Efficient frequency upconversion of coherent radiation from 10.26 to 1.187 μm in a GaSe crystal

Frequency upconversion of laser pulses at 10.26 μm to those at 1.187 μm was achieved in the presence of Nd:YAG laser pulses based on difference-frequency generation in a 10 mm-long GaSe crystal. The highest power conversion efficiency for the parametric conversion was determined to be 20.9%, corresponding to the photon conversion efficiency of 2.42%. This value is two orders of magnitude higher than the highest value reported on GaSe in the literature. The saturation of the output power at 1.187 μm as the input power at 10.26 μm was increased, due to the back conversion, i.e. 1.187 μm + 10.26 μm → 1.064 μm, was clearly evidenced. Such a parametric process has potential for achieving sensitive detections of mid-infrared radiation.     

Multi-order diffractive optical elements for achromatic interconnections at 1.30 μm and 1.55 μm

We propose a class of diffractive components allowing free-space optical systems to operate at the two telecommunication wavelengths simultaneously. These are fifth order diffractive components working at the sixth order at 1.30 μm and at the fifth order at 1.55 μm. Simulation results showing the link efficiency between two single-mode fibres as a function of the wavelength are presented. The width of the two transmission windows depends on the architecture of the whole system, which must be designed in accordance with technological realizability.     

Development of a 4–15 μm infrared GaAs hyperspectral QWIP imager

In the on-going evolution of GaAs quantum well infrared photodetectors (QWIPs) we have developed a four band, 640 × 512, 23 μm × 23 μm pixel array which we have subsequently integrated with a linear variable etalon (LVE) filter providing over 200 spectral bands across the 4–15.4 μm wavelength region. This effort was a collaboration between NASA’s Goddard Space Flight Center (GSFC), the Jet Propulsion Laboratory (JPL) and the Army Research Laboratory (ARL) sponsored by the Earth Science Technology Office of NASA. The QWIP array was fabricated by graded molecular beam epitaxial (MBE) growth that was specifically tailored to yield four distinct bands (FWHM): Band 1; 4.5–5.7 μm, Band 2; 8.5–10 μm, Band 3; 10–12 μm and Band 4; 13.3–14.8 μm. Each band occupies a swath that comprises 128 × 640 elements. The addition of the LVE (which is placed directly over the array) further divides the four “broad” bands into 209 separate spectral bands ranging in width from 0.02 μm at 5 μm to 0.05 μm at 15 μm. The detector is cooled by a mechanical cryocooler to 46 K. The camera system is a fully reflective, f/4.2, 3-mirror system with a 21° × 25° field of view. The project goals were: (1) develop the 4 band GaAs QWIP array; (2) develop the LVE and; (3) implement a mechanical cryocooler. This paper will describe the efforts and results of this undertaking with emphasis on the overall system characteristics.     

Observations of ω0/2 harmonic emission from 0.35μm laser-irradiated plasmas

Observations of ω₀/2 harmonic emission from both spherical and plane targets irradiated by 0.35 μm, 800 ps laser pulses have been obtained with simultaneous high spectral and temporal resolutions of 16 Å and 20 ps respectively. The ω₀/2 harmonic emission spectrum is interpreted as providing a direct measurement of the frequency of the ω₀/2 plasma waves and hence can be used to estimate the electron temperature.     

Near-infrared sources in the 1–1.3 μm region by efficient stimulated Raman emission in glass fibers

Low-loss glass fiber waveguides are found to be excellent media for Raman lasers and amplifiers in the near-infrared region of the spectrum. Multiwavelength emission in the 1–1.3 μm range is readily obtained by efficient stimulated Raman scattering in single-mode silica fibers. With a 1.064 μm pulsed pump of 250 W in a 175-m, 6-μm diameter single-mode silica fiber we observed four orders of Stokes radiation at 1.12 μm, 1.18 μm, 1.23 μm and 1.3 μm, respectively. Our results imply that pulsed tunable stimulated Raman emission in this wavelength region is possible using kW tunable infrared dye lasers near 1 μm as pumps. These sources are useful for studying the dispersion of glass fibers as well as for other spectroscopic applications.     

Pulsewidth-dependence of nonlinear energy deposition and redistribution in Si, GaAs and Ge during 1 μm picosecond irradiation

We have used 1 μm pulses ranging in duration from 4–260 ps to measure the pulsewidth dependence of the nonlinear absorption, melting threshold, and resolidification morphologies of Si, GaAs, and Ge. With these materials, we have been able to quantify a variety of nonlinear absorption processes with a single excitation wavelength. We find that the fluence required to melt Si and GaAs is roughly proportional to the square root of the pulsewidth while that required for Ge is nearly pulsewidth independent. A crystalline-to-amorphous transition is observed in Si for pulses less than 10 ps and in GaAs for all pulsewidths, but no such transition is observed in Ge. These observations are shown to be consistent with the various energy deposition and redistribution mechanisms present in each material. Finally, we have used the active nonlinearities in Si and GaAs to construct optical limiters designed to protect sensitive optical components from intense 1 μm radiation.     

Study of pulse compression from 1.5 μm distributed feedback lasers by a gires-tournois interferometer

In this paper, the compression experiments of picosecond optical pulses from a gain-switched InGaAsP distributed feedback (DFB) laser at a 1.5 μm wavelength range using a Gires-Tournois (G-T) interferometer are reported. Ultrashort optical pulses with a pulsewidth of 6.6 ps, repetition rate of 2.4 GHz, and peak power in excess of 200 mW are obtained. The compression ratio is close to 5. The explanation for the experimental results is given, and the pulse's compression characteristics of a G-T inteferometer are discussed by a computer simulation analysis.     

Transient analysis of degenerate four-wave mixing in saturable absorbers: application to Cr:GSGG at 1.06 μm

We introduce a model of degenerate four-wave mixing in saturable absorbers in the transient regime when the interacting pulses have a duration much shorter than the lifetime of the excited-state level. Our model takes into account of the depletion and the mutual interaction of the pump waves. We study the influence of excited-state absorption on phase conjugate reflectivity. This theory agrees with experimental investigations made in Cr⁴⁺:GSGG with nanosecond pulses at λ₀ = 1.06 μm. A reflectivity of 0.6% is achieved and imaging capabilities are demonstrated.     

Radiative properties of cirrus clouds in the infrared (8–13 μm) spectral region

Atmospheric radiation in the infrared (IR) 8–13 μm spectral region contains a wealth of information that is very useful for the retrieval of ice cloud properties from aircraft or space-borne measurements. To provide the scattering and absorption properties of nonspherical ice crystals that are fundamental to the IR retrieval implementation, we use the finite-difference time-domain (FDTD) method to solve for the extinction efficiency, single-scattering albedo, and the asymmetry parameter of the phase function for ice crystals smaller than 40 μm. For particles larger than this size, the improved geometric optics method (IGOM) can be employed to calculate the asymmetry parameter with an acceptable accuracy, provided that we properly account for the inhomogeneity of the refracted wave due to strong absorption inside the ice particle. A combination of the results computed from the two methods provides the asymmetry parameter for the entire practical range of particle sizes between 1 and 10,000 μm over the wavelengths ranging from 8 to 13 μm. For the extinction and absorption efficiency calculations, several methods including the IGOM, Mie solution for equivalent spheres (MSFES), and the anomalous diffraction theory (ADT) can lead to a substantial discontinuity in comparison with the FDTD solutions for particle sizes on the order of 40 μm. To overcome this difficulty, we have developed a novel approach called the stretched scattering potential method (SSPM). For the IR 8–13 μm spectral region, we show that SSPM is a more accurate approximation than ADT, MSFES, and IGOM. The SSPM solution can be further refined numerically. Through a combination of the FDTD and SSPM, the extinction and absorption efficiencies are computed for hexagonal ice crystals with sizes ranging from 1 to 10,000 μm at 12 wavelengths between 8 and 13 μm.

Calculations of the cirrus bulk scattering and absorption properties are performed for 30 size distributions obtained from various field campaigns for midlatitude and tropical cirrus cloud systems. Ice crystals are assumed to be hexagonal columns randomly oriented in space. The bulk scattering properties are parameterized through the use of second-order polynomial functions for the extinction efficiency and the single-scattering albedo and a power-law expression for the asymmetry parameter. We note that the volume-normalized extinction coefficient can be separated into two parts: one is inversely proportional to effective size and is independent of wavelength, and the other is the wavelength-dependent effective extinction efficiency. Unlike conventional parameterization efforts, the present parameterization scheme is more accurate because only the latter part of the volume-normalized extinction coefficient is approximated in terms of an analytical expression. After averaging over size distribution, the single-scattering albedo is shown to decrease with an increase in effective size for wavelengths shorter than 10.0 μm whereas the opposite behavior is observed for longer wavelengths. The variation of the asymmetry parameter as a function of effective size is substantial when the effective size is smaller than 50 μm. For effective sizes larger than 100 μm, the asymmetry parameter approaches its asymptotic value. The results derived in this study can be useful to remote sensing studies of ice clouds involving IR window bands.     

A DFG spectrometer at 3 μm for high resolution molecular spectroscopy and trace gas detection

We report the realization and characterization of a spectrometer based on difference frequency generation using a periodically poled lithium niobate crystal. As signal and pump lasers we used a diode-pumped Nd–YAG laser (λ=1.064 μm) and an extended cavity semiconductor diode laser (λ=0.785 μm), respectively. The mid-infrared coherent radiation was produced at 3 μm with a maximum power of about 160 nW obtained with 340 mW of signal and only 3.4 mW of pump. That corresponds to an efficiency of 0.01%/Wcm, which is in good agreement with other data available in literature. The generated radiation around 3 μm has allowed us to study fundamental absorption bands of molecules of great atmospheric and physical interest such as water vapor and the hydroxyl free radical. In this work we report preliminary spectroscopic results concerning the ν₁ 5₄₁→6₅₂ H₂O line at 2.968 μm. In particular, for this line we provide the first experimental estimation of self-, N₂- and O₂-broadening coefficients.     

Stimulated four-photon mixing and efficient polychromatic visible light generation in SiO2-based single-mode optical fibers pumped at 1.319 μm

The generation of near-infrared and intense visible light through stimulated multi-wave mixing processes in single-mode silica-based optical fibers pumped by a Q-switched and mode-locked Nd:YAG laser operated at 1.319 μm is described. The experimental results show that intense infrared light around 1.2 μm is produced via selp-hase-matched four-photon mixing at the minimum group velocity dispersion region of pure SiO₂-core and P₂O₅-doped silica fibers. In the visible spectral region, from 580 nm to 600 nm, 20 W peak power 100-ps pulses were generated by pumping single spans of single-mode P₂O₅-doped and undoped SiO₂-core fibers with 1.319-μm laser pulses. The signal light generated in such fibers propagated in the LP₀₂ fiber mode and exhibited a threshold power that depended upon the fiber length and a critical length that was power dependent. Also, it exhibited an asymmetrical spectrum of a few nanometers bandwidth, with a long tail toward high frequencies. For GeO₂-doped silica-based fibers, a multiple-wavelength visible signal propagating in several high-order fiber modes was generated.     

Measurements and interpretation of the absorption of 0.35 μm laser radiation on planar targets

We report on experimental plasma absorption of 0.35 μm radiation incident on plane targets. Absorption fractions between 50 and 98% were found for UV pulses of 90 and 450 ps duration on planar CH, nickel, and gold targets for intensities between 10¹³ and 3 × 10¹⁵ W/cm². The results are in agreement with computer calculations using inverse bremsstrahlung absorption and a thermal electron heat flux limiter between 0.03 and 0.06     

Gas source MBE grown wavelength extended 2.2 and 2.5 μm InGaAs PIN photodetectors

Using homo-junction structure and relative thin linear graded In_xGa_1−xAs as the buffer layer, extended wavelength InGaAs PIN photodetectors with cut-off wavelength of 2.2 and 2.5 μm at room temperature have been grown by using GSMBE, and their performance over a wide temperature range have been extensively investigated. For those 2.2 or 2.5 μm detectors with 100 μm diameter, the typical dark current (V_R = 10 mV) and R₀A are 57 nA/10.3 Ω cm² or 67 nA/12.7 Ω cm² at 290 K, and 84 pA/4.70 kΩ cm² or 161 pA/3.12 kΩ cm² at 210 K respectively. The thermal activation energies of the dark current are 0.447 eV or 0.404 eV for 2.2 or 2.5 μm detectors respectively.     

Transmission experiments in the 1.2-1.6 μm wavelength region using graded-index optical fiber cables

Optical fiber transmission systems with extremely long repeater spacing are very attractive for various applications both in land and undersea communication systems. This paper describes the results of transmission experiments, using low-loss fibers in the 1.2-1.6 μm wavelength region. Graded-index optical fibers having an optimum profile at 1.27 μm were manufactured in cables. Average bandwidth was 1,275 MHz-km, and the average optical loss was 0.6 dB/km. The 52.6-km and 62.3-km repeater spacings were realized at 100 Mb/s and 32 Mb/s transmission, respectively, using InGaAsP/InP LD and Ge-APD. The 21.5-km and 12.0-km repeater spacings at 32 Mb/s were also realized by 1.2μm and 1.5μm LEDS, respectively.     

Pulsed first-overtone CO laser: effective source of IR radiation in spectral range of 2.5–4.0 μm

Spectral properties of radiation of a pulsed electron-beam controlled discharge laser operating on the first-overtone transitions (Δv=2) of CO molecules have been studied both experimentally and theoretically. Various sets of dielectric mirrors with high reflectivity in the wide range of overtone spectrum have been used for the laser resonator. Multiwavelength lasing has been obtained in the wide spectral range of 2.5–4.0 μm. Efficiency of the laser operating on few vibrational transitions within a relatively narrow spectral range comes up to 5% at entirely suppressed fundamental band (Δv=1) lasing. Spectral characteristics of the overtone laser operating on a selected set of vibrational transitions have been analyzed theoretically. A comparison of the experimental and theoretical data has been made.     

τ→μγ and μ→eγ as probes of neutrino mass models

We discuss the possibility of discriminating between different supersymmetric see-saw models by improving the experimental sensitivity to charged lepton flavour violating processes. Assuming a hierarchical neutrino mass spectrum, we classify see-saw models according to how the hierarchy Δm²Δm²_atm is generated, and study the predictions of each class for the branching ratios of τ→μγ and μ→eγ. The process τ→μγ is found to be a particularly promising tool to probe the fundamental see-saw parameters, and especially to identify the origin of the large atmospheric mixing angle. Predictions for μ→eγ are more model-dependent. We point out that, even with an improvement of the experimental sensitivities by three orders of magnitude, both τ→μγ and μ→eγ could escape detection in models where Δm²_atm is determined by one of the lightest right-handed neutrinos.     

Echo-Planar Imaging of Porous Media with Spatial Resolution below 100 μm

A modified version of the echo-planar imaging technique incorporating a Carr–Purcell train of 180° rf pulses (PEPI) has been implemented on a standard spectrometer. It is demonstrated that artifacts in the image due to cumulative errors in the rf field can be reduced by replacing each 180° pulse by a composite sequence of three rf pulses. Artifact-free 3D images at 94 μm voxel resolution are obtained within 15 min. This technique has been applied to study the drying process in an initially water-saturated model porous medium with characteristicT^*₂of order 700 μs.     

Continuous-wave and passively Q-switched Nd:GdVO4 lasers at 1.06 μm end-pumped by laser-diode-array

We demonstrated a diode-end-pumped continuous-wave and passively Q-switched Nd:GdVO₄ laser operating at 1.06 μm wavelength with a three-mirror folded resonator. The maximum continuous-wave output power of 8.18 W was obtained at the incident pump power of 22.5 W, with the corresponding optical conversion efficiency of 36.4%. For Q-switched operation, the maximum average output power was measured to be 4.64 W with the corresponding optical conversion efficiency of 25.8%, when the initial transmission of Cr⁴⁺:YAG crystal was 90%. The shortest pulse width of 83 ns, the largest pulse energy of 20.7 μJ and the highest peak power of 246.7 W were obtained when the Cr⁴⁺:YAG crystal with an initial transmission of 85% was used.     

A simple technique for generating single-mode nanosecond pulses of 10.6 μm radiation

A technique for generating short pulses of 10.6 μm radiation is presented. This technique produces pulses of 10⁻⁹−10⁻⁸ s duration of single-mode radiation with diffraction-limited divergence of the beam and good extraction efficiency of the energy stored in the cavity.     

GaInAsSb/AlGaAsSb lasers in the wavelength range between 2.73 μm and 2.93 μm

Compressively strained multiple quantum well lasers in the GaInAsSb/AlGaAsSb material system are reported. Indium concentrations between 40% and 47.5% were chosen for the GaInAsSb quantum wells. Compressive strains varied between 1.16% and 1.43%. The lasers worked continuous wave at room temperature up to a wavelength of 2.81 μm. For a laser with 2.93 μm wavelength continuous wave operation was found up to a temperature of −23°C. This laser worked in pulsed operation at 15°C.