Low-threshold mid-infrared optical parametric oscillation in periodically poled LiNbO3 synchronously pumped by a Ti:sapphire laser

We report the generation of tunable high-repetition-rate optical pulses in the mid-infrared using synchronously pumped parametric oscillation in periodically poled LiNbO₃ (PPLN). Using a Kerr-lens-mode-locked Ti:sapphire laser as the pump source and a PPLN crystal incorporating grating periods of 21.0–22.4 μm, we have achieved wavelength conversion in the -–4 6μm spectral range in the mid-infrared. The use of a semi-monolithic cavity design and hemispherical focusing has permitted pulse generation in the strong idler absorption region of PPLN, resulting in a simple, compact, all-solid-state configuration with a pump power threshold as low as 17 mW and mid-infrared idler powers of up to 64 mW at 9% extraction efficiency. Signal output powers of up to 280 mW at 35% extraction efficiency are available over the -–1.004 1.140μm spectral range at 80.5 MHz and pulse repetition rates at harmonics of the fundamental frequency up to 322 MHz have also been obtained. Received: 5 December 2000 / Revised version: 23 January 2001 / Published online: 27 April 2001     

Synchronously pumped femtosecond optical parametric oscillator based on AgGaSe2 tunable from 2 μm to 8 μm

The operation of a continuous-wave mode-locked silver gallium selenide (AgGaSe₂) optical parametric oscillator (OPO) is reported. The OPO was synchronously excited by 120-fs-long pulses of 1.55-μm radiation at a repetition rate of 82 MHz. The 1.55-μm radiation is generated by a noncritically phasematched cesium-titanyl-arsenate (CTA)-OPO pumped by a mode-locked Ti:sapphire laser. The AgGaSe₂-OPO generates signal and idler radiation in the range from 1.93 μm to 2.49 μm and from 4.1 μm to 7.9 μm, respectively. Up to 67 mW of signal wave output power has been obtained. The experimentally determined pulse duration and chirp parameters are in reasonable agreement with results from a numerical model taking into account group velocity mismatch, group velocity dispersion, self phase modulation, and chirp enhancement. Received: 6 August 1999 / Revised version: 4 October 1999 / Published online: 3 November 1999     

Optical parametric oscillators for high pulse energy and high average power operation based on large aperture periodically poled KTP and RTA

We report on optical parametric oscillators (OPOs) based on large aperture periodically poled KTiOPO₄ (PPKTP) and RbTiOAsO₄ (PPRTA) pumped with high pulse energy and high average power Q-switched solid-state lasers. The OPOs were pumped with 1064-nm pulses of a diode-pumped Nd:YVO₄ laser at 20 kHz repetition rate. The emitted signal wavelengths were 1.72 μm and 1.58 μm and the idler wavelengths were 2.79 μm and 3.26 μm, respectively. Pumping the PPKTP OPO with 7.2 W and the PPRTA OPO with 8 W average power, 2 W and 1.3 W total OPO output powers were generated. Two-dimensional measurements of the total OPO output power, the signal wavelength and the signal bandwidth in dependence on the crystal location indicated a good uniformity of the quasiphasematching structure over the entire 3-mm-thick crystals. This allowed pumping with larger pump beams and therefore with pulse energies of tens of millijoules. Pumping with different flash-lamp-pumped lasers, good OPO performance and high output pulse energies could be achieved for all pump lasers. Maximum input pulse energies of 56 mJ gave output pulse energies of as much as 18 mJ. The temperature tuning behaviors of both OPOs were measured, showing excellent agreement with calculated temperature tuning curves. New equations for temperature dispersion in RTA are presented. These results show that large-aperture PPKTP and PPRTA crystals are well suited for tunable nanosecond OPO operation with multi-watt average pump power and several tens of millijoules pump pulse energies. Received: 7 September 2001 / Published online: 7 November 2001     

Mid-infrared ZGP OPO pumped by near-degenerate narrowband type-I PPKTP parametric oscillator

The total pulse energy of the signal and idler in a near-degenerate type-I periodically poled KTiOPO₄ (PPKTP) optical parametrical oscillator (OPO) was spectrally confined within a 2 nm spectral bandwidth at 2.13 μm. This was achieved by using a volume Bragg grating as the output coupler. Both the signal and the idler from the PPKTP OPO were then simultaneously used to pump a mid-infrared ZnGeP₂ (ZGP) OPO. The 2 nm bandwidth was narrower than the ZGP crystal acceptance bandwidth and, thus, made efficient conversion in the second OPO possible. A total slope efficiency of 10% from 1.06 μm to the 3.5–5 μm region was demonstrated, generating 250 μJ in the mid-IR with only 3.6 mJ of 1.06 μm pump energy. This corresponds to a Nd:YAG pump to mid-IR conversion efficiency of 7%. PACS 42.65.Yj; 42.72.Ai; 42.40.Eq     

8.30 μm singly resonant ZnGeP2 optical parametric oscillators pumped by a Tm,Ho:GdVO4 laser

A single resonator 8.30 μm ZnGeP₂ (ZGP) optical parametric oscillators (OPO) was reported in the paper. The OPO was pumped by a 10.2-W Tm,Ho:GdVO₄ laser at 8 kHz in a Q-switch mode, a 170-mW idler was obtained at 8.30 μm, and the output power of the idler and signal wave was 1.0 W, corresponding to an optical-optical conversion efficiency of 10.3% and a slope efficiency of 20.9%. Tm,Ho:GdVO₄ laser was pumped by a 30-W fiber-coupled laser diode (LD) at the center wavelength of 801 nm. The output wavelength of Tm,Ho:GdVO₄ laser was at 2.05 μm, and the energy per pulse of 1.28 mJ in 18 ns was achieved at 8 kHz with the peak power of 71.1 kW.     

A compact,widely tunable intracavity PPLN optical parameter oscillator driven by an Nd:YAG/Cr:YAG composite crystal laser

Based on periodically poled lithium niobate (PPLN), a mini intracavity optical parameter oscillator (IOPO) driven by an diode-end-pumped composite Nd³⁺:YAG/Cr⁴⁺:YAG laser was demonstrated. The PPLN wafer has 20 domain reversal periods from 27.8 to 31.6 μm with a step of 0.2 μm between the neighbor periods. The output signal laser of OPO can be widely tunable in the range of 1402–1676 nm by changing the period at a certain temperature of 50°C. Under the diode pump power of 14 W, the maximum average output power of 600 mW at 1534 nm with pulse width of 2.0 ns and repetition rate of 16 kHz was obtained, corresponding to a peak power of 18.7 kW and a single pulse energy of 37.5 μJ, respectively.     

Estimation of required parameters for detection of small smoke plumes by lidar at 1.54 μm

Parameters of eyesafe lidar at 1.54 μm for detection of small plumes of smoke from burning wood or oil have been evaluated. It was assumed that a diode-pumped solid-state Er:glass laser at 1.54 μm or a Nd:YAG laser with a Raman cell or optical-parametric oscillator is used as a light source and that detection of backscattered light is performed with an avalanche photodiode. Ash and soot particle size distributions were taken from experiments. A backscattering coefficient at 1.54 μm for various source of smoke was estimated. In computing the laser energy, range between lidar and smoke, receiver optics diameter, fuel mass burned in unit time, fire source radius, laser pulse duration and visibility were varied. Results of the computations enabled estimation of the required laser energy, which ranges from 0.05 to 1400 mJ depending on the parameters. Received: 5 January 2000 / Revised version: 3 March 2000 / Published online: 11 May 2000     

High-energy, fourth-harmonic generation using CO2 lasers

2 laser to 2.38 μm has been studied experimentally by using tandem AgGaSe₂ and ZnGeP₂ crystals. Up to 24 mJ per pulse of 2.38-μm radiation at a 10% overall conversion efficiency has been achieved with a mode-locked pulse format. A computer model was also developed and its predictions are in reasonable agreement with our experimental data. Received: 6 July 1997/Revised version: 8 December 1997     

Compact X-ray radiograph based on a plasma gun

The results of the experiments on the formation of a plasma emitter with small spatial dimensions for pulsed radiography in the soft X-ray spectral range are presented. Emitting hot plasma was formed as a result of compression of the plasma jet by a current pulse with amplitude I _m = 215 kA and rise time T _fr = 200 ns. For the jet formation, we used a plasma gun based on the arc discharge (I _m = 8.5 kA and T _fr = 6 μs) initiated by breakdown over the surface of a dielectric in vacuum. The experiments were carried out with aluminum, tin, copper, and iron plasma jets. A single emitter, i.e., point Z-pinch (PZ-pinch), was formed when an interelectrode gap of a high current generator of 1.3–1.5 mm was used. The smallest spatial dimensions of the emitting region were obtained with the use of aluminum and tin. For a tin jet, the diameter of the emitting region was 7 ± 2 μm and its height was 17 ± 2 μm. The emission pulse duration at half-height was 2–3 ns. The total emission yield per pulse in the spectral range 1.56–1.90 keV was 30–50 mJ for the aluminum pinch and 10–30 mJ for the tin pinch. The developed method makes it possible to carry out radiographic examination of microobjects (including biological ones) 1–1000 μm in thickness, with spatial (10–20 μm) and time (2–3 ns) resolution.     

A Raman laser system for multi-wavelength satellite laser ranging

~~A Raman laser system for multi-wavelength satellite laser ranging@K.Hamal$Czech Technical University in Prague,Czech @I.Prochazka$Czech Technical University in Prague,Czech @J.Blazej$Czech Technical University in Prague,Czech1. Yang Fumin, Chen Wanzhen, Zhang Zhongping et al., Satellite laser ranging experiment with sub-centimeter single-shot ranging precision at Shanghai Observatory, Science in China, Ser. A, 2002, 32(10): 935-939. 2. Degnan, J. J., Millimeter accurac…     

Efficient continuous wave and Q-switched operation of a dual-end-pumped <Emphasis Type="Italic">c</Emphasis>-cut Tm:YAP laser

An efficient continuous wave (CW) and Q-switched c-cut Tm:YAP laser is reported in this letter. With the dual-end-pumped convex-concave resonator, CW output power up to 13.6 W at 1.99 μm was obtained under a total incident pump power of 50 W. The corresponding slope efficiency was 34.3% and conversion efficiency was 27.2%. The active Q-switched operation of the laser had an average output power of 12.5 W at 10 kHz pulse repetition frequency, with a minimum pulse width of 126 ns. With 6 kHz pulse repetition frequency, the maximum pulse energy of 1.6 mJ was obtained. In addition, using the Tm:YAP laser as a pumping source for gain-switched Cr:ZnSe laser, as much as 4 W output power in the wavelength range of 2.5–2.6 μm was obtained.     

An all-diode-laser-based, dual-cavity AgGaS2 cw difference-frequency source for the 9–11 μm range

2 ) nonlinear crystal is reported. The device uses a standing-wave dual-resonator scheme to enhance both near-infrared lasers. For 7 mW of 778.2-nm and 275 mW of 842.5-nm input powers, 40 nW of 10.2-μm radiation is generated by a preliminary setup. A μW-level range output power is expected after optimization of the device optical components. This compact tunable source will allow Fabry–Pérot high-resolution Doppler-free spectroscopy of spherical molecules, such as OsO₄ or SF₆, in the 9–11 μm range as an alternative source to frequency-stabilized CO₂ lasers. Received: 17 March 1998     

Experimental investigation of pulse diodes side-pumped 2 μm Tm:YAG lasers

The free running and Q-switched operation of 2 μm Tm:YAG lasers side-pumped by pulse laser diodes were reported. In the free running mode the maximum output energies were 102.5 mJ at 1 Hz and 94.6 mJ at 10 Hz, respectively. With an acousto-optic modulator in the laser resonator, 21 mJ 2 μm Q-switched pulse was obtained, with a pulse width of about 330 ns. The dependences of the output energy and the efficiency on the laser resonator parameters were investigated.     

A 9.5-W 82-MHz-repetition-rate picosecond optical parametric generator with cw diode laser injection seeding

We report on an injection-seeded 9.5-W 82-MHz-repetition-rate picosecond optical parametric generator (OPG) based on a 55 mm long crystal of periodically poled lithium niobate (PPLN) with a quasi-phase-matching (QPM) grating period of 29.75 μm. The OPG is excited by a continuously diode pumped mode-locked picosecond Nd:YVO₄ oscillator-amplifier system. The laser system generates 7 ps pulses with a repetition rate of 82.3 MHz and an average power of 24 W. Without injection-seeding the total average output power of the OPG is 8.9 W, which corresponds to an internal conversion efficiency of 50%. The wavelengths of the signal and idler waves were tuned in the range 1.57–1.64 μm and 3.03–3.3 μm, respectively, by changing the crystal temperature from 150 °C to 250 °C. Injection seeding of the OPG at 1.58 μm with 4 mW of single frequency continuous-wave radiation of a distributed-feedback (DFB) diode laser increases the OPG output to 9.5 W (53% conversion efficiency). The injection seeding increases the pulse duration and reduces the spectral bandwidth. When pumped by 10 W of 1.06 μm laser radiation, the duration of the signal pulses increased from 3.6 ps to 5.5 ps while the spectral bandwidth is reduced from 4.5 nm to 0.85 nm. Seeding thus improved the time-bandwidth product from 1.98 to a value of 0.56, much closer to the Fourier limit. Received: 29 April 2002 / Published online: 8 August 2002     

High-efficiency,high-repetition-rate,temperature-tuning optical parametric oscillator based on periodically poled MgO-doped lithium niobate

We report a compact and viable source of high-efficiency, high-repetition-rate, temperature-tuning, mid-IR optical parametric oscillator (OPO) based on periodically poled MgO-doped lithium niobate (PPMgOLN) pumped by a homemade high power AOM Q-switched Nd:YVO₄ laser centered at 1.064 μm. With an optimal plane-concave resonator configuration, average output power of 5.7 W at 2.73 μm was obtained when the pump power was 25 W at the repetition rate of 80 kHz. The conversion efficiency from the 1.064 μm laser to the 2.73 μm laser was 22.8%. Temperature tuning of the OPO yielded a signal wavelength range from 1.67 to 1.75 μm and an idler wavelength in the range of 2.72 to 2.92 μm.     

Efficient and widely step-tunable terahertz generation with a dual-wavelength CO<Subscript>2</Subscript> laser

Coherent terahertz radiation in a widely step-tunable range of 72.3–2706 μm (0.11–4.15 THz) has been generated in GaAs crystal by difference-frequency generation using one CO₂ laser with dual-wavelength output. The peak power of THz pulse reaches 35 W at the wavelength of 236.3 μm, which corresponds to a pulse energy of 2.1 μJ. An average power of 10 μW has been achieved when working repetitively. This efficient terahertz radiation source is more compact and widely tunable than other THz sources pumped by CO₂ laser.     

CO<Subscript>2</Subscript> laser oscillating in the range of 16 μm

The ability of a CO₂ laser to oscillate in the range of 16 (14) μm at room temperature was investigated experimentally and theoretically. The output energy per pulse was ~60 mJ at peak power of ~50 kW. It was necessary to minimize not only harmful losses but also useful ones in both channels 00⁰1–02⁰0 and 02⁰0–0110 and to increase the input energy, i.e., the density of free electrons in the discharge, in order to increase the peak power and energy of 16-μm radiation. The highest values of peak power and energy of radiation were reached at different pressures of the active mixture. The rotational bottleneck effect limiting the peak power and energy of oscillation was important at rather low pressures of the active medium. Oscillation at the R12 line is more preferable than that at the P12 line for use as 9.6-μm dumping radiation.     

Stimulated rotational Raman scattering at multiwavelength under tea CO2 laser pumping with a multiple-pass cell

Stimulated rotational Raman scattering (SRRS) at multiwavelength pumped by TEA CO₂ laser was demonstrated in this paper. Raman mediums were cooled by liquid-N₂ and a multiple-pass cell (MPC) with 25 passes was designed and used. When the para-H2 was pumped by single-longitudinal-mode (SLM) circular polarized TEA CO₂ laser on 10P(20), 9P(20), and 10R(20), 50 mJ 16.95 μm, 350 mJ 14.44 μm, and 536 mJ 16.9 μm radiations were obtained, corresponding to energy conversion efficiency of 1.2, 11.7, and 13.4%, respectively. When the ortho-D₂ was pumped by CO₂ laser on 10R(18), 108 mJ 12.57 μm Raman laser was obtained with energy conversion efficiency of 2.9%.     

Table-top kHz hard X-ray source with ultrashort pulse duration for time-resolved X-ray diffraction

The interaction of ultrashort laser pulses with solid state targets is studied concerning the production of short X-ray pulses with photon energies up to about 10 keV. The influence of various parameters such as pulse energy, repetition rate of the laser system, focusing conditions, the application of prepulses, and the chirp of the laser pulses on the efficiency of this highly nonlinear process is examined. In order to increase the X-ray flux, the laser pulse energy is increased by a 2nd multipass amplifier from 750 μJ to 5 mJ. By applying up to 4 mJ of the pulse energy a X-ray flux of 4×10¹⁰ Fe K _α photons/s or 2.75×10¹⁰ Cu K _α photons/s are generated. The energy conversion efficiency is therefore calculated to η _Fe≈1.4×10⁻⁵ and η _Cu≈1.0×10⁻⁵. The X-ray source size is determined to 15×25 μm². By focusing the produced X-rays using a toroidally bent crystal a quasi-monochromatic X-ray point source with a diameter of 56 μm×70μm is produced containing ≈10⁴ Fe K _α1 photons/s which permits the investigation of lattice dynamics on a picosecond or even sub-picosecond time scale. The lattice movement of a GaAs(111) crystal is shown as a typical application.     

Cr:LiSrAlF6 channel waveguides as broadband fluorescence sources

We report on the production and fluorescence of active channel waveguides in Cr:LiSrAlF₆. We have produced ∼10 μm wide and 5 μm high channel waveguides by He⁺ ion implantation, lithographic patterning and subsequent Ar⁺ ion sputtering. Diode-pumped waveguides emitted 13 μW of fluorescence light with a spectrum ranging from 760 nm to 900 nm at a pump power of 165 mW and a pump wavelength of 660 nm. The compact and cheap optical pump source is a main advantage of this fluorescence material. This makes Cr:LiSrAlF₆ channel waveguides a suitable candidate for a broadband fluorescence source in low-coherence interferometry and other applications in the near-infrared wavelength range. PACS 42.70.Hj; 42.79.Gn; 42.30.Wb