First observation of excited states in 197At: the onset of deformation in neutron-deficient astatine nuclei

Excited states in the Z= 85 nucleus ¹⁹⁷At have been identified for the first time using the recoil-decay-tagging (RDT) technique. The excitation energy of these states is found to be consistent with the systematics of neutron-deficient astatine nuclei and with theoretical calculations indicating that the nucleus may be deformed in its ground state. Received: 8 January 1999     

Identification of the 13/2+ isomer in 199At

The 13/2⁺ isomeric state in the ¹⁹⁹At nucleus has been identified at an excitation energy of 573 keV and its half-life measured to be 580(130) ns using the recoil-decay tagging technique. Received: 19 September 2000 / Accepted: 1 November 2000     

Particle octupole-vibration coupling near 208Pb

High-spin states in ²⁰²Pb and ²⁰³Pb have been investigated by in-beam γ-ray spectroscopy following the reaction ¹⁹⁸Pt(⁹Be,xn). A search for magnetic rotational bands in these isotopes confirmed one of the two bands previously assigned to ²⁰²Pb and revealed a new band in this isotope. No evidence for magnetic rotation has been found in ²⁰³Pb. Received: 24 July 2000 / Accepted: 28 September 2000     

Investigations into the alpha-decay of <Superscript>195</Superscript>At

The low-energy nuclear structure and decay properties of the neutron-deficient isotopes ¹⁹⁵At and ¹⁹¹Bi have been studied. ¹⁹⁵At was produced in the reaction ¹⁴²Nd(⁵⁶Fe,p2n)¹⁹⁵At and ¹⁹¹Bi as the daughter activity of ¹⁹⁵At. The activities were implanted in a position-sensitive silicon detector after being separated from the primary beam by a gas-filled recoil separator. The 1/2⁺ intruder state was determined to be the ground state in ¹⁹⁵At with an alpha-decay energy of E _α = 6953(3) keV and a half-life T _1/2 = 328(20) ms. Another state with an alpha-decay energy E _α = 7075(4) keV and a half-life T _1/2 = 147(5) ms was found to decay to a 148.7(5) keV excited state in ¹⁹¹Bi for which a spin and parity of 7/2^- were deduced. Consequently, the same 7/2^- character was assigned to the initial state at 32(7) keV in ¹⁹⁵At on the basis of unhindered alpha-decay. The 9/2^- state, being the ground state in heavier odd-mass astatine isotopes, was not observed. Received: 16 September 2002 / Accepted: 19 December 2002 / Published online: 25 March 2003 RID="a" ID="a"e-mail: heikki.kettunen@phys.jyu.fi RID="b" ID="b"Present address: Laboratory of Radiochemistry, P.O. Box 55, FIN-00014, University of Helsinki, Finland. RID="c" ID="c"Present address: Radiation and Nuclear Safety Authority, P.O. Box 14, FIN-00881 Helsinki, Finland. Communicated by W. Henning     

The decay of the neutron–rich nucleus 216Bi

The decay of the neutron–rich isotope ²¹⁶Bi, produced by proton–induced spallation at the PS Booster–ISOLDE facility, was investigated by β-γγ, αγ coincidence and spectrum-multiscaling measurements. A new method for reducing isobaric contamination enabled to cover the unknown region “east” of ²⁰⁸Pb for the isobaric chain A=216. The half-life of the β decay of ²¹⁶Bi was found as T_1/2= 135 ± 5 s. Its decay scheme was extended and the possible shell model configurations are proposed. Received: 13 July 1999 / Revised version: 22 September 1999     

High spin states above the α-decaying isomer in 211Po

Prompt and delayed γ-rays in nuclei of the ²⁰⁸Pb region produced in 450 MeV ⁷⁶Ge +²⁰⁸Pb collisions have been studied at GASP. Yrast states above the α-decaying isomer in ²¹¹Po have been located including a 0.25 μs 31/2⁻ isomer at 2135 keV and a 2 μs isomer at 4874 keV. Received: 22 September 1997     

γ Spectroscopy of 209Pb with deep inelastic reactions

High spin states in nuclei around ²⁰⁸Pb were populated in deep inelastic collisions of ⁷⁶Ge, ¹³⁶Xe, and ²⁰⁸Pb projectiles with ²⁰⁸Pb targets at beam energies about 12% above the Coulomb barrier. New states in ²⁰⁹Pb were found by measuring γ-γ-coincidences. They are interpreted as the yrast states that originate from the coupling of one neutron to the lowest excitations of the ²⁰⁸Pb core. The results are discussed in the frame of the shell model. Received: 22 November 1997     

Properties of N=84, even-even nuclei populated in the spontaneous fission of 248Cm

Excited states in the neutron-rich, N=84 nuclei ¹³⁴Sn, ¹³⁶Te and ¹³⁸Xe, populated in the spontaneous fission of ²⁴⁸Cm, were studied to medium spins using the EUROGAM2 array. OXBASH code calculations support the experimental identification of maximum aligned configurations in these isotopes. Empirical shell model calculations agree with the proposed excitation energy of the neutron h_9/2 excitation in the ¹³²Sn region. A discrepancy between the observed and calculated excitation energy of the I^π= 12⁺ level in ¹³⁶Te indicates possible admixtures of collective excitations in this nucleus. Clear signs of collective excitations are observed in ¹³⁸Xe. Received: 10 November 1999 / Revised version: 22 December 1999     

Magnetic properties of the υj15/2 intruder orbital in the superdeformed minimum of 197Pb

This work has established eight cross-talk transitions between the two signature partner superdeformed (SD) bands in ¹⁹⁷Pb with the EUROBALL IV spectrometer. Directional correlations from oriented states measurements confirm the ΔI = 1 character of these transitions. The flat behaviour of the dynamical moment of inertia and the agreement between the experimental and microscopic HF+BCS values of (g _K - g _R)K/Q ₀ suggest that the configuration of the SD bands is based upon the υ[752]5/2^- neutron intruder orbital. The derived effective spin gyromagnetic factor g _s ^eff is found to be not quenched, and is close to the theoretical g _s ^free value. Received: 14 June 2000 / Accepted: 14 September 2000     

New excited superdeformed bands in heavy Pb nuclei: Clue for an octupole softness near the N = 118 gap at large deformation

We report the identification of six new superdeformed (SD) bands in ^197,198Pb observed with the EUROBALL IV spectrometer. The results are interpreted in the framework of cranked Hartree-Fock calculations with approximate projection on the particle number by means of the Lipkin-Nogami method. A mixing between quasi-particle excitations and an octupole vibration is suggested in the two SD isotopes. We have estimated the ordering of the neutron valence orbitals and confirm indirectly a N = 118 SD gap. Received: 20 December 2000 / Accepted: 24 January 2001     

Structure of 136Te and the problem of mass of 134Te

Neutron-rich, N=84 nuclei from the ₁₃₂Sn region, populated in spontaneous fission of ₂₄₈Cm, have been studied with EUROGAM 2. Excited states and their spins and parities in the ₁₃₆Te nucleus were established up to 17ħ. OXBASH code calculations support the experimental identification of maximum aligned configurations in ₁₃₆Te. Empirical shell model calculations for the I_π= 14₊ level in ₁₃₆Te indicate that the adopted mass of the ₁₃₄Te nucleus should be lowered by 200(80) keV. Received: 3 August 1998     

Shape coexistence near the double-midshell nucleus 111Rh

The decay of ¹¹¹Ru obtained from fast on-line chemical and mass separation has been investigated by β-γ-t and γ-γ coincidence techniques. Earlier spin and parity assignments of ¹¹¹Rh levels based on extrapolations of level systematics are confirmed. In particular, the K=1/2 intruder band is supported by the hindrance of E2 transitions between deformed and spherical states and enhancement of intraband E2 transitions. The excitation energies of intruder band members in Rh isotopes show a minimum at ¹⁰⁹Rh₆₄, with two neutrons less than ¹¹¹Rh at the N=66 midshell. This trend, which differs from the one in the higher-Z neighbouring elements Ag and Cd with minima at N=66, follows the evolution of deformation observed in the lower-Z elements Ru and Mo. Received: 25 June 1997 / Revised version: 10 September 1997     

Identification of Rotational Band in Doubly Odd 170Ta

High spin states in ¹⁷⁰Ta have been studied via ¹⁵⁹Tb(¹⁶O,5nγ)¹⁷⁰Ta reaction through excitation functions, K X-γ and γ-γ-t coincidence measurements. Three rotational bands have been identified among which one coupled band and an unfavored δI=2 E2 transition sequence are newly found in this work. The possible quasiparticle configurations of these bands are discussed. Received: 7 November 1997     

High-spin states in 208Pb

High-spin states in ²⁰⁸Pb have been studied by γ-ray-spectroscopy methods in deep inelastic reactions induced by beams of ²⁰⁸Pb, ¹³⁶Xe and ⁷⁶Ge beams on a thick ²⁰⁸Pb target. The 11⁺ ₂ state and new γ-transitions between the one-particle one-hole states of highest spin have been found and electromagnetic matrix elements verified. High-spin states of two-particle two-hole structure have been detected for the first time. The results are compared to shell model calculations with realistic interactions in the complete Kuo-Herling space. Received: 31 October 2000 / Accepted: 26 March 2001     

Observation of intermediate bands feeding the positive-parity yrast band in 155Gd

High-spin states of ¹⁵⁵Gd were populated by using the ¹⁵⁴Sm(α,3nγ)¹⁵⁵Gd reaction at E _α= 33 MeV. γ-γ coincidence, E _γ singles, excitation function, and the DCO ratios were measured. we have identified three intermediate bands with ΔI= 2 feeding the positive yrast band. The bands are interpreted as such candidate bands that are mixed with the negative-parity ground state band. This observation can provide a plausible explanation for unusually large population of the positive-parity yrast band observed in a recent Coulomb excitation. Received: 2 November 1999     

First decay scheme of 113Tc and identification of 113Ru m

Very neutron–rich fission products of the mass chain A=113 obtained from the IGISOL on–line mass separator have been investigated by γγ coincidence techniques and γ-spectra multiscaling. Gamma–rays following β–decay of ¹¹³Tc have been observed for the first time and a new 0.5 s isomeric state has been found in ¹¹³Ru. Received: 10 February 1998     

High-K quasiparticle structures in 159Er and 160Er

A series of new strongly coupled high-K, multi-quasiparticle structures have been observed in the light erbium transitional nuclei, ¹⁵⁹Er and ¹⁶⁰Er. The interpretation of these bands is discussed within the framework of the cranked shell model. These sequences, when taken together with the existing quasiparticle excitations, form a near complete set of low-lying, multi-quasiparticle structures on which a coherent series of aligned angular momentum, band crossing and blocking arguments can be based. The measured B(M1)/B(E2) ratios are compared with geometrical calculations to test the proposed configuration assignments. Received: 19 November 1997     

Intruder states in even-even neutron-rich Pd isotopes

The decays of ¹¹²Rh ^g and ¹¹²Rh ^m obtained as on-line mass separated fission products have been investigated by standard β and γ spectroscopic techniques and γ-γ angular correlations. Low-lying 0⁺ and 2⁺ states are identified in the daughter nucleus ¹¹²Pd. Systematics suggests the existence of an intruder band which is the lowest in ¹¹⁰Pd, i.e. two neutrons before the midshell. Received:13 March 1998     

High-spin structures observed in the 101Tc fission fragment

High-spin states have been studied in ¹⁰¹Tc produced as a fission fragment in the reaction ¹⁷⁶Yb +²⁸Si at 145 MeV. Gamma rays were detected with the EUROGAM2 array. The level scheme of ¹⁰¹Tc has been extended up to 4.2 MeV excitation energy and several band structures are observed. Configurations are assigned to two new bands on the basis of their behaviour and of cranked Hartree-Fock-Bogolyubov calculations. Received: 4 January 1999     

High-spin states in odd-odd 168Lu

High-spin states of odd-odd ¹⁶⁸Lu were observed up to 18ħ for the first time using the ¹⁵⁹Tb(¹³C, 4nγ)¹⁶⁸Lu reaction at E _13C= 58.5 MeV. γ-γ coincidence, E _γ singles, excitation function, and the DCO ratios were measured. Two rotational bands with signature splitting were populated, among which the lower-energy band is identified as π 7/2⁺[404] ⊗ν 5/2⁺[642] in view of alignment and energy systematics. Received: 27 October 1997