Nuclear magnetic moment of the 57Cu ground state

The nuclear magnetic moment of the ground state of (57)Cu(Iota(pi) = 3/2(-), T(1/2) = 196.3 ms) has been measured to be /mu((57)Cu)/ = (2.00 +/- 0.05)mu(N) using the beta-NMR technique. Together with the known magnetic moment of the mirror partner (57)Ni, the spin expectation value was extracted as = -0.078 +/- 0.13. This is the heaviest isospin mirror T = 1/2 pair above the (40)Ca region for which both ground state magnetic moments have been determined. The discrepancy between the present results and shell-model calculations in the full f p shell giving mu((57)Cu) approximately 2.4mu(N) and approximately 0.5 implies significant shell breaking at (56)Ni with the neutron number N = 28.     

Magnetic phase transition and magnetic structure of ground state in CsDyW O

Magnetic phase transition in the CsDyW₂O₈ magnet has been studied by means of low temperature specific heat C ( T ) measurements. The magnetic ordering temperature of the Dy³⁺ sublattice was established to be 1.34 K. The experimental results indicate on the antiferromagnetic character of interactions between Dy³⁺ ions. The behavior of the C ( T ) dependencies above and below T _N is discussed in frames of different theoretical models. The measurements data on temperature and field dependencies of magnetization are used to calculate the exchange and dipole-dipole interactions energy and to determine the possible magnetic structure of the ground state. Received 7 January 2002 / Received in final form 15 May 2002 Published online 7 September 2002     

Crystal and magnetic structures of the oxyphosphates MFePO 5 (M = Fe, Co, Ni, Cu). Analysis of the magnetic ground state in terms of superexchange interactions

We have studied in detail the crystal and magnetic structures of the oxyphosphates MFePO₅ (M: divalent transition metal) using neutron powder diffraction as a function of temperature. All of them are isomorphic to the mixed valence compound α-Fe₂PO₅ with space-group Pnma. No disorder exists between the two metallic sites. The M²⁺O₆ octahedra share edges between them and faces with Fe³⁺O₆ octahedra building zigzag chains running parallel to the b-axis that are connected by PO₄ tetrahedra. The topology of this structure gives rise to a complex pattern of super-exchange interactions responsible of the observed antiferromagnetic order. The magnetic structures are all collinear with the spin directed along the b-axis except for M = Co. The experimental magnetic moments of Cu⁺² and Ni²⁺ correspond to the expected ionic value, on the contrary the magnetic moment of Fe³⁺ is reduced, probably due to covalence effects, and that of Co²⁺ is greater than the spin-only value indicating a non negligible orbital contribution. Using numerical calculations we have established a magnetic phase diagram adapted for this type of crystal structure and determined the constraints to be satisfied by the values of the exchange interactions in order to obtain the observed magnetic structure as the ground state. Received 15 December 2000 and Received in final form 25 June 2001     

Spin polarized current in the ground state of superconductor-ferromagnet-insulator trilayers

We study the ground state properties of a superconductor-ferromagnet-insulator trilayer on the basis of a Hubbard Model featuring exchange splitting in the ferromagnet and electron-electron attraction in the superconductor. We solve the spin-polarized Hartree-Fock-Gorkov equations together with the Maxwell's equation (Ampere's law) fully self-consistently with respect to the order parameter and the current. For certain values of the exchange splitting we find that a spontaneous spin polarized current is generated in the ground state and is intimately related to Andreev bound states at the Fermi level. Moreover, the polarization of the current strongly depends on the band filling. Received 23 September 2002 / Received in final form 13 December 2002 Published online 1st April 2003 RID="a" ID="a"e-mail: m.a.krawiec@bristol.ac.uk     

The 3701 keV neutron g 9/2 single-particle state in 57Ni

The neutron g _9/2 single-particle state in ⁵⁷Ni has been unambiguously identified in a combined measurement of the linear polarization, angular distribution, and angular correlation of γ rays following the fusion-evaporation reaction ²⁸Si(³²S,2pn)⁵⁷Ni at a beam energy of 90 MeV. The linear polarization was measured with a Euroball cluster detector and a prototype of an encapsulated six-fold segmented hexaconical Ge-detector. The spin of the 3701 keV level in ⁵⁷Ni was confirmed to be I= 9/2 and its parity determined to be positive. Received: 24 September 1999 / Revised version: 22 October 1999     

Magnetism and phase separation in the ground state of the Hubbard model

We discuss the ground state magnetic phase diagram of the Hubbard model off half filling within the dynamical mean-field theory. The effective single-impurity Anderson model is solved by Wilson's numerical renormalization group calculations, adapted to symmetry broken phases. We find a phase separated, antiferromagnetic state up to a critical doping for small and intermediate values of U, but could not stabilize a Néel state for large U and finite doping. At very large U, the phase diagram exhibits an island with a ferromagnetic ground state. Spectral properties in the ordered phases are discussed. Received 9 January 2002 Published online 25 June 2002     

Ferrimagnetic ground state of a phenylene polymer with organic radicals

A ferrimagnetic polymer with m-phenylene skeleton as coupling unit is studied with the Hubbard model in the self-consistent mean-field theory. The ferrimagnetic ground state with a total spin S = 1 per unit cell is obtained and originates from the antiferromagnetic correlations between the nearest neighbors. If the on-site electron-electron repulsions at the radical sites and at the phenylene ring sites are different, the gap in energy band structure may disappear and the ferrimagnetic ground state becomes unstable. The charge density and spin density can transfer between the radical sites and the phenylene ring sites due to the competition between the hopping integral and the on-site repulsion at different sites. Received 15 July 2002 Published online 31 December 2002     

Nuclear spins, magnetic moments and α-decay spectroscopy of long-lived isomeric states in 185Pb

Alpha-decay properties of the neutron-deficient isotope ¹⁸⁵Pb were studied at the PSB-ISOLDE (CERN) on-line mass separator using the resonance ionisation laser ion source (RILIS). The nuclei of interest were produced in a 1.4 GeV proton-induced spallation reaction of a uranium graphite target. In contrast to previous studies, two α-decaying isomeric states were identified in ¹⁸⁵Pb. The relative production of the isomers, monitored by their α-counting rates, could be significantly changed when a narrow-bandwidth laser at the RILIS setup was used to scan through the atomic hyperfine structure. Based on the atomic hyperfine structure measurements, along with the systematics for heavier odd-mass lead isotopes, the spin and the parity of these states were interpreted as 3/2^- and 13/2⁺ and their nuclear magnetic moments were deduced. The α-decay energy and half-life value for the I ^π = 13/2⁺ isomer are E _α = 6408(5) keV, T _1/2 = 4.3(2) s, respectively; while for the I ^π = 3/2^- isomer ( T _1/2 = 6.3(4) s) two α-decays with E _α1 = 6288(5) keV, I _α1 = 56(2)% and E _α2 = 6486(5) keV, I _α2 = 44(2)% were observed. By observing prompt α-γ coincidences new information on the low-lying states in the daughter isotope ¹⁸¹Hg was obtained. Received: 7 February 2002 / Accepted: 19 February 2002     

On the magnetic dipole moment of the153Tb ground state

Temperature dependence of the angular distribution anisotropy of the 212·0 keV gamma-ray following the decay of¹⁵³Tb oriented in a gadolinium host was measured at temperatures from 16 to 70 mK. Magnetic dipole hyperfine splitting parameter a₀ for¹⁵³Tb(Gd) and magnetic dipole moment of the¹⁵³Tb ground state were estimated to be ¦a ₀¦1·2×10^–5 eV and ¦¦3·1 nuclear magnetons, respectively.Authors are indebted to Dr. N. A. Lebedev, Yu. V. Yushkewich and the staff of the JINR synchrocyclotron for the preparation of the¹⁵³Tb activity. The participation of Ing. L. Mare, J. Ferencei and S. I. Antonov in the measurements is also acknowledged.     

Extraction of hyperfine anomalies without precise values of the nuclear magnetic dipole moment

A new method for extracting the hyperfine anomaly from experimental hyperfine structure constants is suggested. Instead of independent high-precision measurements of the nuclear magnetic dipole moment, precise measurements of magnetic dipole hyperfine interaction constants for two atomic states and a theoretical analysis can be used. This can lead to determination of hyperfine anomaly for radioactive isotopes where the nuclear magnetic dipole moment is not known with high accuracy. Received: 17 February 1998     

High resolution laser spectroscopy of NaAr: Improved interaction potential for the ground state

The absorption spectrum of NaAr has been investigated with high resolution using a supersonic beam of molecules and a tunable dye laser. About 3 300 absorption lines due to the transition A ² Π ← X and B ² Σ ← X have been observed. In addition, we observed the spectral distribution of the fluorescence for a particular absorption line. From all experimental data the X ² Σ ⁺ interaction potential has been deduced in a fully quantum-mechanical method of approach. The potential is given in terms of an analytical Hartree-Fock-Dispersion function. For the equilibrium parameters of the X state we get R _e = 5.01(1) ? and D _e = 41.6(2) cm ^-1 . Received 28 August 2002 / Received in final form 15 October 2002 Published online 17 December 2002 RID="a" ID="a"Now at Knick Elektronische Messger?te, Beuckestr. 22, 14163 Berlin, Germany. RID="b" ID="b"e-mail: dz@kalium.physik.tu-berlin.de     

Line shape analysis of two-colour photoassociation spectra on the example of the Cs ground state

Two-photon photoassociation spectra in a Λ-type excitation scheme are analysed under the systematically varied experimental conditions of frequency detunings and laser intensities. Line shape fits are presented as well as the investigation of intensity and detuning dependent line shifts. From both we determine the attained spectroscopic precision, that is corrected for a systematic line shift due to the thermal distribution of atoms in the trap. An energy correction for this effect is given. Information about the feasibility of generating translationally cold molecules in a well defined rotational and vibrational level by the photoassociation process is derived from the analysis. Received 21 May 2002 Published online 15 October 2002 RID="a" ID="a"Current address e-mail: christian.lisdat@ptb.de RID="b" ID="b"e-mail: pierre.pillet@lac.u-psud.fr     

Selecting molecules in the vibrational and rotational ground state by deflection

A beam of diatomic molecules scattered off a standing wave laser mode splits according to the rovibrational quantum state of the molecules. Our numerical calculation shows that single state resolution can be achieved by properly tuned, monochromatic light. The proposed scheme allows for selecting non-vibrating and non-rotating molecules from a thermal beam, implementing a laser Maxwell's demon to prepare a rovibrationally cold molecular ensemble. Received 23 August 2000 and Received in final form 17 November 2000     

Effect of thermal ground state correlations on the statistical properties of the Lipkin model

The renormalized random phase approximation for hot finite Fermi systems is evaluated with the use of the thermo field dynamics formalism. This approximation treats vibrations of a hot finite Fermi system as harmonic ones but takes into account the Pauli principle in a more proper way than the usual thermal RPA, thus incorporating a new type of correlations in a thermal ground state. To demonstrate advantages of the approximation and to analyze a range of its validity, it is applied to the exactly solvable Lipkin model. A comparison is made with the exact grand canonical ensemble calculations, results of the thermal Hartree – Fock approximation and the thermal random phase approximation. The intrinsic energy of the system, the heat capacity, the average value of the quasispin operator z-projection and the particle number variance are calculated as functions of temperature. On the whole, the thermal renormalized RPA appears to be a better approximation than the other two. Its advantage is especially evident in the vicinity of the phase transition point. It is found that within TRRPA the phase transition occurs at lower temperature than in THFA and TRPA. Received: 4 January 1999 / Revised version: 10 March 1999     

Nuclear magnetic moment of161Tb

Nuclear orientation measurements on dilute TbGd are analysed to yield the magnetic dipole and electric quadrupole moments of¹⁶¹Tb g.s. and multipole mixing ratios of transitions in¹⁶¹Dy.     

The magnetic moment of the lowest 3/2− state in57Co

The reaction⁵⁴Fe(α, n)⁵⁷Ni has been used to implant⁵⁷Co isotopes in ferromagnetic iron. Theg-factor of the lowest 3/2^? state is determined using the internal field in a constant angle reversed field method. The angular correlation of the 127–1,378 keV cascade is also measured. The result of the angular correlation measurement together with reaction data is consistent withp _3/2 andp _1/2 single particle assignments to the lowest 3/2^? resp. 1/2^? state. In view of this statement the quenching of the magnetic moment is discussed.     

The large probability of the 0+ ground states

We investigate the dominance of 0⁺ states as the lowest states in shell model calculations with random two-body interactions in a single j-shell. We have found an explanation of the large probability of the 0⁺ ground state. Received: 1 May 2001 / Accepted: 4 December 2001     

Evolution of shapes in 59Cu

High-spin states in ⁵⁹Cu were populated using the fusion-evaporation reaction ²⁸Si + ⁴⁰Ca at a beam energy of 122 MeV. The Gammasphere Ge-detector array in conjunction with the 4π charged-particle detector array Microball allowed for the detection of γ-rays in coincidence with evaporated light particles. The resulting extensive high-spin decay scheme of ⁵⁹Cu is presented, which comprises more than 320 γ-ray transitions connecting about 150 excited states. Their spins and parities have been assigned via directional correlations of γ-rays emitted from oriented states. Average quadrupole moments of rotational bands have been determined from the analysis of residual Doppler shifts. Shell model calculations in the fp shell are invoked to study some of the low-spin states, while the experimental characteristics of the rotational bands are analyzed in the configuration-dependent cranked Nilsson-Strutinsky (CNS) approach. Received: 15 February 2002 / Accepted: 23 April 2002     

The sign of the magnetic dipole moment of the ground state of122I

The sign of the nuclear magnetic dipole moment of the ground state of¹²²I has been determined to be positive using a novel experimental technique. The technique investigates the asymmetry of positron emission by detecting the 511 keV gamma-rays produced on the annihilation of the positrons. The method would appear to have general validity for studying the sign of the magnetic moment in other cases where theβ ⁺ decay is relatively simple.