Hard tissue ablation with a free running Er:YAG and a Q-switched CO2 laser: a comparative study

The Er:YAG and the CO₂ laser are competitors in the field of hard tissue ablation. The use of Er:YAG lasers (2.94 μm, pulse length _L of 100 to 200 μs) show smaller areas of thermal defects then ‘‘superpulsed’’ CO₂ lasers with pulse lengths of approximately 100 μs. Only the development of a Q-switched CO₂ laser (9.6 μm, τ_L=250 ns) allowed for similar results. In this paper new results for the Er:YAG and the Q-switched CO₂ laser under the influence of water spray will be presented. Several parameters are of special interest for these investigations: the specific ablation energy, which shows a minimum for the CO₂ laser at an energy density of 9 J/cm ² and a broad shallow minimum in the range of 10 to 70 J/cm² for the Er:YAG laser, and comparison of the cut-shape and depth. Surface effects and cutting velocity are discussed based on SEM pictures. Received: 19 July 2000 / Revised version: 1 November 2000 / Published online: 30 November 2000     

Power scaling of a continuous-wave and passively Q-switched Yb:KLu(WO<Subscript>4</Subscript>)<Subscript>2</Subscript> laser end-pumped by a high-power diode

The power scaling capacity of a diode end-pumped Yb:KLu(WO₄)₂ laser, operating in the continuous-wave (cw) and passively Q-switched regimes, has been investigated. A cw output power of 11.5 W was achieved with an optical-to-optical efficiency of 41% with respect to the incident pump power, while the slope efficiency amounts to 60%. The passively Q-switchedoperation yielded an average output power of 4.3 W at the fundamental wavelength of 1031.7 nm, and 1.15 W of Raman radiation at 1139.3 nm. The total slope efficiency for Q-switched operation was 40%. The highest pulse energy, duration, and peak power were 170 μJ, 2.2 ns, and 77.3 kW for the fundamental radiation, and 51 μJ, 2.3 ns, and 22.2 kW for the Raman radiation. PACS 42.55.Rz; 42.55.Xi; 42.55.Ye     

High-power picosecond LiB3O5 optical parametric oscillators tunable in the blue spectral range

The paper reports on an experimental investigation and numerical analysis of noncritically and critically phasematched LiB₃O₅ (LBO) optical parametric oscillators (OPOs) synchronously pumped by the third harmonic of a cw diode-pumped mode-locked Nd:YVO₄ oscillator–amplifier system. The laser system generates 9.0 W of 355-nm mode-locked radiation with a pulse duration of 7.5 ps and a repetition rate of 84 MHz. The LBO OPO, synchronously pumped by the 355-nm pulses, generates a signal wave tunable in the blue spectral range 457–479 nm. With a power of up to 5.0 W at 462 nm and 1.7 W at 1535 nm the conversion efficiency is 74%. The OPO is characterized experimentally by measuring the output power (and its dependence on the pump power, the transmission of the output coupler and the resonator length) and the pulse properties (such as pulse duration and spectral width). Also the beam quality of the resonant and nonresonant waves is investigated. The measured results are compared with the predictions of a numerical analysis for Gaussian laser and OPO beams. In addition to the blue-signal output visible-red 629-nm radiation is generated by sum-frequency mixing of the 1.535-μm infrared idler wave with the residual 1.064-μm laser radiation. A power of 1.25 W of 1.535-μm idler radiation and 5.7 W of 1.064-μm laser light generated a red 629-nm output power of 2.25 W. Received: 2 February 2000 / Revised version: 28 July 2000 / Published online: 22 November 2000     

Formation of conical microstructures upon laser evaporation of solids

The formation and development of the large-scale periodic structures on a single crystal Si surface are studied upon its evaporation by pulsed radiation of a copper vapor laser (wavelength of 510.6 nm, pulse duration of 20 ns). The development of structures occurs at a high number of laser shots (∼10⁴) at laser fluence of 1–2 J/cm² below optical breakdown in a wide pressure range of surrounding atmosphere from 1 to 10⁵ Pa. The structures are cones with angles of 25, which grow towards the laser beam and protrude above the initial surface for 20–30 μm. It is suggested that the spatial period of the structures (10–20 μm) is determined by the capillary waves period on the molten surface. The X-ray diffractometry reveals that the modified area of the Si substrate has a polycrystalline structure and consists of Si nanoparticles with a size of 40–70 nm, depending on the pressure of surrounding gas. Similar structures are also observed on Ge and Ti. Received: 12 February 2000 / Accepted: 28 March 2000 / Published online: 20 June 2001     

Efficient, single frequency, high repetition rate, PPLN OPO pumped by a prelase Q-switched diode-pumped Nd:YAG laser

Single axial mode operation (<200 MHz optical bandwidth) of a high repetition rate periodically poled lithium niobate optical parametric oscillator (OPO) has been obtained at signal wavelengths between 1.46 μm and 1.64 μm. OPO signal slope efficiencies of 35% have been measured for repetition rates of 5–20 kHz. Single mode operation required spectral narrowing of both the pump laser and the OPO. A simple technique of prelase Q-switching was implemented to reduce the optical bandwidth of the cw diode-pumped Nd:YAG pump laser to <1 GHz. A single intracavity étalon was then sufficient to ensure single frequency oscillation of the OPO signal. The OPO output was stable with a smooth spatial profile and an M ² value of 1.3. Received: 29 September 1999 / Published online: 27 January 2000     

Difference-frequency generation in PPLN at 4.25 μm: an analysis of sensitivity limits for DFG spectrometers

We report difference-frequency generation (DFG) in periodically poled lithium niobate (PPLN) around 4.25 μm using a cw Nd:YAG and an injection-locked diode laser. This system provides a narrow linewidth source at 4.25 μm with near-shot-noise-limited operation. A conversion efficiency close to the theoretical limit is obtained. Detection of CO₂ absorption spectra is demonstrated and further improvements and applications to high sensitivity spectroscopy are discussed. Received: 12 August 1999 / Revised version: 21 January 2000 / Published online: 24 March 2000     

Efficient continuous wave and Q-switched operation of a dual-end-pumped <Emphasis Type="Italic">c</Emphasis>-cut Tm:YAP laser

An efficient continuous wave (CW) and Q-switched c-cut Tm:YAP laser is reported in this letter. With the dual-end-pumped convex-concave resonator, CW output power up to 13.6 W at 1.99 μm was obtained under a total incident pump power of 50 W. The corresponding slope efficiency was 34.3% and conversion efficiency was 27.2%. The active Q-switched operation of the laser had an average output power of 12.5 W at 10 kHz pulse repetition frequency, with a minimum pulse width of 126 ns. With 6 kHz pulse repetition frequency, the maximum pulse energy of 1.6 mJ was obtained. In addition, using the Tm:YAP laser as a pumping source for gain-switched Cr:ZnSe laser, as much as 4 W output power in the wavelength range of 2.5–2.6 μm was obtained.     

Experimental investigation of pulse diodes side-pumped 2 μm Tm:YAG lasers

The free running and Q-switched operation of 2 μm Tm:YAG lasers side-pumped by pulse laser diodes were reported. In the free running mode the maximum output energies were 102.5 mJ at 1 Hz and 94.6 mJ at 10 Hz, respectively. With an acousto-optic modulator in the laser resonator, 21 mJ 2 μm Q-switched pulse was obtained, with a pulse width of about 330 ns. The dependences of the output energy and the efficiency on the laser resonator parameters were investigated.     

Mid-infrared trace gas detection using continuous-wave difference frequency generation in periodically poled RbTiOAsO4

A tunable mid-infrared continuous-wave (cw) spectroscopic source in the 3.4–4.5 μm region is reported, based on difference frequency generation (DFG) in a quasi-phase-matched periodically poled RbTiOAsO₄ (PPRTA) crystal, DFG power levels of 10 μW were generated at approximately 4 μm in a 20-mm long PPRTA crystal by mixing two cw single-frequency Ti:Al₂O₃ lasers operating near 713 nm and 871 nm, respectively, using a laser pump power of 300 mW. A quasi-phase-matched infrared wavelength-tuning bandwidth (FWHM) of ∼12 cm^-1 and a temperature tuning rate of 1.02 cm^-1/°C were achieved. Experimental details regarding the feasibility of trace gas detection based on absorption spectroscopy of CO₂ in ambient air using this DFG radiation source are also described. Received: 23 October 2000 / Revised version: 22 January 2001 / Published online: 27 April 2001     

CW mode locked Nd:YVO4 laser pumped by 20-W laser diode bar

The efficient cw mode locking (cw-ML) regime was demonstrated in Nd:YVO₄ laser by means of saturable absorber mirror (SAM). The 0.3-at.% Nd³⁺ doped 10-mm-long YVO₄ crystal end pumped by 20-W diode module with a beam shaper was applied as a gain medium located in the close vicinity to the rear flat mirror of the first arm of Z-type resonator of 316 cm total length with two curved mirrors of 100-cm curvature radii. The SAM of 2%-saturable absorptance and saturation fluence of 50 μJ/cm² was mounted at the opposite end of a resonator. The developed “dynamically stable” cavity design mitigates detrimental role of thermal aberration in gain medium, enforcing clean perfect mode locking even for the highest pump densities. The cw-ML pulses with 47.5 MHz repetition rate and pulse durations in the range of 15–20 ps were observed for a wide range of pump powers and output coupler losses. In the best case, for 32% of output coupler transmission, up to 6.2 W of average power with near 35% slope efficiency was achieved. The thresholds for Q-switched ML, cw-ML regimes were 2.67 W and 6.13 W of pump power, respectively. For the maximum pump power of 20 W we obtained 133 nJ of pulse energy with 16-ps pulse duration, resulting in a peak power higher than 8 kW. The threshold energy density at SAM giving the QML regime was estimated to be about 30 μJ/cm², threshold of cw-ML regime was 220 μJ/cm².     

Multiwatt, tunable, diode-pumped CW Yb:GdCOB laser

We demonstrate that Yb-doped Ca₄GdO(BO₃)₃ (GdCOB) crystals are suitable for the development of high-power diode-pumped lasers emitting at around 1.04 μm. A 15%-doped Yb:GdCOB crystal was longitudinally pumped with a cw fiber-coupled diode emitting 10 W at 976 nm. While 5.2 W of diode power was absorbed, we obtained 3.2 W of 1043-μm laser light, with a beam quality factor M² equal to 3, and 2.5 W in a diffraction-limited beam. Furthermore, the laser is continuously tunable between 1018 and 1086 nm. Thermal effects have been investigated with a Shack–Hartmann wavefront analyser: although thermal lensing is not negligible, it does not affect the performance of the laser with the resonator design we used. Received: 1 August 2000 / Revised version: 18 September 2000 / Published online: 21 February 2001     

Diode end-pumped Q-switched high-power intracavity frequency-doubled Nd:GdVO4/KTP green laser

A diode-laser-array end-pumped acousto-optically Q-switched intracavity frequency-doubled Nd:GdVO₄/KTP green laser, formed with a three-mirror folded resonator, has been demonstrated. With 15 W of pump power incident upon the Nd:GdVO₄ crystal, a maximum average green output power of 3.75 W was obtained at 50 kHz of pulse repetition frequency, giving an optical conversion efficiency of 25%, whereas the effective intracavity frequency-doubling efficiency was determined to be 72%. At the incident pump power of 12.8 W, the shortest laser pulse was achieved at a pulse repetition rate of 10 kHz, the resulting pulse width, single pulse energy, and peak power were measured to be 35 ns, 108 μJ, and 3.1 kW, respectively. Received: 18 May 2000 / Published online: 20 September 2000     

Open-path trace gas detection of ammonia based on cavity-enhanced absorption spectroscopy

A compact open-path optical ammonia detector is developed. A tunable external-cavity diode laser operating at 1.5 μm is used to probe absorptions of ammonia via the cavity-enhanced absorption (CEA) technique. The detector is tested in a climate chamber. The sensitivity and linearity of this system are studied for ammonia and water at atmospheric pressure. A cluster of closely spaced rovibrational overtone and combination band transitions, observed as one broad absorption feature, is used for the detection of ammonia. On these molecular transitions a detection limit of 100 ppb (1 s) is determined. The ammonia measurements are calibrated independently with a chemiluminescence monitor. Compared to other optical open-path detection methods in the 1–2 μm region, the present result shows an improved sensitivity for contactless ammonia detection by over one order of magnitude. Using the same set-up, a detection limit of 100 ppm (1 s) is determined for the detection of water at atmospheric pressure. Received: 19 January 2000 / Revised version: 6 March 2000 / Published online: 7 June 2000     

Laser-diode-pumped Cr4+, Nd3+:YAG self-Q-switched laser with high repetition rate and high stability

A diode end-pumped self Q-switched Cr⁴⁺, Nd³⁺: YAG laser was established with 30-ns pulse width (FWHM) and 0.5-μJ pulse energy output. In normal pulse pumping operation, the lasing threshold changed greatly from 122 mJ to 2.4 mJ as the pump pulse frequency varied from 1 Hz to 500 Hz due to pumping-induced thermal effect. A pre-pumping method was proposed and the change of the lasing threshold was reduced; programmable Q-pulse output with maximum frequency of 16 kHz and high stability was achieved. Received: 16 January 2001 / Revised version: 21 May 2001 / Published online: 19 September 2001     

Passive Q-switching of 1.44 μm and 1.34 μm diode-pumped Nd:YAG lasers with a V:YAG saturable absorber

Spectroscopic data of a V³⁺:YAG passive Q-switch crystal were measured. The absorption recovery time was determined to be of 37±7 ns and the ground state absorption cross section was estimated to be 0.7×10^-18 cm² at 1.44 μm and 3.5×10^-18 cm² at 1.34 μm. Passively Q-switched operation of diode pumped 1.44 μm and 1.3 μm Nd:YAG lasers was demonstrated using this crystal as saturable absorber. Average output powers of 1.42 W (1.44 μm) and 1.56 W (1.34 μm) and pulse energies of 24 μJ (1.44 μm) and 25 μJ (1.34 μm) were observed, respectively. Received: 19 August 2002 / Published online: 12 February 2003 RID="*" ID="*"Corresponding author. Fax: +49-40/42838-6281, E-mail: kretschmann@physnet.uni-hamburg.de     

Efficient, kHz repetition rate, gain-switched Cr:forsterite laser

We have developed a gain-switched room-temperature Cr:forsterite laser operating at repetition rates of between 1 and 34 kHz, and pumped by a continuous wave, Q-switched Nd:YAG laser. With optimised output coupling, an output pulse energy of 52 μJ was measured at 1.5 kHz repetition rate, corresponding to 11% efficiency and 13% slope efficiency. Threshold pulse energy was 53 μJ. Output power of 370 mW was obtained at 10 kHz repetition rate and 4.4 W pump power. Water cooling was not required for repetition rates up to 10 kHz. In a tunable, folded resonator, the Cr:forsterite wavelength tuned between 1173 and 1338 nm. This laser operated with maximum pulse energy of 34 μJ, efficiency of 13%, and power of 307 mW. The laser output was close to diffraction-limited with M² of 1.2. Received: 6 January 1999 / Published online: 29 July 1999     

Application of mid-infrared cavity-ringdown spectroscopy to trace explosives vapor detection using a broadly tunable (6–8 μm) optical parametric oscillator

A novel instrument, based on cavity-ringdown spectroscopy (CRDS), has been developed for trace gas detection. The new instrument utilizes a widely tunable optical parametric oscillator (OPO), which incorporates a zinc–germanium–phosphide (ZGP) crystal that is pumped at 2.8 μm by a 25-Hz Er,Cr:YSGG laser. The resultant mid-IR beam profile is nearly Gaussian, with energies exceeding 200 μJ/pulse between 6 and 8 μm, corresponding to a quantum conversion efficiency of approximately 35%. Vapor-phase mid-infrared spectra of common explosives (TNT, TATP, RDX, PETN and Tetryl) were acquired using the CRDS technique. Parts-per-billion concentration levels were readily detected with no sample preconcentration. A collection/flash-heating sequence was implemented in order to enhance detection limits for ambient air sampling. Detection limits as low as 75 ppt for TNT are expected, with similar concentration levels for the other explosives. Received: 1 April 2002 / Revised version: 13 June 2002 / Published online: 12 September 2002 RID="*" ID="*"Corresponding author. Fax: +1-408/524-0551, E-mail: mtodd@picarro.com     

All-solid-state cw mode-locked picosecond KTiOAsO4 (KTA) optical parametric oscillator

4 (KTA) optical parametric oscillator (OPO) synchronously pumped by a cw diode-pumped mode-locked Nd:YVO₄ oscillator–amplifier system. The laser system (pumped by 84 W of cw 808-nm diode radiation) generates 7-ps-long pulses at 1.064 μm with a repetition rate of 83.4 MHz and an average power of 29 W. The OPO, synchronously pumped by the 1.064-μm laser pulses, consists of a 15-mm-long KTA crystal (cut for type II noncritical phase-matching) in a folded signal resonant linear resonator. The average powers of the 1.54-μm signal radiation and the 3.47-μm idler radiation are 14.6 W and 6.4 W, respectively. The total OPO output of 21 W corresponds to an internal efficiency of 75%. The experimental investigations include measurements of the OPO output power (and its dependence on the pump power, the transmission of the output coupler, and the resonator length) and of the pulse properties (such as pulse duration and spectral width). The measured results are in good agreement with the predictions of a numerical analysis based on a split-step Fourier method. Received: 4 May 1998     

Stable Q-switch mode-locking of Nd:YVO<Subscript>4</Subscript> lasers with a semiconductor saturable absorber

This paper reports on a passively mode-locked and Q-switched Nd:YVO₄ laser generating picosecond pulses with an average output power exceeding 7 W. In a first step Q-switch mode-locking was obtained by self Q-switching of a mode-locked oscillator with appropriate cavity design, pump power and output coupling. In a second system the Q-switching was actively controlled and stabilized by modulating the resonator internal losses with an acousto-optic modulator. In the Q-switch mode-locking operation the laser provided 12.8 ps long mode-locked pulses with a repetition rate of 80 MHz. The repetition rate of the Q-switch envelope was 185 kHz. The maximum pulse energy of a single ps pulse was 0.55 μJ which is 5.5 times the pulse energy measured for cw mode locking. The total energy of the pulses within the Q-switch envelope was 42 μJ. PACS  42.55.Xi; 42.60.Fc; 42.60.Gd     

Green sub-nanosecond microchip laser based on BiBO crystals

Frequency doubling of a passively Q-switched microchip laser using BiBO crystals is reported. Generation of green second harmonic at 532 nm with pulse energies of 2.4–3.4 μJ and conversion efficiency of 25–35% is demonstrated.