Two-photon resonance degenerate four-wave mixing in a three-level polar molecule (model calculations)

The third-order non-linear susceptibility, ⁽³⁾(; , , –), describing the phase conjugation by degenerate four-wave mixing (DFWM) is calculated for a three-level polar system under a two-photon resonance (TPR) condition. The part of the susceptibility expressed only by the transitional dipole moments and the part resulting from the permanent dipole moments are distinguished. The spectra of ⁽³⁾(; , , –), as well as the DFWM power-reflection and power-transmission spectra near to the TPR, are modelled for polar molecules. The effect of enhanced reflectivity of TPR-DFWM is obtained numerically.     

Dynamic scaling for spin glasses near the de Almeida-Thouless line

We calculate the dynamic local susceptibility () of an Ising spin glass near the de Almeida-Thouless (AT) line within the soft spin dynamics for the Sherrington-Kirkpatrick model. We find a crossover from analytic behaviour of () at =0 above the AT line to a power law behaviour ()(–i) ^v on the AT line and discuss the analytic properties of the crossover function. The frequencyscale is proportional to ^1/v , where measures the distance from the AT line. We determine the spectrum of relaxation times which diverge as ^1–1/v . The average relaxation time diverges as ^–1/v wherev1/2. In addition we determine the absolute frequency scale and prove the consistency of the ansatz of Sompolinsky and Zippelius ()–(0)(–i) ^v at and below the AT line.     

Three-Mode Entangled State Representation of Continuum Variables and Optical Four-Wave Mixing

We establish a new three-mode entangled state representation , of continuum variables, which make up a complete set. Using optical four-wave mixing and a beam splitter transform we can prepare , . Based on , a new number-difference--operational-phase uncertainty relation is established and the corresponding squeezing dynamics is discussed.     

Periodic Thermodynamics

This paper develops the thermodynamics of quantum Floquet systems, i.e., quantum systems driven by an arbitrarily strong periodic perturbation, which are in weak interaction with a heat bath. The physics differs in an essential way from that of undriven systems, because the usual energy conservation law, for interactions between the system and heat bath, is changed to +E=0, ±, ±2,... where is the driving frequency, is the difference of the so-called quasi-energies of the Floquet states and E the excitation energy of the bath. That is, a transition between two given physical Floquet states will be accompanied by bath transitions with many different energy changes, E=–+m, where m is an arbitrary integer. This results in a breakdown of detailed balance. There is a steady state in which the system has periodic fluctuations of period T=2/. The steady state density matrix is diagonal in the Floquet states, with all Floquet states having finite weights, even at zero temperature. Experimentally favorable conditions for studying periodic thermodynamics are briefly discussed.     

QCD sum rule analysis of the coupling constant g ωσγ

We employ QCD sum rules to calculate the coupling constant g by studying the three point -correlation function. Our result complements the analysis of this coupling constant utilizing the experimental value of the ⁰⁰ decay rate studied within the framework of chiral perturbation theory including vector meson and meson intermediate states.     

Cubic nonlinear tensor of a ferromagnet

The nonlinear properties of a ferromagnet are studied. Many-time retarded Green's functions are used to obtain an expression for the cubic nonlinearity tensor with allowance for spatial dispersion of a uniaxial ferromagnet. The components due to the dipole-dipole interaction of the spins and also due to the anisotropy energy are found. A comparative analysis is made of the different components of the cubic nonlinearity tensor in both the nonresonance case and for various resonances, in particular when ₀, 3 2w₀, 2 ₀, 3 ₀ for the case in tripling of the frequency. Here, is the frequency of the incident wave and ₀ is the frequency of uniform precession. It is shown that in the non-resonance case the largest components are those that are nonvanishing when no allowance is made for spatial dispersion; in the resonance cases the largest components are those due to the dipole-dipole interaction of the ferromagnetism spins.Translated from Izvestiya VUZ. Fizika, No. 12, pp. 53–58, December, 1973.     

Dynamical Localization II with an Application to the Almost Mathieu Operator

Several recent works have established dynamical localization for Schrödinger operators, starting from control on the localization length of their eigenfunctions, in terms of their centers of localization. We provide an alternative way to obtain dynamical localization, without resorting to such a strong condition on the exponential decay of the eigenfunctions. Furthermore, we illustrate our purpose with the almost Mathieu operator, H _{, ,} =–+ cos(2(+x)), 15 and with good Diophantine properties. More precisely, for almost all , for all q>0, and for all functions ²( ) of compact support, we show that The proof applies equally well to discrete and continuous random Hamiltonians. In all cases, it uses as input a repulsion principle of singular boxes, supplied in the random case by the multi-scale analysis.     

Ultrasound in spin glasses

The change of the sound velocity v(,T) and the damping of sound waves (,T) in spin glasses are calculated in the frame-work of an Ising model with a random distribution of exchange interactions. The calculation is based on linearized equations of motion for the spins and on an improved mean field approximation which includes the Onsager reaction field. Near to the freezing temperatureT _f and at high temperatures v(,T) and (,T) turn out to be approximately proportional to the real and the imaginary parts of the dynamical susceptibility. For the special case of infinite range interactions atT=T _f one has v(, T_f) ( )^1/2 and (, T_f) (/)^1/2 where is the relaxation time of independent spins. However, already slightly aboveT _f the frequency dependence of both quantities becomes rather small for RKKY spin glasses. At high temperatures both, v(,T) and (,T) vary asT ^–1.SFB 125 Aachen-Jülich-Köln     

Extensible Embeddings of Black-Hole Geometries

Removing a black hole conic singularity by means of Kruskal representation is equivalent to imposing extensibility on the Kasner–Fronsdal local isometric embedding of the corresponding black hole geometry. Allowing for globally non-trivial embeddings, living in Kaluza–Klein-like M ₅ × S ₁ (rather than in standard Minkowski M ₆ ) and parametrized by some wave number k, extensibility can be achieved for apparently forbidden frequencies in the range ₁ (k) ₂ (k). As k 0, _{1, 2} (0) _H (e.g., _H = 1/4M in the Schwarzschild case) such that the Hawking–Gibbons limit is fully recovered. The various Kruskal sheets are then viewed as slices of the Kaluza–Klein background. Euclidean k discreteness, dictated by imaginary time periodicity, is correlated with flux quantization of the underlying embedding gauge field.     

Calculation of the dispersion of the third-order optical nonlinearity in C60 films

Using wave functions determined from ground-state local-density calculations, we have calculated the wave-dispersed free response of the optical nonlinear polarizability ⁽³⁾(–3;,,), for the C₆₀ molecule and ⁽³⁾(–3;,,) i.e. Third-Harmonic Generation (THG) for films using a sum-over-states approach. The influence of screening was determined by applying an external static electric field in separate selfconsistent calculations to evaluate induced dipole moments which was used to determine the static linear and nonlinear polarizabilities. The polarizabilities calculated in the static limit were used to determine an effective screening parameter which was, in turn, used together with an RPA approach to calculate screened wave-dispersed, third-order nonlinear optical properties such as ⁽³⁾(–3;,,) and ⁽³⁾(–3;,,). Comparing evaluated polarizabilities with experimental values we found that the non-resonant free polarizability compares well in absolute magnitude with experimental results. Inclusion of screening results in a polarizability about two orders of magnitude below the experimental values.Paper presented at the 129th WE-Heraeus-Seminar on Surface Studies by Nonlinear Laser Spectroscopies, Kassel, Germany, May 30 to June 1, 1994     

Enhancement of activated decay of metastable states by resonant pumping

We consider the effect of a high-frequency pumping cost on the escape rate of a classical underdamped Brownian particle out of a deep potential well. The energy dependence of the oscillation frequency(E) is assumed to be weak on the scale of thermal energy,_E(0)T(0)T/V₀ (0)[_E(0) is the derivative of(E) atE= 0,V ₀ is the barrier height,V ₀ T]. The quadratic-in- contribution to the decay rate is calculated in two different regimes: (1) for the case of resonance of the pumping frequency with the nth harmonic of the internal motion at an energye, when = n(e); (2) for a rollout region of the basic resonance near the bottom of the potential well, when ¦-(0)¦ and is the damping coefficient. In the latter case the absorption spectrum and the enhancement of the decay rate are calculated as functions of two reduced parameters, the anharmonicity of the potential,v _E (0)T/, and the resonance mismatch, [ —(0)]/. It is shown that the effect of the pumping increases with diminishing ¦v¦ and at small v is proportional tov ^–1. In this regime, the dependence on is stepwise: the pumping contribution is large for v > 0 and small for v < 0. In the frame of our theory, the decay rate is invariant against the simultaneous alternation of the signs of andv. The spectrum of the energy absorption has the standard Lorentzian shape in the absence of anharmonicity,v=0, and with increasing of ¦v¦ shifts and widens retaining its bell-shape form.     

The modular group and super-KMS functionals

Every normal, faithful, self-adjoint functional on a von Neumann algebraA canonically determines a one-parameter-weakly continuous *-automorphism group (the analog of the modular group) and a canonical ₂ grading onA, commuting with . We show that the functional satisfies the weak super-KMS property with respect to and Furthermore, we prove that and are the unique pair of a-weakly continuous one-parameter *-automorphism group and a grading of the algebra, commuting with each other, with respect to which is weakly super-KMS. The above results thus provide a complete extension of the theory of Tomita and Takesaki to the nonpositive case.Supported in part by the National Science Foundation under Grant DMS-8922002.     

Localization in general one dimensional random systems,I. Jacobi matrices

We consider random discrete Schrödinger operators in a strip with a potentialV (n, ) (n a label in and a finite label across the strip) andV an ergodic process. We prove thatH ₀+V has only point spectrum with probability one under two assumptions: (1) Theconditional distribution of {V (n,)} _n=0,1;all conditioned on {V } _n0,1;all has an absolutely continuous component with positive probability. (2) For a.e.E, no Lyaponov exponent is zero.Research partially supported by USNSF grant MCS-81-20833     

Anderson localization for the almost Mathieu equation: II. Point spectrum for λ>2

We prove that for any >2 and a.e. , the pure point spectrum of the almost Mathieu operator (H()) _n = _n-1 + _n+1 + cos(2( +n)) _n contains the essential closure of the spectrum. Corresponding eigenfunctions decay exponentially. The singular continuous component, if it exists, is concentrated on a set of zero measure which is nowhere dense in .     

Some exact models for nonspherical collapse.I

Evolution of incoherent matter distributions with cylindrical, pseudoplanar, and toroidal symmetries is considered. The system is described in terms of the scale factora (R, T) and the anisotropy factor (R, T) of the (x², x³ surfaces. A number of exact solutions is obtained under the assumptions=(a), =(R), and=(T) and their physical properties are breifly discussed. In particular, the solution with=(T) is noncollapsing and describes a matter distribution with unchanging density.     

Theoretical investigation of noncollinear phase-matched parametric four-photon amplification of ultrashort light pulses in isotropic media

The amplification of light signals (angular frequency _S in some isotropic media (D₂O, fused silica, and Schott type SF10 glasses) by noncollinear phase-matched parametric four-photon interaction ₁+_2S+₁ is studied theoretically. Computer simulations are carried out for fundamental and second-harmonic pump pulses of a mode-locked Nd: glass laser. Degenerate interaction (wavelength ₁=₂=1054nm or 527 nm) and nondegenerate interaction (₁=1054nm, ₂=527 nm are considered. Characteristic phase-matching parameters and gain parameters versus wavelength are determined. Limitations by spectral bandwidth, optical absorption, optical damage, self-phase modulation, self-focusing and stimulated Raman scattering are analysed.     

The Schrödinger equation and canonical perturbation theory

LetT ₀(, )+V be the Schrödinger operator corresponding to the classical HamiltonianH ₀()+V, whereH ₀() is thed-dimensional harmonic oscillator with non-resonant frequencies =(₁, ... , _d ) and the potentialV(q ₁, ... ,q _d) is an entire function of order (d+1)^–1. We prove that the algorithm of classical, canonical perturbation theory can be applied to the Schrödinger equation in the Bargmann representation. As a consequence, each term of the Rayleigh-Schrödinger series near any eigenvalue ofT ₀(, ) admits a convergent expansion in powers of of initial point the corresponding term of the classical Birkhoff expansion. Moreover ifV is an even polynomial, the above result and the KAM theorem show that all eigenvalues _n (, ) ofT ₀+V such thatn coincides with a KAM torus are given, up to order , by a quantization formula which reduces to the Bohr-Sommerfeld one up to first order terms in .     

Anderson localization for the almost Mathieu equation: A nonperturbative proof

We prove that for any diophantine rotation angle and a.e. phase the almost Mathieu operator (H()) _n = _n–1 + _n+1 +cos(2(+n)) _n has pure point spectrum with exponentially decaying eigenfunctions for 15. We also prove the existence of some pure point spectrum for any 5.4.     

The role of electronic density of states in metallic Lanthanum

Observations of X-ray photoabsorption in metallic Lanthanum in the vicinity of the 3d _5/2-edge are given. Two separated absorption peaks are detected at the quantum energies =830.6eV and =834.0eV. The results are interpreted according to the model given in communication I–IV [1].     

Mesoscopic spin-flip transport through a quantum dot system responded by ac magnetic fields

We investigate mesoscopic spin transport through a quantum dot (QD) responded by a rotating and an oscillating magnetic fields. The rotating magnetic field rotates with the angular frequency 0 around the z-axis with the tilt angle , while the time-oscillating magnetic field is located in the z-axis with the angular frequency . The spin flip is caused by the rotating magnetic field, and it is the major source of spin current. The Zeeman effect is contributed by the two field components, and it is important as the magnetic fields are strong. The oscillating magnetic field takes significant role due to the spin-photon pumping effect, and the spin current can be generated by it even as 00 for the tilt angle 0. The peak and valley structure appears with respect to the frequency of oscillating field. The generation of spin current is companying with charge current. Spin current displays quite different appearance between the cases in the absence of source-drain bias (eV=0) and in the presence of source-drain bias (eV0). The symmetric spin current disappears to form asymmetric spin current with a negative valley and a positive plateau. The charge current is mainly determined by the source-drain bias, photon absorption, and spin-flip effect. This system can be employed as an ac charge-spin current generator, or ac charge-spin field effect transistor.