Experimental study of pulse compression in a side-pumped Yb-doped double-clad mode-locked fiber laser

We have developed a side-pumped passively mode-locked Yb-doped double-clad fiber laser emitting sub-picosecond pulses at around 1.05 μm. Mode locking is achieved through a polarization additive-pulse mode-locking technique and compression is obtained with a grating pair inserted in the cavity. We have investigated the compression properties of this laser. High-energy pulses are emitted and different behaviors are observed, such as sideband generation, secant-like or Gaussian-like pulse emission. Received: 7 May 2001 / Revised version: 13 November 2001 / Published online: 17 January 2002     

Diode-pumped Cr:LiCAF fs regenerative amplifier system seeded by an Er-doped mode-locked fiber laser

A fs regenerative amplifier based on Cr:LiCAF is demonstrated for the first time. With direct diode pumping, 8 μJ of pulse energy are obtained directly from the amplifier. When seeded by an Er-doped fiber laser, the amplified seed pulses are compressed down to 252 fs, limited by residual net third-order dispersion of the compression gratings and intracavity elements. Pulse broadening due to second- and third-order dispersion is theoretically investigated and compared to experimental results. Dispersion generated by the geometrical cavity arrangement is measured experimentally. Received: 19 November 2001 / Revised version: 28 January 2002 / Published online: 14 March 2002     

Dependence of spectrum on pump-signal angle in BBO-I noncollinear optical-parametric chirped-pulse amplification

A BBO-I noncollinear optical-parametric chirped-pulse amplifier pumped by a Q-switched and frequency-doubled Nd:YAG laser has been demonstrated. At an optimal pump-signal angle, the temporally stretched chirped signal pulses with bandwidth of 36 nm (FWHM) were amplified without any distortion in spectrum. The gain bandwidth was very sensitive to the pump-signal angle. Variation of this angle by about 1.5 mrad may significantly reduce the amplified bandwidth and result in a significant distortion in the amplified spectrum. Received: 5 October 2000 / Revised version: 13 June 2001 / Published online: 19 September 2001     

Multimode to single-mode conversion of a Yb-doped fiber amplifier with a photorefractive Rh:BaTiO3 crystal

We present a technique to convert a multimode-transverse beam obtained from a multimode large core fiber amplifier into a single-mode beam by means of two-wave mixing in an infrared-sensitive Rh:BaTiO₃ crystal. Received: 26 March 2001 / Revised version: 27 March 2001 / Published online: 27 April 2001     

Four-wave mixing of picosecond pulses in hollow fibers: expanding the possibilities of gas-phase analysis

Third-harmonic, difference-frequency, and sum-frequency generation processes in hollow fibers are experimentally studied with 30-ps pulses having an energy of several millijoules. The experimental dependence of the difference-frequency signal on the pressure of the gas filling the fiber agrees well with the results of calculations when the contribution of higher order waveguide modes is taken into consideration, thus indicating the importance of nonlinear-optical processes involving higher order waveguide modes of a hollow fiber. Hollow fibers are also shown to expand the possibilities of nonlinear-optical analysis of gases by allowing the generation of third-harmonic and sum-frequency signals, which vanish in the regime of tight focusing in a medium with normal dispersion. Received: 26 September 2000 / Revised version: 15 January 2001 / Published online: 30 March 2001     

Two-color pump-probe ionization spectroscopy of gaseous water enhanced by preliminary impulsive Raman excitation

We use sub-10-fs pulses at 400 nm and 15-fs pulses at 800 nm to ionize water molecules and their isotopomers HDO and D₂O in a pump–probe scheme. Pulses are generated via spectral broadening of 25-fs pulses of a 1-kHz Ti:sapphire amplifier system by self-phase modulation in a noble-gas-filled hollow waveguide and subsequent compression using chirped mirrors. At this time scale vibronic excitation of the first bending mode of water in the electronic ground state by impulsive Raman scattering is possible (e.g. the fundamental bending mode of H₂O: t_vib=20 fs). The effect of this pre-excitation on the ionization rate is shown. Received: 14 May 2001 / Revised version: 24 August 2001 / Published online: 19 September 2001     

Enhanced spectral broadening of short laser pulses in high-numerical-aperture holey fibers

The influence of the structure of holey-fiber cladding on the spectral broadening of femtosecond laser pulses is experimentally studied. These experiments demonstrate that the spectral broadening of 70-fs pulses of 800-nm Ti:sapphire laser radiation transmitted through 2- and 3-μm-pitch holey fibers can be enhanced by a factor of about 1.5 by increasing the air-filling fraction of the fiber cladding from 16 up to 65%. Received: 23 April 2001 / Revised version: 18 June 2001 / Published online: 18 July 2001     

Two-octave spectral broadening of subnanojoule Cr:forsterite femtosecond laser pulses in tapered fibers

Spectral broadening of femtosecond Cr:forsterite laser pulses is enhanced due to the use of tapered fibers. Supercontinuum generation with unamplified subnanojoule femtosecond Cr:forsterite laser pulses is observed for the first time. With 40-fs 0.6-nJ pulses of 1.25-μm Cr:forsterite laser radiation coupled into a tapered fiber having a taper waist diameter of about 2 μm and a taper waist length of 90 mm, we observed the spectra spanning more than two octaves at the output of the fiber in the regime of anomalous group-velocity dispersion. This result opens the way for the creation of compact femtosecond Cr:forsterite laser plus tapered fiber systems for optical metrology and biomedical applications. Received: 23 October 2001 / Accepted: 16 January 2002 / Published online: 14 March 2002     

Generation of 17-TW 23-fs Pulses with a Two-Stage Ti：Sapphire Amplifier at Repetition Rate 10 Hz

We have developed a two-stage Ti：sapphire amplifier system which can produce 17- TW/23-fs pulses at a repetition rate 10Hz. A birefringent plate is used in the regenerative amplifier to alleviate gain narrowing, while an all- reflective cylindrical-mirror-based pulse stretcher and an acousto-optic programmable dispersive filter （AOPDF） are used to compensate for the higher order dispersion of the system.     

High-power intracavity frequency doubling of a Ti:sapphire femtosecond oscillator

We demonstrate intracavity frequency doubling of a standard femtosecond Ti:sapphire oscillator. The cavity is extended with a pair of focusing mirrors and a 0.5-mm-thick BBO crystal. We achieve a repetition rate of 50 MHz and simultaneously generate 22 mW of 55-fs pulses at 810 nm and 200 mW of 73-fs pulses at 405 nm, which corresponds to 4 nJ per pulse. We create a total of 330-mW, 405-nm light when pumping the Ti:sapphire crystal with 5.7 W from an Ar-ion laser, corresponding to a conversion efficiency of 5.7%. No saturation is found, which implies that higher outputs can be achieved with higher pump rates. Preliminary results from the use of blue pulses as pump in an optical parametric amplifier seeded by pulses from a photonic crystal fiber are presented. Received: 27 January 2003 / Revised version: 27 March 2003 / Published online: 12 May 2003 RID="*" ID="*"Corresponding author. Fax: +45-861/96199, E-mail: tva@chem.au.dk     

Tunable, high-power, narrow-band picosecond IR radiation by optical parametric amplification in KTP

We report on an optical parametric amplifier (OPA) based on two potassium titanyl phosphate (KTP) crystals in a walk-off compensating geometry. An Nd:YLF regenerative amplifier at a 1-kHz repetition rate serves as the pump source. The seed beam is delivered by a synchronously pumped frequency-stabilized optical parametric oscillator (OPO) based on periodically poled lithium niobate (PPLN). At pump intensities of about 7 GW/cm² large amplification factors of more than 10⁴ were achieved, resulting in pulse energies of more than 450 μJ and 350 μJ for the signal and idler pulses, respectively, at a 1-kHz repetition rate. In the saturation regime the time–bandwidth product increases from two to three times the Fourier limit, with a pulse duration of 105 ps and a bandwidth of 12.7 GHz at the highest intensities employed. Received: 2 November 2001 / Published online: 14 March 2002     

Measurement of thermal lensing in a power amplifier of a terawatt Ti:sapphire laser

We have measured detailed thermal lensing in a power amplifier of a terawatt Ti:sapphire laser operating at 50 Hz. The thermal lensing in the amplifier was evaluated by measuring the optical path difference (OPD) using a Shack–Hartmann-type wavefront sensor. It was found that the radial dependence of the OPD was almost quadratic in the pumping region, despite inhomogeneous pumping. Therefore, a simple spherical lens or convex mirror effectively compensates for the thermal lens in our amplifier. We found that the thermal lens profile was temporally stable, and did not degrade the pointing stability of the amplified laser pulses. We also found that the time constant of the thermal distortion in our power amplifier was approximately 0.5 s. Received: 3 September 2001 / Revised version: 23 January 2002 / Published online: 14 March 2002     

High average power ultra-fast fiber chirped pulse amplification system

We report on a high-gain diode-pumped ytterbium-doped fiber-amplifier system delivering pulse energies in the 100-μJ range at high repetition rates (32 kHz) with nearly-diffraction-limited beam quality (M²∼1.7) at a 1060-nm center wavelength. Femtosecond seed-laser pulses are stretched in a commercially available single-mode fiber and compressed after amplification to subpicosecond pulse duration. In a multimode Yb-doped fiber amplifier we have demonstrated average powers of up to 22 W and single-pulse energies of up to 130 μJ. Received: 16 August 2000 / Revised version: 4 September 2000 / Published online: 8 November 2000     

Femtosecond ultraviolet pulses generated using noncollinear optical parametric amplification and sum frequency mixing

We demonstrate the generation of ultraviolet 33-fs pulses with a shot-to-shot energy fluctuation of less than 3% using sum frequency mixing of visible pulses of a noncollinear optical parametric amplifier with sub-40-fs pulses of a 1-kHz Ti:sapphire-amplified system. The pulses are transform-limited (ΔνΔτ=0.36) and tunable in the range from 315 nm to 355 nm with energy above 1 μJ (2.6 μJ at 330 nm). Received: 21 July 2000 / Published online: 8 November 2000     

A dispersionless Michelson interferometer for the characterization of attosecond pulses

A novel application of a free-standing transmission grating as a beam splitter in a Michelson-type interferometer is described. The arrangement can operate in the XUV and soft X-ray spectral region and, therefore, it is well suited for the characterization of attosecond pulses. Using ray-tracing codes, we have analyzed three different setups in which spherical mirrors are employed in conjunction with the transmission grating and have investigated in detail their dispersive characteristics. It is shown that such an arrangement can be made to exhibit group-delay dispersion of ∼1 as² while it provides two co-propagating and converging beams. Received: 12 October 2001 / Revised version: 17 December 2001 / Published online: 7 February 2002     

Generation of high-quality 10-femtosecond laser pulses with intracavity spatial and spectral control

Spatial and spectral control, using an intracavity capillary and a slit, is applied to improve the output pulse quality of a Ti:sapphire laser. Satellite-free 10-fs optical pulses with a smooth spectral and spatial profile have been generated. Employing a root-mean-square formalism for pulse characterization, spatial, spectral and temporal intensity distributions are analyzed for laser pulses with a duration as short as three to four optical cycles. Received: 11 June 2001 / Published online: 18 July 2001     

Compact high gain double-pass optical parametric chirped pulse amplifier

A novel double-pass noncollinear optical parametric chirped pulse amplifier based on an Yb³⁺-doped passively mode-locked fiber laser has been demonstrated in this paper. The signal was double-pass amplified in a single nonlinear crystal by a long pump pulse, and the signal and pump pulses of each pass were completely phase matched in the plane of the maximum effective nonlinearity. Net saturated gain of 2×10⁶ was achieved and the superfluorescence was suppressed by increasing the overlap time between the signal and pump pulses.     

SOA-based actively mode-locked fiber ring laser by forward injecting an external pulse train

An actively mode-locked fiber ring laser based on cross-gain modulation (XGM) in a semiconductor optical amplifier (SOA) is demonstrated to operate stably with a simple configuration. By forward injecting an easily-generated external pulse train, the mode-locked fiber laser can generate an optical-pulse sequence with pulsewidth about 6 ps and average output power about 7.9 mW. The output pulses show an ultra-low RMS jitter about 70.7 fs measured by a RF spectrum analyzer. The use of the proposed forward-injection configuration can realize the repetition-rate tunability from 1 to 15 GHz for the generated optical-pulse sequences. By employing a wavelength-tunable optical band-pass filter in the laser cavity, the operation wavelength of the designed SOA-based actively mode-locked fiber laser can be tuned continuously in a wide span between 1528 and 1565 nm. The parameters of external-injection optical pulses are studied experimentally to optimize the mode-locked fiber laser.     

Directional coupling of optical signals by odd dark beams with mixed phase dislocations

Numerical simulations on the evolution of step-screw and edge-screw optical phase dislocations in bulk saturable self-defocusing nonlinear media are presented, with emphasis on their ability to induce steering waveguides for signal beams (pulses). Two schemes for directional coupling of such signals, both ensuring a reasonable coupling-to-cross-talk efficiency ratio, are investigated. The parameters useful for performance optimization of the couplers are discussed. Received: 19 July 2000 / Revised version: 5 February 2001 / Published online: 27 April 2001