Simultaneous measurement of localized heat release with OH/CH2O-LIF imaging and spatially integrated OH∗ chemiluminescence in turbulent swirl flames

The in-situ and localized observation of heat release in turbulent flames is important for the validation of computational modeling of turbulent flows with combustion. In the present work we obtain localized information on heat release rate (HRR) by the commonly accepted technique of the simultaneous and single-shot planar imaging of OH and CH₂O concentrations by laser-induced fluorescence (LIF). Additionally, we combine this with the simultaneous line-of-sight and temporally resolved chemiluminescence detection of OH^?, spatially integrated within the flame volume, interrogated by the laser sheets used for the HRR imaging technique. The combined diagnostic methods are demonstrated for a swirl-stabilized, premixed turbulent methane/air flame of 30-kW thermal power, and they show the existence of correlations between both HRR-sensitive diagnostic techniques.     

Laser imaging system for determination of three-dimensional scalar gradients in turbulent flames

An imaging system for the measurement of three-dimensional (3D) scalar gradients in turbulent hydrocarbon flames is described. Combined line imaging of Raman scattering, Rayleigh scattering, and CO laser-induced fluorescence (LIF) allows for simultaneous single-shot line measurements of major species, temperature, mixture fraction, and a one-dimensional surrogate of scalar dissipation rate in hydrocarbon flames, while simultaneous use of two crossed, planar LIF measurements of OH allows for determination of instantaneous flame orientation. In this manner the full 3D scalar dissipation can be estimated in some regions of a turbulent flame on a single-shot basis.     

3-D airflow measurement using smoke particles

A new 3-D PIV-technique that is applicable to low velocity airflow in a real space such as indoor airflow is proposed, and its performance is inspected through a simulation and an experimental application. In this technique, two parallel planes separated by short distance are illuminated by a pair of laser light sheets of different colors. The visualized images are separated with optical filters, and recorded on VTRs. The 2-D tracer pattern movement on visualized planes is tracked with pattern tracking and the movement normal to the visualized planes is calculated from the difference of tracer concentration between two planes. The simulation result showed that the algorithm proposed here can calculate 3-D velocity field adequately, but the experimental result showed that the luminous intensity difference between two visualized planes became the main source of experimental errors.     

Temperature dependence of intensities of laser-induced fluorescences of ethylbenzene and naphthalene seeded in gas flow at atmospheric pressure

The present study has been carried out with the aim of developing a technique for measuring two-dimensional gas temperature profiles based on two-color fluorescence induced by a one-color laser. The laser sheet of the fourth harmonic (266 nm) from a Nd:YAG laser induced fluorescence in species doped in a nitrogen gas flow. The LIF spectra of seven fluorescent species, namely acetone, methylethylketone, acetaldehyde ethylbenzene, anisole, aniline, and naphthalene, were measured to select the best prospective pair of fluorescent species for this technique. Ethylbenzene and naphthalene show relatively high LIF intensities and their LIF spectra overlap less with each other than with other species. Also, ethylbenzene has a high temperature dependence while naphthalene has a low temperature dependence. Thus by selecting one portion of wavelengths in the range where ethylbenzene or naphthalene is dominant, the temperature of the gas can be determined using the ratio of LIF intensities of the mixture at the two wavelengths with good temperature sensitivity. In addition, a general principle is presented for finding out an optimum pair of wavelengths to obtain a good temperature sensitivity in those LIF spectra.     

Measurements of three-dimensional mean flame surface area ratio in turbulent premixed Bunsen flames

A data processing scheme with particular emphasis on proper flame contour smoothing is developed and applied to measure the three-dimensional mean flame surface area ratio in turbulent premixed flames. The scheme is based on the two-sheet imaging technique such that the mean flame surface area ratio is an average within a window covering a finite section of the turbulent flame brush. This is in contrast to the crossed-plane tomograph technique which applies only to a line. Two sets of Bunsen flames have been investigated in this work with the turbulent Reynolds number up to 4000 and the Damköhler number ranging from less than unity to close to 10. The results show that three-dimensional effects are substantial. The measured three-dimensional mean flame surface area ratio correlates well with a formula similar to the Zimont model for turbulent burning velocity but with different model constants. Also, the mean flame surface area ratio displays a weak dependency on turbulence intensity but a strong positive dependency on the turbulence integral length scale.     

Laser-based volumetric colour-coded three-dimensional particle velocimetry

We present a method of three-dimensional particle velocimetry with a single digital colour camera using multiple colour illumination to encode image depth over a large volume. A copper vapour laser operating at 511 nm is used to pump an optical fibre producing a multiple-wavelength beam via multiple order stimulated Raman scattering. The beam is dispersed and formed into a stack of thin sheets to illuminate a volume of space. The spatial co-ordinates of particles imaged within the illuminated volume are obtained from their imaged x,y positions with depth discerned from particle hue (set by the wavelength of illumination). The method exhibits an RMS depth error of 3% in relation to the thickness of the illuminated region. This paper reports a proof-of-principle of three-dimensional particle imaging using a multi-wavelength laser source with a view to 3D-3C particle velocimetry.     

Visualization of Crevice Flow in an Engine Using Laser-Induced Fluorescence

A simultaneous visualization technique of reacting and unburned zones using laser-induced fluorescence (LIF) was applied to a high-pressure combustion field in an engine cylinder. Crevice flow from a crevice between a piston and a cylinder wall of a spark ignition gas engine was visualized by LIF of OH and acetone. OH was excited simultaneously with acetone that was seeded into fuel as a tracer by an excitation light at 283.92 nm. Fluorescence signals from each species were detected individually by two intensified CCD cameras using optical band-pass filters which transmit fluorescence wavelength of OH and acetone, respectively. Pressure- and temperature-dependence of LIF signals from each species were evaluated. From the visualized images, it was clarified that oxidation of the crevice flow is stopped at the time of exhaust valve opening. Effects of exhaust port pressure on the oxidation process were investigated.     

Toluene laser-induced fluorescence for in-cylinder temperature imaging in internal combustion engines

A single-laser single-camera imaging technique was demonstrated for in-cylinder temperature distribution measurements in a direct-injection internal combustion engine. The single excitation wavelength two-color detection technique is based on toluene laser-induced fluorescence (LIF). Toluene-LIF emission spectra show a red-shift with increasing temperature. Temperature can thus be determined from the ratio of the signal measured in two separate wavelength ranges independent of the local tracer concentration, laser pulse energy, and the intensity distribution. An image doubling and filtering system is used for the simultaneous imaging of two wavelength ranges of toluene LIF onto the chip of a single camera upon excitation at 248 nm. The measurements were performed in a spark-ignition engine with homogeneous charge and yielded temperature images with a single-shot precision of approximately ±?6%.     

Simultaneously calibrated two-line atomic fluorescence for high-precision temperature imaging in sooting flames

Simultaneously calibrated, non-linear two-line atomic fluorescence (SC-nTLAF) thermometry for application in turbulent sooting flames has been developed to increase the precision of single-shot, planar measurements of gas temperature. The technique has been demonstrated in both steady and turbulent sooting flames, showing good agreements with previous optical measurements. The SC-nTLAF involves imaging simultaneously laser-induced fluorescence (LIF) of atomic indium in both the target flame and a non-sooting calibration flame for which the temperature distribution is known. The LIF intensities from the reference flame enable correction for fluctuations, not only in the laser power, but also in the laser mode. The resulting precision was found to be ±67 K and ±75 K (based on one standard deviation) in the rich and oxidizing regions of a steady sooting flame for which the measured temperature was 1610 K and 1854 K, respectively, with a spatial resolution of 550 × 550 µm². This corresponds to a relative precision of ∼ 4.1%. The resulting precision in the single-shot temperature images for a well-characterized, lifted ethylene jet diffusion flame (fuel jet Reynolds number = 10,000) compares favorably with previously reported data obtained with shifted-vibrational coherent anti-Stokes Raman spectroscopy (CARS), together with increased spatial resolution. The planar imaging also provides more details of the temperature distribution, particularly in the flame brush region, which offers potential for measurement of more parameters, such as gradients and spatial corrections. The new calibration method has also achieved a significant time-saving in both data collection and processing, which is an estimated total of ∼ 60%–70% compared with conventional nTLAF.     

Visualization of soot formation from evaporating fuel films by laser-induced fluorescence and incandescence

Late-evaporating liquid fuel wall-films are considered a major source of soot in spark-ignition direct-injection (SIDI) engines. In this study, a direct-injection model experiment was developed to visualize soot formation in the vicinity of evaporating fuel films. Isooctane is injected by a multi-hole injector into the optically accessible part of a constant-flow facility at atmospheric pressure. Some of the liquid fuel impinges on the quartz-glass windows and forms fuel films. After spark ignition, a turbulent flame front propagates through the chamber, and subsequently sooting combustion is detected near the fuel films. Overlapping laser light sheets at 532 and 1064 nm excite laser-induced fluorescence (LIF) of polycyclic aromatic hydrocarbons (PAH) -potential soot precursors- and laser-induced incandescence (LII) of soot, respectively. The 532 nm light sheet has low fluence to avoid the excitation of LII. The LII and LIF signals are detected simultaneously and spectrally separated on two cameras. In complementary line-of-sight imaging, the fuel spray, chemiluminescence, and soot incandescence are captured with a high-speed color camera. In separate experiments, toluene is added to the isooctane as a fluorescent tracer and excited by pulsed 266 nm flood illumination. From images of the LIF signal, the fuel-films’ thickness and mass evolutions are evaluated. The films survive the entire combustion event. PAH LIF is found in close vicinity of the evaporating fuel films. Soot is found spatially separated from, but adjacent to the PAH, both with high spatial intermittency. Average images additionally indicate that soot is formed with a much higher spatial intermittency than PAH. Images from the color camera show soot incandescence earlier and in a similar region compared to soot LII. Chemiluminescence downstream of the soot-forming region is thought to indicate the subsequent oxidation of fuel, soot, and PAH.     

Quantitative measurement of naphthalene in low-pressure flames by jet-cooled laser-induced fluorescence

We have recently developed a new laser based set-up (Jet-Cooled Laser-Induced Fluorescence) for the analysis of aromatic compounds generated in flames. This method relies on the extraction of the species from the flame via a thin microprobe and their direct analysis inside a supersonic free jet by Laser-Induced Fluorescence (LIF). Under the supersonic conditions of the jet, the vibronic spectra of the molecules become structured as the possibility of electronic transitions is reduced, allowing their selective detection by LIF. In addition, due to the very low quenching efficiency inside the jet, LIF signals can be directly related to the population of the probed species and easily calibrated into absolute concentrations. All of the work presented here has been carried out for naphthalene, which is an important PAH involved in soot formation mechanisms. The calibration procedure is described in detail. We also report a detailed study of the quantitative features of the technique, in particular cooling efficiencies and collision rates as well as some additional potential factors that could bias the quantitative aspect of the method. Finally, the possibilities of the technique for the measurement of PAH within flames in the presence of soot particles along with its accuracy and reproducibility are demonstrated by recording naphthalene mole fractions profiles in several rich CH₄/O₂/N₂ flames. A detection limit of the order of a ppb is demonstrated under flame conditions with and without the presence of soot particles.     

Estimation of the droplet size spread with the laser induced fluorescence/Mie technique

The laser measurement technique based on the ratio between the laser induced fluorescence (LIF) and the scattered light (Mie) intensities of droplets is presently limited to the evaluation of the Sauter mean diameter of the droplets. The important measurement of the droplet size spread is currently missing. An extension of the LIF/Mie technique for the measurement of droplet size spread is proposed here and is evaluated numerically. The method is based on the imperfect relationships between the scattered light intensity and the droplet surface area or the fluorescent light intensity and the droplet volume, which convey additional information that can be used to evaluate the droplet size spread.     

Flame turbulences recorded at 1 kHz using planar laser induced fluorescence upon hot band excitation of OH radicals

Laser-induced fluorescence (LIF) in flames is excited by a diode-pumped all-solid-state disk laser system which operates at a pulse repetition rate of 1 kHz and a tunable wavelength around 1030 nm. The laser fundamental is converted to 343 nm and used to excite into the hot band transition of OH radicals in H₂/O₂ diffusion flames of an industrial burner and in the premixed flame of a microburner. The OH radical emission around 308 nm is resolved spectrally and spatially using a light-sheet technique. Imaging of the planar LIF (PLIF) by a gated camera visualizes the turbulent flame behavior on the millisecond time scale without averaging. To our knowledge this is the first time that an all-solid-state laser providing at the same time a kHz repetition rate as well as pulse energies of up to 5.5 mJ is available for PLIF observation of OH radicals. PACS 33.50.-j; 42.55.Xi; 82.33.Vx     

应用理性优化蚁群算法提高激光三维复制的重现度

三维复制人工耳和打印手枪把激光三维复制技术推向新的一页。激光三维扫描是激光应用中一个新兴的重要领域,在三维复制中扮演着无可替代的角色,其复制精度在目前所有复制技术中是最高的。而重现度标志着复制结果与复制对象几何形状上的一致程度,是激光三维复制最重要的指标。分析了激光三维复制的误差,得出激光扫描的点云数据处理是减小误差、提高重现度的关键所在的结论。主要创新点在于,在传统蚁群算法的基础上,将提出理性优化蚁群算法应用于激光三维复制中的数据处理。经计算对比发现,有效减小了复制的误差,提高了复制的重现度。     

Light-beat measurement of phase fluctuations of a laser beam propagating through a turbulent atmosphere

Real-time processing of phase fluctuations of a laser beam has been considered in association with the phase of a beat signal of light. Two fine light beams, included in the expanded laser beam propagating through an artificially turbulent atmosphere, are shifted in frequency by two successive ultrasonic light modulators at slightly different frequencies, so that they can be photomixed to generate a beat signal whose phase is randomly modulated. The fluctuating phase difference of the two fine beams can be revealed in real-time from the phase of the beat signal. It is immediately processed by a conventional wave-height analyzer, from which a probability density and its variance are simply obtained. When the atmosphere is perturbed by the blower with a heater alone, the probability density takes the Gaussian form and the variance obeys approximately the 5/3-power law as the two beam separation is increased. When the turbulent atmosphere is further disturbed by some metallic mesh, the probability density does not always obey Gaussian statistics, but it depends greatly on the turbulent state of the atmosphere.     

Xe1v离子激光感生荧光用于医用X射线ZnCdS:Ag荧光屏的性能研究

本文叙述了利用同轴结构Xe1v离子激光器的UVλ=365nm激光作为激发光源的激光感生荧光(LIF)实验系统,对医用X射线ZnCdS:Ag荧光屏的发光性能进行了研究.LIF方法能方便而高灵敏地同时测得荧光光谱与寿命,和传统的紫外灯激发及X射线激发的结果一致,可以完全避免X射线对人体的有害辐射.     

Three-dimensional temperature measurement in turbulent thermal convection by extended range scanning liquid crystal thermometry

The usable temperature range of liquid crystal thermometry has been extended and used to measure three-dimensional temperature fields in turbulent thermal convection. The color of the liquid crystals is calibrated against temperature using the standard method in which hue is the single input variable and two new methods: hue/intensity as input variable, and hue, saturation and intensity as input variables to a neural network. Relative to the hue calibration, the new methods extend the range over which temperature can be measured by more than 100%. Three-dimensional temperature measurements of turbulent thermal convection over smooth surfaces were carried out at a flux Rayleigh number of 3 × 10⁹ by scanning a white light sheet normal to the visualized image plane and capturing a number of sequential images at various positions of the light sheet. Stacks of the planar data were composed into three-dimensional temperature distributions. The results indicate the presence of an irregular spoke pattern over the surface and the generation of plumes from the intersections of the patterns, consistent with other investigations.     

Attenuation corrections for in-cylinder NO LIF measurements in a heavy-duty Diesel engine

Quantification of the nitric oxide (NO) concentration inside the cylinder of a Diesel engine by means of laser-induced fluorescence (LIF) measurements requires, amongst others, knowledge of the attenuation of the ultraviolet radiation involved. We present a number of laser diagnostic techniques to assess this attenuation, enabling a correction for laser intensity and detection efficiency of the raw NO LIF data. Methods discussed include overall laser beam transmission, bidirectional laser scattering (bidirectional LIF), spectrally resolved fluorescence imaging, and Raman scattering by N₂. A combination of techniques is necessary to obtain the complete attenuation of laser beam and NO fluorescence. The overall laser beam transmission measurements and bidirectional LIF measurements (the latter yielding spatially resolved transmission) provide evidence of a non-uniform attenuation distribution, with predominant attenuation within or near the piston bowl. Fluorescence imaging of multiple vibrational bands through a spectrograph is shown to be a powerful method for obtaining spatially resolved data on the transmission losses of fluorescence. Special attention is paid to the role of CO₂ and O₂ as UV light absorbers, and the consequences to different excitation-detection schemes for NO. PACS 82.33.Vx; 42.62.Fi; 33.20.t     

Molecular contrast in optical coherence tomography by use of a pump-probe technique

We describe a novel technique for contrast enhancement in optical coherence tomography (OCT) that makes possible molecular-specific imaging for what is believed to be the first time. A pump-probe technique is employed in which a pulsed pump laser is tuned to ground-state absorption in a molecule of interest. The location of the target molecule population is derived from the resulting transient absorption of OCT sample-arm light acting as probe light. A signal processing technique for three-dimensional localization of the transient absorption signal is described, and preliminary results exhibiting OCT contrast from methylene blue dye in multilayer and scattering phantoms are presented.     

2D mixture fraction measurements in a high pressure and high temperature combustion system using NO tracer-LIF

Mixture fraction measurements in a jet-in-cross flow configuration at high pressures (15 bar) and temperatures (above 1000 K) were performed using planar laser induced fluorescence of nitric oxide (NO-PLIF) as trace species. The goal was the evaluation of this tracer LIF technique for the characterization of the mixing of fuel and hot exhaust gas in the mixing channel. The fuel (natural gas (NG) or H₂/N₂/NG mixture) along with the tracer were injected into the crossflow of the exhaust gas and PLIF measurements were performed in different planes. In order to relate the measured NO-LIF signal to fuel concentration and mixture fraction, effects of pressure, temperature and species concentration were taken into account. Numerical calculations and spectroscopic simulations that mimic the experimental conditions were performed to identify excitation schemes that give optimum correlations between the NO-LIF signal and the mixture fraction. The measured NO-PLIF images were transformed into mixture fraction plots using the computed correlations. The paper reports on the experimental challenges encountered during the measurements and the steps taken to overcome those difficulties. Examples of mixture fraction distributions are presented and discussed. The paper concludes with a detailed analysis on the accuracy of the measured mixture fraction values.