Nuclear charge radius,spin and nuclear moments of45Ca by laserspectroscopy

The mean square charge radius, the spin, the magnetic moment and the quadrupole moment of the⁴⁵Ca nucleus have been determined from the isotope shift in the Ca- intercombination line and from the hyperfine structure splitting of the 4s4p³P₁. state. A highly sensitive laserspectroscopic technique in combination with an atomic beam was used in the experiment.     

Measurement of isotope shift and hyperfine splitting of190, 191, 193, 197Pb isotopes by collinear laser spectroscopy

We report here on the measurement of isotope shift and hyperfine splitting of^{190, 191, 193, 197}Pb for the 723 nm atomic optical transition. Detailed analysis of the optical data has been done by combining them with the available muonic and electronicx-ray isotope shift data. The magnetic dipole moments and the electric quadrupole moments of the odd isotopes have been extracted from the hyperfine coupling constants of the atomic states involved in the optical transition used.     

Measurement of isotope shifts,fine and hyperfine structure splittings of the lithium D lines

The lithium D lines were studied using a diode laser that was frequency modulated by an electro-optic modulator, to excite an atomic beam. The transmission of part of the laser beam through an etalon was monitored to correct for the nonlinearity of the laser scan. The results for the ^6,7Li 2 S _1/2 and 2 P _1/2 hyperfine splittings agree very well with the best existing data while those for the D1 isotope shift and ^6,7Li fine structure splittings disagree significantly from data obtained by a previous laser atomic beam experiment. Our result for the D1 isotope shift is very close to the latest value computed using Hylleraas variational theory. Received 8 April 2002 / Received in final form 26 June 2002 Published online 21 January 2003 RID="a" ID="a"e-mail: wvw@yorku.ca     

Isotope shift and hyperfine structure measurements at the242f Am fission isomer

Istope shift and hyperfine structure measurements have been performed for the^242fAm fission isomer with target production rates of only a few per second. The method is based on resonance ionization spectroscopy (RIS) in a buffer gas cell with radioactive decay detection of the ionization process (RADRIS). A relative isotope shift ratioX _exp=IS^242f,241/ IS^243,241=41.7±0.9 has been measured for the 500.02 nm transition corresponding to a nuclear parameter ^242f,241=5.4±0.3 fm². The analysis of the quadrupole moment based on the deformed Fermi-model of the nuclear charge distribution including second order corrections results inQ ₂₀=38.2 ±1.4( _–0.8 ^+0.4 )_model eb. The measurement of the hyperfine structure splitting of the transition at 466.28 nm yields a negativeg-factor and a nuclear spin ofI=2 orI=3.Work supported by the Bundesministerium für Bildung und Forschung under contract 06 MZ 5661.     

Measurement of the antiproton-nucleus annihilation cross-section at very low energies

The ASACUSA collaboration at the Antiproton Decelerator at CERN is planning to measure the hyperfine splitting of the ground state of antihydrogen using an atomic beam line. This will be a measurement of the antiproton magnetic moment, and also a test of the CPT invariance. The planned experimental method and setup, including the radiofrequency resonance cavity, are described, and results of Monte Carlo simulations are shown. These simulations predict that the antihydrogen ground-state hyperfine splitting can be determined with a relative precision of ～10^???7.     

Temperature and concentration gradient effects on heat and mass transfer in micropolar fluid

We report here the development of collinear laser spectroscopy (CLS) system at VECC for the study of hyperfine spectrum and isotopic shift of stable and unstable isotopes. The facility is first of its kind in the country allowing measurement of hyperfine splitting of atomic levels using atomic beams. The CLS system is installed downstream of the focal plane of the existing isotope separator online (ISOL) facility at VECC and is recently commissioned by successfully resolving the fluorescence spectrum of the hyperfine levels in \(^{85,87}\)Rb. The atomic beams of Rb were produced by charge exchange of 8 keV Rb ion beam which were produced, extracted and transported to the charge exchange cell using the ion sources, extractor and the beam-line magnets of the ISOL facility. The laser propagating opposite to the ion / atom beam direction was allowed to interact with the atom beam and fluorescence spectrum was recorded. The experimental set-up and the experiment conducted are reported in detail. The measures needed to be carried out for improving the sensitivity to a level necessary for studying short-lived exotic nuclei have also been discussed.     

Hyperfine structure and isotope shift measurements on 235U and laser separation of uranium isotopes by two-step photoionization

Two-step photoionization of an atomic beam and quadrupole mass analysis have been used for the precise measurement of the isotope shift between uranium isotopes 235 and 238 and the hyperfine structure of ²³⁵U. For the 5915 Å ground-state transition 15 hfs components were found. The residual atomic beam was isotopically enriched by factors 2.5 and 10 for ²³⁵U and ²³⁸U, respectively.     

Spins,moments and charge radii in the isotopic series181Hg-191Hg

The hyperfine structure splitting and the isotope shift in the (6 s^{2 1}S₀ - 6s 6p³P₁,λ=2,537 Å) line of very neutron deficient Hg isotopes were determined by the β radiation detected optical pumping method (β-RADOP). In addition, nuclear magnetic resonance was observed in the atomic ground state. The results are Mean-square nuclear charge radii are calculated. Interpreting the sudden change of nuclear radius between¹⁸⁷Hg and¹⁸⁵Hg δ〈r²〉^187,185=0.42(5)fm² as oblate-prolate shape transition, one obtains δ〈β²〉 =0.054(5).     

New laser setup at the IRIS facility. Magnetic moments and mean squared charge radii of neutron deficient Tl isotopes

A new laser installation for the resonance ionization spectroscopy in a laser ion source and for rare isotope production has been put into operation at the IRIS mass-separator, working on-line with the 1 GeV proton beam of the Petersburg Nuclear Physics Institute synchrocyclotron. Isotope shift and hyperfine splitting of 276.9 nm atomic transition in the long chain of Tl isotopes and isomers have been measured. New data on the magnetic moments and changes in mean squared charge radius for ^{183,184,185,185m,186m2,195m,197m}Tl have been obtained.     

Isotope shifts and hyperfine structure in the transitions of gadolinium

High-resolution resonance ionization mass spectrometry has been used to measure isotope shifts and hyperfine structure in all (J = 2-6) and the transitions of gadolinium (Gd I). Gadolinium atoms in an atomic beam were excited with a tunable single-frequency laser in the wavelength range of 422-429 nm. Resonant excitation was followed by photoionization with the 363.8 nm line of an argon ion laser and resulting ions were mass separated and detected with a quadrupole mass spectrometer. Isotope shifts for all stable gadolinium isotopes in these transitions have been measured for the first time. Additionally, the hyperfine structure constants of the upper states have been derived for the isotopes ^{155, 157} Gd and are compared with previous work. Using prior experimental values for the mean nuclear charge radii, derived from the combination of muonic atoms and electron scattering data, field shift and specific mass shift coefficients for the investigated transitions have been determined and nuclear charge parameters for the minor isotopes ^{152, 154} Gd have been calculated. Received 18 November 1999     

Nuclear charge radii changes of uranium and hafnium isotopes determined by laser spectroscopy

The present work reports measurements of isotope shifts and hyperfine structure in the optical spectra of two high-Z elements: Hf and U. The experiments are based on the observation of the resonance fluorescence in a well collimated atomic beam, excited by a tunable dye laser. The chains of the stable Hf isotopes and of^{233–236, 238}U have been investigated and changes in ms nuclear charge radii have been deduced. The results have been discussed from the point of view of nuclear structure in the investigated regions.     

Hyperfine structure of the ground state muonic <Superscript>3</Superscript>He atom

On the basis of the perturbation theory in the fine structure constant α and the ratio of the electron to muon masses we calculate one-loop vacuum polarisation and electron vertex corrections and the nuclear structure corrections to the hyperfine splitting of the ground state of the muonic helium atom (μ e ³ ₂He). We obtain total results for the ground state hyperfine splitting Δ ν ^hfs = 4166.648 MHz which improves the previous calculation of Lakdawala and Mohr due to new corrections of orders α ⁵ and α ⁶. The remaining differences between our theoretical result and experimental value of the hyperfine splitting lie in the range of theoretical and experimental errors and require the subsequent investigation of higher order corrections.     

A precision measurement of the hyperfine structure of87Sr+

The ground state hyperfine splitting of⁸⁷Sr⁺ was measured with a precision of 1×10^–8. The experiments were performed with an RF ion trap connected to an ISOL (isotope separator on-line), where all the possible transitions between Zeeman sublevels were observed by a laser-microwave double resonance method. The magnetic dipole hyperfine constant was determined to beA=–1 000 473.673 (11) kHz.     

First Measurement of the Nuclear Charge Radii of Short-Lived Lithium Isotopes

A novel method for the determination of nuclear charge radii of lithium isotopes is presented. Precise laser spectroscopic measurements of the isotope shift in the lithium 2s → 3s transition are combined with highly accurate atomic physics calculation of the mass dependent isotope shift to extract the charge-distribution-sensitive information. This approach has been used to determine the charge radii of ^8,9Li for the first time.     

Hyperfine splitting and isotope shift in the optical transition of Eu isotopes and electromagnetic moments of Eu

The laser-induced resonance fluorescence in an atomic beam was used in order to measure the hyperfine splitting of the 4f ⁷ 6s ² and 4f^{7 6s6p} levels in ^151,153,155Eu isotopes. The hfs constants A and B of the unstable ¹⁵⁵Eu were determined for the first time: MHz, MHz and MHz. With these data and after corrections for second-order hyperfine structure perturbations the nuclear moments of ¹⁵⁵Eu were deduced: n.m. and b. In addition new and more precise values of the hfs constants of the excited state for the stable ^151,153Eu were obtained. They are as follows: MHz, MHz and MHz, MHz. The hyperfine anomalies % and % were extracted from the corrected hfs constants. Received 28 July 1999 and Received in final form 14 January 2000     

Isotope shifts and hyperfine structure in calcium 4snp and 4snf F Rydberg states

Isotope shifts and hyperfine structure have been measured in 4snp ¹ P₁ and Rydberg states for all stable calcium isotopes and the radioisotope ⁴¹Ca using high-resolution laser spectroscopy. Triple-resonance excitation via Rydberg state was followed by photoionization with a CO₂ laser and mass selective ion detection. Isotope shifts for the even-mass isotopes have been analyzed to derive specific mass shift and field shift factors. The apparent isotope shifts for ⁴¹Ca and ⁴³Ca exhibit anomalous values that are n-dependent. This is interpreted in terms of hyperfine-induced fine-structure mixing, which becomes very pronounced when singlet-triplet fine-structure splitting is comparable to the hyperfine interaction energy. Measurements of fine-structure splittings for the predominant isotope ⁴⁰Ca have been used as input parameters for theoretical calculation of the perturbed hyperfine structure. Results obtained by diagonalizing the second-order hyperfine interaction matrices agree very well with experimentally observed spectra. These measurements allow the evaluation of highly selective and sensitive methods for the detection of the rare ⁴¹Ca isotope. Received 17 December 1999 and Received in final form 29 March 2000     

Rubidium and proton ENDOR on ion pairs in solution

The E.S.R. spectrum of the o-dimesitoylbenzene anion-alkali cation radical shows unusually large isotropic alkali hyperfine splitting constants. We report a solution ENDOR study of this radical in which both alkali (^85,87Rb) and proton ENDOR spectra were recorded. Both the alkali and proton intensities showed a strong dependence on the metal ion nuclear spin quantum number of the E.S.R. line being saturated. This dependence is attributed to strong flip-flop cross-relaxation induced by modulation of the isotropic alkali hyperfine splitting. The powder E.S.R. spectrum of the complex reveals a small anisotropy of the Rb hyperfine splitting tensor. This indicates a small metal non-s-contribution to the half-filled molecular orbital, which is consistent with the observed relaxation behaviour and the small g shift. The intensity variations in the alkali and proton ENDOR spectra were used to determine the relative signs of all hyperfine splitting constants, and the absolute signs of the hyperfine splitting constants are deduced from a model of the structure of the complex.     

Nuclear radii of thorium isotopes from laser spectroscopy of stored ions

Isotope shifts and hyperfine splittings in optical transitions for atomic ions of the thorium isotopes²²⁷Th to²³⁰Th and²³²Th have been measured by laser spectroscopy on stored ions. From the isotope shift data, changes of the mean square charge radii are determined. A continuous increase of the charge radius with mass numberA is observed, in agreement with droplet model calculations. The results indicate that the odd-even staggering for Th is different from that one of the neighbouring isotones of Fr and Ra. There is some empirical evidence from systematics for an inversion of the staggering and the appearance of an octupole deformation atN ≦137. The hyperfine splitting for²²⁹Th for 3 electronic levels is given.     

Isotope shift in the Ca I resonance line and changes in mean-square nuclear charge radii of the stable Ca isotopes

The isotope shift of all stable Ca isotopes was studied in the Ca I resonance line. Enriched isotopes were used in an atomic beam, passing through the center of a spherical Fabry-Perot interferometer. The measured isotope shifts were separated into mass shift and field shift by comparing the optical isotope shift with δ〈r ²〉 values derived from recent muonic x-ray measurements. The results are discussed together with known data on the isotope shift in the Ca I intercombination line and data from Hartree-Fock calculations. The following mean values are obtained for the change in nuclear charge distribution δ〈r ²〉 [fm²]∶ [40, 42] 0.23(3); [40, 43] 0.13(3); [40, 44] 0.28(4); [40, 46] 0.14(7); [40, 48] 0.00(2).     

Hyperfine splitting and isotope shift in the atomic D2 line of 22,23Na and the quadrupole moment of 22Na

The hyperfine structure of the D₂ optical line in ²²Na and ²³Na has been investigated using high resolution laser spectroscopy of a well-collimated atomic beam. The hyperfine splitting constants A and B for the excited 3p ²P_3/2 level for both investigated sodium isotopes have been obtained. They are as follows: A(22) = 7.31(4) MHz, B(22) = 4.71(28) MHz, A(23) = 18.572(24) MHz, B(23) = 2.723(55) MHz. With this data, using the high precision MCHF calculations for the electric field gradient at the nucleus, the electric quadrupole moment of ²²Na has been deduced: Q_s(22) =+0.185(11) b. The sign of Q_s(22), determined for the first time, indicates a prolate nuclear deformation. A precise value of the isotope shift ^22,23Na in the D₂ line has also been obtained. Received: 26 February 1998 / Revised version: 25 June 1998