclei were studied in the compound reactions²³¹Pa(p, 2n)²³⁰U,^{230, 232}Th(α,2n)^{232, 234}U and²³⁶U(d, pn)²³⁶U. In-beamγ-rays were measured in coincidence with conversion-electrons, which were detected with an iron-free orange spectrometer. The negative-parity levels are observed up to intermediate spins (I<13^?). In addition, the 1^? and 3^? levels in²³⁰U were confirmed by a decay study with an isotope separated²³⁰Pa source. For the heavier isotopes (A≥232) the properties of theK ^π=0^? bands (energies andγ-branchings) are consistent with a vibrational character of these bands. For²³⁰U theK ^π=0^? band lies at rather low energy (E(1^?)=367 keV), and the level spacings within this band are very similar to those of the isotones²²⁸Th and²²⁶Ra, which might indicate the onset of a stable octupole deformation.     

E1-M2-E3 mixing of the 1241.7 keV transition in147Yb

The half-life of theI,K ^π=2, 2^? state at 1318 keV in¹⁷⁴Yb has been measured in the¹⁷³Yb(n, γ) reaction to be 0.486±0.015 ns. This half-life determines the absolute transition probabilities of the gamma-ray transitions to the ground state rotational band yielding the following hindrance factors relative to the Weisskopf estimate:F _W(M 2; 2, 2^?→0, 0⁺)=350;F _W(M2; 2, 2^?→2, 0⁺)≧77F _W(M 2;2, 2^?→4, 0⁺)>740;F _W(E 1; 2, 2^?→2, 0⁺)=4.5×10⁶;F _W(E 3; 2, 2^?→2, 0⁺)≈0.1;F _W(E 3; 2, 2^?→4, 0⁺)≈0.4. These data are compared to analogous transitions in neighboring nuclei.     

States inN=80140Nd populated in the decay of140Pm

The level structure of theN=80,¹⁴⁰Nd has been investigated through the beta decay of^140m Pm and^140g Pm, whose decay half-lives were measured to be 5.95±0.05 min and 9.1±0.5 sec, respectively. Decay schemes for the two isomers have been constructed fromγ-ray measurements. With the help of the beta decayft values and internal conversion electron measurements, spins and parities were deduced for levels in¹⁴⁰Nd. Among the levels a 7^? state at 2222.0 keV and a 5^? state at 2273.3 keV are identified as two-neutron quasiparticle states. The (ie233-01) for^140m Pm and^140g Pm have been deduced as 7^? and 1⁺, respectively. From beta end-point measurements, the decay energies of the two isomers have been determined asQ _EC=6.48±0.07 MeV^140m (Pm) andQ _EC=6.08±0.10 MeV (^140gPm). The results are discussed in the light of nuclear systematics of theN=79 and 80 isotones.     

Winkelkorrelationsmessungen an88Sr

The γγ ande _? ^KL γ directional correlations have been measured for the (898–1836) keV cascade in⁸⁸Sr following the decay of⁸⁸Y. The observed correlation coefficients areA ₂₂(γγ)=?0.0784±0.0042 andA ₂₂(e _? ^KL γ)=0.0102±0.0046. The γγ experiment is consistent with a mixing ratio δ(γ)=0.009±0.005 for the 898 keV transition. Using the result of thee _? ^KL γ experiment the most probable value of the ratio of the penetration matrix element to the normal γ-ray matrix element was determined to be η=0.03±0.30 showing a normal conversion process. This penetration parameter agrees with a hindrance factorH _W(E1)=2.1 · 10^?3 for theE1 transition.     

Decay studies of101m Rh and101g Rh

The level structure of¹⁰¹Ru has been investigated from the decays of^101m Rh and^101g Rh. For the gamma-ray measurements Ge(Li) detectors with effective volumes of 24 and 43 cm³ were used for singles and coincidence work, and several new transitions were observed. Conversion electron spectra from the^101m Rh decay were investigated with a 50 cm double-focussing beta spectrometer.K-conversion coefficients were determined by combining internal conversion and gamma-ray intensities. For the stronger transitions probable multipolarity assignments have been obtained from these coefficients and also fromK/L andL-subshell ratios. All transitions observed were fitted into a decay scheme, in which tentative spin-parity assignments of all states are given.     

Properties of isomeric states and the πd 3/2-vi 13/2 multiplet in194Au

The level structure of¹⁹⁴Au has been studied by observing prompt and delayedγ-rays following¹⁹⁴Pt(p,n) and¹⁹⁵Pt(p,2n) reactions. The conversion electron andγ-ray spectra from the decay of the 0.42s (10^?) and 0.60s (5⁺) isomers at 476 keV and 107.4 keV, respectively, have been measured using the He-jet method. The half-lives of the 6⁺ (278.2 keV, 1.1±0.4 ns), 7⁺ (224.6 keV, 2.6±0.2 ns) and 8⁺ (406.8 keV, 2.9±0.4 ns) members of theπd _3/2-vi _13/2 multiplet have been obtained from the time distributions between cyclotron beam pulses andγ-rays depopulating these levels. A calculation made assuming a pure two-particle configuration for the multiplet predicts very well theB(E2) values for the transitions between the levels of this multiplet but the calculatedB(M1) values are not in agreement with experimental results.     

A Si(Li) detector system for conversion coefficient measurements and application to the decays of51Cr and87Y

An electron detector system with a 3 mm × 100 mm² Si(Li) detector with a cooled FET and vacuum air lock for changing sources was constructed. The absolute efficiency was measured as a function of energy for use in the measurement ofK conversion coefficients. With the Si(Li) and a Ge(Li) detector, theK conversion coefficient of the 320 keV transition in⁵¹V was measured to be 0.00156 ± 0.00008 where theK conversion coefficients of the 661 and 279 keV transitions in¹³⁷Ba and²⁰³Tl were used as standards. From absolute detection efficiency measurements, theK conversion coefficients of the 388 and 483 keV transitions in⁸⁷Sr were measured to be 0.16 ± 0.02 and 0.0024 ± 0.0003, respectively.     

Experimental evidence for anomalous L/M conversion ratio of the 2+→0+ transitions in some deformed even-even nuclei

TheL-subshell andM conversion coefficients ratios of the 2⁺→0⁺ transitions in some deformed even-even nuclei have been determined using a high resolution iron free double focusing beta-ray spectrometer. All possible uncertainties in these measurements have been minimized and properly evaluated. TheL ₁+L ₁₁/L ₁₁₁ ratios for the 2⁺→0⁺ E2 transitions in Dy¹⁶⁰, Er¹⁶⁶, Yb¹⁷⁰, Hd¹⁷⁶ and W¹⁸² are found to be in agreement with the theoretical ones within an experimental error of about 4%. However, large deviations from the theory of about two order of magnitude are observed forL/M conversion ratios. The deviations indicate the possibility of considerable approximation in the theoretical calculation of theM-internal conversion coefficients.     

Gamma-ray-L-x-ray directional correlations in182W

Directional correlations between gamma radiation andL x-rays in¹⁸²W have been measured. The x-rays are emitted following the internal conversion process of the 100.1 keV 2⁺ → 0⁺ transition. The experimental results for anisotropies involving gamma radiation emitted in the 1189.0 keV transition andL x-rays are A(γ?L _l )=?0.073(27),A(γ?L _α)=?0.0102(45),A(γ?L _β)=?0.0031(35), andA(γ?L _γ)=?0.007(13). The value deduced for the coefficientU ₂(e) pertaining to the converted transition isU ₂(e)=0.52(8) in reasonable agreement with the theoretically expected value 0.410. A note is given on the use of internal conversion radial matrix elements.